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Numerical multi-physical optimization of operating condition and current collecting setup for large-area solid oxide fuel cells

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Frontiers in Energy 2024年第3期18卷 356-368页

作者： Chengrong yu Zehua PAN Hongying ZHANG bin CHEN Wanbing GUAN bin MIAO Siew Hwa CHAN Zheng ZHONG Yexin ZHOU School of Science Harbin Institute of TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Deep Earth Sciences and Geothermal Energy Exploitation and Utilization Institute of Deep Earth Sciences and Green EnergyShenzhen UniversityShenzhen 518060China Key Laboratory of Advanced Fuel Cells and Electrolyzers Technology of Zhejiang Province Ningbo Institute of Materials Technology and Engineering of the Chinese Academy of SciencesNingbo 315201China Energy Research Institute at NTU(ERIAN) Nanyang Technological UniversitySingapore 639798Singapore

Due to the depletion of traditional fossil fuels and the aggravation of related environmental problems,hydrogen energy is gaining more attention all over the *** oxide fuel cell(SOFC)is a promising power generation technology operating on hydrogen with a high *** further boost the power output of a single cell and thus a single stack,increasing the cell area is an effective ***,it was recently found that further increasing the effective area of an SOFC single cell with a flat-tubular structure and symmetric double-sided cathodes would result in a lower areal *** this work,a multi-physical model is built to study the effect of the effective area on the cell *** distribution of different physical fields is systematically *** of the cell performance is also pursued by systematically tuning the cell operating condition and the current collection *** improvement of 42%is revealed by modifying the inlet gas flow rates and by enhancing the current *** the future,optimization of cell geometry will be performed to improve the homogeneity of different physical fields and thus to improve the stability of the cell.

关键词： solid oxide fuel cell(SOFC) large effective area flow rate discharge performance current collection

A nitroreductase-responsive nanoprobe with homogeneous composition and high loading for preoperative non-invasive tumor imaging and intraoperative guidance

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Chinese Chemical Letters 2024年第7期35卷 313-318页

作者： Jingqi Xin Shupeng Han Meichen Zheng Chenfeng Xu Zhongxi Huang bin Wang Changmin yu Feifei An yu Ren Institute of Medical Engineering Department of BiophysicsSchool of Basic Medical ScienceHealth Science CenterXi'an Jiaotong UniversityXi'an 710061China School of Public Health Health Science CenterXi'an Jiaotong UniversityXi'an 710061China Key Laboratory of Flexible Electronics(KLOFE)&Institute of Advanced Materials(IAM) Nanjing Tech UniversityNanjing 211816China Department of Breast Surgery the First Affiliated Hospital of Xi'an Jiaotong UniversityXi'an 710061China

Tumor microenvironment(TME)-activatable probes have been proven to effectively increase signal-tobackground ratios(SBRs)and improve the success rate of complete tumor ***,many fluorescence probes have to be loaded into a nanocarrier for tumor targeted delivery,which consequently encounters poor drug loading,heterogeneous composition and non-encapsulated drug aggregates occurred during nanoformulation ***,a nitroreductase(NTR)-activated“OFF-ON”near-infrared fluorescence nanoprobe,named Nano Bodipy,was synthesized by the spontaneous self-assembling of NTRresponsive dye-polyethylene glycol(PEG)amphiphilic polymer in *** NTR-responsive dye acted as the hydrophobic segment in the amphiphilic polymer,yielding a homogeneous composition and a high loading of 12.2 wt%(according to calculation)in the synthesized Nano *** synthesized Nano Bodipy can efficiently accumulate in tumors via the enhanced permeability and retention(EPR)effect,enabling non-invasive tumor-targeted fluorescence imaging and guiding complete tumor *** the synthesized Nano Bodipy entered the tumor cells,they dissociated and were activated by overexpressed *** the real-time fluorescence guide of Nano Bodipy,complete tumor resection surgery was performed successfully.

关键词： Nitroreductase Tumor diagnosis Intraoperative guidance Self-assembly Nanoprobe

Effect of FeSi additive in dual-chamber sample cup on thermal analysis characteristic values and vermiculating rate of compacted graphite iron

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China Foundry 2024年第1期21卷 91-100页

作者： De-quan Shi Ze-yu Liu Gui-li Gao Yi-cheng feng School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China School of Materials Science and Chemical Engineering Harbin University of Science&TechnologyHarbin 150040China School of Mechanical and Energy Engineering Shanghai Technical Institute of Electronics and InformationShanghai 201411China

Thermal analysis plays a key role in the online inspection of molten iron *** solidification process of molten iron can be reflected by thermal analysis curves,and silicon is one of important elements affecting the solidification of molten *** this study,FeSi75 was added in one chamber of the dual-chamber sample cup,and the influences of FeSi75 additive on the characteristic values of thermal analysis curves and vermiculating rate were *** results show that with the increase of FeSi75,the start temperature of austenite formation TALfirstly decreases and then increases,but the start temperature of eutectic growth TSEF,the lowest eutectic temperature TEU,temperature at maximum eutectic reaction rate TEM,and highest eutectic temperature TERkeep always an *** temperature at final solidification point TEShas little *** FeSi75 additive has different influences on the vermiculating rate of molten iron with different vermiculation,and the vermiculating rate increases for lower vermiculation molten iron while decreases for higher *** to the thermal analysis curves obtained by a dual-chamber sample cup with 0.30wt.%FeSi75 additive in one chamber,the vermiculating rate of molten iron can be evaluated by comparing the characteristic values of these *** time differenceΔtERcorresponding to the highest eutectic temperature TERhas a closer relationship with the vermiculating rate,and a parabolic regression curve between the time differenceΔtERand vermiculating rateηhas been obtained within the range of 65%to 95%,which is suitable for the qualified melt.

关键词： FeSi75 additive characteristic value vermiculating rate thermal analysis compacted graphite iron

Stage separation of recoverable liquid launch vehicle by using moving pulsating ball analogue for propellant sloshing

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Chinese Journal of Aeronautics 2024年第2期37卷 360-370页

作者： yu LU Baozeng yuE Bailong HAO Bole MA feng LIU yuanyuan CHANG School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Astronautical Systems Engineering Beijing 100076China

In the process of stage separation of recoverable liquid launch vehicles,because of the large amount of residual fuel in the storage tanks,the influence of liquid sloshing on separation safety must be *** calculation simplicity and operation practicability,the Moving Pulsating Ball Model(MPBM)of large amplitude liquid sloshing is introduced into the calculation of launch vehicle stage *** the dynamic equation of the model with the energy relationship during"breathing movement",the formula calculating the force of liquid on the rigid body is *** with the calculations of commercial CFD calculation software,the accuracy of MPBM model is ***,all the external forces and moments are applied to the rigid body of the stages,so that the translational and rotational dynamic equations of the stages are obtained *** to the relative position of the two stages,the geometric shape of the interstage section and the engine of the second stage,the minimum clearance in the separation process can be decided to guarantee that the separation process is safe.

关键词： Moving Pulsating Ball Model(MPBM) Dynamics of stage separation Large amplitude sloshing Recoverable liquid launch vehicle Flight dynamics

Layered metastructure containing freely-designed local resonators for wave attenuation

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Defence Technology（防务技术） 2024年第2期32卷 23-31页

作者： yu Li Huguang He Jiang feng Hailong Chen fengnian Jin Hualin Fan State Key Laboratory for Disaster Prevention&Mitigation of Explosion&Impact Army Engineering University of PLANanjing 210007China Rocket Force University of Engineering Xi'an 710025China Henan International Joint Laboratory of Dynamics of Impact and Disaster of Engineering Structures Department of Civil EngineeringNanyang Institute of TechnologyNanyang 473004China Guangxi Key Laboratory of Disaster Prevention and Engineering Safety and Key Laboratory of Disaster Prevention and Structural Safety of Ministry of EducationCollege of Civil Engineering and ArchitectureGuangxi UniversityNanning 530004China Research Center of Lightweight Structures and Intelligent Manufacturing State Key Laboratory of Mechanics and Control of Mechanical StructuresNanjing University of Aeronautics and AstronauticsNanjing 210016China

Combining periodic layered structure with three-dimensional cylindrical local resonators,a hybrid metastructure with improved wave isolation ability was designed and investigated through theoretical and numerical *** metastructure is composed of periodic rubber layers and concrete layers embedded with three-dimensional resonators,which can be freely designed with multi local resonant frequencies to attenuate vibrations at required frequencies and widen the attenuation *** metastructure can also effectively attenuate seismic *** with layered rubber-based structures,the metastructure has more excellent wave attenuation effects with greater attenuation and wider bandgap.

关键词： Layered metastructure Local resonator Wave attenuation

Molecular Dynamics Simulation Studies on the Micromorphology and Proton Transport of Nafion/Ti_(3)C_(2)T_(x) Composite Membrane

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Chinese Journal of Polymer Science 2024年第3期42卷 373-387,I0009页

作者： Zhi-yue Han Su-Peng Pei Chun-Yang yu Yong-feng Zhou School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China School of Chemistry&Chemical Engineering Frontiers Science Center for Transformative MoleculesShanghai Key Laboratory of Electrical Insulation and Thermal AgingShanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of Green and High-end Utilization of Salt Lake Resources Chinese Academy of SciencesXining 810008China

The perfluorosulfonic acid(PFSA) membrane doped with two-dimensional conductive filler Ti_(3)C_(2)T_(x) is a fuel cell proton exchange membrane with high application potential. Experimental studies showed that the proton conductivity of Nafion/Ti_(3)C_(2)T_(x) composite membrane is improved significantly compared with that in pure Nafion. However, the microscopic mechanism of doping on the enhancement of membrane performance is remain unclear now. In this work, molecular dynamics simulation was used to investigate the microscopic morphology and proton transport behaviors of Nafion/Ti_(3)C_(2)T_(x) composite membrane at the molecular level. The results shown that there were significant differences about the diffusion kinetics of water molecules and hydroxium ions in Nafion/Ti_(3)C_(2)T_(x) at low and high hydration levels in the nanoscale *** the increase of water content, Ti_(3)C_(2)T_(x) in membrane was gradually surrounded by ambient water molecules to form a hydration layer, and forming a relatively continuous proton transport channel between Nafion polymer and Ti_(3)C_(2)T_(x) monomer. The continuous proton transport channel could increase the number of binding sites of proton and thus achieving high proton conductivity and high mobility of water molecules at higher hydration level. The current work can provide a theoretical guidance for designing new type of Nafion composite membranes.

关键词： Nafion/Ti_(3)C_(2)T_(x)composite membrane Proton transport Molecular dynamics simulation

Elliptical vibration chiseling:a novel process for texturing ultra-high-aspect-ratio microstructures on the metallic surface

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International Journal of Extreme Manufacturing 2024年第2期6卷 449-467页

作者： Zhiwei Li Jianfu Zhang Zhongpeng Zheng Pingfa feng Dingwen yu Jianjian Wang State Key Laboratory of Tribology in Advanced Equipment Department of Mechanical EngineeringTsinghua UniversityBeijing 100084People’s Republic of China Beijing Key Laboratory of Precision/Ultra-precision Manufacturing Equipments and Control Department of Mechanical EngineeringTsinghua UniversityBeijing 100084People’s Republic of China Division of Advanced Manufacturing Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055People’s Republic of China

High-aspect-ratio metallic surface microstructures are increasingly demanded in breakthrough applications,such as high-performance heat transfer enhancement and surface plasmon ***,the fast and cost-effective fabrication of high-aspect-ratio microstructures on metallic surfaces remains challenging for existing *** study proposes a novel cutting-based process,namely elliptical vibration chiseling(EV-chiseling),for the high-efficiency texturing of surface microstructures with an ultrahigh aspect *** conventional cutting,EV-chiseling superimposes a microscale EV on a backward-moving *** tool chisels into the material in each vibration cycle to generate an upright chip with a high aspect ratio through material *** to the tool’s backward movement,the chip is left on the material surface to form a microstructure rather than falling *** one microstructure is generated in one vibration cycle,the process can be highly efficient using ultrafast(>1 kHz)tool vibration.A finite element analysis model is established to explore the process mechanics of ***,a mechanistic model of the microstructured surface generation is developed to describe the microstructures’aspect ratio dependency on the process ***,surface texturing tests are performed on copper to verify the efficacy of *** micro ribs with a spacing of 1–10μm and an aspect ratio of 2–5 have been successfully textured on *** with the conventional EV-cutting that uses a forward-moving tool,EV-chiseling can improve the aspect ratio of textured microstructure by up to 40 *** experimental results also verify the accuracy of the developed surface generation model of ***,the effects of elliptical trajectory,depth of cut,tool shape,and tool edge radius on the surface generation of micro ribs have been discussed.

关键词： metallic microstructure high aspect ratio backward-moving cutting vibration cutting chiseling material deformation

Three anti-inflammatory polysaccharides from Lonicera japonica Thunb.:insights into the structure-function relationships

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Food Science and Human Wellness 2024年第4期13卷 2197-2207页

作者： yu Liu Hongjing Dong Dongxiao Sun-Waterhouse Wenwen Li bin Zhang Jinqian yu Zhichang Qiu Zhenjia Zheng Key Laboratory of Food Nutrition and Health in Universities of Shandong College of Food Science and EngineeringShandong Agricultural UniversityTai’an 271018China Key Laboratory for Applied Technology of Sophisticated Analytical Instruments of Shandong Province Shandong Analysis and Test CenterQilu University of Technology(Shandong Academy of Sciences)Jinan 250014China School of Chemical Sciences The University of AucklandPrivate Bag 92019New Zealand

This study demonstrates the feasibility of producing three polysaccharides(neutral LJP-1,acidic LJP-2 and acidic LJP-3)with significant in vitro and in vivo anti-inflammatory activities from the flowers of Lonicera *** three polysaccharides differed in chemical composition,molecular weight(Mw)distribution,glycosidic linkage pattern,functional groups and *** exhibited excellent protective effects(in a dose-dependent manner)in lipopolysaccharide-injured RAW264.7 macrophages and Cu SO4-damaged zebrafish via reducing NO production and inhibiting the overexpressions of inflammation-related transcription factors,inflammatory proteins and cytokines in the NF-κB/MAPK signaling *** antiinflammatory effects varied owing to their different molecular characteristics and chemical ***,LJP-2 at 400μg/m L was the most ***-2 consisted mainly of→5)-α-L-Araf(1→,→4)-α-LGalp A(1→and→2)-α-L-Rhap(1→residues with terminal T-β-***,honeysuckle flowers are good sources of anti-inflammatory polysaccharides,and precise fractionation enables the production of potent antiinflammatory agents for the development of functional foods and healthcare products.

关键词： Honeysuckle polysaccharides Fractionation Molecular characteristics Anti-inflammatory properties Structure-function relationship

Dynamic simulation analysis of molten salt reactor-coupled air-steam combined cycle power generation system

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Nuclear Science and Techniques 2024年第2期35卷 222-233页

作者： Jing-Lei Huang Guo-bin Jia Li-feng Han Wen-Qian Liu Li Huang Zheng-Han Yang Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201800China University of Chinese Academy of Sciences Beijing 100049China

A nonlinear dynamic simulation model based on coordinated control of speed and flow rate for the molten salt reactor and combined cycle systems is proposed here to ensure the coordination and stability between the molten salt reactor and power *** model considers the impact of thermal properties of fluid variation on accuracy and has been validated with *** study reveals the capability of the control system to compensate for anomalous situations and maintain shaft stability in the event of perturbations occurring in high-temperature molten salt tank outlet ***,the control system’s impact on the system’s dynamic characteristics under molten salt disturbance is also *** results reveal that after the disturbance occurs,the controlled system benefits from the action of the control,and the overshoot and disturbance amplitude are positively correlated,while the system power and frequency eventually return to the initial *** simulation model provides a basis for utilizing molten salt reactors for power generation and maintaining grid stability.

关键词： Molten salt reactor Combined cycle Dynamic characteristic Control