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Direct patterning of reduced graphene oxide/graphene oxide memristive heterostructures by electron-beam irradiation

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Journal of Materials Science & Technology 2020年第3期38卷 237-243页

作者： Olesya O.Kapitanova Evgeny V.Emelin Sergey G.Dorofeev Pavel V.Evdokimov Gennady N.Panin youngmin lee Sejoon lee Lomonosov Moscow State University Leninskie gory119991 MoscowRussia Moscow Institute of Physics and Technology 9 Institutskiy per.DolgoprudnyMoscow Region141701Russia Institute of Microelectronics Technology and High-Purity Materials Russian Academy of SciencesChernogolovkaMoscow district142432Russia Nano Information Technology Academy Dongguk University-SeoulSeoul 04620Korea Quantum-Functional Semiconductor Research Center Dongguk University-SeoulSeoul 04620Korea Department of Semiconductor Science Dongguk University-SeoulSeoul 04620Korea

Memristive heterostructures,composed of reduced graphene oxide with different degree of reduction,were demonstrated through a simple method of‘direct electron-beam writing’on graphene *** with an electron beam at various doses and accelerating voltages made it possible to define highand low-conductivity graphene-oxide *** electron beam-reduced graphene oxide/graphene oxide heterostructure clearly exhibited a nonlinear behavior and a well-controlled resistive switching characteristic at a low operating-voltage range(<1 V).The proposed memristive heterostructures are promising for highly-efficient digital storage and information process as well as for analogous neuromorphic computations.

关键词： Electron beam irradiation Reduced graphene oxide Graphene oxide Memristive heterostructure

电沉积Mo和Mo-Co合金纳米线用于互联电阻的电阻率改性

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Engineering 2024年第1期32卷 127-137页

作者： Jun Hwan Moon Taesoon Kim youngmin lee Seunghyun Kim Yanghee Kim Jae-Pyoung Ahn Jungwoo Choi Hyuck Mo lee Young Keun Kim Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea Department of Materials Science and Engineering Korea Advanced Institute of Science and EngineeringDaejeon 34141Republic of Korea Advanced Analysis Center Korea Institute of Science and TechnologySeoul 02792Republic of Korea Research Resources Division Korea Institute of Science and TechnologySeoul 02792Republic of Korea

Achieving historically anticipated improvement in the performance of integrated circuits is challenging,due to the increasing cost and complexity of the required technologies with each new *** overcome this limitation,the exploration and development of novel interconnect materials and processes are highly desirable in the microelectronics ***(Mo)is attracting attention as an advanced interconnect material due to its small resistivity size effect and high cohesive energy;however,effective processing methods for such materials have not been widely ***,we investigate the electrochemical behavior of ions in the confined nanopores that affect the electrical properties and microstructures of nanoscale Mo and Mo-Co alloys prepared via template-assisted *** in an electrolyte allow the deposition of extremely pure metal materials,due to their interac-tion with metal ions and *** this study,boric acid and tetrabutylammonium bisulfate(TBA)were added to an acetate bath to inhibit the hydrogen evolution *** accelerated the reduction of Mo at the surface by inducing surface conduction on the *** Mo nanowires with a 130 nm diameter synthesized through high-aspect-ratio nanopore engineering exhibited a resistivity of(63.0±17.9)μΩ*** also evaluated the resistivities of Mo-Co alloy nanowires at various compo-sitions toward replacing irreducible conventional barrier/liner *** intermetallic compound formed at a Mo composition of 28.6 at%,the resistivity of the Mo-Co nanowire was(58.0±10.6)μΩcm,indicat-ing its superior electrical and adhesive properties in comparison with those of conventional barriers such as TaN and ***,density functional theory and non-equilibrium Green's function calcula-tions confirmed that the vertical resistance of the via structure constructed from Mo-based materials was 21%lower than that of a conventional Cu/Ta/TaN structure.

关键词： Molybdenum Molybdenum-cobalt Interconnect Microstructure Electrodeposition Density functional theory

Implementation of Dynamic Pictures into Spatially Coarse-Grained Atomic Models

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Implementation of Dynamic Pictures into Spatially Coarse-Gra...

Origin of the giant persistent photoconductivity in LaAlO_(3)/SrTiO_(3)heterostructures probed by noise spectroscopy

The Sixth World Congress on Computational Mechanics in Conjunction with the Second Asian-Pacific Congress on Computational MechanicsⅠ

作者： Sung Youb Kim Sukky Jun Young-Sam Cho Jong Youn Park youngmin lee Seyoung Im Department of Mechanical Engineering Korea Advanced Institute of Science and Technology(KAIST) 373-1 Cruseong-dong Yuseong-gu Daejeon 305-701

As a part of the synthetic multiscale modeling and simulation both in length and time scales, an implementation methodology of dynamic picture into spatially coarse-grained atomic system is presented. For tackling the length-scale limitation of atomistic simulations, employed in this work is the fully nonlocal three-dimensional version of the quasicontinuum method [1]. This coarse-grained atomic system are then implemented into the formulation of the action-derived molecular dynamics (ADMD) that has recently proposed to handle the multiple time-scale atomic systems such as rare-event and slow-mode systems [2-3]. This combination of ADMD and nonlocal quasicontinuum method provides the complete dynamic pathways, not simply minimized configurations, of the large-scale atomic models including energy barrier through a saddle point in phase space. The proposed scheme does not suffer from the unrealistic wave reflection caused by the presence of boundaries or interfaces, which is difficult to avoid in dynamic simulations of scale-bridging models. In this presentation, two typical examples of multiple time-scale problems are simulated. One is the adatom diffusion on (100) metal surface. The energy barrier and the realistic dynamic trajectory of diffusion mechanism are calculated for the coarse-grained quasicontinuum models. The other example is the molecular junction of long carbon nanotubes. For this, we also suggest a nonlocal coarse-graining scheme for large-scale carbon nanotubes. The various dynamic pictures of junction formations through bond-breaking and re-bonding of carbon atoms are examined with the activation energy barriers of the specific atomic recon figuration to take place. It is of note that all the dynamic pathways found are determined only by actual dynamic conditions such as the energy conservation, not by predetermined evolving scenarios of the atomic configurations.

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Journal of Materials Science & Technology 2023年第6期137卷 152-158页

作者： Kitae Eom Jung-Woo lee Gyeongmo Yang youngmin Kim Jaeyoung Jeon Jieun Yeon Hyungwoo lee School of Advanced Materials Science and Engineering Sungkyunkwan University(SKKU)Suwon 16419South Korea KIURI Institute Yonsei UniversitySeoul 03722South Korea Department of Physics Ajou UniversitySuwon 16499South Korea Department of Energy Systems Research Ajou UniversitySuwon 16499South Korea

LaAlO_(3)/SrTiO_(3)(LAO/STO)heterostructures have shown a strong persistent photoconductivity(PPC)at room *** abnormally strong PPC has attracted immense research interest due to its possible applications in optically-tunable electronic *** its promise,the fundamental understanding of the PPC in the LAO/STO heterostructures is still ***,we report that the giant PPC origi-nates from the photo-induced valence change in oxygen vacancies near the LAO/STO *** spec-tral analysis of the photocurrent and the model-fitting study consistently show that the ionized oxygen vacancies near the interface are neutralized during the electron relaxation *** hinder the complete relaxation of the photoexcited electrons by the deeply-located oxygen vacancies and result in the strong *** change in the ionization state distribution of the oxygen vacancies is probed by the per-sistent noise behavior at the frequency between 1 kHz and 20 kHz *** results provide insight into the role of oxygen vacancies in influencing the internal charge distribution and triggering the PPC phenomena in complex oxide heterostructures.

关键词： Persistent photoconductivity LaAlO_(3)/SrTiO_(3)heterostructures Two-dimensional electron gases Oxygen vacancies Low-frequency noise Spectral analyses

Signal processing for real-time identification of similar metals by laser-induced breakdown spectroscopy

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Plasma Science and Technology 2019年第3期21卷 84-91页

作者： Sungho SHIN youngmin MOON Jaepil lee Hyemin JANG Euiseok HWANG Sungho JEONG School of Mechanical Engineering Gwangju Institute of Science and Technology

Laser-induced breakdown spectroscopy(LIBS) is regarded as a promising technique for realtime sorting of scrap metals due to its capability of fast multi-elemental and in-air analysis. This work reports a method for signal processing which ensures high accuracy and high speed during similar metal sorting by LIBS. Similar metals such as aluminum alloys or stainless steel are characterized by nearly the same constituent elements with slight variations in elemental concentration depending on metal type. In the proposed method, the original data matrix is substantially reduced for fast processing by selecting new input variables(spectral lines) using the information for the constituent elements of similar metals. Specifically, principal component analysis(PCA) of full-spectra LIBS data was performed and then, based on the loading plots, the input variables of greater significance were selected in the order of higher weights for each constituent element. The results for the classification test with aluminum alloy, copper alloy,stainless steel and cast steel showed that the classification accuracy of the proposed method was nearly the same as that of full-spectra PCA, but the computation time was reduced by a factor of 20 or more. The results demonstrated that incorporating the information for constituent elements can significantly accelerate classification speed without loss of accuracy.

关键词： laser-induced breakdown spectroscopy classification similar metal reduced number of spectral lines

PGLYRP1 protein as a novel mediator of cellular dialogue in neuroinflammation

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Neural Regeneration Research 2025年第7期20卷 1993-1994页

作者： Anup Bhusal Won-Ha lee Kyoungho Suk Department of Pharmacology School of MedicineKyungpook National UniversityDaeguRepublic of Korea BK21 Plus KNU Biomedical Convergence Program Department of Biomedical ScienceSchool of MedicineKyungpook National UniversityDaeguRepublic of Korea School of Life Sciences BK21 plus KNU Creative BioResearch GroupKyungpook National UniversityDaeguRepublic of Korea Brain Science and Engineering Institute Kyungpook National UniversityDaeguRepublic of Korea

Neuroinflammation has been identified as a crucial element in several neurological disorders. Glial cells play a critical role in directing neuroinflammation, both in deleterious and beneficial ways.

关键词： inflammation considerably

Single-cell and spatial omics:exploring hypothalamic heterogeneity

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Neural Regeneration Research 2025年第6期20卷 1525-1540页

作者： Muhammad Junaid Eun Jeong lee Su Bin Lim Department of Biochemistry&Molecular Biology Ajou University School of MedicineSuwonSouth Korea Department of Biomedical Sciences Graduate School of Ajou UniversitySuwonSouth Korea Department of Brain Science Ajou University School of MedicineSuwonSouth Korea

Elucidating the complex dynamic cellular organization in the hypothalamus is critical for understanding its role in coordinating fundamental body functions. Over the past decade, single-cell and spatial omics technologies have significantly evolved, overcoming initial technical challenges in capturing and analyzing individual cells. These high-throughput omics technologies now offer a remarkable opportunity to comprehend the complex spatiotemporal patterns of transcriptional diversity and cell-type characteristics across the entire hypothalamus. Current single-cell and single-nucleus RNA sequencing methods comprehensively quantify gene expression by exploring distinct phenotypes across various subregions of the hypothalamus. However, single-cell/single-nucleus RNA sequencing requires isolating the cell/nuclei from the tissue, potentially resulting in the loss of spatial information concerning neuronal networks. Spatial transcriptomics methods, by bypassing the cell dissociation, can elucidate the intricate spatial organization of neural networks through their imaging and sequencing technologies. In this review, we highlight the applicative value of single-cell and spatial transcriptomics in exploring the complex molecular-genetic diversity of hypothalamic cell types, driven by recent high-throughput achievements.

关键词： cellular diversity hypothalamus multi-omics single-cell transcriptomics spatial transcriptomics

Generation of brain vascular heterogeneity:recent advances from the perspective of angiogenesis

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Neural Regeneration Research 2025年第7期20卷 2013-2014页

作者： Nathanael J.lee Ryota L.Matsuoka Department of Neurosciences Lerner Research InstituteCleveland ClinicClevelandOHUSA Department of Molecular Medicine Cleveland Clinic Lerner College of MedicineCase Western Reserve UniversityClevelandOHUSA

Heterogeneous proper t i es of vascular endothelial cells in the brain:The brain displays large energy dynamics and consumption,and this high level of metabolic demands is fulfilled by a continuous supply of glucose and oxygen through its vascular *** vasculature consists of highly divergent blood vessel branches,giving rise to a dense network of capillaries that supply blood to all cells across the *** elaborated vascular network is thought to develop via angiogenesis,a process in which new blood vessels grow from pre-existing *** capillaries exhibit organotypic features distinct from other tissues and are formed primarily by two major endothelial cell(EC)types:those that form the semi-permeable blood-brain barrier(BBB)and those that develop highly permeable pores known as fenestrae(Matsuoka et al.,2022).The structural and functional differences between BBB and fenestrated vascular ECs represent a fundamental feature of brain vasculature and form the foundation for both brain function and homeostasis.

关键词： angiogenesis homeostasis network

Tailoring Light–Matter Interactions in Overcoupled Resonator for Biomolecule Recognition and Detection

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Nano-Micro Letters 2025年第1期17卷 262-280页

作者： Dongxiao Li Hong Zhou Zhihao Ren Cheng Xu Chengkuo lee Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore Center for Intelligent Sensors and MEMS(CISM) National University of SingaporeSingapore 117608Singapore

Plasmonic nanoantennas provide unique opportunities for precise control of light–matter coupling in surface-enhanced infrared absorption(SEIRA)spectroscopy,but most of the resonant systems realized so far suffer from the obstacles of low sensitivity,narrow bandwidth,and asymmetric Fano resonance ***,we demonstrated an overcoupled resonator with a high plasmon-molecule coupling coefficient(μ)(OC-Hμresonator)by precisely controlling the radiation loss channel,the resonator-oscillator coupling channel,and the frequency detuning *** observed a strong dependence of the sensing performance on the coupling state,and demonstrated that OC-Hμresonator has excellent sensing properties of ultra-sensitive(7.25%nm^(−1)),ultra-broadband(3–10μm),and immune asymmetric Fano *** characteristics represent a breakthrough in SEIRA technology and lay the foundation for specific recognition of biomolecules,trace detection,and protein secondary structure analysis using a single array(array size is 100×100μm^(2)).In addition,with the assistance of machine learning,mixture classification,concentration prediction and spectral reconstruction were achieved with the highest accuracy of 100%.Finally,we demonstrated the potential of OC-Hμresonator for SARS-CoV-2 *** findings will promote the wider application of SEIRA technology,while providing new ideas for other enhanced spectroscopy technologies,quantum photonics and studying light–matter interactions.

关键词： Plasmonic nanoantennas Light-matter interaction Surface-enhanced infrared absorption Overcoupled Biosensing