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Impact of climate change and human activities on the spatiotemporal dynamics of surface water area in Gansu Province, China

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Journal of Arid Land 2024年第6期16卷 798-815页

作者： LU Haitian zhao Ruifeng zhao Liu LIU Jiaxin LYU Binyang YANG Xinyue College of Geography and Environmental Science Northwest Normal UniversityLanzhou 730070China Key Laboratory of Resource Environment and Sustainable Development of Oasis Gansu ProvinceLanzhou 730070China School of Geography Planning and Spatial SciencesUniversity of TasmaniaHobart TAS 7005Australia School of Chinese Language and Literature Xi'an International Studies UniversityXi'an 710128China Department of Mechanics and Aerospace Engineering Southern University of Science and TechnologyShenzhen 518055China School of Design and Built Environment Curtin UniversityPerth 6102Australia

Understanding the dynamics of surface water area and their drivers is crucial for human survival and ecosystem stability in inland arid and semi-arid *** study took Gansu Province,China,a typical area with complex terrain and variable climate,as the research *** on Google Earth Engine,we used Landsat data and the Open-surface Water Detection Method with Enhanced Impurity Control method to monitor the spatiotemporal dynamics of surface water area in Gansu Province from 1985 to 2022,and quantitatively analyzed the main causes of regional differences in surface water *** findings revealed that surface water area in Gansu Province expanded by 406.88 km2 from 1985 to *** surface water area exhibited significant fluctuations,while permanent surface water area showed a steady ***,terrestrial water storage exhibited a trend of first decreasing and then increasing,correlated with the dynamics of surface water *** change and human activities jointly affected surface hydrological processes,with the impact of climate change being slightly higher than that of human ***,climate change affected the'source'of surface water to a greater extent,while human activities tended to affect the'destination'of surface *** of surface water resources faced by inland arid and semi-arid areas like Gansu Province are ***,we summarized the surface hydrology patterns typical in inland arid and semi-arid areas and tailored surface water'supply-demand'balance *** study not only sheds light on the dynamics of surface water area in Gansu Province,but also offers valuable insights for ecological protection and surface water resource management in inland arid and semi-arid areas facing water scarcity.

关键词： surface water area terrestrial water storage Open-surface Water Detection Method with Enhanced Impurity Control method Google Earth Engine climate change human activities inland arid and semi-arid areas

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渗滤液作基质培养甲烷氧化菌的工艺优化

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环境工程 2014年第9期32卷 65-69页

作者：梅娟赵由才苏州科技学院环境科学与工程学院江苏苏州215009 同济大学污染控制与资源化研究国家重点实验室上海200092

甲烷氧化菌菌液可用来制备高甲烷氧化率的填埋场覆盖材料。分析了渗滤液预处理对甲烷氧化菌培养的影响,优化了渗滤液作基质培养甲烷氧化菌的工艺。结果表明:补充N、P能改善培养效果,使培养液的最高甲烷氧化率提高30%以上,稀释效果不明... 详细信息

甲烷氧化菌菌液可用来制备高甲烷氧化率的填埋场覆盖材料。分析了渗滤液预处理对甲烷氧化菌培养的影响,优化了渗滤液作基质培养甲烷氧化菌的工艺。结果表明:补充N、P能改善培养效果,使培养液的最高甲烷氧化率提高30%以上,稀释效果不明显。甲烷氧化会降低渗滤液中金属元素的浓度,Mn、Fe和Cu等元素含量过低可能成为老龄渗滤液甲烷氧化菌培养的限制因素。

关键词：渗滤液矿化垃圾甲烷氧化菌填埋场

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Ionic liquid-assisted preparation of hydroxyapatite and its catalytic performance for decarboxylation of itaconic acid

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Chinese Journal of Chemical Engineering 2024年第3期67卷 9-15页

作者： Shutong Pang Hualiang An Xinqiang zhao Yanji Wang Hebei Provincial Key Laboratory of Green Chemical Technology and Efficient Energy Saving Tianjin Key Laboratory of Chemical Process SafetySchool of Chemical Engineering and TechnologyHebei University of TechnologyTianjin 300130China

The synthesis of methacrylic acid from biomass-derived itaconic acid is a green route,for it can get rid of the dependence on fossil *** order to solve the problems on this route such as use of a preciousmetal catalyst and a corrosive homogeneous alkali,we prepared a series of hydroxyapatite catalysts by an ionic liquid-assisted hydrothermal method and evaluated their catalytic *** results showed that the ionic liquid[Bmim]BF_(4) can affect the crystal growth of hydroxyapatite,provide fluoride ion for fluorination of hydroxyapatite,and adjust the surface acidity and basicity,morphology,textural properties,crystallinity,and composition of ***[Bmim]BF4 dosage and hydrothermal temperature can affect the fluoride ion concentration in the hydrothermal system,thus changing the degree of fluoridation of *** fluoride-ion concentration can lead to the formation of CaF_(2) and thus significantly decrease the catalytic performance of *** hydrothermal time mainly affects the growth of hydroxyapatite crystals on the c axis,leading to different catalytic *** suitable conditions for the preparation of this fluoridized hydroxyapatite are as follows:a mass ratio of[Bmim]BF4 to calcium salt=0.2:1,a hydrothermal time of 12 h,and a hydrothermal temperature of 130℃.A maximal methacrylic acid yield of 54.7%was obtained using the fluoridized hydroxyapatite under relatively mild reaction conditions(250℃ and 2 MPa of N_(2))in the absence of a precious-metal catalyst and a corrosive homogeneous alkali.

关键词： Ionic liquid Hydroxyapatite Itaconic acid Methacrylic Decarboxylation reaction

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Self-Triggered Set Stabilization of Boolean Control Networks and Its Applications

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IEEE/CAA Journal of Automatica Sinica 2024年第7期11卷 1631-1642页

作者： Rong zhao Jun-e Feng Dawei Zhang the School of Mathematics Shandong UniversityShandong UniversityJinan 250100China

Set stabilization is one of the essential problems in engineering systems, and self-triggered control(STC) can save the storage space for interactive information, and can be successfully applied in networked control systems with limited communication resources. In this study, the set stabilization problem and STC design of Boolean control networks are investigated via the semi-tensor product technique. On the one hand, the largest control invariant subset is calculated in terms of the strongly connected components of the state transition graph, by which a graph-theoretical condition for set stabilization is derived. On the other hand, a characteristic function is exploited to determine the triggering mechanism and feasible controls. Based on this, the minimum-time and minimum-triggering open-loop, state-feedback and output-feedback STCs for set stabilization are designed,respectively. As classic applications of self-triggered set stabilization, self-triggered synchronization, self-triggered output tracking and self-triggered output regulation are discussed as well. Additionally, several practical examples are given to illustrate the effectiveness of theoretical results.

关键词： Boolean control networks(BCNs) output regulation self-triggered control semi-tensor product of matrices set stabilization synchronization

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Illuminating functions of evolutionarily conserved long non-coding RNAs

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Science China Life Sciences 2024年第9期67卷 2043-2044页

作者： Ruiqiao He Fangqing zhao Institute of Zoology Chinese Academy of Sciences Key Laboratory of Systems Health Science of Zhejiang Province Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences

Long non-coding RNAs(lnc RNAs) serve as crucial regulators of gene expression,influencing various physiological processes and disease states(Cabili et al.,2011; Ulitsky and Bartel, 2013; Yao et al.,2019). Dysregulation of certain notable lnc RNAs, such as HOTAIR and MALAT1,has been implicated in a wide range of pathological processes, including tumorigenesis in various human cancers(Gupta et al., 2010; Kim et al., 2018). However,the functions of the majority of lnc RNAs remain elusive.

关键词： LINCRNAS

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Integrated separation-electrochemical detection device based on wood column for online identification of enantiomer

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Nano Research 2024年第3期17卷 1893-1901页

作者： Junli Guo Yuanfei Xue Chenxi zhao Junjian zhao Zhida Gao Ye Mei Yan-Yan Song College of Sciences Northeastern UniversityShenyang 110004China State Key Laboratory of Precision Spectroscopy School of Physics and Electronic ScienceEast China Normal UniversityShanghai 200062China NYU-ECNU Center for Computational Chemistry at NYU Shanghai Shanghai 200062China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

Chiral chemicals have attracted significant interest in the pharmaceutical industry,yet the separation methods to get pure enantiomers from racemic mixture are still *** date,the separation of enantiomers still mainly depends on chromatography using high-cost chiral stationary ***,wood channels were used as the handheld integrated device,and enantiomer separation was simultaneously detected using an electrochemical *** this method,a chiral UIO-66(L-UIO-66)modified enantiomer separation zone and carbonized wood based online detection zone are integrated along a single wood *** on the in situ separation results from the chronoamperometry data,the wood device shows excellent separation ability for a wide range of electrochemically active enantiomers,including 3,4-dihydroxyphenylalanine,amino acids,ascorbic acid,carnitine,and penicillamine with high chirality *** unbiased molecular dynamic simulations indicate that the excellent chiral recognition and separation are attributed to the different barriers from the bound states to the dissociated state of the enantiomers in the homochiral microenvironment of the *** integrated enantiomer separation-electrochemical detection device provides a novel,easy,and low-cost platform for the separation of pure enantiomer from racemic mixture.

关键词： wood column integrated separation-detection device enantioselectivity online sensing free energy barrier

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矿化垃圾生物反应床处理NO_X废气的研究

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环境污染与防治 2005年第4期27卷 271-273页

作者：张华赵由才同济大学污染控制与资源化研究国家重点实验室上海200092

矿化垃圾(稳定化垃圾)是一种良好的生物介质,可作为生物反应床的填料处理NOX废气。实验室研究表明,稳定化垃圾反应床可有效地处理NOX气体,其硝化能力(以N计)可达0.83g/(kg·d)(干重)。NOX去除率受停留时间的影响显著,NOX去除率随着停留... 详细信息

矿化垃圾(稳定化垃圾)是一种良好的生物介质,可作为生物反应床的填料处理NOX废气。实验室研究表明,稳定化垃圾反应床可有效地处理NOX气体,其硝化能力(以N计)可达0.83g/(kg·d)(干重)。NOX去除率受停留时间的影响显著,NOX去除率随着停留时间的缩短而降低。当空床停留时间为1.5min时,NOX气体的平均去除率为76.7%;空床停留时间为15min时,NOX气体的平均去除率为91.0%。在NOX进气负荷低于110mmol/(m3·h)时,NOX消除能力随进气负荷的增加而线性增加。当进气流量一定时,NOX去除能力随着进气NOX浓度的增加而线性增加。

关键词：稳定化垃圾矿化垃圾氮氧化物生物过滤

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制革污泥焚烧特性及焚烧过程中重金属挥发控制研究

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环境科学学报 2011年第6期31卷 1270-1276页

作者：夏凤毅赵由才唐平中国计量学院杭州310018 同济大学污染控制与资源化研究国家重点实验室上海200092 杭州电子科技大学材料与环境科学院杭州310018

以制革污泥为研究对象进行焚烧处理,并对其燃烧特性进行分析.结果发现,制革污泥燃烧过程中并未出现明显的固定碳燃烧区.同时,将制革污泥与煤粉混合后焚烧,结果显示,制革污泥的比例及挥发分的析出对混合燃料的着火燃烧有显著影响,在低温... 详细信息

以制革污泥为研究对象进行焚烧处理,并对其燃烧特性进行分析.结果发现,制革污泥燃烧过程中并未出现明显的固定碳燃烧区.同时,将制革污泥与煤粉混合后焚烧,结果显示,制革污泥的比例及挥发分的析出对混合燃料的着火燃烧有显著影响,在低温段（180~450℃）,制革污泥比例的增大可提高混合试样的活化性能,且燃烧程度加剧.通过添加CaO、橡胶粉等添加剂,可抑制制革污泥焚烧过程中重金属的挥发,当CaO添加量为3%时,对Zn、Pb、Cu和C r等重金属的抑制效果最佳,其挥发率分别降低了5.23%、0.90%、5.59%和4.43%;橡胶粉的添加对于金属元素的挥发有一定的影响,但影响程度非常有限.

关键词：制革污泥煤粉焚烧重金属挥发控制热重分析

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Enhanced photocatalytic nitrogen fixation performance via in situ constructing BiO_(2-x)/NaNbO_(3) heterojunction

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Chinese Journal of Chemical Engineering 2024年第5期69卷 92-100页

作者： Jiayu Zhang Zhihao Zeng Lin Yue Chunran zhao Xin Hu Leihong zhao Xiuwen Wang Yiming He Key Laboratory of the Ministry of Education for Advanced Catalysis Materials College of Chemistry and Materials ScienceZhejiang Normal UniversityJinhua 321004China Heilongjiang Provincial Key Laboratory of Surface Active Agent and Auxiliary School of Chemistry and Chemistry EngineeringQiqihar UniversityQiqihar 161006China Department of Materials Science and Engineering Zhejiang Normal UniversityJinhua 321004China

The fabrication of heterojunction catalysts is an effective strategy to enhance charge separation efficiency,thereby boosting the performance of *** this study,BiO_(2-x)nanosheets were synthesized through a hydrothermal process and loaded onto NaNbO_(3) microcube to construct a series of BiO_(2-x)/NaNbO_(3) heterojunctions for photocatalytic N_(2) *** indicated that 2.5%BiO_(2-x)/NaNbO_(3) had the highest photocatalytic *** NH_(3) production rate under simulated solar light reached 406.4μmol·L^(-1)·g^(-1)·h^(-1),which reaches 2.6 and 3.8 times that of NaNbO_(3) and BiO_(2-x),***_(2-x)nanosheets primarily act as electron trappers to enhance the separation efficiency of charge *** strong interaction between BiO_(2-x)and NaNbO_(3) facilitates the electron migration between ***,the abundant oxygen vacancies in BiO_(2-x)nanosheets may facilitate the adsorption and activation of N_(2),which may be another possible reason of the high photocatalytic activity of the BiO_(2-x)/NaNbO_(3).This study may offer new insights for the development of semiconductor materials in photocatalytic nitrogen fixation.

关键词： Catalyst Solar energy Hydrothermal BiO_(2-x)/NaNbO_(3) Photocatalytic N_(2)-fixation

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Well-dispersed Sb particles embedded on N-doped carbon nanofibers toward high-performance Li-ion battery

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Rare Metals 2024年第7期43卷 2994-3006页

作者： Ying Li Yi-Han zhao Lu-Lu zhao Peng-Fei Wang Ying Xie Ting-Feng Yi School of Materials Science and Engineering Northeastern UniversityShenyang 110819China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China

The alloy-type material Sb is widely used in the anode materials of lithium-ion batteries(LIBs)due to its high theoretical specific ***,its serious volume expansion problem during alloying/dealloying of Li~+limits its practical *** this work,C-Sb composite was constructed as anode material of LIBs by electrospinning route for the first time,Sb was introduced into the polyacrylonitrile-based hard carbon and coal tar pitch-based soft carbon composite amorphous carbon fiber with a diameter of 300-600 nm,which realized high cycling *** C-Sb-2(the mass ratio of polyacrylonitrile to Sb source is 1:2)electrode displayed charge capacities of 1098.5,930.3,841.7,753.5,643.9 and 545.8 mAh·g^(-1)at 0.1,0.2,0.3,0.5,1 and 2 A·g^(-1),*** when the current density returned to 0.1 A·g^(-1),the charge capacity was 939.3 mAh·g^(-1),revealing good stability and *** introduction of Sb into the amorphous carbon improved its conductivity and addressed the volume expansion issue of high specific capacity Sb during charge/***-situ XRD analysis confirmed the high reversibility of the C-Sb-2 during charging and *** functional theory(DFT)calculations revealed the gradual enhancement of the interface interaction between Sb_(x)Li_(y) and amorphous carbon(AMC)with increasing lithium content,contributing to the anchoring of alloy nanoparticles on the AMC surface and buffering the volume change of the ***,the gradual lithiation of Sb facilitated the electron transfer from Sb_(x)Li_(y) to *** findings hold promise for designing lithium storage materials with exceptional performance,highlighting the potential of C-Sb composites as anode materials for efficient next-generation lithium storage.

关键词： Li-ion battery Metallic Sb Carbon Electrospinning Cycling stability

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