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N:ZnO/MoS_(2)-heterostructured flexible synaptic devices enabling optoelectronic co-modulation for robust artificial visual systems

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Nano Research 2024年第3期17卷 1902-1912页

作者： Lei Xu Wenxiao Wang Yang Li yonghui lin Wenjing Yue Kai Qian Qinglei Guo Jeonghyun Kim Guozhen Shen School of Information Science and Engineering University of JinanJinan 250022China School of Microelectronics Shandong UniversityJinan 250101China Department of Electronic Convergence Engineering Kwangwoon UniversitySeoul 01897Republic of Korea School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing 100081China

With the merits of non-contact,highly efficient,and parallel computing,optoelectronic synaptic devices combining sensing and memory in a single unit are promising for constructing neuromorphic computing and artificial visual chip.Based on this,a N:ZnO/MoS_(2)-heterostructured flexible optoelectronic synaptic device is developed in this work,and its capability in mimicking the synaptic behaviors is systemically investigated under the electrical and light signals.Versatile synaptic functions,including synaptic plasticity,long-term/short-term memory,and learning-forgetting-relearning property,have been achieved in this synaptic device.Further,an artificial visual memory system integrating sense and memory is emulated with the device array,and the visual memory behavior can be regulated by varying the light parameters.Moreover,the optoelectronic co-modulation behavior is verified by applying mixed electric and light signals to the array.In detail,a transient recovery property is discovered when the electric signals are applied in synergy during the decay of the light response,of which property facilitates the development of robust artificial visual systems.Furthermore,by superimposing electrical signals during the light response process,a differentiated response of the array is achieved,which can be used as a proof of concept for the color perception of the artificial visual system.

关键词： flexible synaptic device synaptic plasticity optoelectronic synapse robust visual memory optoelectronic co-modulation artificial visual system

Reducing children’s exposure to di(2-ethylhexyl)phthalate in homes and kindergartens in China:Impact on lifetime cancer risks and burden of disease

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Building Simulation 2024年第3期17卷 431-440页

作者： Dongsheng Tao Wen Sun Donghui Mo yonghui lin Wei Lv Daniel Mmereki Yousheng Xu Yanghui Ye Yuanjun Tang Chao Ye Cong Dong Zhongming Bu Zhejiang Ecowell Energy Management Technology Co. LtdHangzhouChina Department of Energy and Environmental System Engineering Zhejiang University of Science and TechnologyHangzhouChina Faculty of Health Sciences School of Clinical MedicineUniversity of the WitwatersrandParktown2193JohannesburgSouth Africa

Exposure to di(2-ethylhexyl)phthalate(DEHP)in the indoor environment has been linked with significant health risks for Chinese children.Multi-phase DEHP concentrations in Chinese residences and kindergartens were estimated using a mass balance model based on the current baseline condition and control strategies(i.e.,increasing ventilation rate,reducing area of sources,using mechanical ventilation systems,and using portable air cleaners).The health benefits of each control strategy were quantified as the reduction in lifetime cancer risks(LCR)and burden of disease(BoD).In the current situation,the mean LCR and disability-adjusted life years(DALY)number attributable to indoor DEHP exposure for Chinese children were around 6.0×10^(−6) and 155 thousand,respectively.The mean LCR and DALY might be reduced by 25%-54%and 16%-40%,respectively,by increasing air exchange rates by 100%,reducing the use of source materials by two-thirds or deploying commercial air cleaners in naturally ventilated buildings.Meanwhile,avoidable DALYs could result in a reduction of mean economic losses of 2.2-5.3 billion RMB.Mechanical ventilation systems with filtration units may not be helpful for reducing children’s health risks.House-specific and tailor-made control measures are critical in lowering indoor exposure to DEHP to promote sustainable buildings and children’s health in China.

关键词： indoor air di(2-ethylhexyl)phthalate children exposure control strategies health benefits

Two NIS1-like proteins from apple canker pathogen(Valsa mali)play distinct roles in plant recognition and pathogen virulence

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Stress Biology 2022年第1期2卷 606-620页

作者： Jiajun Nie Wenjing Zhou yonghui lin Zhaoyang Liu Zhiyuan Yin Lili Huang State Key Laboratory of Crop Stress Biology for Arid Areas College of Plant ProtectionNorthwest A&F University3 Taicheng RoadYangling 712100ShaanxiChina College of Plant Protection China Agricultural UniversityBeijing 100193China

Conserved effectors produced by phytopathogens play critical roles in plant-microbe interactions.NIS1-like proteins represent a newly identified family of effectors distributed in multiple fungal species.However,their biological functions in a majority of pathogenic fungi remain largely elusive and require further investigation.In this study,we characterized two NIS1-like proteins VmNIS1 and VmNIS2 from Valsa mali,the causal agent of apple Valsa canker.Both of these two proteins were predicted to be secreted.Using agroinfiltration,we found that VmNIS1 induced intense cell death,whereas VmNIS2 suppressed INF1 elicitin-triggered cell death in Nicotiana benthamiana.Treatment of N.benthamiana with VmNIS1 recombinant protein produced by Escherichia coli activated a series of immune responses and enhanced plant disease resistance against Phytophthora capsici.In contrast,VmNIS2 suppressed plant immune responses and promoted P.capsici infection when transiently expressed in N.benthamiana.Both VmNIS1 and VmNIS2 were shown to be highly induced at late stage of V.mali infection.By individually knocking out of these two genes in V.mali,however,only VmNIS2 was shown to be required for pathogen virulence as well as tolerance to oxidative stress.Notably,we further showed that C-terminal extension of VmNIS1 was essential for plant recognition and VmNIS2 may escape plant detection via sequence truncation.Our data collectively indicate that VmNIS1 and VmNIS2 play distinct roles in plant recognition and pathogen virulence,which provided new insights into the function of NIS1-like proteins in plant-microbe interactions.

关键词： Valsa mali Effector protein Cell death Plant immunity Virulence

Removal of Crystal Violet from aqueous solution using powdered mycelial biomass of Ceriporia lacerata P2

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Journal of Environmental Sciences 2011年第12期23卷 2055-2062页

作者： yonghui lin Xingbing He Guomin Han Qijian Tian Wenyong Hu College of Biology and Environmental Sciences Jishou University Jishou 416000 China School of Life Science Nanjing University Nanjing 210093 China

A biosorbent prepared from powdered mycelial biomass of Ceriporia lacerata （CLB）, a basidiomycetous fungus, was applied for the uptake of Crystal Violet from aqueous solution. A batch adsorption experiment was used for the biosorption process, involving effect of experimental factors and biosorption kinetics and equilibrium. Biosorption process showed that the removal of Crystal Violet by CLB was effective over wide pH range, and meanwhile was independent on ionic strength. Biosorption capacities of CLB increased with the initial dye concentration increasing, due to an increase in the driving force of the concentration gradient. The adsorbed Crystal Violet amount per unit biomass weight decreased with increasing biosorbent dosage, due to the splitting effect of flux （concentration gradient） between sorbate and biosorbent. A maximum sorption capacity of 239.25 mg/g was observed. Biosorption kinetics was found to be best represented by the pseudo second-order kinetic model. The equilibrium adsorption data was well described by the Koble-Corrigan model. FT-IR （Fourier Transform Infrared Spetroscopy） spectrum showed the presence of O–H, COOH, C=O, C–N, C–H, –NH2 and P–OH in the surface of CLB as functional groups. This study showed CLB can effectively remove CV from dye wastewater.

关键词： biosorption Ceriporia lacerata P2 Crystal Violet equilibrium kinetics

Amorphous gallium oxide homojunction-based optoelectronic synapse for multi-functional signal processing

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半导体学报:英文版 2023年第7期44卷 60-68页

作者： Rongliang Li yonghui lin Yang Li Song Gao Wenjing Yue Hao Kan Chunwei Zhang Guozhen Shen School of Information Science and Engineering University of JinanJinan 250022China School of Microelectronics Shandong UniversityJinan 250101China School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing 100081China

In the era of accelerated development in artificial intelligence as well as explosive growth of information and data throughput,underlying hardware devices that can integrate perception and memory while simultaneously offering the bene-fits of low power consumption and high transmission rates are particularly valuable.Neuromorphic devices inspired by the human brain are considered to be one of the most promising successors to the efficient in-sensory process.In this paper,a homojunction-based multi-functional optoelectronic synapse(MFOS)is proposed and testified.It enables a series of basic electri-cal synaptic plasticity,including paired-pulse facilitation/depression(PPF/PPD)and long-term promotion/depression(LTP/LTD).In addition,the synaptic behaviors induced by electrical signals could be instead achieved through optical signals,where its sen-sitivity to optical frequency allows the MFOS to simulate high-pass filtering applications in situ and the perception capability integrated into memory endows it with the information acquisition and processing functions as a visual system.Meanwhile,the MFOS exhibits its performances of associative learning and logic gates following the illumination with two different wave-lengths.As a result,the proposed MFOS offers a solution for the realization of intelligent visual system and bionic electronic eye,and will provide more diverse application scenarios for future neuromorphic computing.

关键词： optoelectronic synapse gallium oxide filter visual system associative learning logic gate

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高炉原料硫含量与煤气硫含量相关性分析

工业安全与环保 2024年第3期50卷 88-91页

作者：易祥付本全林永辉林钰全武汉钢铁有限公司湖北武汉430080 武汉钢铁有限公司技术中心湖北武汉430086

对某钢铁高炉原料中的焦炭、喷吹煤、烧结矿硫含量进行了统计分析,同时分析了对应区间高炉煤气硫化氢、羰基硫含量,利用统计分析软件分析了高炉各原料中硫含量与高炉煤气中硫化氢、羰基硫的相关性,提出了要降低高炉煤气硫含量,需要适当... 详细信息

对某钢铁高炉原料中的焦炭、喷吹煤、烧结矿硫含量进行了统计分析,同时分析了对应区间高炉煤气硫化氢、羰基硫含量,利用统计分析软件分析了高炉各原料中硫含量与高炉煤气中硫化氢、羰基硫的相关性,提出了要降低高炉煤气硫含量,需要适当降低焦炭、烧结矿的硫含量,适当提高喷吹煤中硫含量。分析的结果对支撑高炉煤气硫含量源头减排提供了数据支撑。

关键词：高炉煤气源头减排二氧化硫数据统计硫含量

Exploring the impact of Nafion modifier on electrocatalytic CO_(2) reduction over Cu catalyst

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Journal of Energy Chemistry 2024年第1期88卷 543-551,I0012页

作者： Yingshi Su yonghui Cheng Zhen Li Yanjia Cui Caili Yang Ziyi Zhong Yibing Song Gongwei Wang lin Zhuang College of Chemistry&Chemical Engineering and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province Shantou UniversityShantou 515063GuangdongChina College of Chemistry and Molecular Sciences Hubei Key Lab of Electrochemical Power SourcesWuhan UniversityWuhan 430072HubeiChina The Institute for Advanced Studies Wuhan UniversityWuhan 430072HubeiChina Department of Chemistry Engineering Guangdong Technion-Israel Institute of Technology(GTIIT)Shantou 515063GuangdongChina Technion-Israel Institute of Technology(IIT) Haifa 32000Israel

Nafion as a universal polymer ionomer was widely applied for nanocatalysts electrode preparation.However,the effect of Nafion on electrocatalytic performance was often overlooked,especially for CO_(2)electrolysis.Herein,the key roles of Nafion for CO_(2)RR were systematically studied on Cu nanoparticles(NPs)electrocatalyst.We found that Nafion modifier not only inhibit hydrogen evolution reaction(HER)by decreasing the accessibility of H_(2)O from electrolyte to Cu NPs,and increase the CO_(2)concentration at electrocatalyst interface for enhancing the CO_(2)mass transfer process,but also activate CO_(2)molecule by Lewis acid-base interaction between Nafion and CO_(2)to accelerate the formation of^(*)CO,which favor of C–C coupling for boosting C_(2)product generation.Owing to these features,the HER selectivity was suppressed from 40.6%to 16.8%on optimal Cu@Nafion electrode at-1.2 V versus reversible hydrogen electrode(RHE),and as high as 73.5%faradaic efficiencies(FEs)of C_(2)products were achieved at the same applied potential,which was 2.6 times higher than that on bare Cu electrode(~28.3%).In addition,Nafion also contributed to the long-term stability by hinder Cu NPs morphology reconstruction.Thus,this work provides insights into the impact of Nafion on electrocatalytic CO_(2)RR performance.

关键词： Nafion modifier CO_(2)reduction Cu nanoparticles In situ ATR-SEIRAS C_(2)product

Degradation of tetracycline by immobilized laccase and the proposed transformation pathway

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Degradation of tetracycline by immobilized laccase and the p...

Applications of Cerrena laccase in biodegradation

全国农业生物化学与分子生物学第十五届学术研讨会

作者： Jie Yang Xinqi Xu yonghui lin Xiuyun Ye Juan lin Fujian Key Laboratory of Marine Enzyme Engineering Fuzhou University Technical Center Fujian Entry-Exit Inspection and Quarantine Bureau

Antibiotics are commonly used in human and veterinary medicine and have attracted increasing attention as emerging contaminants.Laceases are copper-containing oxidases that can oxidize a wide range of phenolic and non-phenolic compounds and have application potentials in wastewater treatment and bioremediation.Magnetic cross-linked enzyme aggregates(M-CLEAs)were prepared for

关键词： laccase tetracycline transformation products antimicrobial activity Methods

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Applications of Cerrena laccase in biodegradation