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Emerging natural clay-based materials for stable and dendrite-free lithium metal anodes: A review

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Chinese Chemical Letters 2025年第2期36卷 161-172页

作者： Haobo wang Fei wang yong Liu Zhongxiu Liu Yingjie miao Wanhong Zhang Guangxin wang Jiangtao Ji Qiaobao Zhang School of Materials Science and Engineering Provincial and Ministerial Co-construction of Collaborative Innovation Center for Non-ferrous Metal new Materials and Advanced Processing Technology Henan University of Science and Technology Faculty of Engineering Huanghe Science and Technology University Henan Key Laboratory of Non-Ferrous Materials Science & Processing Technology Henan University of Science and Technology College of Agricultural Equipment Engineering Henan University of Science and Technology State Key Laboratory of Physical Chemistry of Solid Surfaces College of Materials Xiamen University

Lithium metal is one of the most promising anodes for lithium batteries because of their high theoretical specific capacity and the low electrochemical potential. However, the commercialization of lithium metal anodes(LMAs) is facing significant obstacles, such as uncontrolled lithium dendrite growth and unstable solid electrolyte interface, leading to inferior Coulombic efficiency, unsatisfactory cycling stability and even serious safety issues. Introducing low-cost natural clay-based materials(NCBMs) in LMAs is deemed as one of the most effective methods to solve aforementioned issues. These NCBMs have received considerable attention for stabilizing LMAs due to their unique structure, large specific surface areas, abundant surface groups, high mechanical strength, excellent thermal stability, and environmental friendliness. Considering the rapidly growing research enthusiasm for this topic in the last several years, here, we review the recent progress on the application of NCBMs in stable and dendrite-free *** different structures and modification methods of natural clays are first summarized. In addition, the relationship between their modification methods and nano/microstructures, as well as their impact on the electrochemical properties of LMAs are systematically discussed. Finally, the current challenges and opportunities for application of NCBMs in stable LMAs are also proposed to facilitate their further development.

关键词： Aolid-state electrolyte Li metal anodes Natural clay-based materials Rechargeable batteries Surface modification

Correlation between the rock mass properties and maximum horizontal stress:A case study of overcoring stress measurements

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 39-48页

作者： Peng Li Meifeng Cai Shengjun miao Yuan Li Yu wang Key Laboratory of Ministry of Education for Efficient Mining and Safety of Metal Mines University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Coal Resources and Safe Mining China University of Mining and TechnologyXuzhou 221116China

Understanding the mechanical properties of the lithologies is crucial to accurately determine the horizontal stress *** investigate the correlation between the rock mass properties and maximum horizontal stress,the three-dimensional(3D)stress tensors at 89 measuring points determined using an improved overcoring technique in nine mines in China were adopted,a newly defined characteristic parameter C_(ERP)was proposed as an indicator for evaluating the structural properties of rock masses,and a fuzzy relation matrix was established using the information distribution *** results indicate that both the vertical stress and horizontal stress exhibit a good linear growth relationship with *** is no remarkable correlation between the elastic modulus,Poisson's ratio and depth,and the distribution of data points is scattered and ***,there is no obvious relationship between the rock quality designation(RQD)and *** maximum horizontal stress σ_(H) is a function of rock properties,showing a certain linear relationship with the C_(ERP)at the same *** addition,the overall change trend of σ_(H) determined by the established fuzzy identification method is to increase with the increase of C_(ERP).The fuzzy identification method also demonstrates a relatively detailed local relationship betweenσ_H and C_(ERP),and the predicted curve rises in a fluctuating way,which is in accord well with the measured stress data.

关键词： overcoring stress measurements elastic modulus Poisson's ratio rock quality designation maximum horizontal stress fuzzy identification

Biogenic emission as a potential source of atmospheric aromatic hydrocarbons:Insights from a cyanobacterial bloom-occurring eutrophic lake

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Journal of Environmental Sciences 2025年第5期151卷 497-504页

作者： Hua Fang Ting Wu Shutan Ma Yuqing miao Xinming wang School of Ecology and Environment Anhui Normal UniversityWuhu 241000China Center of Cooperative Innovation for Recovery and Reconstruction of Degraded Ecosystem in Wanjiang City Belt Wuhu 241000China School of Geography and Tourism Anhui Normal UniversityWuhu 241000China State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China CAS Center for Excellence in Deep Earth Science Guangzhou 510640China

As important precursors of ozone(O_(3))and secondary organic aerosol(SOA),reactive aromatic hydrocarbons(AHs)have typically been classified as anthropogenic air ***,biogenic emission can also be a potential source of atmospheric ***,field observations in a eutrophic lake were combined with laboratory incubation experiments to investigate the biogenic AH *** work showed that the water-air fluxes of AHs measured at sites with high cyanobacteria abundance could reach an order of magnitude greater than those at sites with low cyanobacteria abundance,suggesting that cyanobacteria could be the important contributor to measured *** incubation experiments further confirmed the AH emission of cyanobacteria and revealed that the emission could change significantly over the lifespan of cyanobacteria and varied to their growing *** combining field observations and laboratory incubation experiments,it has been suggested that the emission of different AH species from cyanobacteria could be modulated by variable biogeochemical mechanisms and that the biochemical process of toluene could be different from that of other *** study investigates AH emissions from inland aquatic ecosystem and suggests that biogenic emission could be a potential source of atmospheric AHs.

关键词： Aromatic hydrocarbons Biogenic emission Eutrophic lake Cyanobacteria Biosphere-atmosphere exchange

Structural design and controllable preparation of SiC NWs@Fe_(3)O_(4)@NC nanocomposites for electromagnetic wave absorption

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International Journal of Minerals,Metallurgy and Materials 2025年第3期32卷 520-533页

作者： Wenxin Zhao Meng Zhang Yukun miao Chang wang Anguo Cui Liying Yuan Zeqing miao Xiaoqing wang Zhibo wang Haoyu Pang Alan Meng Zhenjiang Li Ting wang College of Materials Science and Engineering Qingdao University of Science and TechnologyQingdao 266042China Shandong Engineering Laboratory for Preparation and Application of High-Performance Carbon-Materials College of Electromechanical EngineeringQingdao University of Science and TechnologyQingdao 266061China Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science MOEShandong Key Laboratory of Biochemical AnalysisCollege of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao 266042China College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042China

Using SiC nanowires(SiCNWs)as the substrate,reflux-annealing and electrodeposition-carbonization were sequentially applied to integrate SiC nanowires with magnetic Fe_(3)O_(4) nanoparticles and amorphous nitrogen-doped carbon(NC)for the fabrication of SiCNWs@Fe_(3)O_(4)@NC *** testing and characterization of this product provided valuable insights into the im-pact of structural and composition changes on its electromagnetic wave absorption *** optimized SiCNWs@Fe_(3)O_(4)@NC nanocomposite,which has 30wt%filler content and a corresponding thickness of 2.03 mm,demonstrates exceptional performance with the minimum reflection loss(RL_(min))of-53.69 dB at 11.04 GHz and effective absorption bandwidth(EAB)of 4.4 *** synergistic effects of the enhanced nanocomposite on electromagnetic wave absorption were thoroughly elucidated using the theories of multiple scattering,polarization relaxation,hysteresis loss,and eddy current ***,a multicomponent electromagnetic wave attenu-ation model was established,providing valuable insight into the design of novel absorbing materials and the enhancement of their absorp-tion *** research demonstrated the significant potential of the SiCNWs@Fe_(3)O_(4)@NC nanocomposite as a highly efficient electromagnetic wave-absorbing material with potential applications in various fields,such as stealth technology and microwave absorption.

关键词： electromagnetic attenuation mechanism multicomponent nanocomposite SiC nanowires structural design

Status analysis on sputtering and erosion evaluation methods of ion optic systems

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Chinese Journal of Aeronautics 2025年第1期38卷 254-270页

作者： Long miao Tongxun YANG Zhengxi ZHU Chang LU Zhiwen WU Ningfei wang School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Chongqing Innovation Center Beijing Institute of TechnologyChongqing 404100China Advanced Aerospace Power and Energy Research Center Beijing Institute of TechnologyZhuhai 519088China

In the past few decades,ion engines have been widely used in deep-space propulsion and satellite *** aim of extending the thruster lifetime is still one of the most important parts during the design stage of ion *** one of the core components of ion engine,the grid assembly of ion optic systems may experience long-term ion sputtering in extreme electro-thermal environments,which will eventually lead to its structural and electron-backstreaming *** this paper,the current studies of the grid assembly erosion process are systematically analyzed from the aspects of sputtering damage process of grid materials,numerical simulations,and measurements of erosion characteristics of grid *** advantages and disadvantages of various erosion prediction models are highlighted,and the key factors and processes affecting the prediction accuracy of grid assembly erosion patterns are *** different types of experimental methods of grid assembly erosion patterns are *** analysis in this paper is of great importance for selecting the sputter-resistant grid materials,as well as establishing the erosion models and measurement methods to accurately determine the erosion rate and failure modes of grid ***,the working conditions and structure parameters of ion optic systems could be optimized based on erosion models to promote the ion engine lifetime.

关键词： Electric propulsion Ion optic systems Sputtering yield Erosion characteristics Erosion pattern measurement Lifetime evaluation

Optimizing hardware-software co-design based on non-ideality in memristor crossbars for in-memory computing

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Science China(Information Sciences) 2025年第2期68卷 354-369页

作者： Pinfeng JIANG Danzhe SONG Menghua HUANG Fan YANG Letian wang Pan LIU Xiangshui miao Xingsheng wang School of Integrated Circuits Huazhong University of Science and Technology Hubei Yangtze Memory Labs

The memristor crossbar, with its exceptionally high storage density and parallelism, enables efficient vector matrix multiplication(VMM), significantly improving data throughput and computational efficiency. However, its analog computing is vulnerable to issues like IR-drop, device-to-device(D2D) variation, and stuck-at-fault(SAF), leading to a substantial decrease in the inference accuracy of neural networks deployed on crossbars. This work presents a hardware-software co-design approach tailored to deal with memristor crossbar non-ideality. We introduce an end-to-end functional array simulator(FAST) for precise and ultra fast end-to-end training, mapping, and evaluation of neural networks on the memristor crossbar. Utilizing the sparsity of the memristor crossbar coefficient matrix, it achieves simulation with low storage and computational resource requirements,dynamically selecting the optimal solution to complete the process. It can also precisely simulate the impact of non-ideal effects such as IR-drop, retention, variation, SAF, and AD/DA precision. Using FAST, we assess memristor crossbar matrix operations under non-ideal conditions, identifying the max throughput and the most energy-efficient crossbar configurations. Additionally,we propose a comparator-based activation function modulation(CAFM) scheme and its corresponding hardware architecture with programmable activation function circuits to address the IR-drop issue, enabling low power and area overheads, resulting in the recovery of neural network accuracy by 54% or more. This is validated within FAST, demonstrating the success of our hardware-software optimization co-design.

关键词： memristor crossbar IR-drop neural network activation function hardware-software co-design

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Was chicken domesticated in northern China?New evidence from mitochondrial genomes

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Science Bulletin 2018年第12期63卷 743-746页

作者： Xun-He Huang Ya-Jiang Wu yong-wang miao Min-Sheng Peng Xing Chen Dan-Lin He Chatmongkon Suwannapoom Bing-wang Du Xian-Yao Li Zhuo-Xian Weng Si-Hua Jin Jiao-Jiao Song Ming-Shan wang Jie-Bo Chen Wei-Na Li Newton Otieno Otecko Zhao-Yu Geng Xiang-yong Qu Yan-Ping Wu Xiu-Rong Yang Jie-Qiong Jin Jian-Lin Han Fu-Sheng Zhong Xi-Quan Zhang Ya-Ping Zhang School of Life Sciences.flaying University.Meizhou 514015.China State Key Laboratory for Conservation and Utilization of Bio-resources in Yunnan Yunnan UniversityKunming 650091China Faculty of Animal Science and Technology.Yunnan Agricultural University.Kunming 650201.China State Key Laboratory of Genetic Resources and Evolution and Yunnan Laboratory of Molecular Biology of Domestic Animals.kunming Institute of Zoology.Chinese Academy of Sciences.Kunming 650223.China College of Animal Sciences.South China Agricultural University.Guangzhou 510642.China School of Agriculture and Natural Resources.University of Phayao.Phayao 56000.Thailand College of Agriculture.Guangdong Ocean University.Zhanjiang 524088.China College of Animal Science and Technology.Shandong Agricultural University.Taian 271018.China College of Animal Science and Technology.Hunan Agricultural University.Changsha 410128.China College of Animal Science and Technology.Anhui Agricultural University.Hefei 230036.China Institute of Animal Science.Jiangxi Academy of Agricultural Sciences.Nanchang 330200.China College of Animal Science and Technology.Guangxi University.Nanning 530004.China Kunming College of Life Science.University of Chinese Academy of Sciences.Kunming 650204.China Southeast Asia Biodiversity Research Institute.Chinese Academy of Sciences(CAS-SEABRI).Yezin 05282.Myanmar CAAS-ILRI Joint Laboratory on Livestock and Forage Genetic Resources.Institute of Animal Science.Chinese Academy of Agricultural Sciences(CAAS).Beijing 100193.China International Livestock Research Institute(ILRI).Nairobi 00100.Kenya

The timing and location of chicken(Gallus gallus domesticus)domestication have remained controversial for over a century[1].Several researchers have proposed China as one of the early centers for chicken domestication[2].This is based on a few archaeological‘‘chicken"remains discovered in China(Table S1).Recently,one investigation detected mitochondrial DNA(mt DNA)haplotypes

关键词：鸡肉中国染色体驯养证据研究人员职业人员 DNA

Improve Strategy for Transient Power Angle Stability Control of VSG Combining Frequency Difference Feedback and Virtual Impedance

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Energy Engineering 2025年第2期122卷 651-666页

作者： Dianlang wang Qi Yin Haifeng wang Jing Chen Hong miao Yihan Chen Substation Management Office Qujing Bureau of CSG EHV Power Transmission CompanyQujing655000China College of Electrical Engineering SichuanUniversityChengdu610065China

As the penetration rate of distributed energy increases,the transient power angle stability problem of the virtual synchronous generator(VSG)has gradually become *** view of the situation that the grid impedance ratio(R/X)is high and affects the transient power angle stability of VSG,this paper proposes a VSG transient power angle stability control strategy based on the combination of frequency difference feedback and virtual *** improve the transient power angle stability of the VSG,a virtual impedance is adopted in the voltage loop to adjust the impedance ratio R/X;and the PI control feedback of the VSG frequency difference is introduced in the reactive powervoltage link of theVSGto enhance the damping ***-orderVSGdynamic nonlinearmodel considering the reactive power-voltage loop is established and the influence of different proportional integral(PI)control parameters on the system balance stability is ***,the impact of the impedance ratio R/X on the transient power angle stability is presented using the equal area *** the simulations,during the voltage dips with the reduction of R/X from 1.6 to 0.8,Δδ_(1)is reduced from 0.194 rad to 0.072 rad,Δf_(1)is reduced from 0.170 to 0.093 Hz,which shows better transient power angle *** results verify that compared with traditional VSG,the proposedmethod can effectively improve the transient power angle stability of the system.

关键词： Transient synchronous stability virtual synchronous generator impedance ratio

Constructing diverse switchable circularly polarized luminescence via a single azobenzene polymer film

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Chinese Chemical Letters 2025年第1期36卷 299-305页

作者： Xiang wang Qingping Song Zixiang He Gong Zhang Tengfei miao Xiaoxiao Cheng Wei Zhang State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials Department of Polymer Science and EngineeringCollege of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123China School of Chemical and Environmental Engineering Anhui Polytechnic UniversityWuhu 241000China Jiangsu Key Laboratory for Chemistry of Low-Dimensional Materials School of Chemistry and Chemical EngineeringHuaiyin Normal UniversityHuaian 223300China

Recently circularly polarized luminescence(CPL)materials have attracted significant *** reversible dynamic property to these materials has been a key focus in cutting-edge fields,such as in high-level information ***,we provided a novel and general strategy involving handednessselective filtration and ground-state chiral self-recovery(CSR)in double film system to address this *** on this strategy,we achieved CPL switch through the reversible modulation of ground-state chirality including absorption and scattering circular dichroism(CD)signals over the full UV-visible wavelength range(365-700 nm)in a single azobenzene polymer(PAzo)*** importantly,by flexibly changing the type of fluorescent films,it is convenient to achieve general excited-state CSR,that is reversible switching of full-color including ideal white(CIE coordinate(0.33,0.33)),as well as room-temperature phosphorescent *** these CPL signals without almost any intensity decay after three cycles of onand-off *** results indicated that the trans-cis isomerization and ordered rearrangement of azobenzene units in PAzo film were the fundamental reasons for realizing CPL ***,based on this system we achieved dynamic visual encryption and decryption process including multiple decryption *** study provides an effective method for constructing a universally applicable chiroptical switch in excited state.

关键词： Circularly polarized luminescence Azobenzene polymer Multiple CPL Chiral switch Information encryption