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Long-term operation optimization of circulating cooling water systems under fouling conditions

Chinese Journal of Chemical Engineering 2024年第1期65卷 255-267页

作者： Jiarui Liang yong Tian Shutong yang yong Wang Ruiqi Yin Yufei Wang School of Chemical Engineering and Environment China University of PetroleumBeijing102249China CHN Energy Xinjiang Chemical Co. LTDUrumqi830092China College of Mechanical and Transportation Engineering China University of PetroleumBeijing 102249China

Fouling caused by excess metal ions in hard water can negatively impact the performance of the circulating cooling water system(CCWS)by depositing ions on the heat exchanger's ***,the operation optimization of CCWS often prioritizes short-term flow velocity optimization for minimizing power consumption,without considering ***,low flow velocity promotes ***,it's crucial to balance fouling and energy/water conservation for optimal CCWS long-term *** study proposes a mixed-integer nonlinear programming(MINLP)model to achieve this *** model considers fouling in the pipeline,dynamic concentration cycle,and variable frequency drive to optimize the synergy between heat transfer,pressure drop,and *** optimizing the concentration cycle of the CCWS,water conservation and fouling control can be *** model can obtain the optimal operating parameters for different operation intervals,including the number of pumps,frequency,and valve local resistance *** experiments on cycle and environmental temperature reveal that as the cycle increases,the marginal benefits of energy/water conservation *** periods with minimal impact on fouling rate,energy/water conservation can be achieved by increasing the cycle while maintaining a low fouling ***,the proposed model has significant energy/water saving effects and can comprehensively optimize the CCWS through its incorporation of fouling and cycle optimization.

关键词： Computer simulation Circulating water system Fouling Concentration cycle Optimization Variable frequency drive

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Modeling analysis of cobalt-based Fischer-Tropsch catalyst particles

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Chinese Journal of Chemical Engineering 2024年第6期70卷 82-92页

作者： Huashuai Wu Gang Wang yong yang yongwang Li College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuan 030024China National Energy Research&Development Center for Coal to Liquid Fuels Synfuels China CompanyLimitedBeijing 101400China

The influences of particle size,shape,and catalyst distribution on the reactivity and hydrocarbon product selectivity of a cobalt-based catalyst for Fischer-Tropsch synthesis were investigated in the present work.A self-consistent kinetic model for Fischer-Tropsch reaction proposed here was found to correlate experimental data well and hence was used to describe the consumption rates of reactants and formation rates of hydrocarbon *** perturbed-chain statistical associating fluid theory equation of state was used to describe vapor-liquid equilibrium behavior associated with Fischer-Tropsch *** interaction between intraparticle diffusion and Fischer-Tropsch reaction was investigated in *** showed that in order to avoid the adverse influence of intraparticle diffusional limitations on catalyst reactivity and product selectivity,the use of small particles is *** eggshell spherical particles are shown to keep the original catalyst reactivity and enhance the selectivity of heavy hydrocarbon *** suitable layer thickness for a spherical particle with a diameter of 2 mm is nearly 0.15 *** the same outer diameter of 2 mm,the catalyst reactivity and heavy product selectivity of hollow cylindrical particles with a layer thickness of 0.25 mm are found to be larger than eggshell spherical *** the viewpoint of catalytic performance,hollow cylindrical particles are a better choice for industrial applications.

关键词： Fischer-Tropsch synthesis Kinetic modeling Vapor-liquid equilibria Numerical simulation Intraparticle diffusion Particle shapes

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Copper-coated Porous Polyimide as Ultralight and Safe Current Collectors for Advanced LIBs

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Chinese Journal of Polymer Science 2024年第4期42卷 521-531页

作者： Cun-Sheng Liu Jun-Qi Hu ting-ting Mao Song-Yi Liao Ru-Ming Feng Yi-Dong Liu yong-Gang Min School of Materials and Energy Guangdong University of TechnologyGuangzhou510006China College of Chemistry and Chemical Engineering Zhongkai University of Agriculture and EngineeringGuangzhou510225China Shanwei Branch of Advanced Energy Science and Technology Guangdong Laboratory Shanwei516600China

Metallic copper is widely used as current collector(CC) for graphite anode of lithium-ion batteries(LIBs) due to its high electrical conductivity and electrochemical stability. However, the large volume density of commercial copper foil(~8.9 g·cm^(-3)) limits the increase of energy density of battery. Here, copper-coated porous polyimide(Cu@PPI) was prepared by vacuum evaporation as collector for the graphite anode. The sandwich structure connects the copper metal on both sides of the collector with excellent electrical conductivity. Compared to commercial Cu foil, Cu@PPI has lighter mass(≤3.9 mg for disc of 12 mm diameter versus 9.9 mg of ~10 μm Cu foil) and lower volume density(≤3.3 g·cm^(-3)). In addition, the porous structure allows of better adhesion of reactive substances and electrochemical properties than pure Cu foils. It is estimated that the energy density of Cu@PPI should be much higher than that of Cu foil. This strategy should be applicable for other current collectors.

关键词： Copper-coated Vacuum evaporation Porous polyimide(PPI) Current collector(CC) LIBs

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Efficient Monolithic Perovskite/Silicon Tandem Photovoltaics

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Energy & Environmental Materials 2024年第3期7卷 272-285页

作者： yong Wang Yu Wang Feng Gao Deren yang State Key Laboratory of Silicon Materials and School of Materials Science and Engineering Zhejiang University ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang University Department of Physics Chemistry and Biology (IFM) Linkping University

Tunable bandgaps make halide perovskites promising candidates for developing tandem solar cells (TSCs),a strategy to break the radiative limit of 33.7%for single-junction solar *** perovskites with marketdominant crystalline silicon (c-Si) is particularly attractive; simple estimates based on the bandgap matching indicate that the efficiency limit in such tandem device is as high as 46%.However,state-of-the-art perovskite/c-Si TSCs only achieve an efficiency of～32.5%,implying significant challenges and also rich *** this review,we start with the operating mechanism and efficiency limit of TSCs,followed by systematical discussions on wide-bandgap perovskite front cells,interface selective contacts,and electrical interconnection layer,as well as photon management for highly efficient perovskite/c-Si *** highlight the challenges in this field and provide our understanding of future research directions toward highly efficient and stable large-scale wide-bandgap perovskite front cells for the commercialization of perovskite/c-Si TSCs.

关键词： 2-terminal electrical interconnection perovskite/silicon tandem photovoltaics photon management wide-bandgap perovskites

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On the Probability of Generating a Primitive Matrix

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Journal of Systems Science & Complexity 2024年第4期37卷 1755-1771页

作者： CHEN Jingwei FENG yong LIU yang WU Wenyuan Chongqing Key Laboratory of Automated Reasoning and Cognition Chongqing Institute of Green and Intelligent TechnologyChinese Academy of SciencesChongqing 400714China Chongqing College University of Chinese Academy of SciencesChongqing 400714China Key Laboratory of Advanced Manufacturing Technology of Ministry of Education Guizhou UniversityyGuiyang 550025China Information Science and Engineering Chongqing Jiaotong UniversityChongqing 400074China

Given a k×n integer primitive matrix A(i.e.,a matrix can be extended to an n×n unimodular matrix over the integers)with the maximal absolute value of entries‖A‖bounded by an integer λ from above,the authors study the probability that the m×n matrix extended from A by appending other m-k row vectors of dimension n with entries chosen randomly and independently from the uniform distribution over{0,1,…,λ-1}is still *** authors present a complete and rigorous proof of a lower bound on the probability,which is at least a constant for fixed m in the range[k+1,n-4].As an application,the authors prove that there exists a fast Las Vegas algorithm that completes a k×n primitive matrix A to an n×n unimodular matrix within expected O(n^(ω)log‖A‖)bit operations,where O is big-O but without log factors,ω is the exponent on the arithmetic operations of matrix multiplication.

关键词： Integer matrix matrix completion probabilistic algorithm unimodular matrix

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Quantum Tunneling Enhanced Hydrogen Desorption from Graphene Surface: Atomic versus Molecular Mechanism

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Chinese Physics Letters 2024年第8期41卷 58-68页

作者： yangwu Tong yong yang Science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China Key Lab of Photovoltaic and Energy Conservation Materials Institute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China

We study the desorption mechanism of hydrogen isotopes from graphene surface using first-principles calculations,with focus on the effects of quantum *** low temperatures,quantum tunneling plays a dominant role in the desorption process of both hydrogen monomers and *** the case of dimer desorption,two types of mechanisms,namely the traditional one-step desorption in the form of molecules(molecular mechanism),and the two-step desorption in the form of individual atoms(atomic mechanism),are studied and *** the ortho-dimers,the dominant desorption mechanism is found to switch from the molecular mechanism to the atomic mechanism above a critical temperature,which is∼300K and 200K for H and D,respectively.

关键词： desorption quantum mechanism

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Sequential bowel necrosis and large gastric ulcer in a patient with a ruptured femoral artery:A case report

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World Journal of Gastrointestinal Surgery 2024年第7期16卷 2337-2342页

作者： Peng Wang ting-Gang Wang An-yong Yu Department of Emergency The Affiliated Hospital of Zunyi Medical UniversityZunyi 563000Guizhou ProvinceChina

BACKGROUND Severe bleeding as a result of a major vascular injury is a potentially fatal event commonly observed in the emergency *** necrosis and gastric ulcers secondary to ischemia are rare due to their rich blood *** this case,we present the case of a patient who was treated successfully following rupture of his femoral artery resulting in bowel necrosis and an unusually large gastric *** SUMMARY A 28-year-old male patient sustained a knife stab wound to the right thigh,causing rupture of his femoral artery and leading to massive *** underwent cardiopulmonary resuscitation and received a large blood *** surgeries confirmed bowel necrosis,and jejunostomy was *** necrotic intestine was removed,the remaining intestine was anastomosed,and the right thigh was *** three surgeries,the patient's overall condition gradually improved,and the patient was discharged from the ***,one day after discharge,the patient was admitted again due to dizziness and melena,and a gastroduodenoscopy revealed a giant banded *** 2 weeks of treatment,the ulcer had decreased in size without *** months after the last surgery,enterostomy and reintroduction surgery were *** patient was fitted with a right lower limb prosthesis one year after *** 3 years of follow-up,the patient did not complain of *** Trauma department physicians need to be aware of the possible serious complications involving the abdomen of trauma patients with massive bleeding.

关键词： Bowel necrosis Gastric ulcer Trauma Femoral artery rupture Ischemia Case report

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Diagnose and treatment for Type D congenital esophageal atresia with tracheoesophageal fistula

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Pediatric Investigation 2024年第1期8卷 37-43页

作者： Dingding Wang yong Zhao Yanan Zhang Kaiyun Hua Yichao Gu Shuangshuang Li Junmin Liao Shen yang ting yang Jiawei Zhao Jinshi Huang Department of Neonatal Surgery Beijing Children’s HospitalCapital Medical UniversityNational Center for Children’s HealthBeijingChina

Importance:Type D esophageal atresia(EA)with tracheoesophageal fistula(TEF)is characterized by EA with both proximal and distal *** is a rare congenital anomaly with a very low ***:To investigate diagnostic and treatment strategies for this rare ***:We retrospectively reviewed the clinicopathological features of patients with EA/TEF treated at our institution between January 2007 and September ***:Among 386 patients with EA/TEF,14(3.6%)had type D EA/*** two patients were diagnosed with proximal TEF *** patients were diagnosed *** patients were missed for diagnosis during the initial surgery but was later confirmed by *** the neonatal period,seven patients underwent a one-stage repair of proximal and distal TEF via thoracoscopy or *** to missed diagnosis and other reasons,the other 7 patients underwent two-stage surgery for repair of the proximal TEF,including cervical incision and *** of the 14 patients experienced postoperative complications including anastomotic leakage,pneumothorax,esophageal stricture,and *** who underwent one-stage repair of distal and proximal TEF during the neonatal period showed a higher incidence of anastomotic leak(4/7).In contrast,only one of seven patients with two-stage repair of the proximal TEF developed an anastomotic ***:Type D EA/TEF is a rare condition,and proximal TEFs are easily *** may aim to diagnose and determine the correct surgical approach.A cervical approach may be more suitable for repairing the proximal TEF.

关键词： Diagnosis Therapy Tracheoesophageal fistula Type D congenital esophageal atresia

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Geochemistry, zircon U–Pb geochronology, and Hf isotopes of S-type granite in the Baoshan block, constraints on the age and evolution of the Proto-Tethys

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Acta Geochimica 2024年第1期43卷 40-58页

作者： Jianjun Zhang Chuanlong Mou Chendong Liu yong Zhang ting Chen Hualiang Li Institute of Geological Survey East China University of TechnologyNanchang 330013China School of Earth Sciences East China University of TechnologyNanchang 330013China Chengdu Geological Survey Center Chengdu 610081China School of Water Resources&Environmental Engineering East China University of TechnologyNanchang 330013China

Geochemistry, zircon U–Pb geochronology, and Hf isotope data for the Early Paleozoic granites in the Baoshan Block reveal the Early Paleozoic tectonic evolution of the Proto-Tethys. The samples are high-K, calcalkaline, strongly peraluminous rocks with A/CNK values of 1.37–1.46, are enriched in SiO2, K2O, and Rb, and are depleted in Nb, P, Ti, Eu, and heavy rare earth elements,which indicates the crystallization fractionation of the granitic magma. Zircon U–Pb dating indicates that they formed in ca. 480 Ma. The Nansa granites have εHf(t) values ranging from-16.04 to 4.36 with corresponding TC DMages of 2.10–0.81 Ga, which suggests the magmas derived from the partial melting of ancient metasedimentary with minor involvement of mantle-derived components. A synthesis of data for the Early Paleozoic igneous rocks in the Baoshan block and adjacent(Tengchong,Qiangtang, Sibumasu, Himalaya, etc.) blocks indicates that these blocks were all aligned along the proto-Tethyan margin of East Gondwana in the Early Paleozoic. The Early Paleozoic S-type granites from Nansa were generated in a high-temperature and low-pressure(HTLP) extensional tectonic setting, which resulted from Andean-type orogeny instead of the final assembly of Gondwana or crustal extension in a non-arc environment. In certain places, an expanding environment may exist in opposition to the tectonic backdrop of the lithosphere’s thickening and shortening, leading the crust to melt and decompress,mantle-derived materials to mix, and a small quantity of peraluminous granite to emerge.

关键词： Baoshan block Early Paleozoic Granite Geochemistry Zircon Geochronology Hf isotope

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Atmospheric chemistry of 2-nitrobenzaldehyde:Initiated by photo-excitation,OH-oxidation,and small TiO_(2) clusters adsorption catalysis

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Journal of Environmental Sciences 2024年第5期139卷 123-137页

作者： Feng-yang Bai Xiang-Huan Liu ting-ting Meng Zhou Yu Yi-Chen Wang Shuang Ni Zhen Zhao Institute of Catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034China

The fate of 2-nitrobenzaldehyde(2-NBA)is of interest in atmospheric chemistry as it is a semi-volatile organic compound with high *** study presents a quantum chemical study of the gas-phase reactions of 2-NBA photo-excitation and OH-oxidation in the absence and presence of small TiO_(2) *** further understand the unknown photolysis mechanism,the photo-reaction pathways of ground singlet state and the lying excited triplet state of 2-NBA were investigated including the initial and subsequent reactions of proton transfer,direct CO,NO_(2),and HCO elimination routes in the presence of O_(2) and ***,the OH-mediated degradation of 2-NBA proceeded via five H-extraction and six OH-addition channels by indirect mechanism,which follows a succession of reaction steps initiated by the formation of weakly stable intermediate *** H-extraction from the-CHO group was the dominant pathway with a negative activation energy of-1.22 kcal/*** calculated rate coefficients at 200–600 K were close to the experimental data in literature within 308-352 K,and the kinetic negative temperature independence was found in both experimental literature and computational ***,2-NBA was favored to be captured onto small TiO_(2) clusters via six adsorption configurations formed via various combination of three types of bonds of Ti…O,Ti…C,and O…H between the molecularly adsorbed 2-NBA and TiO_(2) *** indicted that the chemisorptions of aldehyde oxygen have largest *** results suggested adsorption conformations have a respectable impact on the catalysis *** study is significant for understanding the atmospheric chemistry of 2-nitrobenzaldehyde.

关键词： 2-nitrobenzaldehyde OH radical oxidation Rate coefficient Photolysis mechanism Adsorption catalysis

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