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Liquid metal in prohibiting polysulfides shuttling in metal sulfides anode for sodium-ion batteries

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Journal of Energy Chemistry 2024年第9期96卷 559-567页

作者： Xiaobo Zheng Xinwei Guan Xuan Cheng Xiaoning Li Yang Fu yitong Li Zhi Zheng Weikong Pang Xun Xu Peng Li Tianyi Ma Institute for Superconducting&Electronic Materials Australian Institute for Innovative MaterialsUniversity of WollongongWollongongNSW 2522Australia School of Science RMIT UniversityMelbourneVIC 3000Australia CSIRO Manufacturing ClaytonVIC 3168Australia

Metal sulfides are a class of promising anode materials for sodium-ion batteries(SIBs)owing to their high theoretical specific ***,the reactant products(polysulfides)could dissolve into electrolyte,shuttle across separator,and react with sodium anode,leading to severe capacity loss and safety ***,for the first time,gallium(Ga)-based liquid metal(LM)alloy is incorporated with MoS_(2)nanosheets to work as an anode in *** electron-rich,ultrahigh electrical conductivity,and self-healing properties of LM endow the heterostructured MoS_(2)-LM with highly improved conductivity and electrode ***,LM is demonstrated to have excellent capability for the adsorption of polysulfides(e.g.,Na_(2)S,Na_(2)S_(6),and S_(8))and subsequent catalytic conversion of Na_(2)***,the MoS_(2)-LM electrode exhibits superior ion diffusion kinetics and long cycling performance in SIBs and even in lithium/potassium-ion battery(LIB/PIB)systems,far better than those electrodes with conventional binders(polyvinylidene difluoride(PVDF)and sodium carboxymethyl cellulose(CMC)).This work provides a unique material design concept based on Ga-based liquid metal alloy for metal sulfide anodes in rechargeable battery systems and beyond.

关键词： GalnSn liquid metal alloy MoS_(2) Polysulfides shuttle effects Catalytic conversion Sodium-ion batteries

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电力用户低压采集成功率影响因素研究

农村电气化 2023年第5期 87-89页

作者：向奕同国网重庆市电力公司市北供电分公司重庆渝北401147

为了分析电力用户低压采集成功率的影响因素,将电力用户用电数据传输分为上行通道和下行通道2个方面,分析总结各项因素对通信信道的影响,判断导致采集终端和计量装置采集异常的因素,并提出提高采集成功率相关措施,为计量装置运行维护、... 详细信息

为了分析电力用户低压采集成功率的影响因素,将电力用户用电数据传输分为上行通道和下行通道2个方面,分析总结各项因素对通信信道的影响,判断导致采集终端和计量装置采集异常的因素,并提出提高采集成功率相关措施,为计量装置运行维护、电费准确回收、线损管控提供支撑。

关键词：电力用户终端采集成功率通信信道

Interplay between the atomic structures and superconductivity of two-monolayer Pb films

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Science China(Physics,Mechanics & Astronomy) 2024年第1期67卷 90-98页

作者： Kun Xie Ze Huang Pengju Li Yumin Xia Desheng Cai yitong Gu Yuzhou Liu Fangliang Cai Runxiao Zhang Haohao Shi Ping Cui Shengyong Qin International Center for Quantum Design of Functional Materials(ICQD) University of Science and Technology of ChinaHefei 230026China CAS Key Laboratory of Strongly Coupled Quantum Matter Physics Department of PhysicsUniversity of Science and Technology of ChinaHefei 230026China Hefei National Laboratory University of Science and Technology of ChinaHefei 230088China

Superconductors with reduced dimensionality have been widely explored for their exotic superconducting ***,at the two-dimensional limit,two-monolayer Pb films with two types of structures provide an ideal platform to unveil the underlying superconducting mechanism[Science 324,1314(2009)].Here,by combining scanning tunneling microscopy(STM)with the first-principle calculations,we successfully identify that these two types have different atomic lattice structures with varying stacking phases,which further enables us to calculate the phonon spectrum and electron phonon coupling strength of each *** theoretical calculations are in good agreement with tunneling spectroscopy measurements of the superconducting transition temperatures(T_(c)),which established a correlation between atomic structures and ***,it was observed that the higher T_(c)of these two types also possess higher out-of-plane upper critical magnetic fields(Hc2).These findings will provide important new insights into two-dimensional superconductivity at the atomic level.

关键词： 2 ML Pb films superconductivity atomic structure scanning tunneling microscopy first-principle calculations

强风沙尘环境下车顶复合绝缘子风压分布和形变特性研究

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高压电器 2019年第12期55卷 7-14页

作者：赵玉顺向奕同董冰冰杜斌向念文谷山强合肥工业大学电气与自动化工程学院国网重庆市电力公司江北供电分公司国网电力科学研究院武汉南瑞有限责任公司

高速列车在运行过程中,车顶硅橡胶复合绝缘子伞裙在长期强风沙尘环境下存在撕裂问题。为研究车顶绝缘子在强风沙尘条件下的撕裂原因,伞裙的受力和形变特性,采用流固耦合仿真的方法,计算车顶绝缘子表面的风压分布、探讨风速和来流角度对... 详细信息

高速列车在运行过程中,车顶硅橡胶复合绝缘子伞裙在长期强风沙尘环境下存在撕裂问题。为研究车顶绝缘子在强风沙尘条件下的撕裂原因,伞裙的受力和形变特性,采用流固耦合仿真的方法,计算车顶绝缘子表面的风压分布、探讨风速和来流角度对绝缘子受力和形变特性的影响。结果表明:伞裙上下表面的风压差,形成较大合力作用于伞裙,引起伞裙形变,伞裙表面的风压差越大,伞裙形变越大。伞裙根部会出现应力集中现象。在反复外加力的作用下,伞裙根部的材料寿命明显低于伞裙的其他部位。不同来流角度下,绝缘子伞裙边缘的形变量和伞裙根部的受力明显不同。随着风速从60 m/s到100 m/s的增加,伞裙边缘最大形变量从6.442 8 mm增大到18.561 mm,伞裙根部最大应力从0.180 56 MPa增大到0.496 98 MPa。同时伞裙的结构、直径和倾角显著影响绝缘子的抗风性能。该研究成果为车顶硅橡胶复合绝缘子结构设计与优化提供参考价值。

关键词：车顶复合绝缘子强风沙尘撕裂来流角度风压分布形变特性应力

White light emission in 0D halide perovskite[(CH_(3))_(3)S]_(2)SnCl_(6)·H_(2)O crystals through variation of doping ns^(2) ions

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Frontiers of Optoelectronics 2024年第1期17卷 57-66页

作者： yitong Lin Yu Zhong Yangpeng Lin Jiawei Lin Lei Pang Zhilong Zhang Yi Zhao Xiao‑Ying Huang Ke‑Zhao Du Fujian Provincial Key Laboratory of Advanced Materials Oriented Chemical Engineering Collage of Chemistry and Material ScienceFujian Normal UniversityFuzhou 350007China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Qinghai Environmental Monitoring Center Xining 810000China Strait Institute of Flexible Electronics(SIFE Future Technologies)Fujian Normal University and Strait Laboratory of Flexible Electronics(SLoFE)Fuzhou 350007China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China

With the rapid development of white LEDs,the research of new and efficient white light emitting materials has attracted increasing *** dimensional(0D)organic–inorganic hybrid metal halide perovskites with superior luminescent property are promising candidates for LED application,due to their abundant and tailorable ***,[(CH_(3))_(3)S]_(2)SnCl_(6)・H_(2)O is synthesized as a host for dopant ions Bi^(3+)and Sb^(3+).The Sb^(3+)doped,or Bi^(3+)/Sb^(3+)co-doped,[(CH_(3))3S]_(2)SnCl_(6)・H_(2)O has a tunable optical emission spectrum by means of varying dopant ratio and excitation *** a result,we can achieve single-phase materials suitable for emission ranging from cold white light to warm white *** intrinsic mechanism is examined in this work,to clarify the dopant effect on the optical *** high stability of title crystalline material,against water,oxygen and heat,makes it promising for further application.

关键词： 0D Metal halide White light Perovskite Ions doping Excitation dependent

SnS_(2)nanoparticles embedded in sulfurized polyacrylonitrile composite fibers for high-performance potassium-ion batteries

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Interdisciplinary Materials 2024年第1期3卷 150-159页

作者： Ruiling Li Lijuan Tong yitong Jiang Yaxin Wang Jing Long Xiaochuan Chen Junxiong Wu Xiaoyan Li Yuming Chen Engineering Research Center of Polymer Green Recycling of Ministry of Education Fujian Key Laboratory of Pollution Control&Resource ReuseCollege of Environmental and Resource Sciences and College of Carbon Neutral Modern IndustryFujian Normal UniversityFuzhouFujianChina

Potassium-ion batteries(PIBs)have garnered significant attention as a promising alternative to commercial lithium-ion batteries(LIBs)due to abundant and cost-efficient potassium ***,the large size of potassium ions and the resulting sluggish reaction kinetics present major obstacles to the widespread use of ***,we present a simple method to ingeniously encapsulate SnS_(2)nanoparticles within sulfurized polyacrylonitrile(SPAN)fibers(SnS_(2)@SPAN)for serving as a high-performance PIB *** large interlayer spacing of SnS_(2)provides a fast transport channel for potassium ions during charge–discharge cycles,while the one-dimensional SPAN skeleton offers massive binding sites and shortens the diffusion path for potassium ions,facilitating faster reaction ***,the excellent ductility of SPAN can effectively accommodate the large volume changes that occur in SnS_(2)upon potassium-ion insertion,thereby enhancing the cyclic stability of SnS_(2).Benefiting from the above advantages,the SnS_(2)@SPAN composites exhibit impressive cyclability over 500 cycles at 4 A g−1,with a capacity retention rate close to 100%.This study provides an effective approach for stabilizing high-capacity PIB anode materials with large volume variations.

关键词： electrospinning encapsulation potassium‐ion batteries sulfurized polyacrylonitrile tin disulfide

Surface repair of wide-bandgap perovskites for high-performance all-perovskite tandem solar cells

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Journal of Energy Chemistry 2024年第6期93卷 64-70,I0003页

作者： Xiaojing Lv Weisheng Li Jin Zhang Yujie Yang Xuefei Jia yitong Ji Qianqian Lin Wenchao Huang Tongle Bu Zhiwei Ren Canglang Yao Fuzhi Huang Yi-Bing Cheng Jinhui Tong State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina Key Lab of Artificial Micro-and Nano-Structures of Ministry of Education of China School of Physics and TechnologyWuhan UniversityWuhan 430072HubeiChina Department of Electrical and Electronic Engineering Photonics Research Institute(PRI)Research Institute for Intelligent Wearable Systems(iWEAR)The Hong Kong Polytechnic University999077Hong KongChina Laboratory of Advanced Materials Fudan UniversityShanghai 200438China Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory Foshan 528200GuangdongChina

Wide-bandgap(WBG)perovskite solar cells(PSCs)play a fundamental role in perovskite-based tandem solar ***,the efficiency of WBG PSCs is limited by significant open-circuit voltage losses,which are primarily caused by surface *** this study,we present a novel method for modifying surfaces using the multifunctional S-ethylisothiourea hydrobromide(SEBr),which can passivate both Pb^(-1)and FA^(-1)terminated surfaces,Moreover,the SEBr upshifted the Fermi level at the perovskite interface,thereby promoting carrier *** proposed method was effective for both 1.67 and 1.77 eV WBG PSCs,achieving power conversion efficiencies(PCEs)of 22.47%and 19.90%,respectively,with V_(OC)values of 1.28 and 1.33 V,along with improved film and device *** this advancement,we were able to fabricate monolithic all-perovskite tandem solar cells with a champion PCE of 27.10%,This research offers valuable insights for passivating the surface trap states of WBG perovskite through rational multifunctional molecular engineering.

关键词： Wide-bandgap perovskite Surface defect Multifunctional molecule All-perovskite tandem solar cells

Temporal-spatial Generation of Astrocytes in the Developing Diencephalon

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Neuroscience Bulletin 2024年第1期40卷 1-16页

作者： Wentong Hong Pifang Gong Xinjie Pan Zhonggan Ren yitong Liu Guibo Qi Jun-Liszt Li Wenzhi Sun Woo-Ping Ge Chun-Li Zhang Shumin Duan Song Qin Department of Anatomy Histology and EmbryologySchool of Basic Medical SciencesFudan UniversityShanghai 200032China Academy for Advanced Interdisciplinary Studies Peking UniversityBeijing 100871China Chinese Institute for Brain Research Beijing 102206China School of Basic Medical Sciences Capital Medical UniversityBeijing 100069China Department of Molecular Biology University of Texas Southwestern Medical CenterDallasTexas 75390-9148USA Department of Neurobiology Key Laboratory of Medical Neurobiology of Ministry of Health of ChinaZhejiang University School of MedicineHangzhou 310058China State Key Laboratory of Medical Neurobiology and MOE Frontiers Center for Brain Science Fudan UniversityShanghai 200032China

tAstrocytes are the largest glial population in the mammalian ***,we have a minimal understanding of astrocyte development,especially fate specification in different regions of the *** lineage tracing of the progenitors of the third ventricle(3V)wall via in-utero electroporation in the embryonic mouse brain,we show the fate specification and migration pattern of astrocytes derived from radial glia along the 3V ***,radial glia located in different regions along the 3V wall of the diencephalon produce distinct cell types:radial glia in the upper region produce astrocytes and those in the lower region produce neurons in the *** genetic fate mapping analysis,we reveal that the first population of astrocytes appears along the zona incerta in the *** occurs at an early time point in the dorsal region relative to that in the ventral region of the developing *** transcriptomic analysis of the region-specific 3V wall and lateral ventricle(LV)wall,we identified cohorts of differentially-expressed genes in the dorsal 3V wall compared to the ventral 3V wall and LV wall that may regulate astrogenesis in the dorsal ***,these results demonstrate that the generation of astrocytes shows a spatiotemporal pattern in the developing mouse diencephalon.

关键词： Radial glia Astrocyte specification Lineage tracing Diencephalon Third ventricle

基于顾客等待厌恶的可插队服务系统的定价策略研究

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系统工程理论与实践 2024年第7期44卷 2339-2351页

作者：张怡通徐秀丽燕山大学经济管理学院秦皇岛066004 燕山大学理学院秦皇岛066004

为限制顾客的插队行为,许多服务商考虑为顾客设置插队费用和入场费用,该措施能有效规范顾客的排队秩序,使得服务系统的运营机制高效有序.本文基于可插队排队系统,通过设置等待厌恶心理参数来反映普通顾客排队等待时的心理负效用,探讨策... 详细信息

为限制顾客的插队行为,许多服务商考虑为顾客设置插队费用和入场费用,该措施能有效规范顾客的排队秩序,使得服务系统的运营机制高效有序.本文基于可插队排队系统,通过设置等待厌恶心理参数来反映普通顾客排队等待时的心理负效用,探讨策略性消费者平均等待时间的纵向差异化和有限理性行为规律.数值实验表明并不是插队概率越高社会收益越大,合理的服务定价决策可以减少顾客的插队乱象从而实现社会利益最大化.厘清消费者的插队行为、服务商的定价策略和顾客插队行为下收益增量之间的交互作用机制,不仅为可插队排队系统的定价费用研究提供管理学启示,更重要的是帮助企业和社会消除消费者排队等待时产生的心理不公平感知,提高整体服务效率,确保社会经济可持续发展.

关键词：插队行为等待时间均衡行为等待厌恶定价策略