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Meteorological effects on sources and future projection of nitrogen deposition to lakes in China

Journal of Environmental Sciences 2025年第5期151卷 100-112页

作者： Cheng Shi Hao guo Xue qiao Jingsi Gao ying Chen Hongliang Zhang Department of Biological and Ecological Engineering Oregon State UniversityCorvallisOR 97331USA State Key Laboratory of Organic Geochemistry Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China Institute of New Energy and Low-carbon Technology Sichuan UniversityChengdu 610065China Engineering Technology Development Center of Urban Water Recycling Shenzhen PolytechnicShenzhen 518055China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention Department of Environmental Science and EngineeringFudan UniversityShanghai 200438China IRDR ICoE on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health Fudan UniversityShanghai 200438China

Lake ecosystems are extremely sensitive to nitrogen growth,which leads to water quality degradation and ecosystem health *** depositions,as one of the main sources of nitrogen in water,are expected to change under future climate change ***,it remains not clear how nitrogen deposition to lakes respond to future meteorological *** this study,a source-oriented version of Community Multiscale Air Quality(CMAQ)Model was used to estimate nitrogen deposition to 263 lakes in 2013 and under three RCP scenarios(4.5,6.0 and 8.5)in *** total deposition of 58.2 Gg nitrogen was predicted for all lakes,with 23.3 Gg N by wet deposition and 34.9 Gg N by dry *** and ammonium in aerosol phase are the major forms of wet deposition,while NH3 and HNO_(3)in gas phase are the major forms of dry *** emissions contribute to 57%of wet deposition and 44%of dry *** future meteorological conditions,wet deposition is predicted to increase by 5.5%to 16.4%,while dry deposition would decrease by 0.3%to 13.0%.Changes in wind speed,temperature,relative humidity(RH),and precipitation rates are correlated with dry and wet deposition *** predicted changes in deposition to lakes driven by meteorological changes can lead to significant changes in aquatic chemistry and ecosystem *** from future emission scenarios,different climate scenarios should be considered in future ecosystem health evaluation in response to nitrogen deposition.

关键词： Deposition Nitrogen Lakes CMAQ Meteorological variations

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基于伪逆算法的冷镦坯模具的优化(英文)

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中国有色金属学会会刊：英文版 2012年第S2期22卷 207-213页

作者： Ali HALOUANI Yu-ming LI ABBES Boussad ying-qiao guo GRESPI/MPSE Université de Reims Champagne-Ardenne Moulin de la Housse

基于对最终产品形状的认识,提出一种新的快速的针对多工步轴对称冷锻建模方法—"伪逆法(PIA)"。为了考虑变形路径,引入了一些中间构型并且采用自由表面对这些中间构形进行修正而不采用接触算法。利用等效应力的概念和拉伸曲线,提出了一... 详细信息

基于对最终产品形状的认识,提出一种新的快速的针对多工步轴对称冷锻建模方法—"伪逆法(PIA)"。为了考虑变形路径,引入了一些中间构型并且采用自由表面对这些中间构形进行修正而不采用接触算法。利用等效应力的概念和拉伸曲线,提出了一种新的快速而健壮的塑性积分直接算法。数值试验表明:与增量法相比,伪逆法速度非常快。PIA被用于多工步冷锻工艺预制体模具优化设计过程中,该优化过程以最大限度减少在锻造过程中产生的等效塑性应变和需要的冲压力为目标,预制体模具的形状采用B样条曲线描述,以B样条曲线控制点的纵坐标为设计变量。目标函数的演变表明了模具形状优化对锻造件的质量和节能的重要性。通过与传统增量法的结果相比较,体现出了PIA的高效性和准确性。

关键词：冷锻伪逆算法预制坯设计 B样条形状优化 Pareto前沿

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Sky location of massive black hole binaries in the foreground of Galactic white dwarf binaries

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Science China(Physics,Mechanics & Astronomy) 2025年第1期68卷 93-104页

作者： Pan guo Hong-Bo Jin Cong-Feng qiao Yue-Liang Wu The International Centre for Theoretical Physics Asia-Pacific University of Chinese Academy of SciencesBeijing 100190China Institute for Frontiers in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China The School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China

For space-based gravitational wave(GW)detection,the main noise source for massive black hole binaries(MBHBs)is attributed to approximately 107 double white dwarf binaries in the *** a GW source,the amplitude of the detector response,recorded by a space-based gravitational wave detector,exhibits a modulation effect with a year period when observing the source from various orbital *** the adverse conditions mentioned above,where there is a strong foreground noise and annual modulation in the signals,we employed the wavelet transform and the strong-amplitude relevant orbital position search methods,which allows the weak MBHB sources to achieve higher locating *** detail,for two MBHB sources of lower intensity,the precision of luminosity distance,represented by the ratioΔD_(L)/D_(L) at the 95%confidence level,is enhanced by factors of∼*** angular resolutions,denoted byΔΩs,are enhanced by a factor of∼*** improvements increase the number of detectable GW sources,facilitate multi-messenger follow-up observations and provide constraints on the cosmological constant.

关键词： space-based gravitational wave detection gravitational waves massive black hole binaries

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Atomically Precise Cu Nanoclusters:Recent Advances,Challenges,and Perspectives in Synthesis and Catalytic Applications

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Nano-Micro Letters 2025年第4期17卷 130-165页

作者： Mengyao Chen Chengyu guo Lubing Qin Lei Wang Liang qiao Kebin Chi Zhenghua Tang New Energy Research Institute School of Environment and EnergySouth China University of TechnologyGuangzhou Higher Education Mega CentreGuangzhou 510006People’s Republic of China Petrochemical Research Institute PetroChina Company LimitedBeijing 102206People’s Republic of China Key Laboratory of Functional Inorganic Material Chemistry(Heilongjiang University) Ministry of EducationHarbin 150001People’s Republic of China

Atomically precise metal nanoclusters are an emerging type of nanomaterial which has diverse interfacial metal-ligand coordination motifs that can significantly affect their physicochemical properties and *** that,Cu nanoclusters have been gaining continuous increasing research attentions,thanks to the low cost,diversified structures,and superior catalytic performance for various *** this review,we first summarize the recent progress regarding the synthetic methods of atomically precise Cu nanoclusters and the coordination modes between Cu and several typical ligands and then discuss the catalytic applications of these Cu nanoclusters with some explicit examples to explain the atomical-level structure-performance ***,the current challenges and future research perspectives with some critical thoughts are *** hope this review can not only provide a whole picture of the current advances regarding the synthesis and catalytic applications of atomically precise Cu nanoclusters,but also points out some future research visions in this rapidly booming field.

关键词： Atomically precise Cu nanoclusters Controllable synthesis Catalytic applications Structure-performance relationship Challenges and perspectives

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Structural engineering of high-entropy alloys for advanced electrocatalytic reactions

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Tungsten 2025年第1期7卷 1-31页

作者： qiao Xie ying-Jie Yu Hai-Jun Zhang Ya-Ping Deng Wen Lei The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and Technology Department of Chemical Engineering Waterloo Institute for Sustainable Energy Waterloo Institute for Nanotechnology University of Waterloo

High-entropy alloys(HEAs) have emerged as promising candidates to replace traditional precious metal catalysts,owing to their unique chemical and physical *** review commences by revisiting the fundamental concepts of HEAs,including their synthesis methods and structural control strategies in *** underscores the critical role of meticulously manipulating both macroscopic and microscopic structures of the HEAs to optimize their catalytic performance.A deep understanding of the structure-activity relationship in HEAs across various configurations is pivotal in developing more effective *** review methodically encapsulates the research progress of structural control strategies for HEAs in achieving efficient energy conversion,with the aim of gaining a better understanding of the relationship between structure and *** review concludes by summarizing the current achievements and challenges,and suggestions for potential future directions of HEAs in the fields of energy conversion and environmental purification.

关键词： Electrocatalytic Energy conversion High-entropy alloys Structural modulation

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Understanding amorphous PrO_(x)-based N-doped carbon catalyst as an efficient electrocatalyst for oxygen reduction reaction

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Journal of Rare Earths 2025年第1期43卷 73-80,I0003页

作者： Xiao Man ying Chang Shaohong guo Meilin Jia Jingchun Jia Inner Mongolia Key Laboratory of Green Catalysis and Inner Mongolia Collaborative Innovation Center for Water Environment Safety College of Chemistry and Environmental ScienceInner Mongolia Normal UniversityHohhot010022China

The development of an e fficacious and easily prepared no nprecious metal electrocatalyst is crucial for the oxygen reduction reaction(ORR).This work used a dual template method to prepare the amorphous rare earth-based catalyst PrO_(x)-NC,and optimized the calcination temperature and *** PrO_(x)-NC-900 catalyst has high durability and activity and exhibits superior ORR performance in alkaline electrolytes with an onset potential(E_(0))of 0.96 V and a half-wave potential(E_(1/2))of 0.85 *** research results indicate that the ORR performance of rare earth oxide composite carbon catalysts can be improved by adjusting oxygen vacancies(Ov).In addition,high specific surface area,N rich defect *** oxygen vacancies,and the synergistic effect of oxygen vacancies and N-doped carbon interfacial layer play a significant part in the enhancement of *** performance of the zinc air battery assembled with PrO_(x)-NC-900 is significantly improved,and rare earth oxides and carbon frameworks originating from metal organic frameworks(MOFs)contribute to the oxygen electrocatalyst and electron transfer rate of the zinc air *** catalyst provides promising information for the development of rare earth metal oxide nanostructures as potential candidate materials for ORR in alkaline media.

关键词： Rare earths Metal-organic framework Oxygen reduction reaction Zn-air batteries

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Modeling of Spring Phenology of Boreal Forest by Coupling Machine Learning and Diurnal Temperature Indicators

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Chinese Geographical Science 2025年第1期35卷 38-54页

作者： DENG guorong ZHANG Hongyan HONG ying guo Xiaoyi YI Zhihua EHSAN BINIYAZ School of Hydraulic Engineering Nanchang Institute of TechnologyNanchang 330099China Key Laboratory of Geographical Processes and Ecological Security in Changbai Mountains Ministry of EducationSchool of Geographical SciencesNortheast Normal UniversityChangchun 130024China Urban Remote Sensing Application Innovation Center School of Geographical SciencesNortheast Normal UniversityChangchun 130024China School of Geographical Sciences Inner Mongolia Normal UniversityHohhot 010022China Landscape Ecology and Geoinformation Science Department of GeographyKiel UniversityKiel 24118Germany

The roles of diurnal temperature in providing heat accumulation and chilling requirements for vegetation spring phenology *** previous studies have established a stronger correlation between leaf onset and diurnal temperature than between leaf onset and average temperature,current research on modeling spring phenology based on diurnal temperature indicators remains *** this study,we confirmed the start of the growing season(SOS)sensitivity to diurnal temperature and average temperature in boreal *** estimation of SOS was carried out by employing K-Nearest Neighbor Regression(KNR-TDN)model,Random Forest Regres-sion(RFR-TDN)model,eXtreme Gradient Boosting(XGB-TDN)model and Light Gradient Boosting Machine model(LightGBM-TDN)driven by diurnal temperature indicators during 1982-2015,and the SOS was projected from 2015 to 2100 based on the Coupled Model Intercomparison Project Phase 6(CMIP6)climate scenario *** sensitivity of boreal forest SOS to daytime temperature is greater than that to average temperature and nighttime *** LightGBM-TDN model perform best across all vegetation types,exhibiting the lowest RMSE and bias compared to the KNR-TDN model,RFR-TDN model and XGB-TDN *** incorporating diurn-al temperature indicators instead of relying only on average temperature indicators to simulate spring phenology,an improvement in the accuracy of the model is ***,the preseason accumulated daytime temperature,daytime temperature and snow cover end date emerged as significant drivers of the SOS simulation in the study *** simulation results based on LightGBM-TDN model exhibit a trend of advancing SOS followed by stabilization under future climate *** study underscores the potential of diurn-al temperature indicators as a viable alternative to average temperature indicators in driving spring phenology models,offering a prom-ising new method for simulating spring phenology.

关键词： spring phenology diurnal temperature machine learning future climate scenarios boreal forest

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B2-CuZr reinforced amorphous alloy matrix composites:A review

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China Foundry 2025年第1期22卷 1-11页

作者： Wei guo Run-hua Huang Zhen Zhang Mi Zhao Jin-cheng Wang Yan-qiang qiao Shu-lin Lü Shu-sen Wu State Key Lab of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China School of Aerospace Engineering Huazhong University of Science and TechnologyWuhan 430074China Research Institute of Huazhong University of Science and Technology in Shenzhen Shenzhen 518057GuangdongChina

B2-CuZr phase reinforced amorphous alloy matrix composites has become one of the research hotspots in the field of materials science due to the“transformation-induced plasticity”phenomenon,which makes the composites show better macroscopic plastic deformability and obvious work-hardening behavior compared to the conventional amorphous alloy matrix composites reinforced with ductile ***,the in-situ metastable B2-CuZr phase tends to undergo eutectoid decomposition during solidification,and the volume fraction,size,and distribution of B2-CuZr phase are difficult to control,which limits the development and application of these *** date,much efforts have been made to solve the above problems through composition optimization,casting parameter tailoring,and post-processing *** this study,a review was given based on relevant studies,focusing on the predictive approach,reinforcing mechanism,and microstructure tailoring methods of B2-CuZr phase reinforced amorphous alloy matrix *** research focus and future prospects were also given for the future development of the present composite system.

关键词： amorphous alloy matrix composite B2-CuZr phase plasticity microstructure tailoring

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Plasmonic tandem heterojunctions enable high-efficiency charge transfer for broad spectrum photocatalytic hydrogen production

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Journal of Energy Chemistry 2025年第1期100卷 710-720页

作者： Wenxuan Chen Xiu-Qing qiao guo Hui Bojing Sun Dongfang Hou Meidi Wang Xueqian Wu Tao Wu Dong-Sheng Li College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion MaterialsChina Three Gorges UniversityYichang 443002HubeiChina Hubei Three Gorges Laboratory Yichang 443007HubeiChina College of Chemistry and Materials Science and Guangdong Provincial Key Laboratory of Supramolecular Coordination ChemistryJinan UniversityGuangzhou 510632GuangdongChina

Rational engineering of semiconductor photocatalysts for efficient hydrogen production is of great significance but still challenging,primarily due to the limitations in charge transfer ***,a fascinating plasmonic tandem heterojunction with the hc-CdS/Mo_(2)C@C heterostructure is aimfully prepared for effectively promoting the charge separation kinetics of the CdS photocatalyst via the synergistic strategy of phase junction,Schottky junction,and photothermal *** difference in atomic configuration between cubic-CdS (c-CdS) and hexagonal-CdS (h-CdS) leads to effective charge separation through a typical Ⅱ charge transfer mechanism,and plasmonic Schottky junction further extracts the electrons in the hc-CdS phase junction to realize gradient charge ***,the photothermal effect of Mo_(2)C@C helps to expand the light absorption,accelerate charge transfer kinetics,and reduce the hydrogen evolution energy *** carbon layer provides a fast channel for charge transfer and protects the photocatalyst from *** a result,the optimized hc-CMC photocatalyst exhibits a significantly high photocatalytic H_(2)production activity of 28.63 mmol/g/h and apparent quantum efficiency of 61.8%,surpassing most of the reported *** study provides a feasible strategy to enhance the charge transfer kinetics and photocatalytic activity of CdS by constructing plasmonic tandem heterogeneous junctions.

关键词： Heterojunctions Mo_(2)C LSPR Photocatalyst Phase junction Schottkyjunction Photothermal effect

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Estimation of rice phenology date using integrated HJ-1 CCD and Landsat-8 OLI vegetation indices time-series images

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2015年第10期16卷 832-844页

作者： Jing WANG Jing-feng HUANG Xiu-zhen WANG Meng-ting JIN Zhen ZHOU qiao-ying guo Zhe-wen ZHAO Wei-jiao HUANG Yao ZHANG Xiao-dong SONG Institute of Remote Sensing and Information Application College of Environmental and Resource Sciences Zhejiang University Institute of Remote Sensing and Earth Sciences Hangzhou Normal University

Accurate estimation of rice phenology is of critical importance for agricultural practices and studies. However, the accuracy of phenological parameters extracted by remote sensing data cannot be guaranteed because of the influence of climate, e.g. the monsoon season, and limited available remote sensing data. In this study, we integrate the data of H J-1 CCD and Landsat-8 operational land imager （OLI） by using the ordinary least-squares （OLS） and construct higher temporal resolution vegetation indices （VIs） time-series data to extract the phenological param- eters of single-cropped rice. Two widely used VIs, namely the normalized difference vegetation index （NDVI） and 2-band enhanced vegetation index （EVI2）, were adopted to minimize the influence of environmental factors and the intrinsic difference between the two sensors. Savitzky-Golay （S-G） filters were applied to construct continuous VI profiles per pixel. The results showed that, compared with NDVI, EVI2 was more stable and comparable between the two sensors. Compared with the observed phenological data of the single-cropped rice, the integrated VI time-series had a relatively low root mean square error （RMSE）, and EVI2 showed higher accuracy compared with NDVI. We also demonstrate the application of phenology extraction of the single-cropped rice in a spatial scale in the study area. While the work is of general value, it can also be extrapolated to other regions where qualified remote sensing data are the bottleneck but where complementary data are occasionally available.

关键词： Phenological parameters Intercalibration Vegetation index H J-1 CCD Landsat-80LI

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