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Advances of high-performance LiNi_(1-x-y)Co_(x)M_(y)O_(2) cathode materials and their precursor particles via co-precipitation process

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Particuology 2024年第3期86卷 67-85页

作者： Wenbiao Liang yin Zhao Liyi Shi Zhuyi Wang Yi Wang Meihong Zhang shuai Yuan School of Materials Science and Engineering Shanghai UniversityShanghai200444China Research Center of Nanoscience and Nanotechnology Shanghai UniversityShanghai200444China Emerging Industries Institute Shanghai UniversityJiaxingZhejiang314006China

Layered LiNi_(1-x-y)Co_(x)M_(y)O_(2)(M=Mn or Al)is a promising cathode material for lithium-ion batteries due to its high specific capacity and acceptable manufacturing ***,the polycrystalline LiNi_(1-x-y)Co_(x)M_(y)O_(2) cathode material suffers from disordered orientation of primary particles and poor geometric symmetry of secondary particles,which severely hampers the migration of Lit ***,the resulting anisotropy accelerates the disintegration of the secondary particle structure,significantly affecting the electrochemical performance of the polycrystalline *** spite of less grain boundary,the single-crystal LiNi_(1-x-y)Co_(x)M_(y)O_(2) cathodes still suffer from severe microcracks generated by repeated planar gliding during cycling,which poses a great challenge to the cycling stability of single-crystal ***'s worth noting that the microstructure of the cathode material is mainly inherited from its ***,it is necessary to deeply understand the influence of the microstructure of Ni_(1-x-y)Co_(x)M_(y)(OH)2 on the electrochemical properties of LiNi_(1-x-y)Co_(x)M_(y)O_(2) cathode materials,so as to optimize the production process of preparing high-performance cathode *** this review,we summarize recent advances in the research and development of Ni-rich cathode precursor ***,the challenges faced by the Ni-rich hydroxide precursor materials are presented,including the effect of primary particle morphology and arrangement on the electrochemical performance of cathode materials,the influence of secondary particle morphology on lithium insertion reactions in cathode,and the effect of particle size on the microcracking of single-crystal ***,the presentation of the conventional co-precipitation reactor,the mechanism of precursor particle growth,and the influence of coprecipitation parameters are described in ***,the strategies are systematically discussed to solve the cha

关键词： Lithium-ion batteries Cathode materials Co-precipitation Ni-rich layered oxides Single crystal Precursor particles

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Non-bonding modulations between single atomic cerium and monodispersed selenium sites towards efficient oxygen reduction

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Nano Research 2024年第6期17卷 4753-4763页

作者： Leilei yin shuai Zhang Mingzi Sun Siyuan Wang Bolong Huang Yaping Du Tianjin Key Lab for Rare Earth Materials and Applications Center for Rare Earth and Inorganic Functional MaterialsHaihe Laboratory of Sustainable Chemical TransformationsSmart Sensing Interdisciplinary Science CenterSchool of Materials Science and EngineeringNational Institute for Advanced MaterialsNankai UniversityTianjin 300350China Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHung HomKowloon 999077Hong KongChina Research Centre for Carbon-Strategic Catalysis The Hong Kong Polytechnic UniversityHung HomKowloon 999077Hong KongChina

Currently,dual atomic catalysts(DACs)with neighboring active sites for oxygen reduction reaction(ORR)still meet lots of challenges in the synthesis,especially the construction of atomic pairs of elements from different blocks of the periodic ***,a“rare earth(Ce)-metalloid(Se)”non-bonding heteronuclear diatomic electrocatalyst has been constructed for ORR by rational coordination and carbon support defect ***,the optimized Ce-Se diatomic catalysts(Ce-Se DAs/NC)displayed a half-wave potential of 0.886 V *** hydrogen electrode(RHE)and excellent stability,which surpass those of separate Ce or Se single atoms and most single/dual atomic catalysts ever *** addition,a primary zinc-air battery constructed using Ce-Se DAs/NC delivers a higher peak power density(209.2 mW·cm^(−2))and specific capacity(786.4 mAh·gZn^(−1))than state-of-the-art noble metal catalysts Pt/*** calculations reveal that the Ce-Se DAs/NC has improved the electroactivity of the Ce-N_(4)region due to the electron transfer towards the nearby Se specific activity(SA)***,the more electron-rich Se sites promote the adsorptions of key intermediates,which results in the optimal performances of ORR on Ce-Se DAs/*** work provides new perspectives on electronic structure modulations via non-bonded long-range coordination micro-environment engineering in DACs for efficient electrocatalysis.

关键词： catalyst rare earth oxygen reduction reaction(ORR) metalloid non-bonding modulation

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Highly coordinated Pd overlayers on nanoporous gold for efficient formic acid electro-oxidation

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Nano Research 2021年第10期14卷 3502-3508页

作者： Qinqin Sang shuai yin Feng Liu Huiming yin Jia He Yi Ding Tianjin Key Laboratory of Advanced Functional Porous Materials Institute for New Energy Materials&Low-Carbon TechnologiesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Kunming Institute of Precious Metals Kunming 650106China

Design and fabrication of highly efficient and stable electrocatalysts remain key challenges in green energy technologies such as low-temperature direct liquid fuel *** on in-depth theoretical calculations,here we demonstrate that surface Pd atoms with high coordination numbers(HCNs)can effectively modulate their adsorption energies for CO and OH,and thus achieve very high performance for formic acid electro-oxidation reaction(FAOR).Based on epitaxial coating Pd atomic layers onto nanoporous gold(NPG)thin membranes and a slight further decoration of Au clusters on top,the resulted core-shell structured NPG-Pd-Au electrocatalyst can demonstrate Pd intrinsic and mass activities of 8.62 mA·cm^(-2)and 27.25 A·mg^(-1)respectively at the peak potential around 0.33 V versus saturated calomel electrode toward FAOR,which are far better than those of commercial Pd/C catalysts(1.09 mA·cm^(-2)and 0.32 A·mg^(-1))tested under the same ***,the membrane electrode assemblies based on these low precious metal loading electrodes can achieve an anode Pd power efficiency over 10 W·mg^(-1)in a direct formic acid fuel cell,which is two orders of magnitude higher than that of the commercial Pd/*** results provide new inspirations for the development of revolutionary electrodes for energy technologies in a rational manner.

关键词： Pd nanoporous gold high coordination number formic acid oxidation direct formic acid fuel cell

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超高层建筑安全风险监管分析平台应用现状与问题分析

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建筑技术 2024年第8期55卷 989-993页

作者：丁天一殷帅曹勇于晓龙纪博雅毛晓峰中国建筑科学研究院有限公司建筑环境与能源研究院北京100013 住房和城乡建设部科技与产业化发展中心北京100835

为了尽可能地避免超高层建筑风险的发生,结合信息化、智能化手段的监管分析平台应运而生。调研了目前各类超高层建筑安全风险监管分析平台的应用情况,分析了现有技术和存在的问题,总结了平台技术未来的发展趋势,为该技术平台的发展与应... 详细信息

为了尽可能地避免超高层建筑风险的发生,结合信息化、智能化手段的监管分析平台应运而生。调研了目前各类超高层建筑安全风险监管分析平台的应用情况,分析了现有技术和存在的问题,总结了平台技术未来的发展趋势,为该技术平台的发展与应用提供了一定的参考。

关键词：超高层建筑智能监管平台结构健康监测消防安全监管风险评估

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Research Progress on Economic Forest Water Stress Based on Bibliometrics and Knowledge Graph

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Phyton-International Journal of Experimental Botany 2024年第5期93卷 843-858页

作者： Xin yin shuai Wang Chunguang Wang Haichao Wang Zheying Zong Zeyu Ban College of Mechanical and Electrical Engineering Inner Mongolia Agricultural UniversityHohhot010018China College of Energy and Traffic Engineering Inner Mongolia Agricultural UniversityHohhot010018China Key Laboratory of Biopesticide Creation and Resource Utilization of Universities Inner Mongolia Agricultural UniversityHohhotChina

This study employed the bibliometric software CiteSpace 6.1.R6 to analyze the correlation between thermal infrared,spectral remote sensing technology,and the estimation of economic forest water *** aimed to review the development and current status of this field,as well as to identify future research trends.A search was conducted on the China National Knowledge Infrastructure(CNKI)database using the keyword“water stress”for relevant studies from 2003 to *** visual analysis function of CNKI was used to generate the distribution of annual publication volume,and CiteSpace 6.1.R6 was utilized to create network maps illustrating collaboration among authors and *** study also analyzed the hotspots and frontiers of economic forest water *** a result,a total of 6664 academic journal articles related to water stress were *** collaboration networks were observed among scholars and institutions,with a focus on using crown temperature monitoring to diagnose crop water *** on the research findings,it was evident that the primary research trend involved the use of thermal infrared and spectral remote sensing technology for estimating water stress,making it a future research hotspot.

关键词： Water stress thermal infrared spectral visual analysis knowledge map CiteSpace

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Ultrathin nanoporous metal electrodes facilitate high proton conduction for low-Pt PEMFCs

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Nano Research 2021年第8期14卷 2681-2688页

作者： shuai Shi Xianglong Wen Qinqin Sang shuai yin Kaili Wang Jian Zhang Min Hu Huiming yin Jia He Yi Ding Tianjin Key Laboratory of Advanced Functional Porous Materials Institute for New Energy Materials&Low-Carbon TechnologiesSchool oj Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China

Design of catalyst layers(CLs)with high proton conductivity in membrane electrode assemblies(MEAs)is an important issue for proton exchange membrane fuel cells(PEMFCs).Herein,an ultrathin catalyst layer was constructed based on Pt-decorated nanoporous gold(NPG-Pt)with sub-Debye-length thickness for proton *** the absence of ionomer incorporation in the CLs,these integrated carbon-free electrodes can deliver maximum mass-specific power density of 198.21 and 25.91 kW·gPt^(-1) when serving individually as the anode and cathode,at a Pt loading of 5.6 and 22.0 pg·cm^(-2),respectively,comparable to the best reported nano-catalysts for ***-depth quantitative experimental measurements and finite-element analyses indicate that improved proton conduction plays a critical role in activation,ohmic and mass transfer polarizations.

关键词： nanoporous metal electrode proton exchange membrane fuel cell(PEMFC) ultrathin catalyst layer proton conduction dealloying

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Molecular surface functionalization of In_(2)O_(3) to tune interfacial microenvironment for enhanced catalytic performance of CO_(2) electroreduction

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Nano Research 2024年第3期17卷 1242-1250页

作者： Suwen WangQiang GaoCui Xu shuai Jiang Mengyang Zhang Xianjun yin Hui-Qing Peng Bin Liu Yu-Fei Song State Key Laboratory of Chemical Resource Engineering Beijing Advanced Innovation Center for Soft Matter Science and EngineeringCollege of ChemistryBeijing University of Chemical TechnologyBeijing 100029China

Indium-based materials(e.g.,In_(2)O_(3))are a class of promising non-noble metal-based catalysts for electroreduction of carbon dioxide(CO_(2)).However,competitive hydrogen reduction reaction(HER)on indium-based catalysts hampers CO_(2) reduction reaction(CO_(2)RR)*** herein tune the interfacial microenvironment of In_(2)O_(3) through chemical graft of alkyl phosphoric acid molecules using a facile solution-processed strategy for the first time,which is distinguished from other researches that tailor intrinsic activity of In_(2)O_(3) *** surface functionalization of alkyl phosphoric acids over In_(2)O_(3) is demonstrated to remarkably boost CO_(2) *** example,octadecylphosphonic acid modified In_(2)O_(3) exhibits Faraday efficiency for H_(2) H_(2) H_(2)(FE)of as low as 6.6%and FEHCOOH of 86.5%at-0.67 V ***,which are far superior to parent In_(2)O_(3) counterparts(FE of 24.0%and FEHCOOH of 63.1%).Moreover,the enhancing effect of alkyl phosphoric acid functionalization is found to be closely related to the length of alkyl *** virtue of comprehensive experimental characterizations and molecular dynamics simulations,it is revealed that the modification of alkyl phosphoric acids significantly alters the interface microenvironment of the electrocatalyst,which changes the electrocatalyst surface from hydrophilic and aerophobic to hydrophobic and *** this case,the water molecules are pushed away and more CO_(2) molecules are trapped,increasing local CO_(2) concentration at In_(2)O_(3) active sites,thus leading to the significantly enhanced CO_(2)RR and suppressed *** work highlights the importance of regulating the interfacial microenvironment of inorganic catalysts by molecular surface functionalization as a means for promoting the electrochemical performance in electrosynthesis and beyond.

关键词： carbon dioxide(CO_(2))electroreduction interfacial microenvironment molecular surface functionalization In_(2)O_(3)catalyst water and CO_(2)diffusion

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浅议化妆品中塑料微珠治理

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中国食品药品监管 2024年第4期 108-115页

作者：章为曹菲斐邱颖姮殷帅刘雁鸣胡斌王晓炜湖南省药品检验检测研究院深圳市药品检验研究院国家药品监督管理局化妆品监测评价重点实验室

塑料微珠引起的环境问题对于全球生态保护是一个极大的挑战,开展化妆品中塑料微珠的治理已是大势所趋。本文梳理了化妆品中塑料微珠的定义、危害和国内外政策要求,分析了我国化妆品中塑料微珠的监管现状,并提出了监管对策,以期为相关部... 详细信息

塑料微珠引起的环境问题对于全球生态保护是一个极大的挑战,开展化妆品中塑料微珠的治理已是大势所趋。本文梳理了化妆品中塑料微珠的定义、危害和国内外政策要求,分析了我国化妆品中塑料微珠的监管现状,并提出了监管对策,以期为相关部门持续深化化妆品中塑料微珠治理工作提供参考。

关键词：化妆品塑料微珠定义危害治理

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Clinical relevance of distolingual roots and periodontal status in mandibular first molars: a cross-sectional study employing CBCT analysis

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2024年第3期25卷 244-253页

作者： Feifei MAO Meng WANG shuai ZHOU Yan ZHAO Jiaping HUANG Fengying yin Haiping YANG Pei-hui DING Stomatology Hospital School of StomatologyZhejiang University School of MedicineZhejiang Provincial Clinical Research Center for Oral DiseasesKey Laboratory of Oral Biomedical Research of Zhejiang ProvinceCancer Center of Zhejiang UniversityHangzhou 310016China

Objectives:Distolingual root of the permanent mandibular first molar(PMFM-DLR)has been frequently reported,which may complicate the treatment of *** study aimed to assess the morphological features of PMFM-DLR and investigate the correlation between the morphological features of PMFM-DLR and periodontal status in patients with Eastern Chinese ethnic *** and methods:A total of 836 cone beam computed tomography(CBCT)images with 1497 mandibular first molars were analyzed to observe the prevalence of PMFM-DLR at the patients and tooth levels in Eastern *** them,complete periodontal charts were available for 69 Chinese patients with 103 *** and regression analyses were used to evaluate the correlation between the morphological features of DLR,bone loss,and periodontal clinical parameters,including clinical attachment loss(CAL),probing pocket depth(PPD),gingival recession(GR),and furcation involvement(FI).Results:The patient-level prevalence and tooth-level prevalence of DLR in mandibular first molars were 29.4%and 26.3%,*** linear regression analysis suggested that bone loss at the lingual site and CAL were negatively affected by the angle of separation between distolingual and mesial roots in the transverse section,while they were significantly influenced by age and the angle of separation between distobuccal and mesial roots in the coronal ***:The prevalence of PMFM-DLR in Eastern China was relatively high in our *** morphological features of DLR were correlated with the periodontal status of mandibular first *** study provides critical information on the morphological features of DLR for improved diagnosis and treatment options of mandibular molars with DLR.

关键词： Distolingual root Mandibular first molar Periodontal clinical parameter Clinical attachment loss Cone beam computed tomography(CBCT)

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全屋智能技术研究与实践

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建设科技 2024年第7期 30-33页

作者：邵洋殷帅范培林吴波李杨陈仕京曹峻鹏纪博雅华为终端有限公司深圳5181291 住房和城乡建设部科技与产业化发展中心北京100835 中国建筑科学研究院有限公司北京100013

建筑空间智能化是一个万亿级的新赛道,也是以科技赋能人民“好房子”的关键变量。促进住房改善消费的重点是提供群众喜欢愿意消费的好房子,好房子需要一个大的变量,能显性提升价值,相比传统的住房品质升级,全屋智能是具备划时代的科技特... 详细信息

建筑空间智能化是一个万亿级的新赛道,也是以科技赋能人民“好房子”的关键变量。促进住房改善消费的重点是提供群众喜欢愿意消费的好房子,好房子需要一个大的变量,能显性提升价值,相比传统的住房品质升级,全屋智能是具备划时代的科技特征,既能显性提高居住品质,又满足群众追求潮流和科技感的需求。

关键词：好房子数字家庭全屋智能 PLC

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