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Influence of Nd^(3+) concentration on mid-infrared emission in PbF_(2) crystal co-doped with Ho^(3+) and Nd^(3+) ions

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Journal of Rare Earths 2024年第3期42卷 479-487,I0002页

作者： Yan Chen Juncheng Tan Peixiong Zhang Weibi Zheng Lin Li Lianhan Zhang Zhen Li yin hang Zhenqiang Chen Department of Optoelectronic Engineering Jinan UniversityGuangzhou510632China Guangdong Provincial Engineering Research Centerof Crystal and Laser Technology.Guangzhou 510632China Research Center of Laser Crystal Key Laboratory of High Power Laser MaterialsShanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai201800China

A promising series of Ho_(y)Nd_(x)Pb_((1-x-y))F_2(x = 0, 0.01, 0.02, 0.03, 0.04;y = 0.02) crystals was grown by the Bridgman method. The influence of the Nd^(3+)ions concentration on mid-infrared(~2.0, ~2.9 and ~3.9 μm)fluorescence emissions of Ho^(3+)ions in the PbF_(2) crystal excited by 808 nm laser diode was investigated in this work. The energy transfer mechanism between Nd^(3+)ions and Ho~(3+)ions under different concentrations of the Nd^(3+)ions was systematically analyzed. The results show that the Nd^(3+)ions have good sensitization and deactivation effect on the Ho^(3+)ions to stimulate the mid-infrared fluorescence emissions. The experimental analysis proves that the sensitization efficiency of the Nd^(3+)ions is relatively stable at around 93.45% with varying Nd^(3+)-doping concentrations. Concentration dependence studies indicate that the concentration of the Nd^(3+)ions has significant influence on mid-infrared *** the doping concentration of the Nd^(3+)ions is up to 2.0 at%, the intensity of ~2.0, ~2.9 and ~3.9 μm emissions all reach the maximum. The output characteristics of a 3.9 μm laser are simulated, and it is found that with the increase of the Nd^(3+)-doping concentration, the peak power, pulse width, and peak energy all meet the trend of first increasing and then decreasing, and Ho_(0.02)Nd_(0.02)Pb_(0.96)F_(2) crystal displays the best performance. All the results show that the Nd^(3+)/Ho^(3+)co-doped PbF_(2) crystals might act as a useful optical medium for mid-infrared laser applications.

关键词： Crystal growth Mid-infrared PbF_(2) Rare earth ions

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Size-controlled synthesis and near-infrared photothermal response of Cp^(*)Rh-based metalla[2]catenanes and rectangular metallamacrocycles

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Chinese Chemical Letters 2024年第6期35卷 337-343页

作者： ying Zhao yin-hang Chai Tian Chen Jie Zheng Ting-Ting Li Francisco Aznarez Li-Long Dang Lu-Fang Ma College of Chemistry and Chemical Engineering Henan Key Laboratory of Function-Oriented Porous MaterialsLuoyang Normal UniversityLuoyang 471934China College of Chemistry Zhengzhou UniversityZhengzhou 450001China Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of PolymersDepartment of ChemistryFudan UniversityShanghai 200438China

A variety of research reports on novel supramolecular topologies have been published over the last ***,it is still a great challenge to tap into the inner functional properties of these ***,two tetranuclear metallamacrocycles 1 and 2 and four octonuclear[2]catenanes 3-6 were constructed successfully via a coordination-driven self-assembly strategy,by conscious design and use of the tetramethyl bidentate pyridine ligand L1,and the appropriate selection of six binuclear half-sandwich rhodium building units with different longitudinal *** complexes have been fully characterized by single crystal X-ray diffraction analysis and NMR ***,near-infrared photothermal studies of the obtained[2]catenanes reveal different photothermal response in solid and solution states,which may be attributed to a strong fluorescence quenching effect of the half-sandwich organometallic fragment and different conjugated effect of Cp^(*)Rh based building blocks in the interlocking *** photothermal conversion efficiencies of[2]catenanes 4-6 fall in the range 30.5%-16.5% *** contribution aims to play a key role in the experimental development of Cp^(*)-based photothermal materials.

关键词： Catenanes Photothermal materials Supramolecular topologies Half-sandwich fragment 3,3'-N-donor analogues

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Reductive lipid nanoparticles loaded with vinorelbine inhibit chemotherapy-induced invasion of cancer cells by modulating ENPP2

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Nano Research 2024年第4期17卷 2886-2898页

作者： Xiaoqi Zhao Xuemeng Guo Mei Pang Weigen Qiu Zhenyu Luo Qing Lin Yichao Lu hang yin Sijie Wang Huihui Liu Junlei Zhang Lihua Luo Jian You College of Pharmaceutical Sciences Zhejiang University866 Yuhangtang RoadHangzhou 310058China hangzhou Institute of Innovative Medicine Zhejiang UniversityHangzhou 310058China

Cancer is a predominant culprit behind worldwide death and accounts for up to 10 million deaths every *** is the primary therapeutic method employed for cancer in clinical settings and is essential in controlling tumor *** the advances in this field,tumor invasion and metastasis during treatment remain a significant cause of treatment ***,the underlying mechanisms involving such a disappointing phenomenon are still not fully ***(VNB)extends the lifespan of many cancer patients in the clinic as an emerging chemotherapy drug approved by Food and Drug Administration(FDA).However,VNB-induced tumor metastasis is still an intractable problem,which may be closely related to the abnormal oxidative stress generated during VNB-mediated ***,the study aims to construct a reductive nanosystem loaded with VNB,called VNB-VNP,to improve cancer cure rates and reduce tumor *** the reductive component vitamin E,VNB-VNP can effectively reduce oxidative stress and significantly outperform free VNB in preventing tumor *** transcriptome analysis shows that VNB-VNP can alleviate the over-expression of ectonucleotide pyrophosphatase/phosphodiesterase 2(ENPP2),which may be the main reason why VNB-VNP can inhibit tumor invasion and ***,the research designs a new platform for VNB treatment,which demonstrates promising efficacy in inhibiting neoplastic progression and identifies a new mechanism associated with VNB-induced tumor metastasis,which may offer several valuable references for enhancing chemotherapy efficacy in clinical anti-tumor therapy.

关键词： chemotherapy vinorelbine tumor Invasion lysophosphatidic acid ectonucleotide pyrophosphatase/phosphodiesterase 2(ENPP2)

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Triple the steady-state reaction rate by decorating the In_(2)O_(3)surface with SiO_(x)for CO_(2)hydrogenation

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Journal of Energy Chemistry 2024年第8期95卷 96-105,I0003页

作者： Hao Wang Chun Yang Xiaoyan Yu Mingrui Wang Runze Yang Xiaowa Nie Ben hang yin Alex C.K.Yip Chunshan Song Guanghui Zhang Xinwen Guo State Key Laboratory of Fine Chemicals Frontier Science Center for Smart MaterialsPSU-DUT Joint Center for Energy ResearchSchool of Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina Department of Chemistry the Chinese University of Hong KongHong Kong 999077China Paihau-Robinson Research Institute the MacDiarmid Institute for Advanced Materials and NanotechnologyVictoria University of WellingtonWellington 6012New Zealand Department of Chemical and Process Engineering The University of CanterburyChristchurch 8041New Zealand

Indium oxide(In_(2)O_(3)),as a promising candidate for CO_(2)hydrogenation to C_(1) products,often suffers from sintering and activity decline,closely related to the undesirable structural evolution under reaction *** on the comprehension of the dynamic evolution,this study presents an efficient strategy to alleviate the agglomeration of In_(2)O_(3)nanoparticles by the surface decoration with highly dispersed silica species(SiO_(x)).Various structural characterizations combined with density functional theory calculations demonstrated that the sintering resulted from the over-reduction,while the enhanced stability originated from the anchoring effect of highly stable In-OSi bonds,which hinders the substantial formation of metallic In(In^(0))and the subsequent agglomeration.0.6Si/In_(2)O_(3)exhibited CO_(2)conversion rate of10.0 mmol g^(-1)h^(-1)at steady state vs.3.5 mmol g^(-1)h^(-1)on In_(2)O_(3)in CO_(2)*** steady-state activity was also achieved on Pd-modified *** to the traditional Pd/In_(2)O_(3)catalyst,the methanol production rate of Pd catalyst supported on 0.6Si/In_(2)O_(3)was enhanced by 23%,showing the potential of In_(2)O_(3)modified by SiO_(x)in serving as a platform *** work provides a promising method to design new In_(2)O_(3)-based catalysts with improved activity and stability in CO_(2)hydrogenation.

关键词： CO_(2)hydrogenation In_(2)O_(3)sintering Dynamic structural evolution Surface SiO_(x)modification DFT simulations

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Research progress on the effect of pyroptosis on the occurrence,development,invasion and metastasis of colorectal cancer

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World Journal of Gastrointestinal Oncology 2024年第8期16卷 3410-3427页

作者： Xu Wang Qi-hang yin Lin-Lu Wan Ruo-Lan Sun Gang Wang Jun-Fei Gu De-Cai Tang School of Traditional Chinese Medicine Nanjing University of Chinese MedicineNanjing 210023Jiangsu ProvinceChina Department of Ana and Intestine Surgery The First Affiliated Hospital of Zhengzhou UniversityZhengzhou 450052Henan ProvinceChina

Pyroptosis is a type of programmed cell death mediated by gasdermines(GSDMs).The N-terminal domain of GSDMs forms pores in the plasma membrane,causing cell membrane rupture and the release of cell contents,leading to an inflammatory response and mediating *** plays an important role in inflammatory diseases and malignant *** the further study of pyroptosis,an increasing number of studies have shown that the pyroptosis pathway can regulate the tumor microenvironment and antitumor immunity of colorectal cancer and is closely related to the occurrence,development,treatment and prognosis of colorectal *** review aimed to explore the molecular mechanism of pyroptosis and the role of pyroptosis in the occurrence,development,treatment and prognosis of colorectal cancer(CRC)and to provide ideas for the clinical diagnosis and treatment of CRC.

关键词： Cell pyroptosis Tumor metastasis Colorectal cancer Clinical diagnosis Review

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无人机集群对地攻击时空协同控制策略

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工程科学学报 2024年第9期46卷 1565-1573页

作者：黄振尹航童颖裔张博洋空军工程大学航空工程学院西安710051 北京蓝天科技创新研究中心北京100080 中国人民解放军95894部队北京102200

针对三维战场环境下无人机集群协同对地打击问题,提出了一种基于预设时间收敛的无人机集群时空协同控制方法.首先,对无人机集群对地攻击任务场景及其相关要素进行了分析,并建立了无人机集群、地面运动目标和攻击问题模型.在问题建模的... 详细信息

针对三维战场环境下无人机集群协同对地打击问题,提出了一种基于预设时间收敛的无人机集群时空协同控制方法.首先,对无人机集群对地攻击任务场景及其相关要素进行了分析,并建立了无人机集群、地面运动目标和攻击问题模型.在问题建模的基础上,考虑无人机集群的时空协同策略,设计三维空间无人机集群对地攻击的时空协同控制律.所提出的时空协同控制律能够控制无人机集群在指定的时间内到达期望的攻击位置,实现对地面运动目标的时空协同攻击.通过基于李雅普诺夫函数的理论分析,证明了所提出的控制律能够在预设时间条件下使攻击位置误差变量渐进稳定.仿真结果表明,在地面运动目标转弯运动的情况下,所提出的协同控制律能够实现无人机集群的时空协同,在指定的时间内完成对地面运动目标的多角度协同攻击.

关键词：无人机集群对地攻击时空协同地面运动目标预设时间

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重型柴油车实际道路NO_(x)排放分析方法研究

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汽车工程 2024年第1期46卷 151-160页

作者：吕立群徐龙尹航杨杨葛蕴珊北京理工大学机械与车辆学院北京100081 潍柴动力股份有限公司排放法规室潍坊261061 中国环境科学研究院机动车排污监控中心北京100021

利用PEMS对6辆典型国六重型柴油车开展实际道路排放测试,基于功基窗口法(中国和欧盟)、NTE法(美国EPA)和3B-MAW法(美国CARB)研究了重型柴油车实际道路NO_(x)排放特性,探讨了不同分析方法的特点及适用性。结果表明:基于功基窗口法的NO_(x... 详细信息

利用PEMS对6辆典型国六重型柴油车开展实际道路排放测试,基于功基窗口法(中国和欧盟)、NTE法(美国EPA)和3B-MAW法(美国CARB)研究了重型柴油车实际道路NO_(x)排放特性,探讨了不同分析方法的特点及适用性。结果表明:基于功基窗口法的NO_(x)排放结果符合中国和欧盟的监管要求,但基于NTE法和3B-MAW法的NO_(x)排放合规性具有不确定性。NO_(x)排放数据利用率低导致NTE法无法有效分析实际道路NO_(x)排放,3B-MAW法对NO_(x)排放分类管理值得借鉴。冷起动NO_(x)排放占PEMS试验的47.3%~80.7%,重型柴油车冷起动NO_(x)排放应被重视。然而目前中国、欧盟和美国的重型车实际道路NO_(x)排放分析方法均无法有效评估冷起动NO_(x)排放。因此,下阶段排放法规对冷起动NO_(x)排放的监管应当提出相应测试循环、分析方法和排放限值,切实降低重型柴油车NO_(x)实际排放。

关键词：重型柴油车实际道路NO_(x)排放 NTE法功基窗口法 3B-MAW法

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长江入海热通量及其生态效应

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北京大学学报（自然科学版） 2024年第4期60卷 682-690页

作者：尹航杨善卿梁恩航李斌教育部水沙科学重点实验室北京大学环境科学与工程学院环境工程系北京100871

通过对陆地卫星Landsat 5,7,8长时间序列遥感影像资料的提取和分析,采用实用单通道算法反演1997—2016年长江入海口逐月的长序列水温数据集,同时基于全球径流数据,核算同期长江河口处的多年月均热通量,分析其时空变化规律及对气候变化... 详细信息

通过对陆地卫星Landsat 5,7,8长时间序列遥感影像资料的提取和分析,采用实用单通道算法反演1997—2016年长江入海口逐月的长序列水温数据集,同时基于全球径流数据,核算同期长江河口处的多年月均热通量,分析其时空变化规律及对气候变化和人类热排放的响应特征。在此基础上,结合全球海洋表面温度数据和哥白尼全球海洋颜色与生物–地球–化学数据集,探究长江入海热通量变化对近海水温和近海生态环境的影响。结果表明,长江河口热通量总值为77.5EJ/年,热通量的季节性变化明显,对近海的热作用以输“热”为主,显著强于其他典型大河系统,预计年均向近海输入6.1EJ的热量,增温效应明显。相较海岸带,长江口对近海水域温度的影响程度更大,影响的空间范围更远。可将近海水温的空间影响划分为两个梯度,即温度下降的河流强作用带(0~40km)以及温度上升的海洋强作用带(40km以上)。1997-2016年间,长江口的近海水域温度整体上呈现先增后减的变化规律。进一步的分析表明,长江河口热通量的变化对近海水温产生深刻影响(R^(2)=0.7495),同时与近海初级生产力密切相关(R^(2)=0.9651),说明长江对近海的热输入是调控近海热环境和生态环境的重要因素。

关键词：长江口热通量环境遥感近海生态环境

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GNSS技术在地质灾害安全监测预警系统中的应用

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中国高新科技 2024年第3期 53-55页

作者：尹航北京市矿产地质研究所北京101500

GNSS监测系统利用卫星实现全球定位,对地表任意空间进行定位,获取该地区的有效数据。人工监测受多重因素影响,无法保证监测数据的有效性。而GNSS监测系统以自身多样性优势诞生,不同于常规测量方法,GNSS操作更加简便,能够实现全天候作业... 详细信息

GNSS监测系统利用卫星实现全球定位,对地表任意空间进行定位,获取该地区的有效数据。人工监测受多重因素影响,无法保证监测数据的有效性。而GNSS监测系统以自身多样性优势诞生,不同于常规测量方法,GNSS操作更加简便,能够实现全天候作业。基于此,文章结合实际案例,对GNSS技术在地质灾害安全监测预警系统中的应用进行深入研究,以供参考。

关键词： GNSS技术地质灾害安全监测预警系统实际应用

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发电厂电气测量系统常见故障研究

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电力系统装备 2024年第5期 124-125,166页

作者：尹航江苏华电扬州发电有限公司江苏扬州225007

发电厂电气测量系统在生产过程中经常会出现各种故障,不仅会影响电力生产的正常运行,还可能对设备和人员安全造成威胁。文章对发电厂电气测量系统常见故障进行研究,并提出相应的处理措施,旨在提高电力生产效率,保障设备和人员安全。

关键词：电厂电气测量系统常见故障线路故障系统软件故障

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