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Understanding fundamentals of electrochemical reactions with tender X-rays:A new lab-based operando X-ray photoelectron spectroscopy method for probing liquid/solid and gas/solid interfaces across a variety of electrochemical systems

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Chinese Journal of Catalysis 2022年第11期43卷 2858-2870页

作者： Chiyan Liu Qiao Dong Yong Han yijing zang Hui Zhang Xiaoming Xie Yi Yu Zhi Liu State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China Center for Transformative Science ShanghaiTech UniversityShanghai 201210China School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China University of Chinese Academy of Sciences Beijing 100049China

Electrocatalysis is key to improving energy efficiency,reducing carbon emissions,and providing a sustainable way of meeting global energy ***,elucidating electrochemical reaction mechanisms at the electrolyte/electrode interfaces is essential for developing advanced renewable energy ***,the direct probing of real-time interfacial changes,i.e.,the surface intermediates,chemical environment,and electronic structure,under operating conditions is challenging and necessitates the use of in situ ***,we present a new lab-based instrument commissioned to perform in situ chemical analysis at liquid/solid interfaces using ambient pressure X-ray photoelectron spectroscopy(APXPS).This setup takes advantage of a chromium source of tender X-rays and is designed to study liquid/solid interfaces by the“dip and pull”*** of the main components was carefully described,and the results of performance tests are *** a three-electrode setup,the system can probe the intermediate species and potential shifts across the liquid electrolyte/solid electrode *** addition,we demonstrate how this system allows the study of interfacial changes at gas/solid interfaces using a case study:a sodium–oxygen model ***,the use of APXPS in electrochemical studies is still in the early stages,so we summarize the current challenges and some developmental *** the challenges,we expect that joint efforts to improve instruments and the electrochemical setup will enable us to obtain a better understanding of the composition–reactivity relationship at electrochemical interfaces under realistic reaction conditions.

关键词： Tender X-rays Ambient pressure X-ray photoelectron spectroscopy Electrocatalysis Liquid/solid interface Gas/solid interface

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The critical role of electrochemically activated adsorbates in neutral OER

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Science China Materials 2020年第12期63卷 2509-2516页

作者： Longsheng Zhang Haiyang Yuan Liping Wang Hui Zhang yijing zang Yao Tian Yunzhou Wen Fenglou Ni Hao Song Haifeng Wang Bo Zhang Huisheng Peng State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science and Laboratory of Advanced MaterialsFudan UniversityShanghai 200438China Key Laboratory for Advanced Materials Key Laboratory for Advanced MaterialsCentre for Computational Chemistry and Research Institute of Industrial CatalysisEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesCAS Center for Excellence in Superconducting ElectronicsShanghai 200050China Key Laboratory of Systems Bioengineering School of Chemical Engineering and TechnologySynBio Research PlatformCollaborative Innovation Centre of Chemical Science and EngineeringTianjin UniversityTianjin 300072China

Developing efficient electrocatalysts for the oxygen evolution reaction(OER)under neutral conditions is important for microbial electrolysis cells(MECs).However,the OER kinetics in neutral electrolytes at present are extremely sluggish,resulting in high overpotentials that greatly limit the energy conversion efficiencies of *** studies failed to probe the adsorbates on surface metal sites of catalysts at the atomic scale and elucidate their influence on the catalytic activities,which has impeded the rational design of efficient neutral OER catalysts with optimal surface ***,using in situ transmission electron microscopy(TEM),in situ X-ray photoelectron spectroscopy(XPS)and in situ low-energy ion scattering studies,we have identified,for the first time,that the electrochemically activated adsorbates on surface metal sites play a critical role in boosting the neutral OER activities of Ru-Ir binary oxide(RuxIryO2)*** adsorbate-activated RuxIryO2on a glassy carbon electrode achieved a low overpotential of 324 m V at10 m A cm-2in neutral electrolyte,with a 36-fold improvement in turnover frequency compared with that of Ir *** application in an MEC system,the resulting full cell showed a decreased voltage of 1.8 V,200 m V lower than the best value reported to date,facilitating efficient synthesis of poly(3-hydroxybutyrate)from bioelectrochemical *** functional theory(DFT)studies revealed that the enhanced OER activity of RuxIryO2catalyst arose from local structural distortion of adjacent adsorbate-covered Ru octahedra at the catalyst surface and the consequently decreased adsorption energies of OER intermediates on Ir active center.

关键词： electrocatalysis oxygen evolution reaction adsorbates neutral electrolytes

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State-of-charge Balance Control and Safe Region Analysis for Distributed Energy Storage Systems with Constant Power Loads

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1733-1745页

作者： yijing Wang Yangzhen Zhang Zhiqiang Zuo Xialin Li Department of Electrical and Information Engineering Tianjin UniversityTianjin 300384China

This paper presents a fully distributed state-of-charge balance control (DSBC) strategy for a distributed energy storage system (DESS). In this framework, each energy storage unit (ESU) processes the state-of-charge (SoC) information from its neighbors locally and adjusts the virtual impedance of the droop controller in real-time to change the current sharing. It is shown that the SoC balance of all ESUs can be achieved. Due to virtual impedance, voltage deviation of the bus occurs inevitably and increases with load power. Meanwhile, widespread of the constant power load (CPL) in the power system may cause instability. To ensure reliable operation of DESS under the proposed DSBC, the concept of the safe region is put forward. Within the safe region, DESS is stable and voltage deviation is acceptable. The boundary conditions of the safe region are derived from the equivalent model of DESS, in which stability is analyzed in terms of modified Brayton-Moser's criterion. Both simulations and hardware experiments verify the accuracy of the safe region and effectiveness of the proposed DSBC strategy.

关键词： Constant power load(CPL) distributed control distributed energy storage system(DESS) safe region state-of-charge(SoC)

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Zero-Dynamics Attacks for Multi-Agent Systems Without Velocity Measurements

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Journal of Systems Science & Complexity 2024年第5期37卷 1809-1831页

作者： GAO Jinming WANG yijing ZUO Zhiqiang ZHANG Wentao Tianjin Key Laboratory of Intelligent Unmanned Swarm Technology and System School of Electrical and Information Engineering Tianjin University Continental-NTU Corporate Lab School of Electrical and Electronic Engineering Nanyang Technological University

This paper studies the periodic zero-dynamics attacks(ZDAs) in multi-agent systems without velocity measurements under directed graph. Specifically, two types of attack modes are addressed,i.e., infinite number and finite number of zero-dynamics attacks. For the former case, the authors show that the consensus of the considered system cannot be guaranteed. For the latter case, the dynamic evolution of the agents is investigated and it is found that only attacking the rooted agents can destroy the consensus. Then, a sufficient condition which quantifies whether or not the consensus value is destroyed is given, revealing the relationship among parameters of system model, filter and attack ***, simulations are carried out to verify the effectiveness of the theoretical findings.

关键词： Consensus directed graph multi-agent systems zero-dynamics attacks

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Virtual Power Plants for Grid Resilience: A Concise Overview of Research and Applications

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 329-343页

作者： yijing Xie Yichen Zhang Wei-Jen Lee Zongli Lin Yacov A.Shamash IEEE Department of Electrical Engineering University of Texas at ArlingtonArlingtonTX 76019 USA Charles L.Brown Department of Electrical and Computer Engineering University of VirginiaCharlottesvilleVA 22904 USA Department of Electrical and Computer Engineering Stony Brook UniversityStony BrookNY 11794 USA

The power grid is undergoing a transformation from synchronous generators(SGs) toward inverter-based resources(IBRs). The stochasticity, asynchronicity, and limited-inertia characteristics of IBRs bring about challenges to grid resilience. Virtual power plants(VPPs) are emerging technologies to improve the grid resilience and advance the transformation. By judiciously aggregating geographically distributed energy resources(DERs) as individual electrical entities, VPPs can provide capacity and ancillary services to grid operations and participate in electricity wholesale markets. This paper aims to provide a concise overview of the concept and development of VPPs and the latest progresses in VPP operation, with the focus on VPP scheduling and control. Based on this overview, we identify a few potential challenges in VPP operation and discuss the opportunities of integrating the multi-agent system(MAS)-based strategy into the VPP operation to enhance its scalability, performance and resilience.

关键词： Climate change renewable energy resources resilience smart grids virtual power plants(VPPs)

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FaultMonitoring Strategy for PV System Based on I-V Feature Library

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Energy Engineering 2024年第3期121卷 643-660页

作者： Huaxing Zhao Yanbo Che Gang Wen yijing Chen School of Electrical and Information Engineering Tianjin UniversityTianjin300000China State Grid Shuozhou Electric Power Supply Company Shuozhou036000China China Huaneng Clean Energy Research lnstitute Technology Co. Ltd.Beijing102209China

Long-term use in challenging natural conditions is possible for photovoltaic modules,which are extremely prone to *** to diagnose and address faults in Photovoltaic(PV)power systems in a timely manner can cause permanent damage to PV modules and,in more serious cases,***,research into photovoltaic module defect detection techniques is crucial for the growth of the photovoltaic sector as well as for maintaining national economic prosperity and ensuring public *** the drawbacks of the current real-time and historical data-based methods for monitoring distributed PV systems,this paper proposes a method for monitoring PV systems at the module or string level that can be achieved by monitoring only electrical *** approach doesn’t need a lot of tests to get the operational data of PV modules beforehand and only requires theoretical feature libraries of PV modules through panel parameter *** present operating conditions and the open-circuit and short-circuit faults can be precisely identified by comparing the observed open-circuit voltage and short-circuit current with the corresponding data in the theoretical feature *** that,by comparing the measured maximum power point voltage and current with the corresponding data in the theoretical feature library through the threshold method,aging and shadowing faults can be accurately *** testing was done to see whether the suggested method was *** results show that the proposed technique is able to diagnose open-circuit faults,short-circuit faults,aging faults,and shadowing faults with shadow occlusion above 20%.

关键词： PV system lambert W function threshold method

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The Lightweight Edge-Side Fault Diagnosis Approach Based on Spiking Neural Network

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Computers, Materials & Continua 2024年第6期79卷 4883-4904页

作者： Jingting Mei Yang Yang Zhipeng Gao Lanlan Rui yijing Lin State Key Laboratory of Networking and Switching Technology Beijing University of Posts and TelecommunicationsBeijing100876China

Network fault diagnosis methods play a vital role in maintaining network service quality and enhancing user experience as an integral component of intelligent network *** the unique characteristics of edge networks,such as limited resources,complex network faults,and the need for high real-time performance,enhancing and optimizing existing network fault diagnosis methods is ***,this paper proposes the lightweight edge-side fault diagnosis approach based on a spiking neural network(LSNN).Firstly,we use the Izhikevich neurons model to replace the Leaky Integrate and Fire(LIF)neurons model in the LSNN *** neurons inherit the simplicity of LIF neurons but also possess richer behavioral characteristics and flexibility to handle diverse data *** by Fast Spiking Interneurons(FSIs)with a high-frequency firing pattern,we use the parameters of ***,inspired by the connection mode based on spiking dynamics in the basal ganglia(BG)area of the brain,we propose the pruning approach based on the FSIs of the BG in LSNN to improve computational efficiency and reduce the demand for computing resources and energy ***,we propose a multiple iterative Dynamic Spike Timing Dependent Plasticity(DSTDP)algorithm to enhance the accuracy of the LSNN *** on two server fault datasets demonstrate significant precision,recall,and F1 improvements across three diagnosis ***,lightweight indicators such as Params and FLOPs significantly reduced,showcasing the LSNN’s advanced performance and model *** conclude,experiment results on a pair of datasets indicate that the LSNN model surpasses traditional models and achieves cutting-edge outcomes in network fault diagnosis tasks.

关键词： Network fault diagnosis edge networks Izhikevich neurons pruning dynamic spike timing dependent plasticity learning

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Predesigned covalent organic framework with sulfur coordination: Anchoring Au nanoparticles for sensitive colorimetric detection of Hg(Ⅱ)

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Chinese Chemical Letters 2024年第5期35卷 392-396页

作者： Guorong Li yijing Wu Chao Zhong Yixin Yang Zian Lin Ministry of Education Key Laboratory of Analytical Science for Food Safety and Biology Fujian Provincial Key Laboratory of Analysis and Detection Technology for Food SafetyCollege of ChemistryFuzhou UniversityFuzhou 350108China

Targeted construction of new covalent organic frameworks(COFs)with specific purposes and rationalities to build colorimetric assay platform for environmental pollutant monitoring have attracted increasing ***,it is still challenging due to lack of available coordination sites inside COFs pores and only a slight bonding ability for anchoring *** this work,a two-dimensional(2D)COFs(termed as Tz-COF)with high crystallinity,excellent chemical stability,and abundant sulfur coordination in its skeletons was synthesized and used for the confined growth of Au *** was found that the Au NPs showed significant dispersibility for the support of *** proposed Tz-COF@Au NPs possessed outstanding Hg^(2+)-activated peroxidase-like activity benefited from physicochemical properties of gold amalgam and synergistic effect between COFs and Au NPs to oxidize chromogenic *** on highly efficient activity and distinctive color evolution,the strategy for detecting Hg^(2+)was developed and successfully applied to determine the content of Hg^(2+)in real environmental *** work manifests that a potential strategy to establish a colorimetric assay platform for environmental pollutant monitoring based on the targeted manufacturing of novel COFs with specific functions.

关键词： Covalent organic frameworks Thiazole Sulfur coordination Au nanoparticles Hg^(2+)-activated peroxidase-like activity

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Dynamic 3D holographic projection of vectorial images with a multimode fiber

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Photonics Research 2024年第6期12卷 1344-1350页

作者： JINGHAN ZHUANG PANPAN YU YIFAN LIU yijing WU ZIQIANG WANG YINMEI LI LEI GONG Department of Optics and Optical Engineering University of Science and Technology of ChinaHefei 230026China Advanced Laser Technology Laboratory of Anhui Province Hefei 230026China

An optical multimode fiber(MMF)is capable of delivering structured light modes or complex images with high ***,we present a holographic approach to enable the MMF as a 3D holographic projector with the capability of complete polarization *** harnessing the strong coupling of the spatial and polarization degrees of freedom of light propagating through MMFs,our approach realizes active control of the output intensity and polarization in 3D space by shaping only the wavefront of the incident *** this manner,we demonstrate MMF-based holographic projection of vectorial images on multiple planes via a phase-only ***,dynamic projection of polarization-multiplexed grayscale images is presented with an averaged Pearson correlation coefficient of up to *** work is expected to benefit fiber-based holographic displays,data transmission,optical imaging,and manipulation.

关键词： holographic projection enable

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Highly conductive and tough double-network hydrogels for smart electronics

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SmartMat 2024年第2期5卷 54-66页

作者： Dong Zhang yijing Tang Xiong Gong Yung Chang Jie Zheng Department of Chemical Biomolecularand Corrosion EngineeringThe University of AkronAkronOhioUSA School of Polymer Science and Polymer Engineering The University of AkronAkronOhioUSA R&D Center for Membrane Technology and Department of Chemical Engineering Chung Yuan Christian UniversityTaiwanChina

Development and understanding of highly mechanically robust and electronically conducting hydrogels are extremely important for ever-increasing energy-based *** mixing/blending of conductive additives with hydrophilic polymer network prevents both high mechanical strength and electronic conductivity to be presented in polymer ***,we proposed a double-network(DN)engineering strategy to fabricate PVA/PPy DN hydrogels,consisting of a conductive PPy-PA network via in-situ ultrafast gelation and a tough PVA network via a subsequent freezing/thawing *** resultant PVA/PPy hydrogels exhibited superior mechanical and electrochemical properties,including electrical conductivity of~6.8 S/m,mechanical strength of~0.39 MPa,and elastic moduli of~0.1 *** further transformation of PVA/PPy hydrogels into supercapacitors,they demonstrated a high capacitance of~280.7 F/g and a cycle life of 2000 galvanostatic charge/discharge cycles with over 94.3%capacity retention at the current density of 2 mA/cm2 and even subzero temperatures of−20℃.Such enhanced mechanical performance and electronic conductivity of hydrogels are mainly stemmed from a synergistic combination of continuous electrically conductive PPy-PA network and the two interpenetrating DN *** in-situ gelation strategy is applicable to the integration of ionic-/electrical-conductive materials into DN hydrogels for smart-soft electronics,beyond the most commonly used PEDOT:PSS-based hydrogels.

关键词： conducting polymers double-network hydrogels smart electronics supercapacitors

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