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Upcycling the spent graphite/LiCoO_(2) batteries for high-voltage graphite/LiCoPO_(4)-co-workable dual-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1745-1751页

作者： Miao du Hongyan Lü Kaidi du Shuohang Zheng Xiaotong Wang Xiaotong Deng Ronghua Zeng Xinglong Wu Key Laboratory for UV Light-Emitting Materials and Technology of Ministry of Education Northeast Normal UniversityChangchun 130024China Faculty of Chemistry Northeast Normal UniversityChangchun 130024China School of Chemistry South China Normal UniversityGuangzhou 510006China

The worldwide proliferation of portable electronics has resulted in a dramatic increase in the number of spent lithium-ion batteries(LIBs).However,traditional recycling methods still have limitations because of such huge amounts of spent ***,we proposed an ecofriendly and sustainable double recycling strategy to concurrently reuse the cathode(LiCoO_(2))and anode(graphite)materials of spent LIBs and recycled LiCoPO_(4)/graphite(RLCPG)in Li^(+)/PF^(-)_(6) co-de/intercalation dual-ion *** recycle-derived dualion batteries of Li/RLCPG show impressive electrochemical performance,with an appropriate discharge capacity of 86.2 mAh·g^(-1) at25 mA·g^(-1) and 69%capacity retention after 400 *** recycling of the cathode and anode from spent LIBs avoids wastage of resources and yields cathode materials with excellent performance,thereby offering an ecofriendly and sustainable way to design novel secondary batteries.

关键词： recycle lithium cobalt oxide lithium cobalt phosphate graphite dual-ion batteries spent lithium-ion batteries

Magneto-optical Kerr Effect of Mono-layer NiX_(2)(X=Cl,Br,I):A Density Functional Theory Study

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1121-1128页

作者： FAN Qingqian du Chaochao School of Economics and Management Shanghai Institute of TechnologyShanghai 200235China College of Information Science&Electronic Engineering Zhejiang UniversityHangzhou 310027China

The full-potential linearized augmented plane wave plus local orbital method is utilized for exploring the electronic,magnetic,and magneto-optical properties of the NiX_(2)(X=Cl,Br,and I)single *** first-principles calculation demonstrates that these compounds are ferromagnetic indirect semiconductors,and the energy band gaps of NiX_(2)for X=Cl,Br,and I are 3.888,3.134,and 2.157 eV,*** magnetic moments of Ni atoms in NiX_(2)monolayer are 1.656,1.588,1.449μB,and their magneto-crystalline anisotropy energies are 0.167,0.029,0.090 meV,*** on the macro-linear response theory,we systematically studied the influences of the external magnetic field and out-of-plane strain on the magneto-optical Kerr effect(MOKE)spectrum of the NiX_(2)single *** is found that,when the external magnetic field is perpendicular to the sample plane,the value of the Kerr rotation angle reaches the maximum,and the single-layer NiI_(2)material has a Kerr rotation angle of 1.89°at the photon energy of 1.986 ***,the Kerr rotation spectrum of NiCl_(2)and NiBr_(2)monolayers redshift as the out-of-plane strain increases,while NiI_(2)monolayer *** computation of the MOKE spectrum of NiX_(2)materials provides an opportunity for applications of 2D magnetic material ranging from sensing to data storing.

关键词： magneto-optical Kerr effect(MOKE) first-principles calculations external magnetic field out-of-plane strain

A Nonparametric Model Checking Test for Functional Linear Composite Quantile Regression Models

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Journal of Systems Science & Complexity 2024年第4期37卷 1714-1737页

作者： XIA Lili du Jiang ZHANG Zhongzhan Faculty of Science Beijing University of TechnologyBeijing 100124China

This paper is focused on the goodness-of-fit test of the functional linear composite quantile regression model.A nonparametric test is proposed by using the orthogonality of the residual and its conditional expectation under the null *** proposed test statistic has an asymptotic standard normal distribution under the null hypothesis,and tends to infinity in probability under the alternative hypothesis,which implies the consistency of the ***,it is proved that the test statistic converges to a normal distribution with nonzero mean under a local alternative *** simulations are reported,and the results show that the proposed test has proper sizes and is sensitive to the considered model *** proposed methods are also applied to two real datasets.

关键词： Composite quantile regression consistent test functional data nonparametric test quadratic form

An alternative 2D ICEEMDAN-based denoising method and its application in processing magnetic anomaly data

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Geodesy and Geodynamics 2024年第5期15卷 465-476页

作者： Jun Xu Jinsong du Changqing Yuan School of Geophysics and Geomatics China University of GeosciencesWuhan 430074China Hubei Subsurface Multi-scale Imaging Key Laboratory China University of GeosciencesWuhan 430074China State Key Laboratory of Geological Processes and Mineral Resources China University of GeosciencesWuhan 430074China Key Laboratory of Geological Survey and Evaluation of Ministry of Education China University of GeosciencesWuhan 430074China

due to environmental noise and human factors,magnetic data collected in the field often contain various noises and interferences that significantly affect the subsequent data processing and *** Mode Decomposition(EMD),an adaptive multiscale analysis method for nonlinear and non-stationary signals,is widely used in geophysical and geodetic data *** with traditional EMD,Improved Complete Ensemble EMD with Adaptive Noise(ICEEMDAN)is more effective in addressing the problem of mode *** on the principles of 1D ICEEMDAN,this paper presents an alternative algorithm for 2D ICEEMDAN,extending its application to two-dimensional *** effectiveness of the proposed approach is demonstrated through synthetic signal experiments,which show that the 2D ICEEMDAN exhibits a weaker mode mixing effect compared to the traditional bidimensional EMD(BEMD)***,to improve the performance of the denoising method based on 2D ICEEMDAN and preserve useful signals in high-frequency components,an improved soft thresholding technique is *** magnetic anomaly data testing indicates that our denoising method effectively preserves signal continuity and outperforms traditional soft thresholding *** validate the practical application of this improved threshold denoising method based on 2D ICEEMDAN,it is applied to ground magnetic survey data in the Yandun area of *** results demonstrate the effectiveness of the method in removing noise while retaining essential information from practical magnetic anomaly *** particular,practical applications suggest that 2D ICEEMDAN can extract trend signals more accurately than the *** conclusion,as a potential tool for multi-scale decomposition,the 2D ICEEMDAN is versatile in processing and analyzing 2D geophysical and geodetic data.

关键词： 2D ICEEMDAN Mode mixing effect Magnetic anomaly Denoising Improved soft thresholding

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铣挖机在城市暗挖隧道施工中的应用

铁道建筑技术 2015年第2期 77-79,108页

作者：杜以臣中铁十四局集团有限公司济南250000

长株潭城际铁路树木岭隧道湘府路站~汽车南站站暗挖区间埋深较浅,地面房屋与构造物密集,多次穿越市政道路及河流,采用矿山法开挖,如何控制围岩变形及地表沉降是本工程的一个技术难点。结合工程实际,重点从铣挖机的选型、开挖方法、施工... 详细信息

长株潭城际铁路树木岭隧道湘府路站~汽车南站站暗挖区间埋深较浅,地面房屋与构造物密集,多次穿越市政道路及河流,采用矿山法开挖,如何控制围岩变形及地表沉降是本工程的一个技术难点。结合工程实际,重点从铣挖机的选型、开挖方法、施工步骤进行了论述,并总结分析了铣挖机在隧道施工中的优缺点。现场采用铣挖机开挖与弱爆破相结合的施工方法,通过监控量测表明能很好地控制围岩变形、地表沉降,可为以后城市暗挖隧道施工提供借签。

关键词：铣挖机暗挖隧道监控量测沉降控制

Prediction of subsurface settlement induced by shield tunnelling in sandy cobble stratum

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第1期16卷 192-212页

作者： Fan Wang Xiuli du Pengfei Li Key Laboratory of Urban Security and Disaster Engineering Ministry of EducationBeijing University of TechnologyBeijing100124China

This study focuses on the analytical prediction of subsurface settlement induced by shield tunnelling in sandy cobble stratum considering the volumetric deformation modes of the soil above the tunnel crown.A series of numerical analyses is performed to examine the effects of cover depth ratio(C/D),tunnel volume loss rate(h t)and volumetric block proportion(VBP)on the characteristics of subsurface settle-ment trough and soil volume *** the ground loss variation with depth,three modes are deduced from the volumetric deformation responses of the soil above the tunnel ***,analytical solutions to predict subsurface settlement for each mode are presented using stochastic medium *** influences of C/D,h t and VBP on the key parameters(i.e.B and N)in the analytical expressions are discussed to determine the fitting formulae of B and ***,the proposed analytical solutions are validated by the comparisons with the results of model test and numerical *** show that the fitting formulae provide a convenient and reliable way to evaluate the key ***,the analytical solutions are reasonable and available in predicting the subsurface settlement induced by shield tunnelling in sandy cobble stratum.

关键词： Shield tunnelling Sandy cobble stratum Subsurface settlement Volumetric deformation mode Stochastic medium theory

Highly efficient and wearable thermoelectric composites based on carbon nanotube film/polyaniline

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Journal of Materiomics 2024年第1期10卷 173-178页

作者： Jing Huang Xiaohua Liu Yong du School of Materials Science and Engineering Shanghai Institute of Technology100 Haiquan RoadShanghai201418China

Polyaniline(PANI)was prepared by in-situ polymerization and compounded on the two-dimensional network structural multi-walled carbon nanotube film(CNTF).Compared with the CNT/PANI composites fabricated by using CNT powders or dispersions,the compact and continuous network structure of CNTF/PANI is beneficial to both the thermoelectric and mechanical properties of the *** resultant CNTF/PANI composites with PANI polymerization time of 5 h obtain an electrical conductivity of 1338.4 S/cm and Seebeck coefficient of 63.3μV/K at 360 K,which are 168.7%and 5.7%higher than those of the CNTF(498.1 S/cm and 59.9μV/K at 360 K).Consequently,a maximum power factor of 536.8μW·m^(−1)·K^(−2) at 360 K is acquired,which is about 2 times higher than that of CNTF(181.7μW·m^(−1)·K^(−2) at 360 K).The electrical conductivity of the composites could maintain 93.3%after being bent for 500 times,indicating the excellent *** tensile strength,Young's Modulus and toughness of CNTF/PANI composites(232.3 MPa,3.6 GPa and 20.1 MJ/m^(3),respectively)are 3.5,2.6 and 2.1 times of those of the *** flexible,free-standing,lightweight and high-strength CNTF/PANI composites reveal the excellent thermoelectric performance,which are promising in the applications in wearable thermoelectric devices.

关键词： Carbon nanotube film Polyaniline Thermoelectric performance Mechanical properties

Photoswitchable Spiropyridine Enabled Photoactuation of Polymeric Hydrogels under Physiological pH Conditions

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Chinese Journal of Polymer Science 2024年第10期42卷 1602-1609,I0015页

作者： Cong Liao Meng-Qi du Chuang Li Key Laboratory of Precision and Intelligent Chemistry Department of Polymer Science and EngineeringUniversity of Science and Technology of ChinaAnhui230026China

The incorporation of molecular switches into polymer networks has been a powerful approach for the development of functional polymer materials that display macroscopic actuation and function enabled directly by molecular ***,such materials sometimes require harsh conditions to perform their functions,and the design of new molecular photoswitches that can function under physiological conditions is highly ***,we report the design and synthesis of a spiropyridine-based photoswitchable hydrogel that exhibits light-driven actuation at physiological *** to its high p Ka,spiropyridine maintains its ring-open protonated form at neutral pH,and the resulting hydrogel remains in a swollen *** irradiation with visible light,the ring closure of spiropyridine leads to a decrease in the charge and a reduction in the volume of the *** contracted gel could spontaneously recover to its expanding state in the dark,and this process is highly dynamic and reversible when the light is switched on and ***,the hydrogel shows switchable fluorescence in response to visible *** deformation is observed in the hydrogel thin films upon irradiation from one ***,the independence of this spiropyridine hydrogel from the acidic environment makes it biotolerant and shows excellent *** biocompatible spiropyridine hydrogel might have important biorelated applications in the future.

关键词： Spiropyridine photowitch Polymer hydrogel Photoactuation Physiological pH Biocompatibility

Land use change and its driving factors in the ecological function area:A case study in the Hedong Region of the Gansu Province,China

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Journal of Arid Land 2024年第1期16卷 71-90页

作者： WEI Zhudeng du Na YU Wenzheng School of Geographical Science Nanjing University of Information Science&TechnologyNanjing 210044China

Land use and cover change(LUCC)is important for the provision of ecosystem *** increasing number of recent studies link LUCC processes to ecosystem services and human well-being at different scales ***,the dynamic of land use and its drivers receive insufficient attention within ecological function areas,particularly in quantifying the dynamic roles of climate change and human activities on land use based on a long time *** study utilizes geospatial analysis and geographical detectors to examine the temporal dynamics of land use patterns and their underlying drivers in the Hedong Region of the Gansu Province from 1990 to *** indicated that grassland,cropland,and forestland collectively accounted for approximately 99% of the total land *** initially increased and then decreased after 2000,while grassland decreased with *** contrast,forestland and construction land were continuously expanded,with net growth areas of 6235.2 and 455.9 km^(2),*** 1990 to 2020,cropland was converted to grassland,and both of them were converted to forestland as a *** expansion of construction land primarily originated from *** 2000 to 2005,land use experienced intensified temporal dynamics and a shift of relatively active zones from the central to the southeastern *** yield,economic factors,and precipitation were the major factors accounting for most land use *** impacts on land use changes were stronger before 1995,succeeded by the impact of animal husbandry during 1995-2000,followed by the impacts of grain production and gross domestic product(GDP)after ***,agricultural and pastoral activities,coupled with climate change,exhibited stronger enhancement effects after 2000 through their interaction with population and economic *** patterns closely correlated with ecological restoration projects in China since *** study implies the importance of synergy be

关键词： land use land type geographic detector driving mechanism Hedong Region