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Structurally Flexible 2D Spacer for Suppressing the Electron-Phonon Coupling Induced Non-Radiative Decay in Perovskite Solar Cells

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Nano-Micro letters 2024年第9期16卷 325-340页

作者： Ruikun Cao Kexuan Sun Chang l.u Yuhong Mao Wei Guo Ping Ouyang Yuanyuan Meng Ruijia Tian lisha Xie Xujie lü Ziyi Ge Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China School of Materials Science and Chemical Engineering Ningbo UniversityNingbo 315211People’s Republic of China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Center for High Pressure Science and Technology Advanced Research(HPSTAR) Shanghai 201203People’s Republic of China

This study presents experimental evidence of the dependence of non-radiative recombination processes on the electron-phonon coupling of perovskite in perovskite solar cells(PSCs).Via A-site cation engineering,a weaker electron-phonon coupling in perovskite has been achieved by introducing the structurally soft cyclohexane methylamine(CMA^(+))cation,which could serve as a damper to alleviate the mechanical stress caused by lattice oscillations,compared to the rigid phenethyl methylamine(PEA^(+))*** demonstrates a significantly lower non-radiative recombination rate,even though the two types of bulky cations have similar chemical passivation effects on perovskite,which might be explained by the suppressed carrier capture process and improved lattice geometry *** resulting PSCs achieve an exceptional power conversion efficiency(PCE)of 25.5%with a record-high opencircuit voltage(V_(OC))of 1.20 V for narrow bandgap perovskite(FAPbI_(3)).The established correlations between electron-phonon coupling and non-radiative decay provide design and screening criteria for more effective passivators for highly efficient PSCs approaching the Shockley-Queisser limit.

关键词： Electron-phonon coupling A-site cation engineering Non-radiative recombination

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Pulsations of Three Rapidly Oscillating Ap Stars TIC 96315731,TIC72392575,and TIC 318007796

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Research in Astronomy and Astrophysics 2024年第8期24卷 157-168页

作者： Hai-Jian Zhong Dong-Xiang Shen Chun-Hua Zhu He-lei l.u Su-Fen Guo Guo-liang lü School of Physical Science and Technology Xinjiang UniversityUrumqi 830046China Xinjiang Astronomical Observatory National Astronomical ObservatoriesChinese Academy of SciencesUrumqi 830000China

We analyze the frequencies of three known roAp stars,TIC 96315731,TIC 72392575,and TIC 318007796,using the light curves from the Transiting Exoplanet Survey *** TIC 96315731,the rotational and pulsational frequencies are 0.1498360 day^(-1)and 165.2609 day^(-1),*** the case of TIC 72392575,the rotational frequency is 0.25551 day^(-1).We detect a quintuplet of pulsation frequencies with a center frequency of135.9233 day^(-1),along with two signals within the second pair of rotational sidelobes of the quintuplet separated by the rotation *** two signals may correspond to the frequencies of a dipole *** TIC318007796,the rotational and pulsational frequencies are 0.2475021 day^(-1),192.73995 day^(-1),and196.33065 day^(-1),*** on the oblique pulsator model,we cal.ulate the rotation inclination(i)and magnetic obliquity angle(b)for the stars,which provide the geometry of the pulsation *** the phases of the frequency quintuplets,the pulsation amplitude and phase modulation curves,and the results of spherical harmonic decomposition,we conclude that the pulsation modes of frequency quintuplets in TIC96315731,TIC 72392575,and TIC 318007796 correspond to distorted dipole mode,distorted quadrupole mode,and distorted dipole mode,respectively.

关键词： asteroseismology-techniques photometric-stars oscillations(including pulsations)-stars chemically peculiar

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Enabling robust and hour-level organic long persistent luminescence from carbon dots by covalent fixation

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light(Science & Applications) 2022年第4期11卷 686-696页

作者： Kai Jiang Yuci Wang Cunjian lin licheng Zheng Jiaren Du yixi Zhuang Rongjun Xie Zhongjun li Hengwei lin International Joint Research Center for Photo-responsive Molecules and Materials School of Chemical and Material EngineeringJiangnan University214122 WuxiChina College of Chemistry Zhengzhou University450001 ZhengzhouChina State Key laboratory of Physical Chemistry of Solid Surface Fujian Provincial Key Laboratory of Materials Genomeand College of MaterialsXiamen University361005 XiamenChina

The first carbon dot(CD)-based organic long persistent luminescence(OlPl)system exhibiting more than 1 h of duration was *** contrast to the established OlPl systems,herein,the reported CDs-based system(named m-CDs@CA)can be facilely and effectively fabricated using a household microwave oven,and more impressively,its lPl can be observed under ambient conditions and even in aqueous *** and TEM characterizations,afterglow decay,time-resolved spectroscopy,and ESR analysis were performed,showing the successful composition of CDs ***,the formation of exciplexes and long-lived charged-separated *** studies suggest that the production of covalent bonds between CA and CDs plays pivotal roles in activating lPl and preventing its quenching from oxygen and *** the best of our knowledge,this is a very rare example of an OlPl system that exhibits hourlevel afterglow under ambient ***,applications of m-CDs@C.A in glow-in-the-dark paints for emergency signs and multicolored luminous pearls were preliminarily *** work may provide new insights for the development of rare earth-free and robust OlPl materials.

关键词： luminescence system ambient

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The Impact of Nova Outbursts on the Chemical Abundance of the Interstellar Medium

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Research in Astronomy and Astrophysics 2024年第10期24卷 116-129页

作者： Guoli He Chunhua Zhu Guoliang lü lin li Sufen Guo Helei l.u Jun Gao School of Physical Science and Technology Xinjiang UniversityUrumqi 830017China Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China

Nova outbursts are the results of thermonuclear runaways,which occur when sufficient material accretes on the surfaces of white dwarfs(WDs).using the MESA code,we construct a detailed grid for carbon-oxygen and oxygen-neon-magnesium *** employing population synthesis methods,we conduct a statistical analysis of the distribution of novae in the Milky *** our models,on average,a typical nova system may undergo about8000 eruptions and the Galactic nova rate is~130 yr^(-1).The C,N,and O elements in nova ejecta are strongly affected by the mixing degree between WD core and accreted *** results show that the average value of^(12)C/^(13)C in nova ejecta is about an order of magnitude lower than that on the surface of a red giant,that for^(16)O/^(17)O is about 5 times lower,and that for^(14)N/^(15)N is about 1.5 times *** annual yields of^(13)C,^(15)N,and^(17)O from nova ejection are larger than those from AGB *** indicates that compared to a red giant,nova eruptions are a more important source of the odd-numbered nuclear elements of^(13)C,^(15)N,and^(17)O in the Galactic interstellar medium.

关键词： ISM:abundances (stars:)novae cataclysmic variables (stars:)white dwarfs

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Simulation of rainfall-runoff and watershed convergence process in the upper reaches of Heihe River Basin,July 2002

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Science China Earth Sciences 2004年第z1期47卷 1-8页

作者： GAO Yanhong l.u) Shihua CHENG Guodong Cold and Arid Regions Environmental and Engineering Research Institute Chinese Academy of Sciences Lanzhou 730000 China Cold and Arid Regions Environmental and Engineering Research Institute Chinese Academy of Sciences Lanzhou 730000 China Cold and Arid Regions Environmental and Engineering Research Institute Chinese Academy of Sciences Lanzhou 730000 China

The watershed flow concentration scheme in the distributed hydrology-soil- vegetation model (DHSVM) is coupled with the mesoscale atmospheric model MM5 version 3.5, in which the Oregen States university land surface model (OSulSM) was involved. The flood event which happened in July 2002 in the upper reaches of Heihe river basin is simulated and the surface flow convergence process is shown with this coupled model. It has been concluded that times water head reaches each place of the basin are different. Water amount at each point is split-flow proportionally as the drops in elevation between it and neighbor points. large part of the water amount pass away in greater slope direction and small part pass away in smaller slope *** of the slope convergence makes the atmospheric model redistributes the surface water laterally.

关键词： distributed hydrology-soil-vegetation model, mesoscale atmospheric model, watershed flow concentration process.

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RATIONAl GENERAl SOluTIONS OF HIGHER ORDER AlGEBRAIC ODES

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Journal of Systems Science & Complexity 2013年第2期26卷 261-280页

作者： HuANG Yanli NG l X Chu WINKlER Franz School of Computer Science and Software Engineering Tianjin Polytechnic University Research Institute for Symbolic Computation(RISC) Johannes Kepler University Department of Mathematics Quy Nhon University

This paper generalizes the method of Ng6 and Winkler （2010, 2011） for finding rational general solutions of a first order non-autonomous algebraic ordinary differential equation （AODE） to the case of a higher order AODE, provided a proper parametrization of its solution hypersurface. The authors reduce the problem of finding the rational general solution of a higher order AODE to finding the rational general solution of an associated system. The rational general solutions of the original AODE and its associated system are in computable 1-1 correspondence. The authors give necessary and sufficient conditions for the associated system to have a rational solution based on proper reparametrization of invariant algebraic space curves. The authors also relate invariant space curves to first integrals and characterize rationally solvable systems by rational first integrals.

关键词： Algebraic ODE associated system invariant algebraic space curve rational first integral rational general solution.

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Generalized autoencoder-based fault detection method for traction systems with performance degradation

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High-speed Railway 2024年第3期2卷 180-186页

作者： Cheng C. l.u W. Di l. Wang S. Changchun university of Technology Changchun 130012 China Jilin Institute of Electronics Information Products Inspection Changchun 130012 China

Fault diagnosis of traction systems is important for the safety operation of high-speed trains. long-term operation of the trains will degrade the performance of systems, which decreases the fault detection accuracy. To solve this problem, this paper proposes a fault detection method developed by a Generalized Autoencoder (GAE) for systems with performance degradation. The advantage of this method is that it can accurately detect faults when the traction system of high-speed trains is affected by performance degradation. Regardless of the probability distribution, it can handle any data, and the GAE has extremely high sensitivity in anomaly detection. Finally, the effectiveness of this method is verified through the Traction Drive Control System (TDCS) platform. At different performance degradation levels, our method's experimental results are superior to traditional methods. © 2024 Beijing Jiaotong university

关键词： Fault detection Generalized autoencoder High-speed trains Performance degradation Traction control systems

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Chitin-glucan improves important pathophysiological features of irritable bowel syndrome

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World Journal of Gastroenterology 2024年第16期30卷 2258-2271页

作者： Caroline Valibouze Caroline Dubuquoy Philippe Chavatte Michaël Genin Veronique Maquet Salvatore Modica Pierre Desreumaux Christel Rousseaux Department of Digestive Surgery and Transplantation Lille UniversityLille 59037France Intestinal Biotech Development Facultéde MédicineLille 59045France u1286-INFINITE-Institute for Translational Research in Inflammation Universitéde LilleLille 59000France ulR 2694-METRICS Évaluation des Technologies de santéet des Pratiques MédicalesUniversity of LilleLille 59000France KitoZyme SA Institution SociétéAnonymeZone 2Parc des Hauts SartsRue de MilmortHerstal 4040Belgium Hepato-Gastroenterology Department Lille University HospitalLille 59037France

BACKGROuND Irritable bowel syndrome(IBS)is one of the most frequent and debilitating conditions leading to gastroenterological ***,recommended treatments remain limited,yielding only limited therapeutic ***-glucan(CG)is a novel dietary prebiotic classically used in humans at a dosage of 1.5-3.0 g/d and is considered a safe food ingredient by the European Food Safety *** provide an alternative approach to managing patients with IBS,we performed preclinical molecular,cel.ular,and animal studies to evaluate the role of chitin-glucan in the main pathophysiological mechanisms involved in *** To evaluate the roles of CG in visceral analgesia,intestinal inflammation,barrier function,and to develop computational molecular *** Visceral pain was recorded through colorectal distension(CRD)in a model of long-lasting colon hypersensitivity induced by an intra-rectal administration of TNBS[15 milligrams(mg)/kilogram(kg)]in 33 Sprague-Dawley *** pressure was regularly assessed during the 9 wk-experiment(weeks 0,3,5,and 7)in animals receiving CG(n=14)at a human equivalent dose(HED)of 1.5 g/d or 3.0 g/d and compared to negative control(tap water,n=11)and positive control(phloroglucinol at 1.5 g/d HED,n=8)*** anti-inflammatory effect of CG was evaluated using clinical and histological scores in 30 C57bl6 male mice with colitis induced by dextran sodium sulfate(DSS)administered in their drinking water during 14 ***-29 cells under basal conditions and after stimulation with lipopolysaccharide(lPS)were treated with CG to evaluate changes in pathways related to analgesia μ-opioid receptor(MOR),cannabinoid receptor 2(CB2),peroxisome proliferator-activated receptor alpha,inflammation[interl.ukin(Il)-10,Il-1b,and Il-8]and barrier function[mucin 2-5AC,cl.udin-2,zonula occludens(ZO)-1,ZO-2]using the real-time PCR *** modelling of CG,lPS,lipoteichoic acid(lTA),and phospholipomannan(PlM)was developed,and the abili

关键词： Chitin-glucan Irritable bowel syndrome Abdominal pain Inflammation Intestinal barrier Molecular modelling Microbial cell walls chelation

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Effect of indirect non-thermal plasma on particle size distribution and composition of diesel engine particles

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Plasma Science and Technology 2017年第11期19卷 59-66页

作者： linbo Gu yixi CAI Yunxi SHI Jing WANG Xiaoyu Pu Jing TIAN Runlin FAN School of Automotive and Traffic Engineering Jiangsu University Zhenjiang 212013 People＇s Republic of China

To explore the effect of the gas source flow rate on the actual diesel exhaust particulate matter（PM）, a test bench for diesel engine exhaust purification was constructed, using indirect nonthermal plasma technology. The effects of different gas source flow rates on the quantity concentration, composition, and apparent activation energy of PM were investigated, using an engine exhaust particle sizer and a thermo-gravimetric analyzer. The results show that when the gas source flow rate was large, not only the maximum peak quantity concentrations of particles had a large drop, but also the peak quantity concentrations shifted to smaller particle sizes from 100 nm to 80 nm. When the gas source flow rate was 10l min^-1, the total quantity concentration greatly decreased where the removal rate of particles was 79.2%, and the variation of the different mode particle proportion was obvious. Non-thermal plasma（NTP） improved the oxidation ability of volatile matter as well as that of solid carbon. However, the NTP gas source rate had little effects on oxidation activity of volatile matter, while it strongly influenced the oxidation activity of solid carbon. Considering the quantity concentration and oxidation activity of particles, a gas source flow rate of 10l min^-1 was more appropriate for the purification of particles.

关键词： diesel engine particulate matter non-thermal plasma gas source flow rate

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Focal distance tabu search

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Science China(Information Sciences) 2021年第5期64卷 5-16页

作者： Fred GlOVER Zhipeng lü Meta-Analytics Inc. School of Computer Science and Technology Huazhong University of Science and Technology

Focal distance tabu search modifies a standard tabu search algorithm for binary optimization by augmenting a periodic diversification step that drives the search away from a current best(or elite) solution until the objective function deteriorates beyond a specified threshold or until attaining a lower bound on the distance from the originating solution. The new augmented algorithm combines the threshold and lower bound approaches by introducing an initial focal distance for the lower bound which is updated when the diversification step is completed. However, rather than terminating the diversification step at the customary completion point, focal distance tabu search(TS) retains the focal distance bound through additional search phases designed to improve the objective function, drawing on a strategy proposed with strategic *** algorithm realizes this strategy by partitioning the variables into two sets which are managed together with an abbreviated tabu search process. An advanced version of the approach drives the search away from a collection of solutions rather than a single originating solution, introducing the concept of a signature solution to guide the search. The method can be employed to augment a variety of other metaheuristic algorithms such as those using threshold procedures, late acceptance hill climbing, iterated local search, breakout local search, GRASP, and path relinking.

关键词： tabu search diversification strategic oscillation adaptive partitioning metaheuristics

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