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Skill-assessments of statistical and Ensemble Kalman Filter data assimilative analyses using surface and deep observations in the Gulf of Mexico

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Frontiers of Earth Science 2013年第3期7卷 271-281页

作者： Zhibin SUN Lie-Yauw OEY yi-hui zhou Universities Space Research Association Columbia MD 21044 USA Princeton University AOS Sayre Hall Forrestal Campus Princeton NJ 08544 USA Department of Biostatistics University of North Carolina Chapel Hill NC 27599 USA

A new data assimilation algorithm （Quasi- EnKF） in ocean modeling, based on the Ensemble Kalman Filter scheme, is proposed in this paper. This algorithm assimilates not only surface measurements （sea surface height）, but also deep （-2000 m） temperature observations from the Gulf of Mexico into regional ocean models. With the use of the Princeton Ocean Model （POM）, integrated for approximately two years by assimilating both surface and deep observations, this new algorithm was compared to an existing assimilation algorithm （Mellor-Ezer Scheme） at different resolutions. The results show that, by comparing the observations, the new algorithm out-performs the existing one.

关键词： data assimilation deep observation Gulf of Mexico

A simple route for preparation of TRIP-assisted Si-Mn steel with excellent performance using direct strip casting

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International Journal of Minerals,Metallurgy and Materials 2024年第10期31卷 2173-2181页

作者： hui Xu Lejun zhou Wanlin Wang Yang yi School of Metallurgy and Environment Central South UniversityChangsha 410083China National Center for International Research of Clean Metallurgy Central South UniversityChangsha 410083China

The complex producing procedures and high energy-consuming limit the large-scale production and application of advanced high-strength steels(AHSSs).In this study,the direct strip casting(DSC)technology with unique sub-rapid solidification characteristics and cost advantages was applied to the production of low-alloy Si-Mn steel with the help of quenching&partitioning(Q&P)concept to address these *** this method with the conventional compact strip production(CSP)process,the initial microstructure formed under different solidification conditions and the influence of heat treatment processes on the final mechanical properties were *** results show that the initial structure of the DSC sample is a dual-phase structure composed of fine lath martensite and bainite,while the initial structure of the CSP sample consists of pearlite and *** volume fraction and carbon content of retained austenite(RA)in DSC samples are usually higher than those in CSP samples after the same Q&P *** samples typically demonstrate better comprehensive mechanical properties than the CSP *** DSC sample partitioned at 300℃ for 300 s(DSC-Pt300)achieves the best comprehensive mechanical properties,with yield strength(YS)of 1282 MPa,ultimate tensile strength(UTS)of 1501 MPa,total elongation(TE)of 21.5%,and product of strength and elongation(PSE)as high as 32.3 GPa·%.These results indicate that the excellent mechanical properties in low-alloy Si-Mn steel can be obtained through a simple process(DSC-Q&P),which also demonstrates the superiority of DSC technology in manufacturing AHSSs.

关键词： direct strip casting sub-rapid solidification quenching and partitioning TRIP-assisted AHSSs microstructure

Variations and future projections of glacial discharge of Urumqi River Headwaters,eastern Tien Shan(1980s-2017)

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Advances in Climate Change Research 2024年第3期15卷 537-546页

作者： hui ZHANG Fei-Teng WANG Ping zhou yi-Da XIE State Key Laboratory of Cryospheric Science Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China Key Laboratory of Cryospheric Science and Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China

To address data scarcity on long-term glacial discharge and inadequacies in simulating and predicting hydrological processes in the Tien Shan,this study analysed the observed discharge at multiple timescales over 1980se2017 and projected changes within a representative glacierized high-mountain region:eastern Tien Shan,Central *** processes were simulated to predict changes under four future scenarios(SSP1,SSP2,SSP3,and SSP5)using a classical hydrological model coupled with a glacier dynamics *** rates at annual,monthly(June,July,August)and daily timescales were obtained from two hydrological gauges:Urumqi Glacier No.1 hydrological station(UGH)and Zongkong station(ZK).Overall,annual and summer discharge increased significantly(p<0.05)at both stations over the study *** intra-annual variations mainly resulted from differences in their recharge *** simulations show that a tipping point in annual discharge at UGH may occur between 2018 and 2024 under the four SSPs *** discharge is predicted to cease earlier at ZK than at *** relates to glacier type and size,suggesting basins with heavily developed small glaciers will reach peak discharge sooner,resulting in an earlier freshwater supply *** findings serve as a reference for research into glacial runoff in Central Asia and provide a decision-making basis for planning local water-resource projects.

关键词： Observed glacial discharge Temporal variations Urumqi River Headwaters Eastern Tien Shan Simulation and projection

Upcycling municipal solid waste to sustainable hydrogen via two-stage gasification-reforming

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Journal of Energy Chemistry 2024年第9期96卷 611-624页

作者： hui zhou Shuzhuang Sun yikai Xu Yeshui Zhang Shouliang yi Chunfei Wu Department of Energy and Power Engineering Tsinghua UniversityBeijing 100084China School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001HenanChina Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center Frontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China School of Engineering University of AberdeenAberdeen AB243UEUK U.S.Department of Energy National Energy Technology LaboratoryPittsburghPA 15236USA School of Chemistry and Chemical Engineering Queen’s University BelfastBelfast BT71NNUK

As global municipal solid waste(MSW)quantities continue to escalate,serious socio-environmental challenges arise,necessitating innovative ***-to-hydrogen(WTH)via two-stage gasification-reforming(TSGR)presents an emergent technology for MSW upcycling,offering to ease waste management burdens and bolster the burgeoning hydrogen *** early initiatives to advance TSGR technology,a cohesive and critical analysis of cutting-edge knowledge and strategies to enhance hydrogen production remains *** review aggregates literature on MSW upcycling to hydrogen via TSGR,with a focus on optimizing process control and catalytic *** underscores technological avenues to augment hydrogen output,curtail catalyst costs,and refine system ***,the review illuminates the potential for integrating chemical and calcium looping into TSGR processes,identifying opportunities,and pinpointing *** review concludes with a summary of the current state of techno-economic analysis for this technology,presenting outstanding challenges and future research directions,with the ultimate goal of transitioning WTH from theoretical to practical application.

关键词： Municipal solidwaste Upcycling Gasification Reforming Hydrogen

Construction of ZnO@CDs@Co_(3)O_(4) sandwich heterostructure with multi-interfacial electron-transfer toward enhanced photocatalytic CO_(2) reduction

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Chinese Chemical Letters 2024年第4期35卷 147-152页

作者： Xiuzheng Deng yi Ke Jiawen Ding yingtang zhou hui Huang Qian Liang Zhenhui Kang Advanced Catalysis and Green Manufacturing Collaborative Innovation Center CNPC-CZU Innovation AllianceSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316004China

Photocatalytic conversion of CO_(2) into small-molecule chemical feedstocks can meet the growing demand for energy and alleviate the global warming. Herein, a p-n ZnO@CDs@Co_(3)O_(4) heterojunction with sandwich structure was constructed by calcination method of self-assembled ZIF-8@CDs@ZIF-67. The ZnO@CDs@Co_(3)O_(4) with well-defined interfacial structure exhibited the significantly enhanced photocatalytic CO_(2) reduction activity, and the optimal catalyst indicated the(CO + CH_(4)) evolution rate of 214.53μmol g^(-1)h^(-1) under simulated solar light, which was superior to ZnO, Co_(3)O_(4) and binary ZnO@Co_(3)O_(4).The internal cavity, exposed active sites, multiple interfaces and constructed p-n heterojunction can facilitate the light harvesting and photoexcited electron transfer. Besides, after introduction of CDs placed in the middle layer between ZnO and Co_(3)O_(4), CDs with excellent photoelectric property further promoted charge separation and migration. This work represents an appealing strategy to construct well-defined photocatalysts for boosting CO_(2) photoreduction.

关键词： Metal-organic framework Photocatalytic CO_(2) reduction Carbon dots p-n heterojunction Sandwich heterostructure

Effect of forging on the microstructure and texture of a high Nb containing γ-TiAl alloy

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Journal of Central South University 2024年第6期31卷 1763-1773页

作者： TAO hui LI hui-zhong WANG Li zhou Rui CHE yi-xuan CHEN Yong-hui LIANG Xiao-peng School of Materials Science and Engineering Central South UniversityChangsha 410083China State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China Key Laboratory of Nonferrous Metal Materials Science and Engineering Central South UniversityChangsha 410083China Department of Materials Science and Engineering City University of Hong KongKowloon 999077Hong KongChina

The effect of forging on the microstructure and texture evolution of a high Nb containing Ti-45Al-7Nb-0.3W(at.%)alloy was investigated by X-ray diffractometer(XRD),scanning electron microscopy(SEM),and transmission electron microscopy(TEM).The results show that the as-cast alloy is mainly composed of α_(2)/γ lamellar colonies with a mean size of 70μm,but the hot-forged pancake displays a near duplex microstructure(DP).Kinking and bending of lamellar colonies,deformation twinning and dynamic recrystallization(DRX)occur during hot ***,dense dislocations in theβphase after forging suggest that the high-temperature β phase with a disordered structure is favorable for improving the hot-workability of the *** the common TiAl casting texture,the solidification process of the investigated as-cast alloy with high Nb content is completely via the β phase region,resulting in the formation of aγ fiber texture where theγ aligns parallel to the heat-flow *** comparison,the relatively strongand weaktexture components in the as-forged alloy are attributed to the deformation *** annealing,static recrystallization occurs at the twin boundary and intersections,which weakens the deformation texture.

关键词： high Nb containingγ-TiAl alloy forging microstructure texture βphase

An Experimental Study on the Effect of a Nanofluid on Oil-Water Relative Permeability

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Fluid Dynamics & Materials Processing 2024年第6期20卷 1265-1277页

作者： hui Tian Dandan Zhao Yannan Wu Xingyu yi Jun Ma Xiang zhou Baikouquan Oil Production Plant PetroChina Xinjiang Oilfield CompanyKaramay834000China Research Institute of Petroleum Exploration Development PetroChina Liaohe OilfieldPanjin124010China Petroleum Engineering School Southwest Petroleum UniversityChengdu610500China Oil and Gas Development Haosheng Xincheng Energy TechnologyLtd.of SicuanChengdu610213China

The low porosity and low permeability of tight oil reservoirs call for improvements in the current technologies for oil *** chemical solutions with large molecular size cannot effectively flow through the nanopores of the *** this study,the feasibility of Nanofluids has been investigated using a high pressure high temperature core-holder and nuclear magnetic resonance(NMR).The results of the experiments indicate that the specified Nanofluids can enhance the tight oil recovery *** water and oil relative permeability curve shifts to the high water saturation side after Nanofluid flooding,thereby demonstrating an increase in the water wettability of the *** the Nanofluid flooding process the oil recovery was enhanced by 15.1%,compared to waterflooding *** T2 spectra using the NMR show that after Nanofluid flooding,a 7.18%increment in oil recovery factor was gained in the small pores,a 4.9%increase in the middle pores,and a 0.29%increase in the large *** results confirm that the Nanofluids can improve the flow state in micro-sized pores inside the core and increase the ultimate oil recovery factor.

关键词： Tight oil reservoir nanofluid relative permeability nuclear magnetic resonance T2 spectrum

Oxidation of emerging organic contaminants by in-situ H_(2)O_(2) fenton system

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Green Energy & Environment 2024年第3期9卷 417-434页

作者： Yuqin Ni Chuxiang zhou Mingyang Xing yi zhou State Environmental Protection Key Lab of Environmental Risk Assessment and Control on Chemical Processes School of Resources&Environmental EngineeringEast China University of Science and TechnologyShanghai200237China Key Laboratory for Advanced Materials and Institute of Fine Chemicals National Engineering Laboratory for Industrial Wastewater TreatmentSchool of Chemistry and Molecular EngineeringEast China University of Science and Technology130 Meilong RoadShanghai200237China Department of Applied Natural Sciences Technische Hochschule LubeckMonkhofer Weg 23923562 LubeckGermany

The existence and risk of emerging organic contaminants(EOCs)have been under consideration and paid much effort to degrade these *** system is one of the most widely used technologies to solve this *** original Fenton system relies on the hydroxyl radicals produced by Fe(Ⅱ)/H_(2)O_(2) to oxidize the organic ***,the application of the Fenton system is limited by its low iron cycling efficiency and the high risks of hydrogen peroxide transportation and *** introduction of external energy(including light and electricity etc.)can effectively promote the Fe(Ⅲ)/Fe(Ⅱ)cycle and the reduction of oxygen to produce hydrogen peroxide in *** review introduces three in-situ Fenton systems,which are electro-Fenton,Photo-Fenton,and chemical *** mechanism,influencing factors,and catalysts of these three in-situ Fenton systems in degrading EOCs are discussed *** review strengthens the understanding of Fenton and in-situ Fenton systems in degradation,offering further insight into the real application of the in-situ Fenton system in the removal of EOCs.

关键词： In-situ H_(2)O_(2)production Fenton Emerging organic contaminants Photocatalysis Electrocatalysis

Stabilization/solidification mechanisms of tin tailings and fuming slag-based geopolymers for different heavy metals

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Frontiers of Environmental Science & Engineering 2024年第5期18卷 43-55页

作者： Xian zhou Zhengfu Zhang hui Yang School of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China Kunming Metallurgical Research Institute Co. Ltd.Kunming650031China

Tin mine tailings(TMT)and fuming slag(FS)contain many heavy metals(As,Cr,Cu,Zn and Mn)that cause severe pollution to the ***,geopolymers were prepared using TMT,FS and flue gas desulfurization gypsum(FGDG)to immobilize heavy metals,and their compressive strength and heavy metal leaching toxicity were *** was first determined that T4F5(TMT:FS=4:5)sample exhibited the highest compressive strength(7.83 MPa).T4F5 achieved 95%immobilization efficiency for As and Cr,and nearly 100%for Cu,Zn and Mn,showing good immobilization performance.A series of characterization analyses showed that heavy metal cations can balance the charge in the geopolymer and replace Al in the geopolymer structure to form covalent *** addition,about 2%–20%of heavy metal Fe was immobilized in hydration products,heavy metal hydroxides and non-bridging Si–O and Al–O coordination with silica-aluminate ***_(3)^(3−) was oxidized into AsO_(4)^(3−),which may form Ca–As or Fe–As ***_(2)O_(7)^(2−)was converted to CrO_(4)^(2−)under alkaline environment and then combined with OH−to form Cr(OH)3 ***^(2+)may react directly with dissolved silicate to form Mn_(2)SiO_(4) and also form Mn(OH)_(2) *** unstable Mn(OH)_(2) can be further oxidized to MnO_(2).The heavy metal cations were immobilized in the silicoaluminate lattice,while the anions tended to form insoluble *** results may benefit the industry and government for better handling of TMT,FS and solid wastes containing the abovementioned five heavy metals.

关键词： Heavy metals Cementitious materials Tin tailings Stabilization/solidification Redox