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Nanosheet-coated synthetic wood with enhanced flame-retardancy by vacuum-assisted sonocoating technique

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Nano Research 2022年第10期15卷 9440-9446页

作者： Zhi-Yuan Ma Xiao-Feng Pan Ze-Lai Xu Zhi-Long Yu Bing Qin yi-chen yin Yu-cheng Gao Shu-Hong Yu Department of Chemistry Institute of Biomimetic Materials&ChemistryAnhui Engineering Laboratory of Biomimetic MaterialsDivision of Nanomaterials&ChemistryHefei National Laboratory for Physical Sciences at the MicroscaleInstitute of EnergyHefei Comprehensive National Science CenterUniversity of Science and Technology of ChinaHefei 230026China Department of Modern Mechanics University of Science and Technology of ChinaHefei 230027China

Compared to natural woods,synthetic woods have superior mechanical stability,thermal insulation,and flame retardancy owing to their hierarchically cellular microstructures and intrinsic advantages of the thermosetting *** the long-time fire resistance is very important to the practical *** this study,we present a novel coating strategy by a vacuum-assisted sonication technique(sonocoating)with a rectorite nanosheet dispersion to create a uniform nanocoating on the channel walls of synthetic *** to ultrasonic energy and vacuum pressure,the nanosheet dispersion can penetrate deep down to form a layered nanocoating on the channel *** coated synthetic woods can withstand fire(400-600℃)for more than 10 min with 62%mass retainment,surpassing uncoated synthetic woods and natural ***,as a lightweight and strong composite with enhanced flame-retardant performance,the coated synthetic woods have huge potential applications in safe and energy-efficient buildings.

关键词： synthetic wood sonocoating vacuum infiltration rectorite nanosheets flame-retardant

Bio-inspired low-tortuosity carbon host for high-performance lithium-metal anode

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National Science Review 2019年第2期6卷 247-256页

作者： yi-chen yin Zhi-Long Yu Zhi-Yuan Ma Tian-Wen Zhang Yu-Yang Lu Tao Ma Fei Zhou Hong-Bin Yao Shu-Hong Yu Department of Chemistry CAS Center for Excellence in Nanoscience Hefei Science Center of CAS University of Science and Technology of China Hefei National Laboratory for Physical Sciences at the Microscale University of Science and Technology of China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of China

Lithium metal is one of the most promising anode materials for high-energy-density Li batteries. However,low stability caused by dendrite growth and volume change during cycling hinders its practical ***, we report an ingenious design of bio-inspired low-tortuosity carbon with tunable vertical micro-channels to be used as a host to incorporate nanosized Sn/Ni alloy nucleation sites, which can guide Li metal’s plating/stripping and meanwhile accommodate the volume change. The pore sizes of the vertical channels of the carbon host can be regulated to investigate the structure–performance correlation. After compositing Li, the bio-inspired carbon host with the smallest pore size（～14 μm） of vertical channels exhibits the lowest overpotential(～18 mV at 1 mA cm;), most stable tripping/plating voltage profiles,and best cycling stability（up to 500 cycles） in symmetrical cells. Notably, the carbon/Li composite anode is more rewarding than Li foil when coupled with LiFePO;in full cells, exhibiting a much lower polarization effect, better rate capability and higher capacity retention（90.6% after 120 cycles）. This novel bio-inspired design of a low-tortuosity carbon host with nanoalloy coatings may open a new avenue for fabricating advanced Li-metal batteries with high performance.

关键词： bio-inspiration low-tortuosity carbon host lithium metal micro-channels nucleation sites

Expression of hepatitis B virus surface antigens induces defective gonad phenotypes in Caenorhabditis elegans

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World Journal of Virology 2017年第1期6卷 17-25页

作者： yi-yin chen Li-Wei Lee Wei-Ning Hong Szecheng J Lo Department of Biomedical Science College of Medicine Chang Gung University Graduate Institute of Biomedical Science College of Medicine Chang Gung University

AIM To test whether a simple animal, Caenorhabditis elegans(C. elegans), can be used as an alternative model to study the interaction between hepatitis B virus antigens(HBs Ag) and host factors. METHODS Three plasmids that were able to express the large, middle and small forms of HBs Ags(LHBs Ag, MHBs Ag, and SHBs Ag, respectively) driven by a ubiquitous promoter(fib-1) and three that were able to express SHBs Ag driven by different tissue-specific promoters were constructed and microinjected into worms. The brood size, egglaying rate, and gonad development of transgenic worms were analyzed using microscopy. Levels of m RNA related to endoplasmic reticulum stress, enpl-1, hsp-4, pdi-3 and xbp-1, were determined using reverse transcription polymerase reaction(RT-PCRs) in three lines of transgenic worms and dithiothreitol(DTT)-treated wild-type worms. RESULTS Severe defects in egg-laying, decreases in brood size, and gonad retardation were observed in transgenic worms expressing SHBs Ag whereas moderate defects were observed in transgenic worms expressing LHBs Ag and MHBs Ag. RT-PCR analysis revealed that enpl-1, hsp-4 and pdi-3 transcripts were significantly elevated in worms expressing LHBs Ag and MHBs Ag and in wild-type worms pretreated with DTT. By contrast, only pdi-3 was increased in worms expressing SHBs Ag. To further determine which tissue expressing SHBs Ag could induce gonad retardation, we substituted the fib-1 promoter with three tissue-specific promoters(myo-2 for the pharynx, est-1 for the intestines and mec-7 for the neurons) and generated corresponding transgenic animals. Moderate defective phenotypes were observed in worms expressing SHBs Ag in the pharynx and intestines but not in worms expressing SHBs Ag in the neurons, suggesting that the secreted SHBs Ag may trigger a cross-talk signal between the digestive track and the gonad resulting in defective phenotypes. CONCLUSION Ectopic expression of three forms of HBs Ag that causes recognizable pheno

关键词： Hepatitis B virus Caenorhabditis elegans Green fluorescence proteins Endoplasmic reticulum stress Gonad retardation Surface antigens

CsPbI_(2)Br epitaxial shell for efficient PbS quantum dot solar cells

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Nano Research 2024年第12期17卷 10302-10308页

作者： Sami Ur Rahman Yong-Hui Song Zhen-Yu Ma Xiao-Lin Tai Bai-Sheng Zhu yi-chen yin Li-Zhe Feng Jing-Ming Hao Guan-Jie Ding Kuang-Hui Song Ya-Lan Hu Tieqiang Li Jixian Xu Hong-Bin Yao Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China Department of Applied Chemistry University of Science and Technology of ChinaHefei 230026China Department of Material Science and Engineering University of Science and Technology of ChinaHefei 230026China

Lead sulfide quantum dots(PbS QDs)are promising candidates for high-performance solar cells due to their tunable bandgaps and low-cost solution ***,low carrier mobility and numerous surface defects restrict the performance of the fabricated solar ***,we report the synthesis of novel PbS-perovskite core-shell QDs to solve the low carrier mobility problem of PbS QDs via a facile hot injection ***_(2)Br shell enabled strain-free epitaxial growth on the surface of PbS QDs because of 98%lattice *** results demonstrate a significant improvement in the photoluminescence and stability of the synthesized PbS-CsPbI_(2)Br QDs upon shell formation,attributed to the effective suppression of surface defects by the epitaxial shell of CsPbI_(2)*** a result,the obtained solar cell based on PbS-CsPbI_(2)Br core-shell QD exhibits a power conversion efficiency(PCE)of 8.43%,two times higher than that of pristine PbS ***,the construction of PbS-CsPbI_(2)Br core-shell structures represent a promising strategy for advancing the performance of PbS QDs-based optoelectronic devices.

关键词： lead chalcogenide perovskites core-shell epitaxial growth solar cell

Low cost and low density chloride solid electrolyte for all solid state cathode with high active material ratio

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Nano Research 2024年第10期17卷 8826-8833页

作者： Hao-Yuan Tan Mei-Yu Zhou Zhongyuan Huang Jin-Da Luo Jing-Tian Yang Jian-Ping Wang Ye-Chao Wu Xiao-Bin cheng Zi-Wei Wang Xu-Dong Hao Linjun Wang Ke Gong yi-chen yin yinguo Xiao Hong-Bin Yao Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China Department of Applied Chemistry University of Science and Technology of ChinaHefei 230026China School of Advanced Materials Peking University Shenzhen Graduate SchoolShenzhen 518055China

Chloride solid electrolytes(SEs)have attracted widespread attention due to their high room-temperature ionic conductivity and excellent cathode ***,the conventionally selected central metal elements(e.g.,In,Y and Ta)are usually rare and heavy,inevitably causing the high cost and high density of the obtained chloride ***,by choosing abundant and light Mg and Al as central metal elements,we develop a cheap and low density Li_(1.2)Mg_(0.95)Al_(0.3)Cl_(4)SE for high active material ratio in all solid state *** replacement of Mg^(2+)by Al^(3+)in the framework yields vacancies and lowers the non-lithium metal ions occupancy at Mg/Li co-occupied 16d site,effectively relieving the blocking effects by Mg^(2+)in the pristine spinel Li_(2-2x)Mg_(1+x)Cl_(4).Thus,a significantly improved room-temperature conductivity of 3.08×10^(-4)S·cm^(-1)is achieved,two orders of magnitude higher than that of Li_(1.2)Mg_(1.4)Cl_(4).More attractively,its low density of only 1.98 g·cm-3 enables low SE mass ratio in cathodes(only 16 wt.%)with still effective electrolyte/cathode contact and lithium-ion conduction *** charged to potential of 4.30 V,the asfabricated Li_(1.2)Mg_(0.95)Al_(0.3)Cl_(4)-based solid lithium battery with uncoated NCM523 cathode can be cycled for over 100 cycles with a capacity retention of 86.68%at room temperature.

关键词： chloride solid electrolytes low cost low density Li+conductivities

Lipase and pancreatic amylase activities in diagnosis of acute pancreatitis in patients with hyperamylasemia

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Hepatobiliary & Pancreatic Diseases International 2005年第4期4卷 600-603页

作者： Rong-Wei Yang, Zhe-Xin Shao, yi-yi chen, Zhou yin and Wen-Juan Wang Clinical Laboratory, First Affiliated Hospital, Zhejiang University School of Medicine, Hangzhou 310003, China and Clinical Laboratory, Zhejiang Xinhua Hospital, Hangzhou 310003 , China Clinical Laboratory First Affiliated Hospital Zhejiang University School of Medicine Hangzhou 310003 China.

BACKGROUND: Measurement of total serum amylase (AMY) is the most widely used biochemical test for the diagnosis of acute pancreatitis, but it is commonly considered a nonspecific marker. To improve the biochemical diagnosis of acute pancreatitis, lipase ( LIP ) and pancreatic amylase (PAMY) have been tested in recent years. The present study was designed to evaluate whether serum LIP and pancreatic PAMY tests could replace total amylase test to improve diagnostic efficiency in the evaluation of acute pancreatitis in patients with hyperamylasemia. METHODS: LIP and PAMY values were determined in serum samples from 92 patients with hyperamylasemia. Reference values for each enzyme were derived from serum samples of 147 healthy subjects. The activities of LIP and PAMY in patients with various diseases were shown directly by the boxplot graph. The diagnostic accuracy of LIP and PAMY was defined as the area under the receiver operating characteristic (ROC) curve. Their sensitivity and specificity in detecting acute pancreatitis at varying cutoff points were shown by the curve, and the best cutoff value for each enzyme was shown by the modified ROC curve. The diagnostic values of LIP, PAMY and LIP + AMY with each upper limit of reference range (ULR) were compared with the corresponding best cutoff values. RESULTS: The references values of LIP and PAMY were 12.2-47.6 U/L and 28-95 U/L, respectively. These values in patients with acute pancreatitis were higher than those patients with other diseases. The areas under the ROC curve ( AUC) of LIP and PAMY were 0. 799 and 0. 792, respectively, With the best diagnostic cutoff point of maximum (sensitivity + specificity) -100%, we obtained values of 97.9 U/L(LIP97.9 =2. 06 × ULR) for LIP and 209 U/L (PAMY209 =2.20 ×ULR) for PAMY. The best cutoff values for LIP, PAMY and LIP +AMY demonstrated the specificity, positive predictive value, and diagnostic efficiency higher than the corresponding ULRs. CONCLUSIONS: Serum LIP and PAMY are

关键词： pancreatic injury lipase pancreatic amylase

水氮耦合对烤烟生育期内土壤酶活性动态变化的影响

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华北农学报 2011年第5期26卷 159-163页

作者：刘美玉陈益银习向银陈亚西南大学资源环境学院重庆400715 酉阳烟草分公司重庆409800 雅安市农业局四川雅安625000

在网室盆栽条件下,采用3水平灌水量(40,60,80 L/株)×4水平施氮量(0,3,7,12 g/株),以烤烟K326为试验材料,研究了水氮耦合对烤烟生育期内土壤过氧化氢酶、蔗糖酶、脲酶和酸性磷酸酶活性动态变化的影响。结果表明,植烟土壤4种酶活性随生... 详细信息

在网室盆栽条件下,采用3水平灌水量(40,60,80 L/株)×4水平施氮量(0,3,7,12 g/株),以烤烟K326为试验材料,研究了水氮耦合对烤烟生育期内土壤过氧化氢酶、蔗糖酶、脲酶和酸性磷酸酶活性动态变化的影响。结果表明,植烟土壤4种酶活性随生育时期推进均呈先上升后下降的趋势,且在旺长期或现蕾期达最高。在相同生育时期和相同灌水水平下,随着施氮水平的提高,植烟土壤过氧化氢酶、蔗糖酶和酸性磷酸酶活性均呈先增加后降低的变化趋势,且过氧化氢酶和蔗糖酶以3 g/株施氮水平下活性最高,酸性磷酸酶活性以7 g/株施氮水平达最高;而脲酶活性则随着施氮量的增加而增加,在12 g/株施氮水平下达最高。在相同生育时期和相同施氮量下,以灌水处理为60L/株和80 L/株的植烟土壤4种酶活性均较高,而低灌水处理(40 L/株)的土壤酶活性均较低。综合所有指标,在该试验条件下,当灌水量为60～80 L/株、施氮量3～7 g/株,烤烟生育期内4种土壤酶均保持较高的活性。

关键词：水氮耦合烤烟酶活性

Electrocatalytic cleavage of a lignin β-O-4 model compound and coupling with nitrogen-containing aromatics using Prussian blue analogue-derived nickel–cobalt spinel

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Journal of Energy Chemistry 2025年第1期100卷 628-636页

作者： yi Qi Xueying chen Bowen Liu Xuliang Lin Xueqing Qiu Yanlin Qin Guangdong Provincial Key Laboratory of Plant Resources Biorefinery School of Chemical Engineering and Light Industry Guangdong University of Technology Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center Guangdong Basic Research Center of Excellence for Ecological Security and Green Development Guangdong University of Technology

Electrochemical conversion of lignin for the production of high-value heterocyclic aromatic compounds has great *** demonstrate the targeted synthesis and cation modulation of NiCo2O4spinel nanoboxes,synthesized via cation exchange and calcination *** catalysts exhibit excellent efficacy in the electrocatalytic conversion of lignin model compounds,specifically 2-phenoxy-1-phenylethanol,into nitrogen-containing aromatics,achieving high conversion rates and *** catalysts were synthesized via a cation exchange and calcination oxidation process,using Prussian blue nanocubes as *** porous architecture and polymetallic composition of the NiCo2O4spinel demonstrated superior performance in electrocatalytic oxidative coupling,achieving a 99.2 wt%conversion rate of the 2-phenoxy-1-phenylethanol with selectivities of 37.5 wt%for quinoline derivatives and 31.5 wt%for *** innovations include the development of a sustainable one-pot synthesis method for quinoline derivatives,the elucidation of a multistage reaction pathway involving CAO bond cleavage,hydroxyaldol condensation,and CAN bond formation,and a deeper mechanistic understanding derived from DFT *** work establishes a new strategy for lignin valorization,offering a sustainable route to produce high-value nitrogen-containing aromatics from renewable biomass under mild conditions,without the need for additional reagents.

关键词： Spinel Biomass valorization Electrocatalysis Lignin oxidation Coupling

Unleashing the Potential of Electroactive Hybrid Biomaterials and Self‑Powered Systems for Bone Therapeutics

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Nano-Micro Letters 2025年第2期17卷 463-497页

作者： Shichang Liu Farid Manshaii Jinmiao chen Xinfei Wang Shaolei Wang Junyi yin Ming Yang Xuxu chen Xinhua yin Yunlei Zhou Honghui Hospital Xi’an Jiaotong UniversityXi’an 710018People’s Republic of China Department of Bioengineering Henry Samueli School of Engineering and Applied ScienceUniversity of California Los AngelesLos Angeles 90095USA Hangzhou Institute of Technology Xidian UniversityHangzhou 311231People’s Republic of China

The incidence of large bone defects caused by traumatic injury is increasing worldwide,and the tissue regeneration process requires a long recovery time due to limited self-healing *** bioelectrical phenomena have been well recognized as critical biophysical factors in bone remodeling and *** by bioelectricity,electrical stimulation has been widely considered an external intervention to induce the osteogenic lineage of cells and enhance the synthesis of the extracellular matrix,thereby accelerating bone *** ongoing advances in biomaterials and energy-harvesting techniques,electroactive biomaterials and self-powered systems have been considered biomimetic approaches to ensure functional recovery by recapitulating the natural electrophysiological microenvironment of healthy bone *** this review,we first introduce the role of bioelectricity and the endogenous electric field in bone tissue and summarize different techniques to electrically stimulate cells and ***,we highlight the latest progress in exploring electroactive hybrid biomaterials as well as self-powered systems such as triboelectric and piezoelectric-based nanogenerators and photovoltaic cell-based devices and their implementation in bone tissue ***,we emphasize the significance of simulating the target tissue’s electrophysiological microenvironment and propose the opportunities and challenges faced by electroactive hybrid biomaterials and self-powered bioelectronics for bone repair strategies.

关键词： Electroactive biomaterials Self-powered bioelectronics Bone regeneration Bone tissue