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Atmospheric fate of typical liquid crystal monomers in the tropospheric gas,liquid,and granular phases

Journal of Environmental Sciences 2024年第2期136卷 348-360页

作者： yanru huo Zexiu An Mingxue Li Jinchan Jiang Yuxin Zhou Ju Xie Jianguo Zhang Maoxia He Environment Research Institute Shandong UniversityQingdao 266237China College of Plant Protection Hebei Agricultural UniversityBaoding 071000China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225002China Jinan Environmental Research Academy Jinan 250000China

Mineral aerosol particles significantly impact environmental risk prediction of liquid crystal monomers(LCMs).In this work,we investigated the reaction mechanisms and kinetics of three typical LCMs(4-cyano-3,5-difluorophenyl 4-ethylbenzoate(CEB-2F),4-cyano-3-fluorophenyl 4-ethylbenzoate(CEB-F),and 4-cyanophenyl 4-ethylbenzoate(CEB))with ozone(O_(3))in the atmospheric gas,liquid,and particle phases employing density functional theory(DFT).Here,O_(3)is prone to add to the benzene ring without F atom(s)in the selected LCMs.The ozonolysis products are aldehydes,carboxylic acids,epoxides,and unsaturated hydrocarbons containing aromatic rings.Those products undergo secondary ozonolysis to generate small molecular compounds such as glyoxal,which is beneficial for generating secondary organic aerosol(SOA).Titanium dioxide(TiO_(2)),an essential component of mineral aerosol particles,has good adsorption properties for LCMs;however,it slightly reduces the reactivity with O_(3).At 298 K,the reaction rate constant of the selected LCMs reacting with O_(3)in the gas and atmospheric liquid phases is(2.74–5.53)×10^(-24)cm^(3)/(mol·sec)and 5.58×10^(-3)–39.1 L/(mol·sec),while CEB-2F reacting with O_(3)on(TiO_(2))_(6)cluster is 1.84×10^(-24)cm^(3)/(mol·sec).The existence of TiO_(2)clusters increases the persistence and long-distance transportability of LCMs,which enlarges the contaminated area of LCMs.

关键词： Liquid crystal monomers(LCMs) Ozonolysis TiO_(2)clusters Adsorption Toxicity assessment

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Introduction to a recently released dataset entitled CSNCD:A Comprehensive Dataset of Chinese Seismic Network

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Earthquake Research Advances 2024年第1期4卷 1-3页

作者： yanru An China Earthquake Networks Center Beijing 100045China

China and its adjacent regions are heavily affected by earthquake disasters,which has led to strong demand and vigorous development of the Chinese Seismic Network(CSN).Since 2004,China Earthquake Networks Center(CENC)has been authorized by China Earthquake Administration(CEA)to take charge of CSN management,mainly observing product output and quality control.

关键词： Seismic Earthquake earthquake

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Sawtooth-enhanced bend sensor for gesture recognition

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Science China Technological Sciences 2024年第6期67卷 1727-1736页

作者： BAI yanru ZHANG ZiHang WANG HaoYu GUO Rui LI XiSheng School of Automation and Electrical Engineering University of Science and Technology Beijing School of Advanced Engineering University of Science and Technology Beijing School of Precision Instrument and Opto-Electronics Engineering Tianjin University School of Computer and Communication Engineering University of Science and Technology Beijing

Gesture recognition has diverse application prospects in the field of human-computer interaction. Recently, gesture recognition devices based on strain sensors have achieved remarkable results, among which liquid metal materials have considerable advantages due to their high tensile strength and conductivity. To improve the detection sensitivity of liquid metal strain sensors,a sawtooth-enhanced bending sensor is proposed in this study. Compared with the results from previous studies, the bending sensor shows enhanced resistance variation. In addition, combined with machine learning algorithms, a gesture recognition glove based on the sawtooth-enhanced bending sensor is also fabricated in this study, and various gestures are accurately identified. In the fields of human-computer interaction, wearable sensing, and medical health, the sawtooth-enhanced bending sensor shows great potential and can have wide application prospects.

关键词： liquid metal bending sensor gesture recognition machine learning

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Strain engineering of Pt-based electrocatalysts for oxygen reaction reduction

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Frontiers in Energy 2024年第2期18卷 241-262页

作者： Zeyu WANG yanru LIU Shun CHEN Yun ZHENG Xiaogang FU Yan ZHANG Wanglei WANG State Key Laboratory of Solidification Processing Atomic Control and Catalysis Engineering LaboratorySchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China State Key Laboratory of Oral and Maxillofacial Reconstruction and Regeneration National Clinical Research Center for Oral DiseasesShaanxi Key Laboratory of StomatologyDepartment of Dental MaterialsSchool of StomatologyThe Fourth Military Medical UniversityXi’an 710032China Institute of New Energy Materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China Key Laboratory of Marine Chemistry Theory and Technology(Ministry of Education) College of Chemistry and Chemical EngineeringOcean University of ChinaQingdao 266100China

Proton exchange membrane fuel cells(PEMFCs)are playing irreplaceable roles in the construction of the future sustainable energy system.However,the insufficient performance of platinum(Pt)-based electrocatalysts for oxygen reduction reaction(ORR)hinders the overall efficiency of PEMFCs.Engineering the surface strain of catalysts is considered an effective way to tune their electronic structures and therefore optimize catalytic behavior.In this paper,insights into strain engineering for improving Pt-based catalysts toward ORR are elaborated in detail.First,recent advances in understanding the strain effects on ORR catalysts are comprehensively discussed.Then,strain engineering methodologies for adjusting Ptbased catalysts are comprehensively discussed.Finally,further information on the various challenges and potential prospects for strain modulation of Pt-based catalysts is provided.

关键词： strain engineering Pt-based catalysts oxygen reduction reaction(ORR) catalytic performance proton exchange membrane fuel cells(PEMFCs)

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Mussel-inspired Methacrylic Gelatin-dopamine/Ag Nanoparticles/Graphene Oxide Hydrogels with Improved Adhesive and Antibacterial Properties for Applications as Wound Dressings

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Journal of Wuhan University of Technology(Materials Science) 2024年第2期39卷 512-521页

作者：宿正楠 HU yanru MENG Lihui OUYANG Zhiyuan LI Wenchao ZHU Fang XIE Bin 吴庆知 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Biomedical Material and Engineering Center of Hubei ProvinceWuhan University of TechnologyWuhan 430070China

A novel strategy was developed to prepare the methacrylic gelatin-dopamine(GelMA-DA)/Ag nanoparticles(NPs)/graphene oxide(GO) composite hydrogels with good biocompatibility,mechanical properties,and antibacterial activity.Mussel-inspired DA was utilized to modify the GelMA molecules,which imparts good adhesive performance to the hydrogels.GO,interfacial enhancer,not only improves mechanical properties of the hydrogels,but also provides anchor sites for loading Ag NPs through numerous oxygencontaining functional groups on the surface.The experimental results show that the GelMA/Ag NPs/GO hydrogels have good biocompatibility,and exhibit a swelling rate of 202±16%,the lap shear strength of 147±17 kPa,and compressive modulus of 136±53 kPa,in the case of the Ag NPs/GO content of 2 mg/mL.Antibacterial activity of the hydrogels against both gram-negative and gram-positive bacteria is dependent on the Ag NPs/GO content derived from the release of Ag^(+).Furthermore,the GelMA/Ag NPs/GO hydrogels possess good adhesive ability,which is resistant to highly twisted state when stuck on the surface of pigskin.These results demonstrate promising potential of the GelMA-DA/Ag NPs/GO hydrogels as wound dressings for biomedical applications in clinical and emergent treatment.

关键词： GelMA dopamine,graphene oxide adhesion antibacterial ability

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Feasibility of condensate water recycle of split air handling unit in Chinese University buildings

Energy and Built Environment

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Energy and Built Environment 2024年第2期5卷 309-315页

作者： Xiang Deng Yiyun Shen Senwang Yang Jingyang Feng Si Wang Dongyue Li yanru Li College of Architecture and Urban-Rural Planning Sichuan Agricultural UniversityDujiangyan CampusChengdu611130China

Recycling the condensate water of the air conditioner could be explored as an alternative water source to con-tribute to building the green campus.This paper explored the condensate water production through actual mea-surement based on a split air handling unit(SAHU)in a university building.Then,the statistical analysis was used to analyze the recycling feasibility and the impact factors of the condensate water production in 31 Chinese provincial capital cities to obtain the recycling potential map of the condensate water generated from a SAHU.Results showed that:(1)In the measurement,the amount of condensate water produced by a single split air conditioner was 1.6 kg from 12:40 to 13:40.Therefore,the daily output of condensate water of the air condi-tioner with the university operation schedule could reach 52.99 kg during the main air-conditioning season.(2)Among the 31 provincial capital cities in China,the largest condensate water outputs could be found in the Hot Summer and Warm Winter zone and the Hot Summer and Cold Winter zone,with an average monthly output of 1600 kg and 1100 kg,respectively.(3)Regression analysis showed that the dry-bulb temperature and dew point temperature of outdoor air had the highest positive and significant influence on condensate water production.The objective of this study is to provide theoretical guidance for the design and energy conservation evaluation of the feasibility of SAHU condensate water recycling in universities.

关键词： Condensate water Recycling Regression analysis Split air handling unit University buildings

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Distribution of polarization squeezed light through a 20 km fiber channel

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Science China(Information Sciences) 2024年第5期67卷 343-344页

作者： Chao LI Siyu REN yanru YAN Yalin LI Meihong WANG Xiaolong SU State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Opto-Electronics Shanxi University Collaborative Innovation Center of Extreme Optics Shanxi University

Polarization squeezed light plays a key role in quantum memory by transferring quantum information between atoms and photons [1], and has potential applications in quantum precision measurement [2]. For polarization squeezed light, the quantum variance of at least one Stokes operator is smaller than that of the coherent state.Compared with the quadrature squeezed state, polarization squeezed light has the following advantages: one is that it is a bright beam, and the other is that it can be measured directly without using a local oscillator.

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Photocatalytic oxidation of methane to methanol over zinc titanate supported silver catalysts

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Journal of Rare Earths 2024年第5期42卷 899-906,I0004页

作者： Yuyan Gan Jinbi Huang Qian Lv yanru Li Lizhi Wu YU Tang Yuanxing Fang Pengfei Zhu Li Tan Institute of Molecule Catalysis and In-Situ/Operando Studies State Key Laboratory of Photocatalysis on Energy and EnvironmentCollege of ChemistryFuzhou UniversityFuzhou350108China School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi'an 70021China

The direct activation of methane under mild condition to achieve highly selective of oxygenates is a challenging project.In this study,a well dispersed silver supported ZnTiO_(3) catalyst was prepared to achieve selective preparation of methanol from methane and water under mild condition.X-ray diffraction,transmission electron microscopy and X-ray photoelectron spectroscopy characterizations demonstrate that silver species are uniformly dispersed on ZnTiO_(3) surface in the form of metallic silver nanoparticles.The photoelectric characterizations reveal that the addition of silver species enhances light absorption and promotes charge separation of the catalysts.Under the reaction conditions of 50℃and 3 MPa,the methanol is obtained as the only liquid product over the designed Ag/ZnTiO_(3) catalyst under light irradiation.In this photocatalytic process,the holes generated by ZnTiO_(3) activate water to produce intermediate·OH,which further reacts with methane to synthesize methanol.The silver species as co-catalysts extend the light absorption range of ZnTiO_(3) as well as promote charge separation.

关键词： Photocatalytic Methane oxidation Zinc titanate Silver Methanol

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Assessing the conservation impact of Chinese indigenous chicken populations between ex-situ and in-situ using genome-wide SNPs

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Journal of Integrative Agriculture 2024年第3期23卷 975-987页

作者： Wenting Li Chaoqun Gao Zhao Cai Sensen Yan yanru Lei Mengya Wei Guirong Sun Yadong Tian Kejun Wang Xiangtao Kang College of Animal Science and Technology Henan Agricultural UniversityZhengzhou 450002China The Shennong Laboratory Zhengzhou 450002China

Conservation programs require rigorous evaluation to ensure the preservation of genetic diversity and viability of conservation populations. In this study, we conducted a comparative analysis of two indigenous Chinese chicken breeds, Gushi and Xichuan black-bone, using whole-genome SNPs to understand their genetic diversity, track changes over time and population structure. The breeds were divided into five conservation populations(GS1, 2010, ex-situ;GS2, 2019, ex-situ;GS3, 2019, in-situ;XB1, 2010, in-situ;and XB2, 2019, in-situ) based on conservation methods and generations. The genetic diversity indices of three conservation populations of Gushi chicken showed consistent trends, with the GS3 population under in-situ strategy having the highest diversity and GS2 under ex-situ strategy having the lowest. The degree of inbreeding of GS2 was higher than that of GS1 and GS3. Conserved populations of Xichuan black-bone chicken showed no obvious changes in genetic diversity between XB1 and XB2. In terms of population structure, the GS3 population were stratified relative to GS1 and GS2. According to the conservation priority, GS3 had the highest contribution to the total gene and allelic diversity in GS breed, whereas the contribution of XB1 and XB2 were similar. We also observed that the genetic diversity of GS2 was lower than GS3, which were from the same generation but under different conservation programs(in-situ and ex-situ). While XB1 and XB2 had similar levels of genetic diversity. Overall, our findings suggested that the conservation programs performed in ex-situ could slow down the occurrence of inbreeding events, but could not entirely prevent the loss of genetic diversity when the conserved population size was small, while in-situ conservation populations with large population size could maintain a relative high level of genetic diversity.

关键词： genome-wide SNPs conservation genetic diversity ex-situ in-situ

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Translating solitons in Rof linear Weingarten type

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Acta Mathematica Sinica,English Series 2024年

作者： Yu Fu Rafael López yanru Luo Dan Yang School of Data Science and Artificial Intelligence.Dongbei University of Finance and Economics Departamento de Geometría y Topología.Universidad de Granada School of Economics Dongbei University of Finance and Economics School of Mathematics.Liaoning University

In this paper,we consider λ-translating solitons in R3.These surfaces are critical points of the weighted area when the density is a coordinate function.If λ=0,these surfaces evolve by translations along the mean curvature flow.We give a full classification of λ-translating solitons that satisfy a linear Weingarten relation between their curvatures.These surfaces are planes,circular cylinders,grim reapers and certain types of cylindrical surfaces.We also prove that planes and circular cylinders are the only λ-translating soliton with constant squared norm of the second fundamental form.

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