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In Situ Polymer Gel Electrolyte in Boosting Scalable Fibre Lithium Battery Applications

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Nano-Micro Letters 2024年第11期16卷 170-173页

作者： Jie luo Qichong Zhang Key Laboratory of Multifunctional Nanomaterials and Smart Systems Chinese Academy of SciencesSuzhou Institute of Nano-Tech and Nano-Bionics398 Ruoshui RoadSuzhou 215123People’s Republic of China

The poor interfacial stability not only deteriorates fibre lithium-ion batteries(FLBs)performance but also impacts their scalable *** efficiently address these challenges,*** Peng team proposed a generalized channel structures strategy with optimized in situ polymerization technology in their recent *** resultant FLBs can be woven into different-sized powering textiles,providing a high energy density output of 128 Wh kg^(-1) and simultaneously demonstrating good durability even under harsh *** a promising strategy expands the horizon in developing FLB with particular polymer gel electrolytes,and significantly ever-deepening understanding of the scaled wearable energy textile system toward a sustainable future.

关键词： High-performance fibre lithium batteries Gel electrolytes Channel structures Stable interface Scalable application

Catalyst design and structure control for photocatalytic refineries of cellulosic biomass to fuels and chemicals

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Journal of Energy Chemistry 2024年第7期94卷 102-127页

作者： Lulu Sun Nengchao luo State Key Laboratory of Catalysis Dalian National Laboratory for Clean EnergyDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina

Lignocellulosic biomass is the largest renewable hydrocarbon resource on *** cellulose,one of the major components of lignocellulose,powered by solar energy is a promising way of providing lowcarbon-footprint energy chemicals such as H_(2),HCOOH,CO,and transportation ***-of-the-art biorefineries target the full use of biomass feedstocks as they have a maximum collection radius of 75-100 km,requesting efficient and selective photocatalysts that significantly influence the outcome of photocatalytic ***-performed photocatalysts can harvest a broad solar spectrum and are active in breaking the chemical bonds of cellulose,decreasing the capital investments of ***,photocatalysts should control the selectivity of cellulose conversion,originating target products to level down separation *** separation in photocatalysts and interfacial charge transfer between photocatalysts and cellulose affect the activity and selectivity of cellulose refineries to H2 and carbonaceous *** account for the challenges above,this review summarizes photocatalysts for the refineries of cellulose and downstream platform molecules based on the types of products,with the structure features of different types of photocatalysts discussed in relation to the targets of either improving the activity or product *** addition,this review also sheds light on the methods for designing and regulating photocatalyst structures to facilitate photocatalytic refineries of cellulose and platform molecules,meanwhile summarizing proposed future research challenges and opportunities for designing efficient photocatalysts.

关键词： Photocatalysts Biorefineries Cellulose Fuels Hydrogen

表面修饰纳米晶纤维素及其在双马来酰亚胺树脂中的应用

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复合材料学报 2020年第6期37卷 1334-1343页

作者：巩桂芬邢韵李泽辛浩曹景飞罗艳梅哈尔滨理工大学材料科学与工程学院哈尔滨150040

采用硫酸水解法制备了纳米晶纤维素(NCC),以N,N-羰基二咪唑(CDI)为活化剂,甲代烯丙基醇(MPO)为改性剂,通过化学取代得到含有烯丙基碳酸酯的纳米晶纤维素(PCNCC);以4,4′-二氨基二苯甲烷双马来酰亚胺(MBMI)、3,3′-二烯丙基双酚A(BBA)及... 详细信息

采用硫酸水解法制备了纳米晶纤维素(NCC),以N,N-羰基二咪唑(CDI)为活化剂,甲代烯丙基醇(MPO)为改性剂,通过化学取代得到含有烯丙基碳酸酯的纳米晶纤维素(PCNCC);以4,4′-二氨基二苯甲烷双马来酰亚胺(MBMI)、3,3′-二烯丙基双酚A(BBA)及双酚A双烯丙基醚(BBE)为原料制备了复合材料基体(MBAE)。采用FTIR、XRD、TEM和碘值法等对化学修饰的产物进行分析和表征。结果表明,当PCNCC中烯丙基碳酸酯的取代率为16.4%时,既能保持晶型不变,同时能在BBE中稳定悬浮;PCNCC中烯丙基碳酸酯的取代率过小或过大时均不适宜用作PCNCC/MBAE复合材料的增强相。利用原位聚合法将PCNCC掺杂在MBAE基体中制备PCNCC/MBAE复合材料,考察PCNCC质量分数对PCNCC/MBAE复合材料力学性能、介电性能及热性能的影响规律。结果显示,当PCNCC质量分数为0.2 wt%时,PCNCC/MBAE复合材料的弯曲强度和弯曲模量分别为148.1 MPa和6 GPa,较MBAE基体分别提高了50.5%和82.9%;冲击强度为13.9 kJ/m^2,较MBAE基体提高54.8%;玻璃化转变温度Tg由纯MBAE的240.4℃提高到257.8℃。此时PCNCC/MBAE复合材料的介电常数明显提高,而介电损耗达到最低值。为扩展纳米晶纤维素及双马来酰亚胺树脂的应用提供了理论依据。

关键词：纳米晶纤维素化学改性 4,4′-二氨基二苯甲烷双马来酰亚胺(MBMI) 复合材料性能

Detecting APT-Exploited Processes through Semantic Fusion and Interaction Prediction

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Computers, Materials & Continua 2024年第2期78卷 1731-1754页

作者： Bin luo Liangguo Chen Shuhua Ruan Yonggang luo School of Cyber Science and Engineering Sichuan UniversityChengdu610065China Key Laboratory of Data Protection and Intelligent Management(Sichuan University) Ministry of EducationChengdu610065China Cyber Science Research Institute Sichuan UniversityChengdu610065China

Considering the stealthiness and persistence of Advanced Persistent Threats(APTs),system audit logs are leveraged in recent studies to construct system entity interaction provenance graphs to unveil threats in a ***-based provenance graph APT detection approaches require elaborate rules and cannot detect unknown attacks,and existing learning-based approaches are limited by the lack of available APT attack samples or generally only perform graph-level anomaly detection,which requires lots of manual efforts to locate attack *** paper proposes an APT-exploited process detection approach called ThreatSniffer,which constructs the benign provenance graph from attack-free audit logs,fits normal system entity interactions and then detects APT-exploited processes by predicting the rationality of entity ***,ThreatSniffer understands system entities in terms of their file paths,interaction sequences,and the number distribution of interaction types and uses the multi-head self-attention mechanism to fuse these ***,based on the insight that APT-exploited processes interact with system entities they should not invoke,ThreatSniffer performs negative sampling on the benign provenance graph to generate non-existent edges,thus characterizing irrational entity interactions without requiring APT attack *** last,it employs a heterogeneous graph neural network as the interaction prediction model to aggregate the contextual information of entity interactions,and locate processes exploited by attackers,thereby achieving fine-grained APT *** results demonstrate that anomaly-based detection enables ThreatSniffer to identify all attack *** to the node-level APT detection method APT-KGL,ThreatSniffer achieves a 6.1%precision improvement because of its comprehensive understanding of entity semantics.

关键词： Advanced persistent threat provenance graph multi-head self-attention graph neural network

Precision regulation of plant aromatic amino acid homeostasis

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Science China(Life Sciences) 2024年第6期67卷 1316-1317页

作者： Jie luo Yazhouwan National Laboratory(YNL) Sanya 572025China School of Breeding and Multiplication(Sanya Institute of Breeding and Multiplication) Hainan UniversitySanya 572025China

The aromatic amino acids(AAAs)phenylalanine(Phe),tyrosine(Tyr),and tryptophan(Trp)are not only building blocks of proteins,but also precursors of numerous primary and specialized metabolites(Schenck and Maeda,2018).For instance,Trp is a precursor of the phytohormone auxin and the plant defense compounds indole glucosinolates,while Phe serves as a precursor of lignin,coumarin and *** plant natural products such as morphine and vitamin E are derived from Tyr,and have been employed in human medicine and nutrition(Schenck and Maeda,2018;Wu et al.,2022;Yokoyama et al.,2021).

关键词： aromatic instance coumarin

骨性Ⅱ类错[牙合]伴牙列拥挤的正畸疗效10年随访一例

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中华口腔医学杂志 2018年第9期53卷 612-615页

作者：罗燕梅叶杨丹许潾于福建医科大学附属口腔医院正畸科福州350002

错[牙合]畸形的矫治目标是平衡、稳定和美观。一个高质量的正畸病例矫治完成后应达到矫治疗效稳定而不复发，而稳定的疗效与错[牙合]诊断、矫治设计、矫治技术的准确运用等因素有重要关系。现报道1例通过减数矫治解决骨性Ⅱ类错[牙合]... 详细信息

错[牙合]畸形的矫治目标是平衡、稳定和美观。一个高质量的正畸病例矫治完成后应达到矫治疗效稳定而不复发，而稳定的疗效与错[牙合]诊断、矫治设计、矫治技术的准确运用等因素有重要关系。现报道1例通过减数矫治解决骨性Ⅱ类错[牙合]伴牙列拥挤患者的正畸疗效及其10年随访观察结果。

关键词：骨性Ⅱ类错[牙合] 正畸疗效牙列拥挤随访观察错[牙合]畸形矫治目标矫治技术减数矫治

THE GRADIENT ESTIMATE OF SUBELLIPTIC HARMONIC MAPS WITH A POTENTIAL

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Acta Mathematica Scientia 2024年第4期44卷 1189-1199页

作者： Han luo School of Mathematical Sciences Fudan UniversityShanghai 200433China

In this paper,we investigate subelliptic harmonic maps with a potential from noncompact complete sub-Riemannian manifolds corresponding to totally geodesic Riemannian *** some suitable conditions,we give the gradient ... 详细信息

关键词： sub-Riemannian manifolds subelliptic harmonic maps with potential gradient estimate Liouville Theorem

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自然因子对四川植被NDVI变化的地理探测

地理学报 2019年第9期74卷 1758-1776页

作者：彭文甫张冬梅罗艳玫陶帅徐新良四川师范大学地理与资源科学学院成都610068 西南土地资源评价与监测教育部重点实验室四川师范大学成都610068 中国科学院资源环境科学数据中心北京100101

许多研究已表明基于遥感的植被指数在地表过程和全球变化研究中具有重要作用,对认识植被变化的驱动因素具有重要意义,但自然因子对植被变化影响仍然难以量化。应用地理探测器模型,研究四川地区自然因子变化对植被分布的空间模式和植被... 详细信息

许多研究已表明基于遥感的植被指数在地表过程和全球变化研究中具有重要作用,对认识植被变化的驱动因素具有重要意义,但自然因子对植被变化影响仍然难以量化。应用地理探测器模型,研究四川地区自然因子变化对植被分布的空间模式和植被变化的交互影响,并确定了促进植被生长的各主要自然因子最适宜特征。结果表明:①2000-2015年,四川植被覆盖度状况良好,中高、高植被覆盖面积之和均超过94%;归一化植被指数(NDVI)转化表现为NDVI> 0.4以上区域转化明显,中高和高植被覆盖区面积分别呈显著下降和上升趋势;植被覆盖时空变化差异显著,植被覆盖较高区域位于四川盆地东北部、川西北高原地区,植被覆盖较低区域分布于四川盆地中部城市密集区域。②土壤类型、高程和年均温度变化等因子较好地解释了植被状况的可变性。③自然因子对植被NDVI影响存在交互作用,自然因子协同效应呈现相互增强和非线性增强关系,两种因子交互作用增强了单因子的影响。④研究揭示的促进植被生长的各主要因子最适宜特征,有助于更好地理解自然因素对植被NDVI变化的影响及其驱动机制。

关键词：植被NDVI 自然因子地理探测器模型四川省

Single-cell RNA sequencing in juvenile idiopathic arthritis

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Genes & Diseases 2024年第2期11卷 633-644页

作者： Xiwen luo Xuemei Tang Department of Rheumatology and Immunology Children’s Hospital of Chongqing Medical UniversityChongqing 400014China Chongqing Key Laboratory of Child Infection and Immunity Ministry of Education Key Laboratory of Child Development and DisordersNational Clinical Research Center for Child Health and DisordersChina International Science and Technology Cooperation Base of Child Development and Critical DisordersChildren's Hospital of Chongqing Medical UniversityChongqing 400014China

Juvenile idiopathic arthritis (JIA) is one of the most common chronic inflammatory rheumatic diseases in children,with onset before age 16 and lasting for more than 6 *** is a highly heterogeneous condition with various consequences for health and quality of *** some JIA patients,early detection and intervention remain *** a result,further investigation of the complex and unknown mechanisms underlying JIA is *** in technology now allow us to describe the biological heterogeneity and function of individual cell populations in *** this review,we hope to provide novel ideas and potential targets for the diagnosis and treatment of JIA by summarizing the current findings of single-cell RNA sequencing studies and understanding how the major cell subsets drive JIA pathogenesis.

关键词： Juvenile idiopathic arthritis Macrophage Macrophage activation syndrome Monocyte Single-cell RNA sequencing Synoviocyte T cell