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Three-dimensional porous bimetallic metal–organic framework/gelatin aerogels: A readily recyclable peroxymonosulfate activator for efficient and continuous organic dye removal

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Chinese Journal of Chemical Engineering 2024年第7期71卷 193-202页

作者： Wenlong Xiang Xian Zhang Rou Xiao yanhui Zhang College of Chemistry Chemical Engineering and EnvironmentFujian Province Key Laboratory of Morden Analytical Science and Separation TechnologyMinnan Normal UniversityZhangzhou 363000China Fujian Provincial University Key Laboratory of Pollution Monitoring and Control Minnan Normal UniversityZhangzhou 363000China

As promising catalysts for the degradation of organic pollutants,metal–organic frameworks(MOFs)often face limitations due to the particle agglomeration and challenging recovery in liquid-catalysis application,stemming from their powdery *** macroscopic structures from pulverous MOF is thus of great importance for broadening their practical *** this study,three-dimensional porous MOF aerogel catalysts were successfully fabricated for degrading organic dyes by activating peroxymonosulfate(PMS).MOF/gelatin aerogel(MOF/gA)catalysts were prepared by directly integrating bimetallic FeCo-BDC with gelatin solutions,followed by freeze-drying and low-temperature *** FeCo-BDC-0.15/gA/PMS system exhibited remarkable performance in degrading various organic dyes,eliminating 99.2%of rhodamine B within a mere 5 *** to the gA/PMS system,there was over a 300-fold increase in the reaction rate ***,high removal efficiency was maintained across varying conditions,including different solution pH,co-existing inorganic anions,and natural water *** trapping experiments and electron paramagnetic resonance analysis revealed that the degradation involved radical(SO_(4)^(-)·)and non-radical routes(^(1)O_(2)),of which ^(1)O_(2) was ***,even after a continuous 400-min reaction in a fixed-bed reactor at a liquid hourly space velocity of 27 h^(-1),the FeCo-BDC/gA composite sustained a degradation efficiency exceeding 98.7%.This work presents highly active MOF-gelatin aerogels for dye degradation and expands the potential for their large-scale,continuous treatment application in organic dye wastewater management.

关键词： Catalyst Environment Wastewater Metal–organic framework gelatin aerogel Peroxymonosulfate

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Influence of Kerr Effect on Second-Order Nonlinearity Induced Transparency

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Wuhan University Journal of Natural Sciences 2024年第1期29卷 67-73页

作者： ZHANg Zhiqiang ZHOU yanhui College of Architectural Engineering Zhengzhou Business UniversityZhengzhou 451200HenanChina Quantum Information Research Center Shangrao Normal UniversityShangrao 334001JiangxiChina

We theoretically study the effect of Kerr effect on the second-order nonlinearity induced transparency in a double-resonant optical cavity *** show that in the presence of the Kerr effect,as the strength of the Kerr effect increases,the absorption curve exhibits an asymmetric-symmetric-asymmetric transition,and the zero absorption point shifts with the increase of the Kerr ***,by changing the strength of the Kerr effect,we can control the width of the transparent window,and the position of the zero-absorption point and meanwhile change the left and right width of the absorption *** asymmetry absorption curve can be employed to improve the quality factor of the cavity when the frequency detuning is tuned to be around the right *** simple dependence of the zeroabsorption point on the strength of Kerr effect suggests that the strength of Kerr effect can be measured by measuring the position of the zero-absorption point in a possible application.

关键词： Kerr effect second-order nonlinearity induced transparency nonlinear optics quantum optics

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generation of input spectrum for electrolysis stack degradation test applied to wind power PEM hydrogen production

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global Energy Interconnection 2024年第4期7卷 462-474页

作者： yanhui Xu guanlin Li Yuyuan gui Zhengmao Li School of Electrical and Electronic Engineering North China Electric Power UniversityBeijing 102206P.R.China School of Electrical Engineering Aalto UniversityFinland

Hydrogen production by proton exchange membrane electrolysis has good fluctuation adaptability,making it suitable for hydrogen production by electrolysis in fluctuating power sources such as wind ***,current research on the durability of proton exchange membrane electrolyzers is *** the typical operating conditions of wind power electrolysis for hydrogen production can provide boundary conditions for performance and degradation tests of electrolysis *** this study,the operating condition spectrum of an electrolysis stack degradation test cycle was *** on the rate of change of the wind farm output power and the time-averaged peak-valley difference,a fluctuation output power sample set was *** characteristic quantities that played an important role in the degradation of the electrolysis stack were *** reduction of the operating data was performed using principal component *** analysis of the data segments was completed using an improved gaussian mixture clustering *** the annual output power data of wind farms in Northwest China with a sampling rate of 1 min as an example,the cyclic operating condition spectrum of the proton-exchange membrane electrolysis stack degradation test was *** preliminary simulation analysis,the typical operating condition proposed in this paper effectively reflects the impact of the original curve on the performance degradation of the electrolysis *** study provides a method for evaluating the degradation characteristics and system efficiency of an electrolysis stack due to fluctuations in renewable energy.

关键词： Hydrogen production by electrolysis of water Wind power Proton exchange membrane electrolyzer gaussian mixture model Cyclic operating condition

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Stabilizing iridium sites via interface and reconstruction regulations for water oxidation in alkaline and acidic media

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Journal of Energy Chemistry 2024年第2期89卷 355-363,I0009页

作者： Weibin Chen yanhui Song Lei Li Junjie guo Zhan Lin guangdo.g Provincial Key Laboratory of Plant Resources Biorefinery School of Chemical Engineering and Light IndustryGuangdong University of TechnologyGuangzhou 510006GuangdongChina Key Laboratory of Interface Science and Engineering in AdvancedMaterials Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024ShanxiChina

Exploring effective iridium(Ir)-based electrocatalysts with stable iridium centers is highly desirable for oxygen evolution reaction(OER).Herein,we regulated the incorporation manner of Ir in Co_(3)O_(4)support to stabilize the Ir sites for effective *** anchored on the surface of Co_(3)O_(4)in the form of Ir(OH)_6 species,the created Ir-OH-Co interface leads to a limited stability and poor acidic OER due to Ir *** doped into Co_(3)O_(4)lattice,the analyses of X-ray absorption spectroscopy,in-situ Raman,and OER measurements show that the partially replacement of Co in Co_(3)O_(4)by Ir atoms inclines to cause strong electronic effect and activate lattice oxygen in the presence of Ir-O-Co interface,and simultaneously master the reconstruction effect to mitigate Ir dissolution,realizing the improved OER activity and stability in alkaline and acidic *** a result,Ir_(lat)@Co_(3)O_(4)with Ir loading of 3.67 wt%requires 294±4 mV/285±3 mV and 326±2 mV to deliver 10 mA cm^(-2)in alkaline(0.1 M KOH/1.0 M KOH)and acidic(0.5 M H_(2)SO_(4))solution,respectively,with good stability.

关键词： Interface effect Reconstruction Ir dissolution Ir-O-Co Oxygen evolution reaction

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Lactate:a prospective target for therapeutic intervention in psychiatric disease

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Neural Regeneration Research 2024年第7期19卷 1473-1479页

作者： yanhui Cai Haiyun guo Tianle Han Huaning Wang Department of Psychiatry Xijing HospitalFourth Military Medical UniversityXi’anShaanxi ProvinceChina Department of Anesthesiology and Perioperative Medicine Xijing HospitalFourth Military Medical UniversityXi’anShaanxi ProvinceChina

Although antipsychotics that act via monoaminergic neurotransmitter modulation have considera ble therapeutic effect,they cannot completely relieve clinical symptoms in patients suffering from psychiatric disorde *** may be attributed to the limited range of neurotransmitters that are regulated by psychotropic *** findings indicate the need for investigation of psychotropic medications that target less-studied neurotransmitte *** these candidate neurotransmitters,lactate is developing from being a waste metabolite to a glial-neuronal signaling molecule in recent *** studies have suggested that cerebral lactate levels change considerably in numerous psychiatric illnesses;animal experiments have also shown that the supply of exogenous la ctate exerts an antidepressant *** this review,we have described how medications targeting newer neurotransmitte rs offer promise in psychiatric diseases;we have also summarized the advances in the use of lactate(and its corresponding signaling pathways)as a signaling *** addition,we have described the alterations in brain lactate levels in depression,anxiety,bipolar disorder,and schizophrenia and have indicated the challenges that need to be overcome before brain lactate can be used as a therapeutic target in psychopharmacology.

关键词： antidepressant anxiety bipolar disorder depression lactate psychiatric disease psychopharmacology schizophrenia signal molecular therapeutics

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Atomic-level insights into the initial oxidation mechanism of high-entropy diborides by first-principles calculations

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Journal of Materiomics 2024年第2期10卷 423-430页

作者： Yiwen Liu Hulei Yu Hong Meng yanhui Chu School of Materials Science and Engineering South China University of TechnologyGuangzhou510641China

Understanding the initial oxidation mechanism is critical for studying the oxidation resistance of high-entropy ***,related studies are ***,the initial oxidation mechanism of(Zr_(0.25)Ti_(0.25)Nb_(0.25)Ta_(0.25))B_(2)high-entropy diborides(HEB_(2)-1)is investigated by first-principles calculations at the atomic *** employing the two-region model method,the most stable surface of HEB_(2)-1 is determined to be(1120)*** dissociative adsorption process of the oxygen molecule on the HEB_(2)-1-(1120)surface is predicted to proceed spontaneously,where OeO bond breaks and each oxygen atom is chemisorbed on the most preferable hollow *** adsorption energy and the diffusion barrier of the oxygen atom on the(1120)surface of HEB_(2)-1 are in the vicinity of the average level of the cor-responding four individual *** addition,ab initio molecular dynamics simulations indicate a high initial oxidation resistance of HEB_(2)-1 at 1000 *** results are beneficial to further designing the high-entropy diborides with excellent oxidation resistance.

关键词： High-entropy diborides Oxidation First-principles calculations

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A promising application of bulk metallic glasses in torque sensor

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Science China(Technological Sciences) 2024年第8期67卷 2505-2514页

作者： LU WenHao MA Jiang WANg Chao LIU yanhui Institute of Physics Chinese Academy of SciencesBeijing 100190China Shenzhen Key Laboratory of High Performance Nontraditional Manufacturing College of Mechatronics and Control EngineeringShenzhen UniversityShenzhen 518060China

Torque sensors are essential components of robotic joints. In the past, structure optimization of force-sensing elements has been the common approach to improve the performance of the torque sensors. In this work, we demonstrate a torque sensor with bulk metallic glasses as a force-sensing element. Compared with the sensors made of stainless steel and aluminum alloy, the use of bulk metallic glass as a force-sensing element significantly improves sensor sensitivity, linearity, repeatability, hysteresis, and measuring range. Our work not only opens up a new avenue for the application of bulk metallic glasses, but also provides opportunities for enhancing the performance of force/torque sensors through materials optimization.

关键词： bulk metallic glasses amorphous alloys force sensors

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Phylogenetic study on Scenedesmacae with the description of a new genus Coccoidesmus ***.(Chlorophyceae,Chlorophyta)and chloroplast genome analyses

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Journal of Oceanology and Limnology 2024年第4期42卷 1272-1285页

作者： Qinghua WANg Ying HOU yanhui LI Ying SHI guoxiang LIU College of Biological Sciences and Technology Taiyuan Normal UniversityJinzhong 030619China Shanxi Vocational University of Engineering Science and Technology Jinzhong 030619China Key Laboratory of Algal Biology Institute of HydrobiologyChinese Academy of SciencesWuhan 430072China

Members of the family Scenedesmaceae are some of the most common algal taxa in inland ecosystems,and they are widely distributed in freshwaters,aerial,and sub-aerial *** the continuous updating of methods,the classic morphological taxonomy of this family needs to be *** recent years,many genera of Scenedesmaceae have been established via the use of molecular *** phylogenetic relationships within Scenedesmaceae were analyzed using different molecular markers and morphological data,and the new freshwater genus Coccoidesmus Wang,Hou et Liu *** *** new species in this genus were also *** analysis based on tufA genes revealed that the new genus formed an independent clade closely related to ***,these two genera are characterized by significant morphological differences in colony arrangement and cell *** chloroplast genome of the type species was assembled and annotated,and analyses of genome structure and sequences were *** genome data could help clarify the phylogenetic relationships within this family.

关键词： phylogenetic Scenedesmaceae Coccoidesmus morphology chloroplast genome

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Evaluation of rainfall threshold models for debris flow initiation in the Jiangjia gully,Yunnan Province,China

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Journal of Mountain Science 2024年第6期21卷 1799-1813页

作者： YANg Hongjuan ZHANg Shaojie HU Kaiheng WEI Fangqiang LIU yanhui State Key Laboratory of Mountain Hazards and Engineering Resilience Institute of Mountain Hazards and EnvironmentChinese Academy of SciencesChengdu 610299China Chongqing Institute of green and Intelligent Technology Chinese Academy of SciencesChongqing 400714China Chongqing School University of Chinese Academy of SciencesChongqing 400714China China Institute of geo-Environment Monitoring Beijing 100081China

Systematically determining the discriminatory power of various rainfall properties and their combinations in identifying debris flow occurrence is crucial for early warning *** this study,we evaluated the discriminatory power of different univariate and multivariate rainfall threshold models in identifying triggering conditions of debris flow in the Jiangjia gully,Yunnan Province,*** univariate models used single rainfall properties as indicators,including total rainfall(R_(tot)),rainfall duration(D),mean intensity(I_(mean)),absolute energy(Eabs),storm kinetic energy(E_(s)),antecedent rainfall(R_(a)),and maximum rainfall intensity over various durations(I_(max_dur)).The evaluation reveals that the I_(max_dur)and Eabs models have the best performance,followed by the E_(s),R_(tot),and I_(mean)models,while the D and R_(a)models have poor ***,the I_(max_dur)model has the highest performance metrics at a 40-min *** used logistic regression to combine at least two rainfall properties to establish multivariate threshold *** results show that adding D or R_(a)to the models dominated by Eabs,E_(s),R_(tot),or I_(mean)generally improve their performances,specifically when D is combined with I_(mean)or when R_(a)is combined with Eabs or E_(s).Including R_(a)in the I_(max_dur)model,it performs better than the univariate I_(max_dur)model.A power-law relationship between I_(max_dur)and R_(a)or between Eabs and R_(a)has better performance than the traditional I_(mean)–D model,while the performance of the E_(s)–R_(a)model is *** evaluation reemphasizes the important role of the maximum intensity over short durations in debris flow *** also highlights the importance of systematically investigating the role of R_(a)in establishing rainfall thresholds for triggering debris *** the regional variations in rainfall patterns worldwide,it is necessary to evaluate the findings of this study across diverse watersheds.

关键词： Rainfall threshold Logistic regression Maximum rainfall intensity Absolute energy Antecedent rainfall

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Nano-effect enhanced cooperative luminescence of Yb^(3+) clusters in bulk materials

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Journal of Rare Earths 2024年第3期42卷 473-478,I0002页

作者： Daguang Li Jiahao Cui yanhui do.g Hao Cui Dan Zhao Weiping Qin State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun130012China

In order to improve the multi-ion cooperative transition, we proposed and exploited a novel nanoscale effect, namely the nanoshell effect in bulk materials. Based on the effect, an optimal material structure was designed by coating the surfaces of Ca F_(2):Yb^(3+)micron size particles with ZrO_(2). An about 2 times higher intensity of cooperative luminescence is observed upon laser excitation at 980 nm. Dynamical analysis exhibits that the novel effect plays a key role in improving the performance of cooperative transitions. Our results also suggest that the nanoshell effect in bulk materials is likely to be significant in some special cases, which have not been reported yet in the literature.

关键词： Yb^(3+)cluster ZrO_(2) Nanoshell Enhancement Cooperative luminescence Rare earths

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