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Bioinspired Tactile Sensation Based on Synergistic Microcrack-Bristle Structure Design toward High Mechanical Sensitivity and Direction-Resolving Capability

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Research 2024年第1期2023卷 611-624页

作者： Yiqun Zhang Qi Liu Wenjuan Ren yangyang Song Hua Luo yangyang Han Liang He Xiaodong Wu Zhuqing Wang School of Mechanical Engineering Sichuan UniversityChengdu 610065China Med+X Center for Manufacturing West China HospitalSichuan UniversityChengdu 610041China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu 610065China

Natural tactile sensation is complex,which involves not only contact force intensity detection but also the perception of the force direction,the surface texture,and other mechanical ***,the vast majority of the developed tactile sensors can only detect the normal force,but usually cannot resolve shear force or even distinguish the directions of the ***,we present a new paradigm of bioinspired tactile sensors for resolving both the intensity and the directions of mechanical stimulations via synergistic microcrack-bristle structure design and cross-shaped configuration *** microcrack sensing structure gives high mechanical sensitivity to the tactile sensors,and the synergistic bristle structure further amplifies the sensitivity of the *** cross-shaped configuration engineering of the synergistic microcrack-bristle structure further endows the tactile sensors with good capability to detect and distinguish the directions of the applied mechanical *** as-fabricated tactile sensors exhibit a high sensitivity(25.76 N^(−1.),low detection limit(5.4 mN),desirable stability(over 2,500 cycles),and good capability to resolve both mechanical intensity and directional *** promising application scenarios,surface texture recognition and biomimetic path explorations are successfully demonstrated with these tactile *** newly proposed tactile sensation strategy and technology have great potential applications in ingenious tactile sensation and construction of various robotic and bionic prostheses with high operational dexterity.

关键词： crack sensation directions

Stereoselective Synthesis of 2-Deoxy-α-N-Glycosides from Glycals with 1.4,2-Dioxazol-5-ones

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Chinese Journal of Chemistry 2024年第18期42卷 2147-2152页

作者： Zhenpeng Shen Guoyin Yin yangyang Li The Institute for Advanced Studies Wuhan UniversityWuhanHubei 430072China

The synthesis of N-glycosides has received significant attention due to their crucial role in carbohydrate *** considerable advancements developed in the construction of N-glycosides,methods for the stereoselective construction of 2-deoxy-α-N-glycosides are still ***,we disclosed a nickel-catalyzed hydroamination of glycals under mild *** transformation could allow for the stereoselective synthesis of an array of 2-deoxy-α-N-glycosides with excellentα-***-catalyzed glycosylation reactions,particularly those involving anomeric C(sp")-metal bond formation,have proven to be an effective and stereoselective strategy for producing various ***,with highlight of the application of this reaction,y-sugar amino acidderivatives weresynthesized.

关键词： 2-Deoxy-α-N-glycosides Nickel catalysis Stereoselectivity Glycals Hydroamination Amides Glycosylation Alkenes ComprehensiveSummary

A blockchain-empowered authentication scheme for worm detection in wireless sensor network

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Digital Communications and Networks 2024年第2期10卷 265-272页

作者： Yuling Chen Xiong Yang Tao Li Yi Ren yangyang Long State Key Laboratory of Public Big Data College of Computer Science and TechnologyGuizhou UniversityGuiyang550025China School of Computing Science University of East AngliaNorwichNR57TJUK

Wireless Sensor Network(WSN)is a distributed sensor network composed a large number of nodes with low cost,low performance and *** special structure of WSN brings both convenience and *** example,a malicious participant can launch attacks by capturing a physical ***,node authentication that can resist malicious attacks is very important to network ***,blockchain technology has shown the potential to enhance the security of the Internet of Things(IoT).In this paper,we propose a Blockchain-empowered Authentication Scheme(BAS)for *** our scheme,all nodes are managed by utilizing the identity information stored on the ***,the simulation experiment about worm detection is executed on BAS,and the security is evaluated from detection and infection *** experiment results indicate that the proposed scheme can effectively inhibit the spread and infection of worms in the network.

关键词： Wireless Sensor Network(WSN) Node authentication Blockchain Tangle Worm detection

The configuration of Au^(δ+)-ZrO_(2)^(δ−)species induced activation enhances electrocatalytic CO_(2)to formate conversion

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Nano Research 2024年第7期17卷 6006-6015页

作者： Yongjian Jia Yadi Zhang Mengque Lin yangyang Cheng Yanjie Xu National Engineering Research Center for Technology and Equipment of Environmental Deposition Lanzhou Jiaotong UniversityLanzhou 730070China Key Lab of Opt-Electronic Technology and Intelligent Control of Ministry of Education Lanzhou Jiaotong UniversityLanzhou 730070China School of Environmental Engineering and Chemistry Luoyang Institute of Science and TechnologyLuoyang 471023China

Electrochemical CO_(2)conversion into value-added chemicals is a promising technology to solve the greenhouse effect and recycle chemical ***,the electrochemical CO_(2)reduction reaction(e-CO_(2)RR)is seriously compromised by weak CO_(2)adsorption and a rough CO_(2)activation process based on the chemical inertness of the CO_(2)molecule and the formed fragile metal–C/O *** this paper,we designed and fabricated Au particles embedded in ZrO_(2).The configuration of Au particles being of positive charge and ZrO_(2)with negative charge is induced and generated by metal–support interactions(MSIs).As a result,Au/ZrO_(2)@C presents a big difference in the CO_(2)conversion compared with the known work,affording a formate yield of 1.2.5μmol·cm^(−2)·h^(−1.at−1.1.V *** hydrogen electrode(RHE),and a max formate Faradaic efficiency of up to 94.1.at−0.9 V *** superior performance was attributed to the activated Au–ZrO_(2)interface to form the Au^(δ+)*** insitu Fourier transform infrared(FTIR)spectroscopy and theoretical calculations show that the MSIs configuration can be inclined to the*OCO intermediate generation on Au^(δ+)species activating CO_(2)molecules and then accelerate the formation of the*OCHO intermediate in e-CO_(2)RR,thereby favoring the CO_(2)conversion to formate.

关键词： electrochemical CO_(2)reduction reaction(e-CO_(2)RR) Au_(δ+)species formic acid *OCHO intermediate metal-support interactions

A novel tunnel waterproof-drainage system based on double-bonded waterproofing materials and its seepage characteristics

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Frontiers of Structural and Civil Engineering 2024年第9期18卷 1321-1336页

作者： Xiaohe SUN Chenghua SHI Guoqing XIAO yangyang GE Chengyong CAO School of Civil Engineering Central South UniversityChangsha 410075China PowerChina ZhongNan Engineering Corporation Limited Changsha 410014China State Key Laboratory of Special Functional Waterproof Materials Beijing Oriental Yuhong Waterproof Technology Co.Ltd.Beijing 101111China College of Civil and Transportation Engineering Shenzhen UniversityShenzhen 518060China

Double-bonded spray membrane waterproofing materials have excellent waterproofing performance and can improve the load-bearing capacity of tunnel linings,leading to an increasing global ***,due to the double-bonded capability of spray membrane materials,traditional interlayer drainage methods cannot be *** limitation makes it difficult to use them in drainage-type tunnels,significantly restricting their range of *** this regard,a novel tunnel waterproof-drainage system based on double-bonded spray membrane materials was proposed in this *** proposed drainage system primarily comprises upper drainage sheets and bottom drainage blind pipes,both located in the tunnel circumferential direction,as well as longitudinal drainage pipes within the ***,numerical calculation methods are employed to analyze the seepage characteristics of this system,revealing the water pressure distribution around the *** results indicate that in the novel waterproof-drainage system,the water pressure in the secondary lining exhibits a“mushroom-shaped”distribution in the circumferential direction,while the water pressure in the longitudinal direction exhibits a“wave-like”***,comparative results with other waterproof-drainage systems indicate that under typical working conditions with a water head of 1.0 m and a rock permeability coefficient of 1.^(−6)m/s,the maximum water pressure in the secondary lining of the novel waterproof-drainage system is 0.6 *** represents a significant reduction compared to fully encapsulated waterproofing and traditional drainage systems,which respectively reduce the water pressure by 65%and 30%.The applicability analysis of the double-bonded waterproofing and drainage system reveals that it can reduce at least 40%of the static water pressure in any groundwater *** novel drainage system provides a valuable reference for the application of double-bonded spray membr

关键词： tunnel drainage spray-applied waterproofing membrane numerical simulation water pressure

Experimental investigation of the inhibition of deep-sea mining sediment plumes by polyaluminum chloride

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International Journal of Mining Science and Technology 2024年第1期34卷 91-104页

作者： Fengpeng Zhang Xuguang Chen Jiakang Wei yangyang Zhang Weikun Xu Hao Li College of Engineering Ocean University of ChinaQingdao 266100China Shandong Province Key Laboratory of Ocean Engineering Ocean University of ChinaQingdao 266100China China Merchants Marine and Offshore Research Institute Co. Ltd.Shenzhen 518000China National Deep Sea Center Qingdao 266237China

Deep-sea sediment disturbance may occur when collecting polymetallic nodules,resulting in the creation of plumes that could have a negative impact on the ecological *** study aims to investigate the potential solution of using polyaluminum chloride(PAC)in the water *** effects of PAC are examined through a self-designed simulation system for deep-sea polymetallic nodule collection and sediment samples from a potential deep-sea mining *** experimental results showed that the optimal PAC dose was found to be 0.75 g/*** with the test conditions without the addition of PAC,the presence of PAC leads to a reduction in volume,lower characteristic turbidity,smaller diffusion velocity,and shorter settling time of the *** indicates that PAC inhibits the entire development process of the *** addition of PAC leads to the flocculation of mm-sized particles,resulting in the formation of cm-sized *** flocculation of particles decreases the rate of erosion on the seabed by around 30%.This reduction in erosion helps to decrease the formation of ***,when the size of suspended particles increases,it reduces the scale at which they ***,the settling velocity of flocs(around 1.^(-2) m/s)is much higher that of compared to sediment particles(around 1.^(-5) m/s),which effectively reduces the amount of time the plume remains in suspension.

关键词： Deep-sea mining Deep-sea polymetallic nodules Sediment plume Polyaluminum chloride Jet impact Particle flocculation

Tribological properties of low-temperature time-dependent pretreated graphite for mechanical seal pairs in high-speed turbopump

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Friction 2024年第2期12卷 305-318页

作者： yangyang ZHAO Guoyuan ZHANG Junqian WANG He WANG Weigang ZHAO Qunfeng ZENG School of Mechano-Electronic Engineering Xidian UniversityXi’an 710071China Xi’an Aerospace Propulsion Institute Xi’an 710071China Key Laboratory of Education Ministry for Modern Design and Rotor-Bearing System Xi’an Jiaotong UniversityXi’an 710049China

The friction coefficient and wear rate of pretreated graphite with liquid nitrogen were obtained by using a ball-on-disk tester,and the wear of GCr1.–graphite seal pairs with the low-temperature time-dependent pretreatment was discussed by comparing the wear *** results show that liquid nitrogen pretreatment can affect the hardness and interlayer spacing of *** range of the friction coefficients of pretreated graphite changes from 0.1. to *** the increase of liquid nitrogen pretreatment time,the wear mechanism of graphite would change from dominated three-body wear to adhesion *** experimental results of the mechanical seal with liquid nitrogen pretreatment show that the wear rate of stator is less than 0.001.5 mm^(3)·N^(−1.·m^(−1.,and the graphite shows a good low-temperature compatibility.

关键词： graphite low-temperature pretreatment mechanical seal friction and wear

Nickel-Catalyzed Stereoselective Migratory Carboboration of 1.4-Cyclohexadiene

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Chinese Journal of Chemistry 2024年第4期42卷 356-362页

作者： Yaoyu Ren Lujin Wang Chao Ding yangyang Li Guoyin Yin The Institute for Advanced Studies Wuhan UniversityWuhanHubei430072 China

Multi-substituted cyclohexanes play a crucial role as scaffolds in bioactive *** significant progress has been made in synthesizing substituted cyclohexanes,methods for the stereoselective assembly of 1.3-disubstituted cyclohexanes remain *** study presents a novel approach involving nickel catalysis to achieve stereoselective carboboration of 1.*** innovative process allows for the simultaneous introduction of a boron group and an aryl or an alkyl fragment into the 1.4-cyclohexadiene framework under mild conditions,with exclusive regioselectivity and excellent cis *** resulting products feature a double carbon bond and the incorporation of the boron group,offering significant potential for subsequent transformations and downstream applications.

关键词： 1.4-Cyclohexadiene Carboboration Nickel Chain-walking Stereoselectivity Difunctionalization

Programmable meta-holography dynamics enabled by grating-modulation

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Photonics Research 2024年第7期12卷 1522-1526页

作者： RUNLONG RAO SHUAI WAN ZHE LI yangyang SHI ZHONGYANG LI Electronic Information School Wuhan UniversityWuhan 430072China Wuhan Institute of Quantum Technology Wuhan 430206China School of Microelectronics Wuhan UniversityWuhan 430072China Suzhou Institute of Wuhan University Suzhou 215123China

Towards next-generation intelligent display devices, it is urgent to find a cheap and convenient dynamic optical control method. Conventional gratings are widely used as cheap diffractive elements due to their effective optical control capabilities. However, they are limited within multi-function or complex optical modulation due to the lack of accurate control of the amplitude/phase at pixel-level. Here, a metasurface-assisted grating-modulation system is originally proposed to achieve switchable multi-fold meta-holographic dynamics. By incorporating metasurfaces with traditional gratings and tuning their relative coupling positions, the modulation system gains the optical modulation capability to realize complex optical functionalities. Specifically, by varying the grating periods/positions relative to the metasurface, 2–8 holographic image channels are programmed to be dynamically exhibited and switched. The proposed metasurface-assisted grating-modulation approach enjoys cost-effective convenience, strong encoding freedom, and facile operation, which promises programmable optical displays,optical sensors, optical information encryption/storage, etc.

关键词： tuning switched holographic