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New possibility for PET plastic recycling by a tailored hydrolytic enzyme

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Green Energy & Environment 2024年第2期9卷 163-165页

作者： Shijie Yu Qinghai Li yanguo zhang.hui zhou Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Beijing Key Laboratory of CO_(2)Utilization and Reduction TechnologyDepartment of Energy and Power EngineeringTsinghua UniversityBeijing 100084China

Plastic waste puts a huge burden on the ecosystem due to the current lack of mature recycling ***(ethylene terephthalate)(PET)is one of the most produced plastics in the *** decomposition holds the promise of recovering monomers from PET plastic,and the monomers can be used to regenerate new PET ***,there are still limitations in the activity and thermal stability of the existing PET *** recent study by Lu et *** a novel PET hydrolase via machine learning-aided *** obtained PET hydrolase showed excellent activity and thermal stability in the hydrolysis of PET and is capable of directly degrading large amounts of postconsumer PET *** approach provides an effective method for recycling PET waste and is expected to improve the current state of plastic pollution worldwide.

关键词： Plastic waste Poly(ethylene terephthalate) Hydrolysis Machine learning Enzymatic depolymerization Hydrolases

Stabilization/solidification mechanisms of tin tailings and fuming slag-based geopolymers for different heavy metals

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Frontiers of Environmental Science & Engineering 2024年第5期18卷 43-55页

作者： Xian zhou Zhengfu zhang.hui Yang School of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China Kunming Metallurgical Research Institute Co. Ltd.Kunming650031China

Tin mine tailings(TMT)and fuming slag(FS)contain many heavy metals(As,Cr,Cu,Zn and Mn)that cause severe pollution to the ***,geopolymers were prepared using TMT,FS and flue gas desulfurization gypsum(FGDG)to immobilize heavy metals,and their compressive strength and heavy metal leaching toxicity were *** was first determined that T4F5(TMT:FS=4:5)sample exhibited the highest compressive strength(7.83 MPa).T4F5 achieved 95%immobilization efficiency for As and Cr,and nearly 100%for Cu,Zn and Mn,showing good immobilization performance.A series of characterization analyses showed that heavy metal cations can balance the charge in the geopolymer and replace Al in the geopolymer structure to form covalent *** addition,about 2%–20%of heavy metal Fe was immobilized in hydration products,heavy metal hydroxides and non-bridging Si–O and Al–O coordination with silica-aluminate ***_(3)^(3−) was oxidized into AsO_(4)^(3−),which may form Ca–As or Fe–As ***_(2)O_(7)^(2−)was converted to CrO_(4)^(2−)under alkaline environment and then combined with OH−to form Cr(OH)3 ***^(2+)may react directly with dissolved silicate to form Mn_(2)SiO_(4) and also form Mn(OH)_(2) *** unstable Mn(OH)_(2) can be further oxidized to MnO_(2).The heavy metal cations were immobilized in the silicoaluminate lattice,while the anions tended to form insoluble *** results may benefit the industry and government for better handling of TMT,FS and solid wastes containing the abovementioned five heavy metals.

关键词： Heavy metals Cementitious materials Tin tailings Stabilization/solidification Redox

Spatial Distribution Feature Extraction Network for Open Set Recognition of Electromagnetic Signal

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 279-296页

作者： hui zhang Huaji zhou Li Wang Feng zhou The Ministry Key Laboratory of Electronic Information Countermeasure and Simulation Xidian UniversityXi’an710071China Science and Technology on Communication Information Security Control Laboratory Jiaxing314033China

This paper proposes a novel open set recognition method,the Spatial Distribution Feature Extraction Network(SDFEN),to address the problem of electromagnetic signal recognition in an open *** spatial distribution feature extraction layer in SDFEN replaces convolutional output neural networks with the spatial distribution features that focus more on inter-sample information by incorporating class center *** designed hybrid loss function considers both intra-class distance and inter-class distance,thereby enhancing the similarity among samples of the same class and increasing the dissimilarity between samples of different classes during ***,this method allows unknown classes to occupy a larger space in the feature *** reduces the possibility of overlap with known class samples and makes the boundaries between known and unknown samples more ***,the feature comparator threshold can be used to reject unknown *** signal open set recognition,seven methods,including the proposed method,are applied to two kinds of electromagnetic signal data:modulation signal and real-world *** experimental results demonstrate that the proposed method outperforms the other six methods overall in a simulated open ***,compared to the state-of-the-art Openmax method,the novel method achieves up to 8.87%and 5.25%higher micro-F-measures,respectively.

关键词： Electromagnetic signal recognition deep learning feature extraction open set recognition

Soil disturbance evaluation of soft clay based on stress-normalized smallstrain stiffness

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第3期16卷 990-999页

作者： yanguo zhou Yu Tian Junneng Ye Xuecheng Bian Yunmin Chen MOE Key Laboratory of Soft Soils and Geoenvironmental Engineering Institute of Geotechnical EngineeringCenter for Hypergravity Experiment and Interdisciplinary ResearchZhejiang UniversityHangzhou310058China Ningbo Rail Transit Group Co. Ltd.Ningbo315010China

Soil disturbance includes the change of stress state and the damage of soil *** field testing indices reflect the combined effect of both changes and it is difficult to identify the soil structure disturbance directly from these *** the present study,the small-strain shear modulus is used to characterize soil structure disturbance by normalizing the effective stress and void ratio based on Hardin *** procedure for evaluating soil sampling disturbance in the field and the further disturbance during the subsequent consolidation process in laboratory test is proposed,and then validated by a case study of soft clay *** seismic testing in the field,portable piezoelectric bender elements for the drilled sample and bender elements in triaxial apparatus for the consolidated sample were used to monitor the shear wave velocity of the soil from intact to disturbed and even remolded *** is found that soil sampling disturbance degree by conventional thin-wall sampler is about 30%according to the proposed procedure,which is slightly higher than that from the modified volume compression method proposed by Hong and Onitsuka(1998).And the additional soil disturbance induced by consolidation in laboratory could reach about 50%when the consolidation pressure is far beyond the structural yield stress,and it follows the plastic volumetric strain quite well.

关键词： Natural clay Soil sample disturbance Shear wave velocity Small-strain shear modulus Hardin equation

FPGA implementation of 500-MHz high-count-rate high-time-resolution real-time digital neutron-gamma discrimination for fast liquid detectors

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Nuclear Science and Techniques 2024年第8期35卷 101-113页

作者： hui‑Yin Shen Jing‑Long zhang Jie zhang Jian‑Hang zhou College of Nuclear Technology and Automation Engineering Chengdu University of TechnologyChengdu 610059China Southwestern Institute of Physics P.O.Box 432Chengdu 610041China

Fast neutron flux measurements with high count rates and high time resolution have important applications in equipment such as *** this study,real-time neutron and gamma discrimination was implemented on a self-developed 500-Msps,12-bit digitizer,and the neutron and gamma spectra were calculated directly on an FPGA.A fast neutron flux measurement system with BC-501A and EJ-309 liquid scintillator detectors was developed and a fast neutron measurement experiment was successfully performed on the HL-2 M tokamak at the Southwestern Institute of Physics,*** experimental results demonstrated that the system obtained the neutron and gamma spectra with a time accuracy of 1 *** count rates of up to 1 Mcps,the figure of merit was greater than 1.05 for energies between 50 keV and 2.8 MeV.

关键词： Neutron-gamma discrimination Liquid scintillation detector Real-time spectrum analyzer

Variations and future projections of glacial discharge of Urumqi River Headwaters,eastern Tien Shan(1980s-2017)

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Advances in Climate Change Research 2024年第3期15卷 537-546页

作者： hui zhang Fei-Teng WANG Ping zhou Yi-Da XIE State Key Laboratory of Cryospheric Science Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China Key Laboratory of Cryospheric Science and Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China

To address data scarcity on long-term glacial discharge and inadequacies in simulating and predicting hydrological processes in the Tien Shan,this study analysed the observed discharge at multiple timescales over 1980se2017 and projected changes within a representative glacierized high-mountain region:eastern Tien Shan,Central *** processes were simulated to predict changes under four future scenarios(SSP1,SSP2,SSP3,and SSP5)using a classical hydrological model coupled with a glacier dynamics *** rates at annual,monthly(June,July,August)and daily timescales were obtained from two hydrological gauges:Urumqi Glacier No.1 hydrological station(UGH)and Zongkong station(ZK).Overall,annual and summer discharge increased significantly(p<0.05)at both stations over the study *** intra-annual variations mainly resulted from differences in their recharge *** simulations show that a tipping point in annual discharge at UGH may occur between 2018 and 2024 under the four SSPs *** discharge is predicted to cease earlier at ZK than at *** relates to glacier type and size,suggesting basins with heavily developed small glaciers will reach peak discharge sooner,resulting in an earlier freshwater supply *** findings serve as a reference for research into glacial runoff in Central Asia and provide a decision-making basis for planning local water-resource projects.

关键词： Observed glacial discharge Temporal variations Urumqi River Headwaters Eastern Tien Shan Simulation and projection

Discrimination of pharmacodynamic components and volatile compounds of Poria cocos cultivated with five different materials based on GC-IMS analysis

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Food Quality and Safety 2024年第1期8卷 135-144页

作者： Yinan Wang Fei zhou hui Wang Jinping zhang Hongxia Xu Research Institute of Subtropical Forestry Chinese Academy of ForestryHangzhouChina Chun‘an County Thousand-island Lake Forest Farm HangzhouChina

Objectives:The chemical constituents of Poria cocos grown with different substrates vary significantly;thus,identifying and comparing their biomarkers are *** and Methods:Herein,the chemical constituents of Poria cocos obtained with five different substrates were assessed using gas chromatography–ion mobility spectrometry(GC-IMS),high-performance liquid chromatography and multivariate statistical ***:The content of moisture,ash,alcohol-soluble matter,and heavy metals,except for those of the miscellaneous wood Poria cocos,conform to the specifications defined in the Chinese Pharmacopoeia(Edition 2020),and the polysaccharide contents are all greater than 57%.Conclusions:Based on GC-IMS and the established fingerprints,87 compounds were detected,70 of which were identified in each *** statistical analysis revealed seven compounds(two esters,three alcohols,and two aldehydes),which could be considered as potential marker compounds for discrimination.

关键词： Poria cocos cultivation material pharmacodynamic component gas chromatography-ion mobility spectrometry(GC-IMS) volatile compound.

Influence of varied drought types on soil conservation service within the framework of climate change:insights from the Jinghe River Basin,China

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Journal of Arid Land 2024年第2期16卷 220-245页

作者： BAI Jizhou LI Jing RAN hui zhou Zixiang DANG hui zhang Cheng YU Yuyang School of Geography and Tourism Shaanxi Normal UniversityXi'an 710119China College of Geomatics Xi'an University of Science and TechnologyXi'an 710054China

Severe soil erosion and drought are the two main factors affecting the ecological security of the Loess Plateau,*** the influence of drought on soil conservation service is of great importance to regional environmental protection and sustainable ***,there is little research on the coupling relationship between *** this study,focusing on the Jinghe River Basin,China as a case study,we conducted a quantitative evaluation on meteorological,hydrological,and agricultural droughts(represented by the Standardized Precipitation Index(SPI),Standardized Runoff Index(SRI),and Standardized Soil Moisture Index(SSMI),respectively)using the Variable Infiltration Capacity(VIC)model,and quantified the soil conservation service using the Revised Universal Soil Loss Equation(RUSLE)in the historical period(2000-2019)and future period(2026-2060)under two Representative Concentration Pathways(RCPs)(RCP4.5 and RCP8.5).We further examined the influence of the three types of drought on soil conservation service at annual and seasonal *** NASA Earth Exchange Global Daily Downscaled Projections(NEX-GDDP)dataset was used to predict and model the hydrometeorological elements in the future period under the RCP4.5 and RCP8.5 *** results showed that in the historical period,annual-scale meteorological drought exhibited the highest intensity,while seasonal-scale drought was generally weakest in autumn and most severe in *** intensity of all three types of drought will increase over the next 40 years,with a greater increase under the RCP4.5 scenario than under the RCP8.5 ***,the intra-annual variation in the drought intensity of the three types of drought becomes smaller under the two future scenarios relative to the historical period(2000-2019).Soil conservation service exhibits a distribution pattern characterized by high levels in the southwest and southeast and lower levels in the north,and this pattern has remained

关键词： meteorological drought hydrological drought agricultural drought soil conservation service Variable Infiltration Capacity(VIC)model Revised Universal Soil Loss Equation(RUSLE) Jinghe River Basin

Modeling human gastric cancers in immunocompetent mice

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Cancer Biology & Medicine 2024年第7期21卷 553-570页

作者： Weihong zhang Shilong Wang hui zhang Yan Meng Shi Jiao Liwei An Zhaocai zhou Department of Stomatology Department of Medical UltrasoundShanghai Tenth People's HospitalTongji University Cancer CenterTongji University School of MedicineShanghai 200072China State Key Laboratory of Genetic Engineering School of Life SciencesZhongshan HospitalFudan UniversityShanghai 200032China Collaborative Innovation Center for Cancer Personalized Medicine School of Public HealthNanjing Medical UniversityNanjing 211166China

Gastric cancer(GC)is a major cause of cancer-related mortality *** is determined by multiple(epi)genetic and environmental factors;can occur at distinct anatomic positions of the stomach;and displays high heterogeneity,with different cellular origins and diverse histological and molecular *** heterogeneity has hindered efforts to fully understand the pathology of GC and develop efficient *** the past decade,great progress has been made in the study of GC,particularly in molecular subtyping,investigation of the immune microenvironment,and defining the evolutionary path and *** mouse models,particularly immunocompetent models that mimic the cellular and molecular features of human GC,in combination with organoid culture and clinical studies,have provided powerful tools for elucidating the molecular and cellular mechanisms underlying GC pathology and immune evasion,and the development of novel therapeutic ***,we first briefly introduce current progress and challenges in GC study and subsequently summarize immunocompetent GC mouse models,emphasizing the potential application of genetically engineered mouse models in antitumor immunity and immunotherapy studies.

关键词： Gastric cancer heterogeneity mouse model GEMM immunocompetent