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Effects of surface chlorine atoms on charge distribution and reaction barriers for photocatalytic CO_(2)reduction

Nano Materials Science 2024年第2期6卷 235-243页

作者： Wendong Zhang Wenjun Ma Yuerui Ma Peng Chen Qingqing Ye Yi Wang Zhongwei Jiang Yingqing ou Fan Dong Chongqing Key Laboratory of Green Synthesis and Application&Chongqing Key Laboratory of Inorganic Functional Materials College of ChemistryChongqing Normal UniversityChongqing401331China Suzhou Industrial Technology Research Institute of Zhejiang University Jiangsu215000China Department of Chemistry Faculty of ScienceNational University of SingaporeSingapore117543Singapore yangtze Delta Region Institute(Huzhou)&Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaHuzhou313001China

Photocatalytic CO_(2)reduction to produce high value-added carbon-based fuel has been proposed as a promising approach to mitigate global warming issues.However,the conversion efficiency and product selectivity are still low due to the sluggish dynamics of transfer processes involved in proton-assisted multi-electron reactions.Lowering the formation energy barriers of intermediate products is an effective method to enhance the selectivity and productivity of final products.In this study,we aim to regulate the surface electronic structure of Bi_(2)WO_(6)by doping surface chlorine atoms to achieve effective photocatalytic CO_(2)reduction.Surface Cl atoms can enhance the absorption ability of light,affect its energy band structure and promote charge separation.Combined with DFT calculations,it is revealed that surface Cl atoms can not only change the surface charge distribution which affects the competitive adsorption of H_(2)O and CO_(2),but also lower the formation energy barrier of intermediate products to generate more intermediate*COOH,thus facilitating CO production.Overall,this study demonstrates a promising surface halogenation strategy to enhance the photocatalytic CO_(2)reduction activity of a layered structure Bi-based catalyst.

关键词： Surface chlorine atoms Charge distribution Reaction barriers Photocatalytic CO_(2)reduction Bi_(2)WO_(6)

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一种电力变压器短路累积机械损伤评价方法

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电工技术学报 2024年第8期39卷 2578-2590页

作者：欧强罗隆福李勇杨贤周腊吾西南科技大学信息工程学院绵阳621010 湖南大学电气与信息工程学院长沙410082 广东电网有限责任公司电力科学研究院广州510080 长沙理工大学电气与信息工程学院长沙410114

多次短路会逐渐积累绕组机械损伤,最终导致电力变压器损坏。然而,目前缺乏一种量化评估方法来评估此类损伤,这对电网的安全运行构成了威胁。因此,该文提出一种考虑绕组的非线性特点和累积过程的电力变压器绕组短路累积机械损伤评价方法... 详细信息

多次短路会逐渐积累绕组机械损伤,最终导致电力变压器损坏。然而,目前缺乏一种量化评估方法来评估此类损伤,这对电网的安全运行构成了威胁。因此,该文提出一种考虑绕组的非线性特点和累积过程的电力变压器绕组短路累积机械损伤评价方法,为评估绕组短路对电力变压器的影响提供了新的途径。该方法采用阻尼比和可靠性损失系数作为特征量,通过指数型曲线来模拟绕组机械弱化过程。同时考虑变压器的初始承受短路的能力、短路电流幅值和故障次数等影响因素,量化了短路损伤与绕组动态机械寿命之间的关系。此外,通过对一台110 kV电力变压器进行多次短路破坏性试验,验证了该评价方法的正确性。最后,阐述了提出的评价方法适用于不同的校核控制方法,并强调了控制阻尼比在减少累积损伤方面的积极作用。

关键词：电力变压器短路累积损伤可靠性评价

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Effective groundwater level recovery from mining reduction: Case study of Baoding and Shijiazhuang Plain area

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地下水科学与工程:英文版 2023年第3期11卷 278-293页

作者： Tian Nan Chen Yue Wen-geng Cao En-lin Mu yang ou Zhen-sheng Lin Wei Kang Institute of Hydrogeology and Environmental Geology Chinese Academy of Geological SciencesShijiazhuang 050061China Key Laboratory of Groundwater Sciences and Engineering Ministry of Natural ResourcesShijiazhuang 050061China Water Resources Management Center Ministry of Water ResourcesBeijing 100053China North China University of Water Resources and Electric Power Zhengzhou 450046China Hebei GEO University Shijiazhuang 05003China

The effective recovery of water level is a crucial measure of the success of comprehensive groundwater over-exploitation management actions in North China.However,traditional evaluation method do not directly capture the relationship between mining and other equilibrium elements.This study presents an innovative evaluation method to assess the water level recovery resulting from mining reduction based on the relationship between variation in exploitation and recharge.Firstly,the recharge variability of source and sink terms for both the base year and evaluation year is calculated and the coefficient of recharge variationβis introduced,which is then used to calculate the effective mining reduction and solve the water level recovery value caused by the effective mining reduction,and finally the water level recovery contribution by mining reduction is calculated by combining with the actual volume of mining reduction in the evaluation area.This research focuses on Baoding and Shijiazhuang Plain area,which share similar hydrogeological conditions but vary in groundwater exploitation and utilization.As the effect of groundwater level recovery with mining reduction was evaluated in these two areas as case study.In 2018,the results showed an effective water level recovery of 0.17 m and 0.13 m in the shallow groundwater of Shijiazhuang and Baoding Plain areas,respectively.The contributions of recovery from mining reduction were 76%and 57.98%for these two areas,respectively.It was notable that the water level recovery was most prominent in the foothill plain regions.From the evaluation results,it is evident that water level recovery depends not only on the intensity of groundwater mining reduction,but also on its effectiveness.The value of water level recovery alone cannot accurately indicate the intensity of mining reduction,as recharge variation significantly influences water level changes.Therefore,in practice,it is crucial to comprehensively assess the impact of mining reduction on water level recovery by combining th

关键词： Water level recovery Water balance Effective mining reduction Coefficient of recharge variation Water level recovery contribution

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COVID-19 transmission and control in land public transport:A literature review

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Fundamental Research 2024年第3期4卷 417-429页

作者： Qiqi Luo Wenbing Liu Jiayuan Liao Zhongli Gu Xiaodan Fan Zhiwen Luo Xuelin Zhang Jian Hang Cuiyun ou School of Atmospheric Sciences Sun Yat-sen Universityand Southern Marine Science and Engineering Guangdong LaboratoryZhuhai 519082China Key Laboratory of Urban Meteorology China Meteorological AdministrationBeijing 100089China China Meteorological Administration Xiong'an Atmospheric Boundary Layer Key Laboratory Xiong'an 070001China Key Laboratory of Tropical Atmosphere-Ocean System(Sun Yat-sen University) Ministry of EducationZhuhai 519000China Guangdong Fans-tech Agro Co. LtdYunfu 527300China Welsh School of Architecture Cardiff UniversityCardiff CF103XQUnited Kingdom

Land public transport is an important link within and between cities,and how to control the transmission of COVID-19 in land public transport is a critical issue in our daily lives.However,there are still many inconsistent opinions and views about the spread of SARS-CoV-2 in land public transport,which limits our ability to implement effective interventions.The purpose of this review is to overview the literature on transmission characteristics and routes of the epidemic in land public transport,as well as to investigate factors affecting its spread and provide feasible measures to mitigate the infection risk of passengers.We obtained 898 papers by searching the Web of Science,Pubmed,and WHO global COVID database by keywords,and finally selected 45 papers that can address the purpose of this review.Land public transport is a high outbreak area for COVID-19 due to characteristics like crowding,inadequate ventilation,long exposure time,and environmental closure.Different from surface touch transmission and drop spray transmission,aerosol inhalation transmission can occur not only in short distances but also in long distances.Insufficient ventilation is the most important factor influencing long-distance aerosol transmission.Other transmission factors(e.g.,interpersonal distance,relative orientation,and ambient conditions)should be noticed as well,which have been summarized in this paper.To address various influencing factors,it is essential to suggest practical and efficient preventive measures.Among these,increased ventilation,particularly the fresh air(i.e.,natural ventilation),has proven to effectively reduce indoor infection risk.Many preventive measures are also effective,such as enlarging social distance,avoiding face-to-face orientation,setting up physical partitions,disinfection,avoiding talking,and so on.As research on the epidemic has intensified,people have broken down many perceived barriers,but more comprehensive studies on monitoring systems and prevention measures in land public transport are still n

关键词： Land transportation Infection risk Transmission route Mitigation measures COVID-19

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基于改进DeepLabv3+模型的桥梁裂缝图像分割方法

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吉林大学学报（工学版） 2024年第1期54卷 173-179页

作者：谭国金欧吉艾永明杨润超吉林大学交通学院长春130022 吉林省公路管理局长春130021

针对桥梁中的裂缝病害智能化检测,深度学习方法中DeepLabv3+分割模型因其提出了新的Encoder-Decoder结构,其融合了目标的高层语义信息与浅层特征并采用了深度分离卷积的方式,取得了优越的图像分割效果。但是,在编码模块训练过程中逐渐... 详细信息

针对桥梁中的裂缝病害智能化检测,深度学习方法中DeepLabv3+分割模型因其提出了新的Encoder-Decoder结构,其融合了目标的高层语义信息与浅层特征并采用了深度分离卷积的方式,取得了优越的图像分割效果。但是,在编码模块训练过程中逐渐缩减输入数据的空间维度导致有用信息丢失,对尺度大小不一的小目标的识别带来一定的局限性。为了提高网络的分割性能,本文提出了一种基于改进DeepLabv3+的图像分割方法。通过增加的YOLOF模块与Resnet模块,进一步扩大感受野同时获取到更精确的裂缝特征图,为了验证本文改进算法的有效性,将大量实际桥梁裂缝图像作为原始数据集,将其与当前具有代表性的图像分割模型(如Mask R-CNN、DeepLabv3+)在相同数据集上进行对比。结果表明,本文算法在裂缝像素精度上相比Mask R-CNN、DeepLabv3+分别提高了12%与8%,平均像素精确度达到91.99%,平均交并比达到了81.43%,更加适用于桥梁裂缝分割任务,具有工程实际应用意义。

关键词：桥梁工程桥梁裂缝检测 DeepLabv3+ 像素精度图像分割

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Microbial Quality and Molecular Identification of Enterotoxigenic Staphylococcus Strains Isolated from Dried, Smoked, and Braised Fish Sold in ouagadougou Markets

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Advances in Microbiology 2024年第1期14卷 59-76页

作者： Arouna ouédraogo Ganamé Abasse ouédraogo Henri Sidabéwindin ouédraogo François Tchoumbougnang Cheikna Zongo Aly Savadogo Laboratoire de Biochimie et d’Immunologie Appliqué es (LABIA) Universit&eacute Joseph Ki-Zerbo Ouagadougou Burkina Faso Laboratoire de Valorisation et Contrô le de Qualit&eacute Institut des Sciences Halieutiques Universit&eacute de Douala Douala Cameroon

Background: The investigation of toxin genes in strains involved in staphylococcal food poisoning contributes to food safety. The aim of this study was to isolate and identify enterotoxigenic Staphylococcus strains from dried, smoked, and braised fish sold in ouagadougou markets. Methodology: Staphylococci were isolated using standard microbiology methods. Staphylococcus strains were identified using API Staph kit (Reference # 20500, BioMerieux S.A., Marcy l'Etoile, France). The molecular identification of isolated Staphylococcus aureus strains was specifically confirmed by PCR using the Staur4 and Staur6 primers. The genes encoding enterotoxins, enterotoxin-like toxins, exfoliative toxins, and TSST-1 toxin were detected by multiplex PCR using specific primers from Inquaba Biotec West Africa Ltd, Africa's Genomics Company. Results: The results of the microbiological quality assessment indicated that most of the samples analyzed were found to be of unsatisfactory microbiological quality according to the Staphylococcus aureus microbiological criteria (m = 102). Overall, only 12.55% of samples were satisfactory, while 97.45% were unsatisfactory. The STAPH API gallery allowed the identification of the following species: Staphylococcus aureus, Staphylococcus xylosus, Staphylococcus lugdunensis, Staphylococcus hominis, Staphylococcus haemolyticus, Staphylococcus lentus, Staphylococcus sciuri and Staphylococcus capitis. Of the 108 Staphylococcus isolates, 81 (75%) showed at least one (1) toxin gene. Among the 21 toxin genes tested in this study, 20 genes were detected in all strains analyzed. The staphylococcal toxin genes detected were present in both Staphylococcus aureus and the other coagulase-negative strains isolated in this study. In addition, these genes are found individually or in association in certain strains. The most frequent genes detected in toxin gene-positive strains were: the tsst-1 gene in 45 isolated strains (41.7%), sei (16/14.8%), seg (13/12%), ser (7/6.5%) sec (6/5.5%), and sea (5/4.6%) for staph

关键词： Fish Stapholocuccus Toxin Genes ouagadougou

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Brassinosteroid Signaling Recruits Histone 3 Lysine-27 Demethylation Activity to FLOWERING LOCUS C Chromatin to Inhibit the Floral Transition in Arabidopsis

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Molecular Plant 2018年第9期11卷 1135-1146页

作者： Zicong Li yang ou Zhicheng Zhang Jianming Li Yuehui He Shanghai Center for Plant Stress Biology & National Key Laboratory of Plant Molecular Genetics CAS Center for Excellence in Molecular Plant Sciences Chinese Academy of Sciences (CAS) Shanghai 201602 China University of Chinese Academy of Sciences Beijing 100049 China Shanghai Center for Plant Stress Biology Shanghai Institutes for Biological Sciences Chinese Academy of Sciences Shanghai 201602 China These authors contributed equally to this article

The steroid hormone brassinosteroid （BR） plays a broad role in plant growth and development. As the retarded growth in BR-insensitive and BR-deficient mutants causes a strong delay in days to flowering, BR signaling has been thought to promote the floral transition inArabidopsis. In this study, using a developmental measure of flowering time, we show that BR signaling inhibits the floral transition and promotes vegetative growth in the Arabidopsis accessions Columbia and Enkheim-2. We found that BR signaling promotes the expression of the potent floral repressor FLOWERING LOCUS C （FLC） and three FLC homologs to inhibit flow- ering. In the presence of BR, the transcription factor BRASSINAZOLE-RESISTANT1 （BZR1）, together with BES1 -INTERACTING MYC-like proteins （BIMs）, specifically binds a BR- responsive element in the first intron of FLC and further recruits a histone 3 lysine 27 （H3K27） demethylase to downregulate levels of the repressive H3K27 trimethylation mark and thus antagonize Polycomb silencing at FLC, leading to its activation. Taken together, our findings demonstrate that BR signaling inhibits the floral transition inArabidopsis by a novel molecular mechanism in which BR signals are transduced into FLC activation and consequent floral repression.

关键词： brassinosteroid BR signaling flowering time BZR1 Polycomb silencing FLOWERING LOCUS C

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局部受热锈蚀预应力混凝土梁力学性能试验研究

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铁道科学与工程学报 2024年第2期21卷 681-696页

作者：杨鸥刘智宇葛鹏吕博文风工程与桥梁工程湖南省重点实验室(湖南大学) 湖南长沙410082 湖南大学土木工程学院湖南长沙410082

随着我国基础建设的发展,大量混凝土桥梁在恶劣环境影响下发生腐蚀和老化,腐蚀桥梁结构的灾害破坏机理研究对桥梁结构的运营安全具有重要意义。为研究已经锈蚀受损的桥梁在局部受热状态下的高温力学性能,设计10根预应力混凝土梁试件。... 详细信息

随着我国基础建设的发展,大量混凝土桥梁在恶劣环境影响下发生腐蚀和老化,腐蚀桥梁结构的灾害破坏机理研究对桥梁结构的运营安全具有重要意义。为研究已经锈蚀受损的桥梁在局部受热状态下的高温力学性能,设计10根预应力混凝土梁试件。其中对照组的2根试件在常温下加载,试验变量为预应力筋初始应力,试验组的8根试件在高温下加载,试验变量分别为钢筋锈蚀、预应力筋初始应力、初始荷载。首先,基于电化学原理对4根预应力混凝土梁进行钢筋加速锈蚀处理,然后利用复合高温试验炉对8根预应力混凝土梁(4根锈蚀、4根未锈蚀)在跨中进行三面受火试验。最后,采用数值方法对局部受热预应力混凝土梁进行了仿真分析。研究结果表明:局部受热条件下,预应力混凝土梁的承载能力会发生明显降低,下降幅度约为11.3%~14.9%;钢筋锈蚀导致的混凝土开裂会对预应力混凝土梁的抗火性能产生不利影响,主要表现为2个方面,1)相同试验条件下,锈蚀后的试件预应力增量更大;2)锈蚀试件在局部受热条件下承载能力下降幅度更大,约为19.4%~21.9%;增大预应力筋的初始应力可以减小预应力混凝土梁在局部受热时的高温蠕变变形;局部高温作用下预应力混凝土梁对初始荷载较为敏感,当试件初始荷载值提升20%时,三分点位移量约增大60%。研究成果可以为实际锈蚀桥梁的防火设计和灾后应急提供理论依据。

关键词：预应力混凝土梁局部受热钢筋锈蚀火灾试验温度场

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Growth hormone promotes the reconstruction of injured axons in the hypothalamo-neurohypophyseal system

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Neural Regeneration Research 2024年第10期19卷 2249-2258页

作者： Kai Li Zhanpeng Feng Zhiwei Xiong Jun Pan Mingfeng Zhou Weizhao Li Yichao ou Guangsen Wu Mengjie Che Haodong Gong Junjie Peng Xingqin Wang Songtao Qi Junxiang Peng Department of Neurosurgery Institute of Brain DiseasesNanfang HospitalSouthern Medical UniversityGuangzhouGuangdong ProvinceChina

Previous studies have shown that growth hormone can regulate hypothalamic energy metabolism, stress, and hormone release. Therefore, growth hormone has great potential for treating hypothalamic injury. In this study, we established a specific hypothalamic axon injury model by inducing hypothalamic pituitary stalk electric lesions in male mice. We then treated mice by intraperitoneal administration of growth hormone. our results showed that growth hormone increased the expression of insulin-like growth factor 1 and its receptors, and promoted the survival of hypothalamic neurons, axonal regeneration, and vascular reconstruction from the median eminence through the posterior pituitary. Altogether, this alleviated hypothalamic injury-caused central diabetes insipidus and anxiety. These results suggest that growth hormone can promote axonal reconstruction after hypothalamic injury by regulating the growth hormone-insulin-like growth factor 1 axis.

关键词： arginine vasopressin growth hormone hypothalamo-neurohypophyseal system hypothalamus injury insulin-like growth factor 1 oxytocin regeneration

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Lithium-Ion Charged Polymer Channels Flattening Lithium Metal Anode

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Nano-Micro Letters 2024年第4期16卷 379-393页

作者： Haofan Duan Yu You Gang Wang Xiangze ou Jin Wen Qiao Huang Pengbo Lyu Yaru Liang Qingyu Li Jianyu Huang Yun‑Xiao Wang Hua‑Kun Liu Shi Xue Dou Wei‑Hong Lai Hunan Provincial Key Laboratory of Thin Film Materials and Devices School of Material Sciences and EngineeringXiangtan UniversityXiangtan 411105People’s Republic of China Guangxi Key Laboratory of Low Carbon Energy Materials School of Chemical and Pharmaceutical ScienceGuangxi Normal UniversityGuilin 541004People’s Republic of China Institute for Superconducting and Electronic Materials Australian Institute of Innovative MaterialsUniversity of WollongongInnovation CampusSquires WayNorth WollongongNSW 2500Australia Institute of Energy Materials Science University of Shanghai for Science and TechnologyShanghai 200093People’s Republic of China

The concentration difference in the near-surface region of lithium metal is the main cause of lithium dendrite growth.Resolving this issue will be key to achieving high-performance lithium metal batteries(LMBs).Herein,we construct a lithium nitrate(LiNO_(3))-implanted electroactiveβphase polyvinylidene fluoride-co-hexafluoropropylene(PVDF-HFP)crystalline polymorph layer(PHL).The electronegatively charged polymer chains attain lithium ions on the surface to form lithium-ion charged channels.These channels act as reservoirs to sustainably release Li ions to recompense the ionic flux of electrolytes,decreasing the growth of lithium dendrites.The stretched molecular channels can also accelerate the transport of Li ions.The combined effects enable a high Coulombic efficiency of 97.0%for 250 cycles in lithium(Li)||copper(Cu)cell and a stable symmetric plating/stripping behavior over 2000 h at 3 mA cm^(-2)with ultrahigh Li utilization of 50%.Furthermore,the full cell coupled with PHL-Cu@Li anode and Li Fe PO_(4) cathode exhibits long-term cycle stability with high-capacity retention of 95.9%after 900 cycles.Impressively,the full cell paired with LiNi_(0.87)Co_(0.1)Mn_(0.03)O_(2)maintains a discharge capacity of 170.0 mAh g^(-1)with a capacity retention of 84.3%after 100 cycles even under harsh condition of ultralow N/P ratio of 0.83.This facile strategy will widen the potential application of LiNO_(3)in ester-based electrolyte for practical high-voltage LMBs.

关键词： Polymer ionic channel Li metal batteries Artificial protective layer Uniform Li deposition Electrochemical performances

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