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Progress in Natural Science:Materials International 2009年第6期19卷 719-726页

作者： yang cui, chenghai wang disaster reduction key laboratory of gansu province, college of atmospheric sciences, lanzhou university, lanzhou 730000, china disaster reduction key laboratory of gansu province College of Atmospheric Sciences Lanzhou University Lanzhou 730000 China

The sensible and latent heat fluxes during the transition season over the western Tibetan Plateau from the NCEP-1 (NCEP/NCAR Reanalysis 1), AR-Ⅱ (NCEP-DOE Reanalysis 2) and ERA40 reanalysis datasets were compared and analyzed. The results show that the phase change in soil moisture has a significant effect on the sensible and latent heat fluxes over the western Tibetan Plateau (TP) due to the freezing-thawing processes during the transition from the dry to the wet period. The uncertainties in the sensible and latent heat fluxes over the western TP are quite high in the reanalysis data, and depend largely on the success of the soil moisture simulations in the models. Improving the hydrological process simulations in the land-surface models in seasonally frozen ground and in the active frozen soil layer may be an effective way of enhancing the reliability of the surface heat fluxes from the reanalysis data over the Tibetan Plateau.

关键词： Western Tibetan Plateau Surface heat fluxes Reanalysis data Transition season Freezing-thawing process

A piecewise-integration method for simulating the influence of external forcing on climate

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Progress in Natural Science:Materials International 2008年第10期18卷 1239-1247页

作者： Zhifu Zhang Chongjian Qiu chenghai wang key laboratory of Arid Climatic Changing and Reducing disaster of gansu province,college of atmospheric sciences,lanzhou university.lanzhou 730000.china key laboratory of Arid Climatic Changing and Reducing disaster of gansu province College of Atmospheric Sciences Lanzhou University Lanzhou 730000 China

Climate drift occurs in most general circulation models (GCMs) as a result of incomplete physical and numerical representation of the complex climate system,which may cause large uncertainty in sensitivity experiments evaluating climate response to changes in external *** solve this problem,we propose a piecewise-integration method to reduce the systematic error in climate sensitivity studies. The observations are firstly assimilated into a numerical model by using the dynamic relaxation technique to relax to the current state of atmosphere,and then the assimilated fields are continuously used to reinitialize the simulation to reduce the error of climate simulation. When the numerical model is integrated with changed external forcing,the results can be split into two parts,background and pertur- bation fields,and the background is the state before the external forcing is *** piecewise-integration method is used to con- tinuously reinitialize the model with the assimilated field,instead of the ***,the simulation error of the model with the external forcing can be *** this way,the accuracy of climate sensitivity experiments is greatly *** with a simple low-order spectral model show that this approach can significantly reduce the uncertainty of climate sensitivity experiments.

关键词： Climate model External forcing Sensitivity experiment Low-order spectral model Dynamic relaxation technique

Stabilizing perovskite precursors with the reductive natural amino acid for printable mesoscopic perovskite solar cells

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Journal of Energy Chemistry 2024年第3期90卷 32-39,I0003页

作者： Wenjing Hu Jian yang Chuang yang Xufeng Xiao Chaoyang wang Zhaozhen cui Qiaojiao Gao Jianhang Qi Minghao Xia Yaqiong Su Anyi Mei Hongwei Han Michael Gratzel Center for Mesoscopic Solar Cells Wuhan National Laboratory for OptoelectronicsKey Laboratory of Materials Chemistry for Energy Conversion and Storage of Ministry of Education Huazhong University of Science and TechnologyWuhan 430074HubeiChina School of Chemistry Xi'an Key Laboratory of Sustainable Energy Materials ChemistryState Key Laboratory of Electrical Insulation and Power EquipmentXi'an Jiaotong UniversityXi'an 710049ShaanxiChina

Solution processability significantly advances the development of highly-efficient perovskite solar ***,the precursor solution tends to undergo irreversible degradation reactions,impairing the device performance and ***,we utilize a reductive natural amino acid,Nacetylcysteine(NALC),to stabilize the precursor solution for printable carbon-based hole-conductorfree mesoscopic perovskite solar *** find that I_(2) can be generated in the aged solution containing methylammonium iodide(MI) in an inert atmosphere and speed up the MA-FA^(+)(formamidinium) reaction which produces large-size cations and hinders the formation of perovskite *** effectively stabilizes the precursor via its sulfhydryl group which reduces I_(2) back to I^(-)and provides H^(+).The NALC-stabilized precursor which is aged for 1440 h leads to devices with a power conversion efficiency equivalent to 98% of that for devices prepared with the fresh ***,NALC improves the device power conversion efficiency from 16.16% to 18.41% along with enhanced stability under atmospheric conditions by modifying grain boundaries in perovskite films and reducing associated defects.

关键词： Perovskite solar cells Perovskite precursor Degradation Stabilization Reductive natural amino acid

Dusty cloud radiative forcing derived from satellite data for middle latitude regions of East Asia

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Progress in Natural Science:Materials International 2006年第10期16卷 1084-1089页

作者： HUANG Jianping , wang Yujie, wang Tianhe and YI Yuhong ( college of atmospheric sciences, lanzhou university, lanzhou 730000, china gansu Provincial Meteorological Bureau, lanzhou 730020, china) college of atmospheric sciences Lanzhou University Lanzhou 730000 China gansu Provincial Meteorological Bureau Lanzhou 730020 China

The dusty cloud radiative forcing over the middle latitude regions of East Asia was estimated by using the 2-year (July 2002-June 2004) data of collocated clouds and the Earth's radiant energy system (CERES) scanner and moderate resolution imaging spectroradiometer (MODIS) from Aqua Edition IB SSF (single scanner footprint). The dusty cloud is defined as the cloud in dust storm environment or dust contaminated clouds. For clouds growing in the presence of dust, the instantaneous short-wave (SW) forcing at the top of the atmosphere (TOA) is about - 275. 7 W/m for cloud over dust (COD) region. The clouds developing in no-dust cloud (CLD) regions yield the most negative short-wave (SW) forcing ( - 311.0 W/m2), which is about 12.8% stronger than those in COD regions. For long-wave (LW) radiative forcing, the no-dust cloud (CLD) is around 102.8 W/m2 , which is 20% less than the LW forcing from COD regions. The instantaneous TOA net radiative forcing for the CLD region is about - 208.2 W/m2, which is 42.1 % larger than the values of COD regions. The existence of dust aerosols under clouds significantly reduces the cooling effect of clouds.

关键词： dust storm cloud radiative forcing global warming dust aerosol-cloud-climate interaction.

Performance Design of High-Temperature Chloride Salts as Thermal Energy Storage Material

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Journal of Thermal Science 2024年第2期33卷 479-490页

作者： ZHAO Le wang Jingyao cui Liu LI Baorang DU Xiaoze WU Hongwei key laboratory of Power Station Energy Transfer Conversion and System(North china Electric Power university) Ministry of EducationBeijing102206China School of Energy and Power Engineering Lanzhou University of TechnologyLanzhou730050China School of Physics Engineering and Computer ScienceUniversity of HertfordshireHatfieldAL109ABUK

The chloride salts have great potential used as high-temperature thermal energy storage(TES) medium for the concentrated solar power *** this study,LiCl,KCl and CaCl_(2) were selected as energy storage materials in order to further broaden the working temperature of ternary chloride salt and improve its energy storage *** new high-temperature energy storage ternary chloride composed of LiCl,KCl,and CaCl_(2) was developed based on the phase diagram generated by *** components of LiCl-KCl-CaCl_(2) with the mass ratio of 37.85%-53.38%-8.77%,30.90%-13.82%-55.28% and 1.78%-18.61%-79.61% were developed,of which the corresponding melting temperature(T_(m)) 340.93,433.57 and 626.85℃,respectively,was obtained *** that T_(m) of the third group of salts was too high,only the first two groups of salts were *** test showed that the actual melting point was only 0.46% and 1.64% different from the melting point predicted by *** thermal properties of the two ternary chloride salts were also *** solid and liquid-specific heat of ternary salts was determined by DSC using sapphire as the standard *** vapor pressure and decomposition temperature of ternary chloride salts were *** results showed that the vapor pressure of salt 1 was almost constant below 650℃ by ***,the TG results showed that the upper working temperature of salt 1 was 650℃ under the air *** addition,the ternary chloride salts after short-term cycling still exhibited excellent thermal properties,which revealed that these good thermal properties make them have broad application prospects in high-temperature thermal energy storage systems.

关键词： chloride salts thermal energy storages thermal properties thermal stability

Molecular design of recyclable thermosetting polyimide and its composite with excellent mechanical and tribological properties

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Friction 2024年第3期12卷 452-461页

作者： Xiaoyue wang Zenghui yang Tingmei wang Qihua wang Xinrui ZHANG Song LI key laboratory of Science and Technology on Wear and Protection of Materials Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China State key laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Recyclability of thermosetting polymers and their composites is a challenge for alleviating environmental pollution and resource *** this study,solvent-recyclable thermosetting polyimide(PI)and its composite were successfully *** tensile strength,elongation at break,and Young’s modulus of PI are 108.70±7.29 MPa,19.35%±3.89%,and 2336.42±128.00 MPa,*** addition of reduced graphene oxide(RGO)not only enhances the mechanical properties of PI but also endows it with excellent tribological *** PI illustrates a high recycling efficiency of 94.15%,but the recycled composite exhibits inferior mechanical *** recycling and utilization of PI and its composite are realized through imine bonds(-C=N),which provides new guidance for solving the problem of environmental pollution and resource waste and is potential application in the field of sustainable tribology.

关键词： thermosetting polyimide(PI) recyclability dynamic covalent bonds friction and wear polymer composites

Understanding the Low Predictability of the 2015/16 El Niño Event Based on a Deep Learning Model

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Advances in atmospheric sciences 2024年第7期41卷 1313-1325页

作者： Tingyu wang Ping HUANG Xianke yang Center for Monsoon System Research Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China National Space Science Center Chinese Academy of SciencesBeijing 100190China State key laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China college of Plant Science and Technology Huazhong Agricultural UniversityWuhan 430070China

The 2015/16 El Niño event ranks among the top three of the last 100 years in terms of intensity,but most dynamical models had a relatively low prediction skill for this event before the summer ***,the attribution of this particular event can help us to understand the cause of super El Niño–Southern Oscillation events and how to forecast them *** present study applies attribute methods based on a deep learning model to study the key factors related to the formation of this event.A deep learning model is trained using historical simulations from 21 CMIP6 models to predict the Niño-3.4 *** integrated gradient method is then used to identify the key signals in the North Pacific that determine the evolution of the Niño-3.4 *** crucial signals are then masked in the initial conditions to verify their roles in the *** addition to confirming the key signals inducing the super El Niño event revealed in previous attribution studies,we identify the combined contribution of the tropical North Atlantic and the South Pacific oceans to the evolution and intensity of this event,emphasizing the crucial role of the interactions among them and the North *** approach is also applied to other El Niño events,revealing several new precursor *** study suggests that the deep learning method is useful in attributing the key factors inducing extreme tropical climate events.

关键词： ENSO attribution deep learning ENSO prediction extreme El Niño

Exploring formation mechanism and source attribution of ozone during the 2019 Wuhan Military World Games:Implications for ozone control strategies

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Journal of Environmental sciences 2024年第2期136卷 400-411页

作者： Lei Zhang Lili wang Runyu wang Nan Chen Yuan yang Ke Li Jie Sun Dan Yao Yuesi wang Minghui Tao yang Sun Institute of atmospheric Physics Chinese Academy of SciencesBeijing 100029China university of the Chinese Academy of sciences Beijing 100049China Hubei Ecological Environment Monitoring Center Station Wuhan 430072China Guizhou Research and Designing Institute of Environmental sciences Guizhou Academy of Environmental Science and DesignGuiyang 550081China Jiangsu key laboratory of atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China School of Environment Key Laboratory for Yellow River and Huai River Water Environment and Pollution ControlMinistry of EducationHenan Normal UniversityXinxiang 453007China key laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China

A series of emission reduction measures were conducted in Wuhan,Central china,to ensure good air quality during the 7th Military World Games(MWG)in October *** better understand the implications for ozone(O_(3))pollution control strategies,we applied integrated analysis approaches based on the de-weathered statistical model,parameterization methods,chemical box model,and positive matrix factorization *** the MWG,concentrations of O_(3),NO_x,and volatile organic compound(VOCs),OFP(O_(3)formation potential),L_(OH)(OH radical loss rate)were 83μg/m^(3),43μg/m^(3),26 ppbv,188μg/m^(3),and 3.9 s^(-1),respectively,which were 26%,18%,3%,15%,and 13%lower than pre-MWG values and 6%,39%,30%,33%,and 50%lower than post-MWG values,*** removing meteorological influence,O_(3)and its precursors during the MWG decreased largely compared with post-MWG values,and only O_(3),NO_(2),and oxygenated VOCs(OVOCs)declined compared with pre-MWG values,which revealed the emission reduction measures during the MWG played an important role for O_(3)*** six VOCs sources,the mass contributions of biomass burning and solvents usage during the MWG decreased largely compared with pre-MWG values.O_(3)production was sensitive to VOCs and the key species were aromatics,OVOCs,and alkenes,which originated mainly from solvents usage,biomass burning,industrial-related combustion,and vehicle *** O_(3)concentration during the strict control was mainly caused by OVOCs reduction due to biomass burning ***,the O_(3)abatement strategies of Wuhan should be focused on the mitigation of high-reactivity VOCs.

关键词： VOCs Ozone Wuhan Military World Games Source apportionment Relative incremental reactivity Random forest

Emission and optical characteristics of brown carbon in size-segregated particles from three types of Chinese ships

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Journal of Environmental sciences 2024年第8期142卷 248-258页

作者： Fengqin yang Fan Zhang Zeyu Liu Yingjun Chen Yan Zhang Can Wu Yali Lei Shijie Liu Binyu Xiao Xinyi Wan Yubao Chen Yong Han Min cui Cheng Huang Gehui wang key Lab of Geographic Information Science of the Ministry of Education School of Geographic SciencesEast China Normal UniversityShanghai 200241China Institute of Eco-Chongming 20 Cuiniao Rd.ChongmingShanghai 202150China State Environmental Protection key laboratory of Formation and Prevention of the Urban Air Pollution Complex Shanghai Academy of Environmental SciencesShanghai 200233China Shanghai key laboratory of atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science and EngineeringFudan UniversityShanghai 200438China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China Department of Civil and Environmental Engineering and State key laboratory of Marine Pollution The Hong Kong Polytechnic UniversityKowloon 100872Hong KongChina college of Environmental Science and Engineering Yangzhou UniversityYangzhou 225009China

Brown carbon(BrC)is one of the important light absorption substances that have high light absorption ability under short wavelength ***,limit studies have focused on the BrC emission from *** this study,size-segregated particulate matters(PM)were collected from three different types of ships,light absorption characteristics and size distribution of methanol-soluble BrC and water-soluble BrC in PM from ship exhausts were *** showed that four-stroke low-power diesel fishing boat(4-LDF)had the highest mass concentrations of methanol-soluble organic carbon(MSOC)and water-soluble organic carbon(WSOC),followed by 2-stroke high-power heavy-fuel-oil vessel(2-HHV),and fourstroke high-power marine-diesel vessel(4-HMV).While 2-HHV had obviously higher light absorption coefficients of methanol-soluble BrC(Abs365,M)and water-soluble BrC(Abs365,W)in unit weight of PM than the other two types of *** tested ships presented comparable or higher absorption efficiency of BrC in water extracts(MAE365,W)compared with other BrC emission *** of BrC was concentrated in fine particles,and the particle size distributions of both Abs365,Mand Abs365,Wshowed bimodal patterns,peaking at0.43–0.65μm and 4.7–5.8μm,***,different particle size distributions were found for MAE365,Mbetween diesel and heavy fuel oil ***,different wavelength dependence in particles with different size were also *** exhaust could be confirmed as a non-ignorable BrC emission source,and complex influencing factor could affect the light absorption characteristics of ship *** size should also be considered when light absorption ability of BrC was evaluated.

关键词： Ship emission Brown carbon Light absorption Size distribution

A kinetic resolution accompanied chirality transformation process for asymmetric synthesis of chiral phenol, oxaziridine, and α-hydroxyl cyclic ketone

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Science china Chemistry 2024年第9期67卷 2989-2997页

作者： Pengxin wang Xiaoyong Zhang Lingqing wang Rui wang Dongxu yang key laboratory of Preclinical Study for New Drugs of gansu province School of Basic Medical Sciences & Research Unit of Peptide ScienceChinese Academy of Medical Sciences Lanzhou University State key laboratory of Bioactive Substance and Function of Natural Medicines Institute of Materia Medica Chinese Academy of Medical Sciences and Peking Union Medical College School of sciences Great Bay University Institute of Systems and Physical Biology Shenzhen Bay Laboratory

Chirality transformation is a basic, attractive, and important strategy for obtaining enantioenriched products with desired chiral elements. The reported chirality conversion reaction often involves the process from one type of chirality to another one. To better utilize the chirality transformation strategy for obtaining two or more products with different chiral elements in a single reaction, a new method of kinetic resolution accompanied by a chirality transformation protocol is proposed and successfully realized in this study. This process is used for the asymmetric oxidation of phenol compounds along with the kinetic resolution of oxaziridines. A wide scope of products, including axially chiral phenols, oxaziridines, and α-hydroxyl cyclic ketones were smoothly obtained in high levels of yields and enantioselectivities in the developed method. These products can be readily used for the synthesis of various types of chiral ligands, which are potential choices for other catalytic asymmetric reactions.

关键词： chirality transformation kinetic resolution accompanied axially chiral phenols chiral oxaziridines

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