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Advances in Manufacturing 2024年第1期12卷 94-107页

作者： yan Liu qiu Tang Xin-Cheng Tian School of Control Science and Engineering Shandong UniversityJinan250061People’s Republic of China Engineering Research Center of Intelligent Unmanned System Ministry of EducationJinan250061People’s Republic of China School of Mechanical and Electronic Engineering Shandong Jianzhu UniversityJinan250101People’s Republic of China

The automatic cutting of intersecting pipes is a challenging task in *** improved automation and accuracy,this paper proposes a model-driven path planning approach for the robotic plasma cutting of a branch pipe with a single ***,it summarizes the intersection forms and introduces a dual-pipe intersection *** on this model,the moving three-plane structure(a description unit of the geometric characteristics of the intersecting curve)is constructed,and a geometric model of the branch pipe with a single Y-groove is ***,a novel mathematical model for plasma radius and taper compensation is ***,the compensation model and groove model are integrated by establishing movable ***,to prevent collisions between the plasma torch and workpiece,the torch height is planned and a branch pipe-rotating scheme is *** the established models and moving frames,the planned path description of cutting robot is provided in this novel *** accuracy of the proposed method is verified by simulations and robotic cutting experiments.

关键词： Automatic groove cutting of intersecting pipes Model-driven robot path planning Plasma beam radius and taper compensation

A new nonfullerene acceptor with an extended π conjugation core enables ternary organic solar cells approaching 19%efficiency

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Nano Research 2024年第5期17卷 4062-4068页

作者： Chunyan Liu Nailiang qiu Zhengjin Li yan Lu School of Materials Science and Engineering Tianjin Key Laboratory for Photoelectric Materials and DevicesKey Laboratory of Display Materials and Photoelectric DevicesMinistry of EducationTianjin University of TechnologyTianjin 300384China School of Chemistry Chemical Engineering and MaterialsJining UniversityQufu 273155China

In organic solar cells(OSCs),it is an effective way to improve the power conversion efficiency(PCE)by adding a guest component with appropriate absorption and energy levels in the host ***,a new nonfullerene acceptor(NFA)named TBF-2.l was developed by the strategy of expanding theπconjugated core of 2.2.-(((4,4,9,9-tetrahexyl-4,9-dihydro-s-indaceno[1,2.b:5,6-b’]dithiophene-2.7-diyl)bis(methaneylylidene))bis(5,6-dichloro-3-oxo-2.3-dihydro-1H-indene-2.1-diylidene))dimalononitrile(IDT-4Cl)with two benzene *** increase of benzene units,TBF-2.l exhibits higher lowest unoccupied molecular orbital(LUMO)level of-3.75 eV than that of one benzene unit based NFA IDT-4Cl and fluorene core based NFA F-2.l,which facilitates enhancing the open-circuit voltage(V_(oc))of ternary ***,TBF-2.l film shows a medium optical bandgap with the absorption range from 500-800 nm,being well complementary with the wide bandgap polymer donor D18 and narrow bandgap NFA ***,a remarkable PCE of 18.92.with a high short-circuit current density(J_(sc))of 2..40 mA·cm^(-2.,a fill factor(FF)of 0.749,especially an outstanding V_(oc) of 0.92. V was achieved for the optimal ternary device based on D18:TBF-2.l:CH-6F,surpassing the binary counterpart(17.08%).The findings provide insight into the development of new guest acceptors for obtaining more efficient OSCs.

关键词： medium optical bandgap high lowest unoccupied molecular orbital(LUMO)level the third component ternary organic solar cell high open-circuit voltage

Clustering for Bivariate Functional Data

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Acta Mathematicae Applicatae Sinica 2024年第3期40卷 613-629页

作者： Shi-yun CAO yan-qiu ZHOU yan-ling WAN Tao ZHANG School of Science Guangxi University of Science and TechnologyLiuzhou 545006China School of Marxism Guangxi University of Science and TechnologyLiuzhou 545006China Key Laboratory of Intelligent Information Processing and Graph Processing Guangxi University of Science and TechnologyLiuzhou 545006China

In this paper,we consider the clustering of bivariate functional data where each random surface consists of a set of curves recorded repeatedly for each *** k-centres surface clustering method based on marginal functional principal component analysis is proposed for the bivariate functional data,and a novel clustering criterion is presented where both the random surface and its partial derivative function in two directions are *** addition,we also consider two other clustering methods,k-centres surface clustering methods based on product functional principal component analysis or double functional principal component *** results indicate that the proposed methods have a nice performance in terms of both the correct classification rate and the adjusted rand *** approaches are further illustrated through empirical analysis of human mortality data.

关键词： bivariate functional data -centres surface clustering functional principal component analysis partial derivative function

Fuzzy-Model-Based Finite Frequency Fault Detection Filtering Design for Two-Dimensional Nonlinear Systems

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IEEE/CAA Journal of Automatica Sinica 2024年第10期11卷 2099-2110页

作者： Meng Wang Huaicheng yan Jianbin qiu Wenqiang Ji Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationSchool of Information Science and EngineeringEast China University of Science and TechnologyShanghai 200237China Research Institute of Intelligent Control and Systems School of AstronauticsHarbin Institute of TechnologyHarbin 150080China School of Artificial Intelligence Hebei University of TechnologyTianjin 300401China IEEE

This article studies the fault detection filtering design problem for Roesser type two-dimensional(2.D)nonlinear systems described by uncertain 2.D Takagi-Sugeno(T-S)fuzzy ***,fuzzy Lyapunov functions are constructed and the 2.D Fourier transform is exploited,based on which a finite frequency fault detection filtering design method is proposed such that a residual signal is generated with robustness to external disturbances and sensitivity to *** has been shown that the utilization of available frequency spectrum information of faults and disturbances makes the proposed filtering design method more general and less conservative compared with a conventional nonfrequency based filtering design ***,with the proposed evaluation function and its threshold,a novel mixed finite frequency H_(∞)/H_(-)fault detection algorithm is developed,based on which the fault can be immediately detected once the evaluation function exceeds the ***,it is verified with simulation studies that the proposed method is effective and less conservative than conventional non-frequency and/or common Lyapunov function based filtering design methods.

关键词： Fault diagnosis finite frequency specifications mixed H_(∞)/H_(-)performance two-dimensional nonlinear systems

Colorimetric Detection of Acid Phosphatase and Malathion Using NiCo_(2.O_(4)Nanosheets as Peroxidase-Mimicking Activity

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Journal of Analysis and Testing 2024年第2期8卷 170-179页

作者： Jia Chen Zerong Long yan Li Hongdeng qiu Xinjiang Uygur Autonomous Product Quality Supervision and Inspection Institute Urumqi830000China CAS Key Laboratory of Chemistry of Northwestern Plant Resources and Key Laboratory for Natural Medicine of Gansu Province Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

The establishment of a low-cost and facile approach for the assay of acid phosphatase(ACP)and its inhibitor is a research *** this paper,we successfully synthesized NiCo_(2.O_(4)nanosheets with peroxidase-mimicking activity in alkaline deep eutectic solvents(DESs)composed of NaOH and PEG-2.0,which can catalyze 3,3',5,5'-tetramethylbenzidine(TMB)to the oxidation state TMB(ox-TMB)in the presence of *** to L-ascorbic acid-2.phosphate can be hydrolyzed into ascorbic acid by ACP,the peroxidase-like activity of NiCo_(2.O_(4)nanosheets is ***,the addition of malathion,an inhibitor of ACP,can inhibit the activity of ACP and thus limit the production of ascorbic acid(AA).Therefore,a colorimetric approach can be established for highly sensitive and selective detection of ACP and malathion with detection limits of 0.032.U/L and 0.65 nmol/L,*** importantly,this method can be successfully applied to malathion detection in environmental samples tap water and food cucumber juice,indicating that it has potential application prospects in environmental and agricultural fields.

关键词： NiCo_(2.O_(4)nanosheets Acid phosphatase Malathion Peroxidase-mimicking activity Colorimetric

Robust-augmentation nonlinear dynamic inversion control of over-actuated coaxial high-speed helicopter in transition mode

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Chinese Journal of Aeronautics 2024年第8期37卷 404-420页

作者： Yuqing qiu yan LI Jinxi LANG Yuxian LIU Zhong WANG School of Automation Northwestern Polytechnical UniversityXi’an 710129China

As the elevator and rudder can be used actively for control,in addition to the rotors,Coaxial High-speed Helicopters(CHHs)have the problems of control redundancy and changing control authority in the transition *** paper presents a robust-augmentation transitioning flight control design for a CHH under the adverse conditions of parametric uncertainties and external ***,based on control characteristic analysis,an Adaptive Filtered Nonlinear Dynamic Inversion(AFNDI)controller is proposed for the angular rate to handle the effect of unknown unstructured uncertainties and external *** analysis proves that the presented angular rate controller can guarantee steady-state and transient ***,the attitude angle and velocity controllers are also ***,an Incremental-based Nonlinear Prioritizing Control Allocation(INPCA)method is designed to take into account control surface transition and changing control authority,which efficiently distributes the required moments between coaxial rotors and aero-surfaces,and avoids the control reversal problem of the yaw *** the proposed control architecture,the low-pass filter is introduced to alleviate the adverse influence of time delay and measurement ***,the effectiveness of the proposed controller is demonstrated through nonlinear numerical simulations,and is compared with existing *** results show that the proposed control law can improve both capabilities of disturbance rejection and fast response,and works satisfactorily for the CHH transitioning control characteristic.

关键词： Coaxial high-speed helicopter Transition mode Attitude control Control allocation Robust adaptive control

Exceptional reversed yield strength asymmetry in a rare-earth free Mg alloy containing quasicrystal precipitates

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Journal of Magnesium and Alloys 2024年第2期12卷 687-699页

作者： Qiang yang Shuhui Lv Zixiang yan Zefeng Xie Xin {2. State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022PR China School of Materials Science and Engineering Changchun University of Science and Technology130022PR China

This work reports an exceptional reversed yield strength asymmetry at room temperature for a rare-earth free magnesium alloy containing a mass of fine dispersed quasicrystal(I-phase)*** exhibiting traditional basal texture,it owns an exceptional CYS/TYS as high as~*** back-scattered diffraction(EBSD)and transmission electron microscopy(TEM)examinations indicate pyramidal and prismatic dislocations plus tensile twinning being activated after immediate yielding in compression while basal and non-basal dislocations in tension.I-phase particles transferred the concentrated stress by self-twinning to provide the driving force for tensile twin initiating in neighboring grains,thereby significantly increasing the critical resolved shear stress of tensile twinning to possibly the level of pyramidal slip,finally leading to the dominance of pyramidal slip plus tensile twinning in texture *** results in a higher contribution on yield strength by~55 MPa in compression than in tension,which reasonably agrees with the experimental yield strength difference(~38 MPa).It can be concluded that I-phase particles influence deformation modes in tension and in compression,finally result in reversed yield strength asymmetry.

关键词： Magnesium alloy Reversed yield strength asymmetry Transmission electron microscopy(TEM) Twinning Dislocations

Electrochemistry and DFT study of galvanic interaction on the surface of monoclinic pyrrhotite(001)and galena(100)

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International Journal of Mining Science and Technology 2024年第8期34卷 1151-1162页

作者： Tingsheng qiu Kaiwei Ding Huashan yan Liu yang Hao Wu Guanfei Zhao Xianhui qiu College of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou 341000China Jiangxi Provincial Key Laboratory of Low-Carbon Processing and Utilization of Strategic Metal Mineral Resources Ganzhou 341000China Jiangxi Environmental Engineering Vocational College Ganzhou 341000China

The electrochemical interaction between galena and monoclinic pyrrhotite was investigated to examine its impact on the physical and chemical properties of the mineral *** investigation employed techniques such as electrochemistry,metal ion stripping,X-ray photoelectron spectroscopy,and quantum *** electrochemical test results demonstrate that the galena surface in the electro-couple system exhibits a lower electrostatic potential and higher electrochemical activity compared to the monoclinic pyrrhotite surface,rendering it more susceptible to oxidation *** pyrrhotite significantly amplifies the corrosion rate of the galena *** charge population calculations indicate that electrons are consistently transferred from galena to monoclinic pyrrhotite,with the number of electron transfers on the mineral surface increasing as the interaction distance *** analysis of state density revealed a shift in the surface state density of galena towards lower energy levels,resulting in decreased reactivity and increased difficulty for the reagent to adsorb onto the mineral ***,monoclinic pyrrhotite exhibited an opposite *** X-ray photoelectron spectroscopy(XPS)test results indicate that galvanic interaction leads to the formation of hydrophilic substances,PbS_(x)O_(y) and Pb(OH)_(2.,on the surface of ***,the surface of monoclinic pyrrhotite not only adsorbs Pb^(2.)but also undergoes S^(0) formation,thereby augmenting its hydrophobic nature.

关键词： Electrochemistry Galvanic interaction Monoclinic pyrrhotite Galena Density functional theory

First-principles study on the electronic structure of Pb_(10−x)Cu_(x)(PO_(4))_(6)O(x=0,1)

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Journal of Materials Science & Technology 2024年第4期171卷 66-70页

作者： Junwen Lai Jiangxu Li Peitao Liu yan Sun Xing-qiu Chen Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China

Recently,Lee et *** the experimental discovery of room-temperature ambient-pressure super-conductivity in a Cu-doped lead-apatite(LK-99)(arXiv:2.07.12.08,arXiv:2.07.12.37).Remarkably,the claimed superconductivity can persist up to 400 K at ambient *** the experimental im-plication,the electronic structure of LK-99 has not yet been ***,we investigate the electronic structures of LK-99 and its parent compound using first-principles calculations,aiming to elucidate the doping effects of *** results reveal that the parent compound Pb_(10)(PO_(4))_(6)O is an insulator,while Cu doping induces an insulator-metal transition and thus volume *** band structures of LK-99 around the Fermi level are featured by a half-filled flat band and a fully-occupied flat *** two very flat bands arise from both the 2. orbitals of 1/4-occupied O atoms and the hybridization of the 3d orbitals of Cu with the 2. orbitals of its nearest-neighboring O ***,we observe four van Hove singularities on these two flat ***,we show that the flat band structures can be tuned by including electronic correlation effects or by doping different *** find that among the considered doping elements(Ni,Cu,Zn,Ag,and Au),both Ni and Zn doping result in the gap opening,whereas Au exhibits doping effects more similar to Cu than *** work establishes a foundation for fu-ture studies to investigate the role of unique electronic structures of LK-99 in its claimed superconducting properties.

关键词： First-principles calculations Density functional theory Electronic structur e Superconductivity Flat bands Strongly correlated electrons

Simultaneous removal of 1,2.dichlorobenzene and furan over Mn-Ce-Fe oxide catalyst:Catalytic activity and product analysis

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Journal of Rare Earths 2024年第5期42卷 972-979,I0006页

作者： Juan qiu Minghui Tang Yaqi Peng Xuanhao Guo Shengyong Lu Jianhua yan Taizhou Institute of Zhejiang University Taizhou 318000China State Key Laboratory for Clean Energy Utilization Institute for Thermal Power EngineeringZhejiang UniversityHangzhou 310027China

The Mn-Ce-Fe mixed oxide(MCFe)was prepared by co-precipitation and the catalytic performance was tested by using 1,2.dichlorobenzene(1,2.DCB)and furan as model molecules of PCDD/*** effect of O_(2.concentration,SO_(2. and NO on the catalytic activity was *** 2.0℃,the MCFe oxide catalyst presents significant simultaneous removal efficiency of 75.2.%and 100%for 1,2.DCB and furan,***-Emmett-Teller(BET)method(BET),X-ray diffraction(XRD),scanning electron microscopy(SEM),X-ray photoelectron spectroscopy(XPS),Fourier transform infrared spectroscopy(FTIR),H_2.temperature programmed reduction(H_(2.-TPR),NH_(3)-temperature programmed desorption(NH_3-TPD)and O_(2.-TPD were used to characterize the catalysts before and after the *** tests suggest that the oxidation behavior of furan occurred prior to that of 1,*** to the intermediate products detected by gas chromatography-mass spectrometry(GC-MS),the by-products include chlorinated hydrocarbons,long-chain hydrocarbons,ketone,*** catalytic oxidation reaction paths are proposed.

关键词： 1 2.dichlorobenzene Furan Catalytic oxidation Product analysis Rare earths