检索结果-南通市图书馆

Rare Metals 2024年第9期43卷 4333-4343页

作者： Qiang Zhang Yuan-Hao Cheng Wei Liu hui-Nan Che yan-hui ao Key Laboratory of Integrated Regulation and Resource Development On Shallow Lakes Ministry of EducationCollege of EnvironmentHohai UniversityNanjing 210098China

The utilization of piezo-photocatalytic technol ogy for environmental remediation under full spectrum solar light is promising but still ***,one dimensional Bi_(2)S_(3)nanowires,which can utilize both mechanical energy and near-infrared(NIR)light to remov hexavalent chromium(Cr(Ⅵ))efficiently,were synthe sized by a restrained growth *** reaction rat constants of Cr(Ⅵ)reduction in piezo-photocatalyti process under NIR(800–2500 nm)reached 0.334 min^(-1)which were 3.2 and 12.4 times as that of single piezo and photocatalytic *** formation of polarized electri fields and one-dimensional structure allow ultrafast sepa ration of charge carriers,thereby promoting the catalyti ***,due to the strong penetrability o NIR light,the piezo-photocatalysis performance in turbid solutions under NIR light(0.188 min^(-1))was even com parable to that under visible light(0.186 min^(-1)).Thi study provides a new concept on the development of piezo photocatalytic technology for environmental remediation by utilization of NIR light and natural mechanical energy.

关键词： Piezo-photocatalysis NIR light Bi_(2)S_(3)nanowires Cr(Ⅵ)

Ultrafast photocatalytic degradation of nitenpyram by 2D ultrathin Bi2WO6:mechanism,pathways and environmental factors

在线全文

学校读者我要写书评

暂无评论

Rare Metals 2022年第7期41卷 2439-2452页

作者： Yuan-Hao Cheng Juan Chen hui-Nan Che yan-hui ao Bin Liu Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes of Ministry of Education College of EnvironmentHohai UniversityNanjing 210098China School of Chemical and Biomedical Engineering Nanyang Technological UniversitySingapore 637459Singapore

As a common insecticide,nitenpyram(NTP)seriously threatens the human health and environmental *** this work,a visible-light-responsive photocata-lyst two-dimensional(2D)Bi_(2)WO_(6) was synthesized and applied to degrade *** with bulk Bi_(2)WO_(6),the 2D Bi_(2)WO_(6)exhibits better photocatalytic performance for NTP degradation under visible-light *** enhanced activity can be ascribed to the unique 2D struc-ture which would induce to higher efficiency of carrier ***,hole(h+)plays a major role(and·O^(2-))in the degradation of *** on the interme-diates detected by high-performance liquid chromatogra-phy-mass spectrometry(HPLC-MS),the degradation pathway of NTP was *** addition,the influence of typical environmental factors(pH,water matrix,inorganic cations and common anions)on the degradation of NTP was also *** work not only helps people to understand the degradation of pesticides in actual water bodies,but also provides reference for the subsequent treatment of agricultural wastewater.

关键词： Photocatalysis Two-dimensional(2D)Bi_(2)WO_(6) Nitenpyram Degradation pathway

Modular assembly of Co4-thiacalix[4]arene units and Keggin-type SiW12O40 for visible-light photothermal conversion

在线全文

学校读者我要写书评

暂无评论

Tungsten 2025年第1期7卷 112-119页

作者： Jia-hui Li Qing Zhao Dong-ao Mao Kun Zhou Bao-Kuan Chen yan-Feng Bi School of Petrochemical Engineering Liaoning Petrochemical University

The construction of metal-organic coordination clusters（MCCs） using modular secondary building units is an important method for preparing functional *** this study,two new MCCs modularly assembled from Keggin-type {SiW12O40}H4TC4A=p-tert-Butylthiacalix[4]arene(SiW12) units and thiacalixarene-supported Co4-thiacalix[4]arene(Co4-TC4A polynuclear second-building units（PSBUs,H4TC4A=p-tert-Butylthiacalix[4]arene） are *** two MCCs,abbreviated as Co4-SiW12and Co8-SiW12,were structurally characterized by single-crystal X-ray *** Co4-SiW12is a supramolecular structure involving cation-anion interactions between Co4-TC4A PSBUs and ***8-SiW12features "barbell-like" shapes with two Co4-TC4A coordinatively linked to a Keggin-type SiW12unit on opposite via W-O_t-Co *** coordination of Co4-TC4A to SiW12in Co8-SiW12resulted in significantly improved photothermal conversion performances compared with Co4-SiW12and pure SiW12or ***-gap determination and photophysical analysis combined with density functional theory calculations indicated the binding mode between Co4-TC4A PSBUs and SiW12,which considerably influences the way of electron transport and the conversion ability of visible light to heat.

关键词： Modular construction Photothermal conversion Polyoxometalate Thiacalixarene

The interaction between KIF21A and KANK1 regulates dendritic morphology and synapse plasticity in neurons

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Neural Regeneration Research 2025年第1期20卷 209-223页

作者： Shi-yan Sun Lingyun Nie Jing Zhang Xue Fang Hongmei Luo Chuanhai Fu Zhiyi Wei Ai-hui Tang Hefei National Research Center for Physical Sciences at the Microscale CAS Key Laboratory of Brain Function and DiseaseMinistry of Education Key Laboratory for Membrane-less Organelles and Cellular DynamicsDivision of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefeiAnhui ProvinceChina CAS Center for Excellence in Molecular Cell Sciences Division of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Department of Neurobiology School of Life SciencesSouthern University of Science and TechnologyShenzhenGuangdong ProvinceChina Brain Research Center Southern University of Science and TechnologyShenzhenGuangdong ProvinceChina

Morphological alterations in dendritic spines have been linked to changes in functional communication between neurons that affect learning and ***-4 KIF21A helps organize the microtubule-actin network at the cell cortex by interacting with KANK1;however,whether KIF21A modulates dendritic structure and function in neurons remains *** this study,we found that KIF21A was distributed in a subset of dendritic spines,and that these KIF21A-positive spines were larger and more structurally plastic than KIF21A-negative ***,the interaction between KIF21A and KANK1 was found to be critical for dendritic spine morphogenesis and synaptic *** of either KIF21A or KANK1 inhibited dendritic spine morphogenesis and dendritic branching,and these deficits were fully rescued by coexpressing full-length KIF21A or KANK1,but not by proteins with mutations disrupting direct binding between KIF21A and KANK1 or binding between KANK1 and *** down KIF21A in the hippocampus of rats inhibited the amplitudes of long-term potentiation induced by high-frequency stimulation and negatively impacted the animals’cognitive *** together,our findings demonstrate the function of KIF21A in modulating spine morphology and provide insight into its role in synaptic function.

关键词： actin cytoskeleton dendrite KANK1 KIF21A microtubule spine morphology spine synaptic plasticity talin1

MoS2 synaptic transistor with one-step manufacture

在线全文

学校读者我要写书评

暂无评论

Science China(Information Sciences) 2025年第1期68卷 357-365页

作者： Yihao GUO yang WANG Wenjie DENG Yi WU Jingtao LI Kexin LI Yuehui ZHao Songlin YU Xiaoting WANG Yongzhe ZHANG hui yan Key Laboratory of Optoelectronics Technology of Education Ministry of China Faculty of Information TechnologyBeijing University of Technology Key Laboratory of Advanced Functional Materials Ministry of Education Faculty of Materials and ManufacturingBeijing University of Technology The 11th Research Institute of Electronics Technology Group Corporation

The synaptic transistor,which is a neuromorphic device with brain-like functions,has garnered significant attention due to characteristics such as low energy consumption,high integration,multiple functions,and high computational ***,the current synaptic transistor possesses a complicated structure and involves complex manufacturing steps,which is not conducive to low-cost,large-scale bionic ***,we introduce a simple MoS2synaptic transistor exhibiting robust synaptic *** transistor utilizes magnetron sputtering manufacture to combine the process of device metal electrode deposition and the introduction of defect states,which helps streamline the manufacturing process into a single *** long-term potentiation and long-term depression in photoelectric coordination are initially ***,biological functions,such as double pulse facilitation and the transformation behavior of short-term memory to long-term memory,are thoroughly evaluated,along with learning-forgetting-relearning ***,the device exhibits robust synaptic plasticity until incident light angles down to 30° to imitate the multi-to-one axon-cellular ***,a classical simulation of Pavlov's dog conditioned reflex is demonstrated along with the multiview extraction *** experimental results demonstrate a promising synaptic transistor with a simple structure,manufacturing technique,and excellent *** further indicates the potential for large-scale integration of bionic neuromorphic systems.

关键词： process optimization artificial synaptic device one-stepmanufacture synaptic plasticity bionic simulation

同方期刊数据库

A robust and transparent nanosilica-filled silicone rubber coating with synergistically enhanced mechanical properties and barrier performance

在线全文

学校读者我要写书评

暂无评论

Journal of Materials Science & Technology 2023年第20期151卷 219-226页

作者： Shiyao Du hui yan Zihe Liu ao Tang Ying Li Institute of Metal Research Chinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China Shenyang National Laboratory for Materials Science Northeastern UniversityShenyang 110819China

Implantable electronic devices(IEDs)are widely used by human beings to achieve medical treatment and diagnosis ***,ideal encapsulation of IEDs is still far from perfect as full prevention of body fluid diffusion into the coating remains ***,we develop a high-performance composite coating for IED encapsulation by introducing SiO_(2) nanoparticles into silicone rubber,which synergistically enhances mechanical properties and improves barrier *** fabricating composite coatings with different nanosilica contents,3%nanosilica is proved to be an optimal additive content with an excellent combination of improved fracture strength(from 2.5 MPa to 4.5 MPa),increased coating resistance(from 10^(4) to 10^(9) cm^(2))and ideal coating *** and electrochemical characterizations subsequently confirm substantially enhanced mechanical properties and barrier performance of the composite coating,which effectively resist crack propagation and impede penetrations of water and chloride ions through the *** calculations further uncover that modified SiO_(2) particles with enriched methyl groups endow a strong bridging effect to interact with silicone rubber monomer,which,together with anti-agglomeration property of methyl groups,contributes to a pronounced improvement in mechanical performance of nanosilica-filled silicone *** from the enhanced mechanical and barrier properties,the as-fabricated nanosilica-filled silicone rubber demonstrates superior protection for the encapsulated circuits with a significantly improved lifetime(709.1 h)compared to that of circuits coated by pure silicone rubber(472.8 h)and bare circuit boards(1 h),which offers great values for packaging material design in future IED encapsulation.

关键词： Organic coatings Implantable electronic devices Nanosilica DFT calculation Mechanical property

Based on non-targeted metabolomics for differential components screening of Rosae Chinensis Flos and Rosae Rugosae Flos and their quality evaluation

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Traditional Medicine Research 2025年第2期10卷 1-15页

作者： Xu Liang Ni-hui Zhang Zhi-Lai Zhan Guang-Lu Chang yan Gao Xia Li Wen-Yuan Gao School of Pharmaceutical Science and Technology Faculty of MedicineTianjin UniversityTianjin 300193China State Key Laboratory for Quality Ensurance and Sustainable Use of Dao-di Herbs China Academy of Chinese Medical SciencesBeijing 100700China Key Laboratory of Modern Chinese Medicine Resources Research Enterprises Tianjin 300402China

Background:Rosa chinensis *** Rosa rugosa *** not only of ornamental value,but also edible flowers and the flower buds have been listed in the Chinese Pharmacopoeia as traditional *** two plants have some differences in efficacy,but the flower buds are easily confused for similar *** addition,large-scale cultivation of ornamental rose flowers may lead to a decrease in the effective components of medicinal ***,it is necessary to study the chemical composition and make quality evaluation of Rosae Chinensis Flos(Yueji)and Rosae Rugosae Flos(Meigui).Methods:In this study,40 batches of samples including Meigui and Yueji from different regions in China were collected to establish high-performance liquid chromatography ***,the fingerprints data was analyzed using principal component analysis,hierarchical cluster analysis,and partial least squares discriminant analysis analysis chemometrics to obtain information on intergroup differences,and non-targeted metabolomic techniques were applied to identify and compare chemical compositions of samples which were chosen from groups with large *** compounds were screened by orthogonal partial least-squares discriminant analysis and S-plot,and finally multi-component quantification was performed to comprehensively evaluate the quality of Yueji and ***:The similarity between the fingerprints of 40 batches roses and the reference print R was 0.73 to 0.93,indicating that there were similarities and differences between the *** principal component analysis and hierarchical cluster analysis of fingerprints data,the samples from different origins and varieties were intuitively divided into four *** least-squares discriminant analysis analysis showed that Meigui and Yueji cluster into two categories and the model was reliable.A total of 89 compounds were identified by high resolution mass spectrometry,mainly were flavonoids and flavon

关键词： Rosa chinensis Jacq. Rosa rugosa Thunb. metabolomics chemometrics multiple component quantification quality evaluation

CALCULATION OF ELASTIC DAMPING CHARACTERISTICS OF ROTOR SUPPORT MADE OF METAL RUBBER MATERIAL UNDER VARIABLE LOADS

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Mechanical Engineering 2007年第6期20卷 33-37页

作者： JIANG Hongyuan yan hui ao Hongrui ALEXANDER M Ulanov School of Mechatronics Engineering Harbin Institute of Technology Harbin 150001 China Department of Aircraft and Engine Structure Design Samara State Aerospace University Samara 443086 Russia

A metal rubber（MR） dry friction damper was designed based on the load supported by the rotor. An experimental apparatus for obtaining hysteresis loops of support under the precession load was designed. The elastic-damping characteristics of the ring-shaped MR damper used as a rotor support under variable loads were presented by studying the hysteresis loops of the damper. The vibration rigidity and the energy dissipation coefficient were calculated from the hysteresis loops, based on the description of the deformation process of the MR element with simple structure in a dimensionless coordinating system. The calculation results showed that the energy dissipation coefficient in the inner of MR element and on the boundary between the damper and the frame of the rotor support were approximately equal. The comparison of the hysteresis loops for a precession load and a one-axial load indicated a large difference when the coefficient of the energy dissipation and the stiffness of the MR damper were concerned.

关键词： Rotor support Precession load Stiffness Energy dissipation coefficient Metal rubber

In situ growth of NiSe@Co_(0.85)Se heterointerface structure with electronic modulation on nickel foam for overall water splitting

在线全文

学校读者我要写书评

暂无评论

Rare Metals 2021年第6期40卷 1373-1382页

作者： Wen-Long Ding yan-hui Cao hui Liu ao-Xuan Wang Cui-Juan Zhang Xue-Rong Zheng Key Laboratory for Green Chemical Technology of Ministry of Education State Key Laboratory of Chemical EngineeringSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China Department of Physics and Astronomy University of CaliforniaIrvineCA 92697USA Tianjin Kaben New Materials Technology Co. Ltd.Tianjin 300350China

Constructing heterointerface engineering has becoming an effective and general strategy for developing highly efficient and durable nonnoble electrocatalysts for catalyzing both hydrogen evolution reaction(HER)and oxygen evolution reaction(OER).In this work,we synthesized a self-supporting heterogeneous NiSe@Co_(0.85)Se/NF electrocatalyst using a facile in situ selenization of transition metal precursors that coated on the nickel foam(NF)in polyol *** NF was used as both conductive substrate and nickel source,ensuring superior electronic conductivity for *** NiSe@-Co_(0.85)Se/NF exhibited remarkable bifunctional electrocatalytic activities with HER overpotential of 168 mV and OER overpotential of 258 mV to achieve 10 mA·*** water splitting system using NiSe@Co_(0.85)Se/NF as both anode and cathode electrodes achieved a current density of 10 mA·cm^(-2) at 1.61 V with nearly 100% faradaic efficiency and impressively long-term *** efficient bifunctional catalytic performance of NiSe@-Co_(0.85)Se/NF should be attributed to the electronic modulation and synergistic effect between NiSe and Co_(0.85)Se,the intrinsic metallic conductivity and the enlarged active sites *** work provides a facile method for developing heterogeneous bifunctional catalysts for advanced electrochemical energy conversion technologies.

关键词： NiSe@Co_(0.85)Se/NF Heterointerface structure Electronic modulation Bifunctional electrocatalyst Overall water splitting

噻吩酰亚胺衍生物二阶非线性光学性质的DFT研究

在线全文

学校读者我要写书评

暂无评论

原子与分子物理学报 2025年第1期42卷 20-28页

作者：蔺彬彬闫慧君哈尔滨学院食品工程学院化学系哈尔滨150086

采用密度泛函理论(DFT)CAM-B3LYP方法,计算研究了12个设计的噻吩酰亚胺衍生物的电子光谱和二阶非线性光学性质.结果表明,此类化合物有较大的第一超极化率β_(tot)值和β_(vec)值,且β_(tot)值和β_(vec)值随引入氰基数目的增加而显著增... 详细信息

采用密度泛函理论(DFT)CAM-B3LYP方法,计算研究了12个设计的噻吩酰亚胺衍生物的电子光谱和二阶非线性光学性质.结果表明,此类化合物有较大的第一超极化率β_(tot)值和β_(vec)值,且β_(tot)值和β_(vec)值随引入氰基数目的增加而显著增大.给/吸电子基团引起的电荷转移变化对体系β_(tot)值和β_(vec)值的影响大于分子六元杂环中N杂原子位置变化对其影响.

关键词：噻吩酰亚胺衍生物密度泛函理论二阶非线性光学性质电子光谱

维普期刊数据库博看期刊