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Molecular Dynamics Simulation of Shock Response of CL-20 Co-crystals Containing Void Defects

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Defence Technology（防务技术） 2024年第1期31卷 364-374页

作者： Changlin Li Wei Yang Qiang Gan yajun wang Lin Liang Wenbo Zhang Shuangfei Zhu Changgen Feng State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China School of Materials Science&Engineering Beijing Institute of TechnologyBeijing 100081China

To investigate the effect of void defects on the shock response of hexanitrohexaazaisowurtzitane(CL-20)co-crystals,shock responses of CL-20 co-crystals with energetic materials ligands trinitrotoluene(TNT),1,3-dinitrobenzene(DNB),solvents ligands dimethyl carbonate(DMC) and gamma-butyrolactone(GBL)with void were simulated,using molecular dynamics method and reactive force *** is found that the CL-20 co-crystals with void defects will form hot spots when impacted,significantly affecting the decomposition of molecules around the *** degree of molecular fragmentation is relatively low under the reflection velocity of 2 km/s,and the main reactions are the formation of dimer and the shedding of nitro *** existence of voids reduces the safety of CL-20 co-crystals,which induced the sensitivity of energetic co-crystals CL-20/TNT and CL-20/DNB to increase more *** has occurred under the reflection velocity of 4 km/s,energetic co-crystals are easier to polymerize than solvent co-crystals,and are not obviously affected by *** results show that the energy of the wave decreases after sweeping over the void,which reduces the chemical reaction frequency downstream of the void and affects the detonation performance,especially the solvent co-crystals.

关键词： CL-20 co-crystals Molecular dynamics simulation Reactive forcefield Impact response Hot spot Void defect

Evaluation of the Oxidation Reactivity and Behavior of Exhaust Soot Particles from Diesel Engines with Different Emission Levels

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China Petroleum Processing & Petrochemical Technology 2024年第2期26卷 72-80页

作者： wang yajun Lin Lei Xing Jianqiang LüXu Yang He Song Haiqing SINOPEC Research Institute of Petroleum Processing Co. Ltd.Beijing 100083China State Key Laboratory of Engines Tianjin UniversityTianjin 300072China

The aim of this study was to investigate the oxidation reactivity and behavior of exhaust particulate matter(PM)from diesel *** samples from two diesel engines(1K,CY4102)with different emission levels were collected by a thermophoretic system and a quartz *** oxidation reactivity,oxidation behaviors,and physicochemical properties of the PM samples were analyzed using thermogravimetric analysis(TGA),high-resolution transmission electron microscopy(HRTEM),Fourier-transform infrared spectrometry(FTIR),and Raman *** results showed that there was a great difference in the oxidation reactivity of soot particles emitted by the two different diesel engines.A qualitative analysis of the factors influencing oxidation reactivity showed that the nanostructure,degree of graphitization,and relative concentration of aliphatic C—H functional groups were the most important factors,whereas no significant correlation was found between the primary particle size and activation energy of the diesel *** on the oxidation behavior analysis,the diesel soot particles exhibited both internal and surface oxidation modes during the oxidation *** oxidation was dominant during the initial stage,and as oxidation progressed,the mode gradually changed to internal *** oxidation mode of soot particles from the 1K engine was significantly higher than that of CY4102.

关键词： diesel engine soot particles oxidation reactivity oxidation behavior

Liquid-metals-induced formation of MXene/polyacrylamide composite organohydrogels for wearable flexible electronics

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Nano Research 2024年第3期17卷 1913-1922页

作者： Minying Wu Bin Chen Xueliang Fan Tong Ye Yuanyuan Fang Qian Zhang Fangzhou Zhou yajun wang Yi Tang Department of Chemistry Fudan UniversityShanghai 200433China College of Chemistry&Materials Engineering Wenzhou UniversityWenzhou 325027China

Organohydrogels have demonstrated superior environmental adaptability and frost resistance compared to conventional hydrogels,thereby prompting considerable interests in the development and design of innovative ***,we report an effective one-pot method for fabricating MXene/polyacrylamide(MXene/PAM)composite organohydrogel(MAOH)by employing Ga liquid metals(Ga LMs)as a highly reactive component in the induced free radical polymerization reaction,without the need for additional heating or cross-linking *** synthetic protocol addresses the time-consuming and organic solvent waste concerns associated with traditional solvent displacement methods for organohydrogel *** incorporation of MXene not only highly enhances the conductivity but also confers improved mechanical properties of *** MAOH exhibits excellent environmental adaptability(>7 d),sustained moisture retention,remarkable self-healing capabilities,and outstanding mechanical properties under low temperatures(-20℃).It demonstrates exceptional performance in micro-motion monitoring,rapid response time(125 ms),superior stretchability,and a broad range of strains(0.3%–600%).Therefore,the designed MAOH has great potential for applications in diverse fields such as prosthetics,electronic skin,human–machine interaction,and smart terminals.

关键词： organohydrogels MXene conductivity mechanical properties environmental adaptability

Comprehensive genomic analysis of early and late-onset hepatocellular carcinoma

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Genes & Diseases 2024年第4期11卷 77-81页

作者： Jialin Yang Chao Chen Song wang Yaru Zhang Jiaohui Pang yajun wang Qiuxiang Ou Hao Jiang Juying Liu Department of Radiation Oncology Sichuan Cancer Hospital&InstituteSichuan Cancer CenterSchool of MedicineUniversity of Electronic Science and Technology of ChinaChengduSichuan 610041China Jinling Hospital Department of OncologyNanjing Medical UniversityNanjingJiangsu 210002China Geneseeq Research Institute Nanjing Geneseeq Technology Inc.NanjingJiangsu 210000China Department of Oncology Haian Hospital of Traditional Chinese MedicineHaianJiangsu 226600China Interventional Therapy Department Jiangsu Cancer Hospital&Jiangsu Institute of Cancer Research&The Affiliated Cancer Hospital of Nanjing Medical UniversityNanjingJiangsu 210009China

Hepatocellular carcinoma(HCC)is the major histologic type of primary liver cancer,accounting for approximately 75%of liver cancer cases.'Despite many advancements in its treatment,the prognosis and drug response of HCC patients are ***,there is an unmet clinical need to explore genomic aberrations underlying early-and lateonset HcC,which might facilitate drug discovery and provide personalized biomarker-driven treatment options for these patients.

关键词： patients prognosis cancer

Impact of Different Rates of Nitrogen Supplementation on Soil PhysicochemicalProperties and Microbial Diversity in Goji Berry

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Phyton-International Journal of Experimental Botany 2024年第3期93卷 467-486页

作者： Xiaojie Liang Wei An Yuekun Li yajun wang Xiaoya Qin Yanhong Cui Shuchai Su State Key Laboratory of Efficient Production of Forest Resources The College of ForestryBeijing Forestry UniversityBeijing100083China National Wolfberry Engineering Research Center Wolfberry Science Research InstituteNingxia Academy of Agriculture and Forestry SciencesYinchuan750002China

Goji berry(Lycium barbarum L.)is substantially dependent on nitrogen fertilizer application,which can signiﬁ-cantly enhance fruit yield and Goji berry industrial development in Ningxia,*** study aimed to analyze the functions of differential nitrogen application rates including low(N1),medium(N2),and high(N3)levels in soil microbial community structure(bacterial and fungal)at 2 diverse soil depths(0-20,20-40 cm)through high-throughput sequencing technology by targeting 16S RNA gene and ITS1&ITS2 *** the observed physicochemical parameters exhibited signiﬁcant improvement(p0.05)differences among three group treatments(N1,N2,and N3).Furthermore,the functional enrichment analysis demonstrated signiﬁcant(p<0.05)enrichment of quorum sensing,cysteine and methionine metabolism,and transcriptional machinery for bacterial communities,while various saprotrophic functional roles for fungal ***,moderately reducing the use of N-supplemented fertilizers is conducive to increasing soil nitrogen utilization rate,which can contribute to sustainable agriculture practices through improved soil quality,and microbial community structure and functions.

关键词： Goji berry production Ningxia,China differential nitrogen supplementation rates 16S RNA gene and IT1&IT2 region sequencing soil physicochemical properties

Highly dispersed Ru nanospecies on N-doped carbon/MXene composite for highly efficient alkaline hydrogen evolution

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Chinese Chemical Letters 2024年第4期35卷 153-159页

作者： Minying Wu Xueliang Fan Wenbiao Zhang Bin Chen Tong Ye Qian Zhang Yuanyuan Fang yajun wang Yi Tang Department of Chemistry Shanghai Key Laboratory of Molecular Catalysis and Innovative Materialsand Laboratory of Advanced MaterialsFudan UniversityShanghai 200438China College of Chemistry&Materials Engineering Wenzhou UniversityWenzhou 325027China

Hydrogen has emerged as a promising environmentally friendly energy source. The development of lowcost, highly active, stable, and easily synthesized catalysts for hydrogen evolution reactions(HER) remains a significant challenge. This study explored the synthesis of nitrogen-doped MXene-based composite catalysts for enhanced HER performance. By thermally decomposing RuCl_(3) coordinated with melamine and formaldehyde resin, we successfully introduced nitrogen-doped carbon(N–C) with highly dispersed ruthenium(Ru) onto the MXene surface. The calcination temperature played a crucial role in controlling the size of Ru nanoparticles(Ru NPs) and the proportion of Ru single-atom(Ru SA), thereby facilitating the synergistic enhancement of HER performance by Ru NPs and Ru SA. The resulting catalyst prepared with a calcination temperature of 600℃, Ti_(3)C_(2)T_x-N/C-Ru-600(TNCR-600), exhibited exceptional HER activity(η10= 17 m V) and stability(160 h) under alkaline conditions. This work presented a simple and effective strategy for synthesizing composite catalysts, offering new insights into the design and regulation of high-performance Ru-based catalysts for hydrogen production.

关键词： HER activity Highly dispersed Ru-based catalysts MXene Alkaline condition

Emergence of highly pathogenic avian influenza A(H5N8)clade 2.3.4.4b viruses in grebes in Inner Mongolia and Ningxia,China,in 2021

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Journal of Integrative Agriculture 2024年第1期23卷 348-353页

作者： Qiuzi Xu Xinru Lü Yi Li Hua Luo Zhen Zhang Xiang Li Rongxiu Qin Qing An Fengyi Qu Zhenliang Zhao Chengbo Zhang Weidong wang Yuecheng Li yajun wang Xiangwei Zeng Zhijun Hou Jingqiang Ren Yulong wang Yanbing Li Hongliang Chai College of Wildlife and Protected Area Northeast Forestry UniversityHarbin 150040China Harbin Veterinary Research Institute Chinese Academy of Agricultural SciencesHarbin 150040China Wenzhou Key Laboratory for Virology and Immunology Institute of VirologyWenzhou UniversityWenzhou 325000China Ordos Forestry and Grassland Administration Ordos 017000China Monitoring Center for Terrestrial Wildlife Epidemic Diseases Yinchuan 750000China

Highly pathogenic avian influenza(HPAI)subtype H5Nx viruses have spread globally and are a major concern for poultry,wild birds,mammals,and even humans(de Vries et al.2015;Zeng et al.2022).The hemagglutinin(HA)genes of H5 subtype viruses have evolved into multiple clades and some of these clades have been further divided into subclades(Cui et al.2022).Clade 2.***.4.4H5N8 HPAI viruses(HPAIVs)have caused several waves of disease outbreaks in wild birds and domestic poultry(wang et al.2022).

关键词： poultry Ningxia influenza

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教师拓展性学习的理论解析与实践检证

教育研究与实验 2024年第4期 87-96页

作者：王亚军四川师范大学基础教育研究院成都610066

无论是职前的“研中习”,还是职后的“教中学”,这两种教师养成模式常陷入理论与实践二维背离的窠臼。拓展性学习理论力求弥合二者的裂痕,把学习视为一种活动,主张将之置于多元素共构的“活动系统”中考察;视为一种拓展,即一种新概念和... 详细信息

无论是职前的“研中习”,还是职后的“教中学”,这两种教师养成模式常陷入理论与实践二维背离的窠臼。拓展性学习理论力求弥合二者的裂痕,把学习视为一种活动,主张将之置于多元素共构的“活动系统”中考察;视为一种拓展,即一种新概念和新实践活动生成的知识创新和集体行动;视为一种循环,即一种基于矛盾驱动的拓展圈循环。循此理路,教师拓展性学习在价值上是对不确定性的寻绎;在空间上它发生于“个体-团队-组织”多级学习网络;在时间上它发生于打破“过去-现在-未来”的边界中。而设定学习目标,统整教师发展与学校绩效;规制学习过程,统一知识集体创新与知识迁移运用;创构学习中介,运用四级矛盾和形成性干预驱动学习,能够勾勒教师拓展性学习的生发机制,建构一个强调社群学习、知识创生和实践转化连续统一的教师拓展性学习模型。

关键词：教师学习拓展性学习知识共创学习中介

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基于边缘计算的船舶通信网络负载均衡研究

中国造船 2024年第3期65卷 122-134页

作者：张博文马国军王亚军江苏科技大学海洋学院镇江212003

在边缘计算环境中,随着任务数量的增加,船舶通信网络服务器节点会出现负载不均衡的现象,针对此问题,提出了一种基于改进蚁群和帝国竞争算法相融合的任务调度算法。首先在蚁群算法中设计负载均衡因子优化启发函数,改善低负载节点的选择问... 详细信息

在边缘计算环境中,随着任务数量的增加,船舶通信网络服务器节点会出现负载不均衡的现象,针对此问题,提出了一种基于改进蚁群和帝国竞争算法相融合的任务调度算法。首先在蚁群算法中设计负载均衡因子优化启发函数,改善低负载节点的选择问题,在信息素更新时引入精英蚂蚁策略,加快算法收敛速度;其次将帝国竞争算法得到的最优解集映射到蚁群算法的信息素初始化分布上;最后调用改进的蚁群算法选取性能较好的服务器节点,以实现船舶通信网络的负载均衡。试验结果表明,相比于其他任务调度算法,所提算法减少了任务执行时间和设备能耗,并且能够降低船舶通信网络系统开销,提高负载均衡度。

关键词：边缘计算船舶通信网络负载均衡蚁群算法帝国竞争算法