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Design and construction of size-controlled CoO/CS catalysts for Fischer–Tropsch synthesis

Nano Research 2024年第4期17卷 2520-2527页

作者： Wei Sun Ting Kuang Guiyou Wei Yue Li yaqin Liu Shuai Lyu Yuhua Zhang Jinlin Li Li Wang Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education&Hubei Key Laboratory of Catalysis and Materials Science South-Central Minzu UniversityWuhan 430074China Hubei Key Laboratory of Biomass Fibers and Eco-dyeing&Finishing College of Chemistry and Chemical EngineeringWuhan Textile UniversityWuhan 430200China

The use of supported Co-based catalysts is widespread in various catalytic reactions due to their unique *** structural sensitivity of these catalysts is closely linked to their particle size and crystal ***,comprehending the structure–activity relationship requires the development of well-defined Co-based ***,we employed a colloidal wet chemical process and a heterogeneous nucleation method to prepare well-defined Co-based catalysts supported by inert carbon *** nanospheres’surface possesses abundant functional groups that efficiently capture metal complexes and facilitate the nucleation and growth of CoO *** adjusting the Co source concentration,solvent molar ratio,and nucleation growth kinetics,we successfully prepared CoO/carbon sphere(CS)catalysts with different particle sizes and crystal *** influence of metallic face-centered cubic(fcc)-Co^(0) particle size in the range of 6.6–17.6 nm on the performance of Fischer–Tropsch synthesis(FTS)using well-defined CoO/CS catalysts has been *** result demonstrated that the turnover frequency(TOF)remained constant for CoO/CS catalysts with metallic fcc-Co^(0) particle size larger than 7.7 ***,both the selectivity and the activity changed for CoO/CS catalysts with smaller particles(<7.7 nm).Significantly,when metallic fcc-Co^(0) particle size was reduced from 17.6 to 7.7 nm,the cobalt time yield increased to 6.7μmolCO·gCo^(-1)·s^(-1),indicating improved catalytic *** the same time,the CH_(4) selectivity decreased to 4.9%,suggesting a higher preference for hydrocarbon *** findings demonstrate the importance of particle size in Co catalyzed Fischer–Tropsch *** use of well-defined CoO/CS catalysts offers valuable insights into the structure–activity relationship,leading to a better understanding of Co catalyzed Fischer–Tropsch synthesis.

关键词： Fischer–Tropsch synthesis(FTS) cobalt size effects phase effects carbon nanospheres

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Manipulating the Macroscopic and Microscopic Morphology of Large-Area Gravure-Printed ZnO Films for High-Performance Flexible Organic Solar Cells

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Energy & Environmental Materials 2024年第2期7卷 229-239页

作者： Zhenguo Wang Jingbo Guo yaqin Pan Jin Fang Chao Gong Lixin Mo Qun Luo Jian Lin Changqi Ma School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026China i-Lab&Printable Electronics Research Center Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of Sciences(CAS)Suzhou 215123China Beijing Engineering Research Center of Printed Electronics Beijing Institute of Graphic CommunicationBeijing 102600China Jiangxi Institute of Nanotechnology Chinese Academy of Sciences(CAS)Nanchang 330200China

Gravure printing is a promising large-scale fabrication method for flexible organic solar cells(FOSCs)because it is compatible with two-dimension patternable roll-to-roll ***,the unsuitable rheological property of ZnO nanoinks resulted in unevenness and looseness of the gravure-printed ZnO interfacial *** we propose a strategy to manipulate the macroscopic and microscopic of the gravure-printed ZnO films through using mixed solvent and poly(vinylpyrrolidone)(PVP)*** regulation of drying speed effectively manipulates the droplets fusion and leveling process and eliminates the printing ribbing structure in the macroscopic *** additive of PVP effectively regulates the rheological property and improves the microscopic compactness of the *** this method,large-area ZnO∶PVP films(28×9 cm^(2))with excellent uniformity,compactness,conductivity,and bending durability were *** power conversion efficiencies of FOSCs with gravure-printed AgNWs and ZnO∶PVP films reached 14.34%and 17.07%for the 1 cm^(2)PM6:Y6 and PM6∶L8-BO flexible *** efficiency of 17.07%is the highest value to date for the 1 cm^(2)*** use of mixed solvent and PVP addition also significantly enlarged the printing window of ZnO ink,ensuring high-quality printed thin films with thicknesses varying from 30 to 100 nm.

关键词： flexible organic solar cell gravure printing large-area flexible interfacial layer rheology properties zinc oxide

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Large-Area Gravure-Printed AgNWs Electrode on Water/Oxygen Barrier Substrate for Long-Term Stable Large-Area Flexible Organic Solar Cells

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Chinese Journal of Chemistry 2024年第5期42卷 478-484页

作者： Hao Wang yaqin Pan Yunfei Han Zhuo Chen Tianyu Liu Lianping Zhang Qun Luo Chang-Qi Ma Printable Electronics Research Center & i-Lab Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of Sciences (CAS)SuzhouJiangsu215123 China Nano Science and Technology Institute University of Science and Technology of China166 Ren Ai RoadSEID SIPSuzhouJiangsu215123 China

Large-area AgNWs electrodes(25 cm×10 cm)were fabricated through roll-to-roll printing on the polyvinyl alcohol(PVA)modified water and oxygen barrier *** modification of the barrier film with PVA improved the wettability of silver nanowires on the barrier films and led to the formation of homogenous large-area AgNWs *** mechanical flexibility,especially the adhesion force between the silver electrode and the barrier film substrate was dramatically improved through PVA *** efficiency of 13.51%for the flexible OSCs with an area of 0.64 cm2 was achieved based on the PET/barrier film/PVA/AgNWs *** long-term stability showed the flexible OSCs based on the PET/barrier film/PVA/AgNWs electrode have a significantly improved stability relative to the device on PET/AgNWs electrode,and comparable air stability as the rigid device with glass/ITO *** unencapsulated devices maintained nearly 50%of the original efficiency after storage for 600 h in *** a simple top encapsulation,the flexible devices remained at 60%of the initial efficiency after 2000 h in the ***,the flexible AgNWs electrode based on the barrier film would have the potential to improve the air storage stability of organic flexible solar cells.

关键词： Flexible organic solar cell AgNWs electrode Air storage stability Barrier films substrate Energy conversion Flexible electronics Interface

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A novel dual serotonin transporter and M-channel inhibitor D01 for antidepression and cognitive improvement

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Acta Pharmaceutica Sinica B 2024年第3期14卷 1457-1466页

作者： yaqin Wei Xiangqing Xu Qiang Guo Song Zhao Yinli Qiu Dongli Wang Wenwen Yu Yani Liu KeWei Wang School of Pharmacy Xuzhou Medical UniversityXuzhou 221004China Institute of Pharmaceutical Research Jiangsu Nhwa Pharmaceutical Co.Ltd.&Jiangsu Key Laboratory of Central Nervous System Drug Research and DevelopmentXuzhou 221116China Department of Pharmacology School of PharmacyQingdao University Medical CollegeQingdao 266073China Institute of Innovative Drug Qingdao UniversityQingdao 266021China Center for Brain Science and Brain-Inspired Intelligence Guangdong-Hong Kong-Macao Greater Bay AreaGuangzhou 510515China

Cognitive dysfunction is a core symptom common in psychiatric disorders including depression that is primarily managed by antidepressants lacking efficacy in improving *** this study,we report a novel dual serotonin transporter and voltage-gated potassium Kv7/KCNQ/M-channel inhibitor D01(a 2-methyl-3-aryloxy-3-heteroarylpropylamines derivative)that exhibits both anti-depression effects and improvements in cognition.D01 inhibits serotonin transporters(K_(i)=30.1±6.9 nmol/L)and M channels(IC_(50)=10.1±2.4μmol/L).D01 also reduces the immobility duration in the mouse FST and TST assays in a dose-dependent manner without a stimulatory effect on *** administrations of D01(20 and 40 mg/kg)can significantly shorten the immobility time in a mouse model of chronic restraint stress(CRS)-induced depression-like ***,D01 dose-dependently improves the cognitive deficit induced by CRS in Morris water maze test and increases the exploration time with novel objects in normal or scopolamine-induced cognitive deficits in mice,but not ***,D01 reverses the long-term potentiation(LTP)inhibition induced by *** together,our findings demonstrate that D01,a dual-target serotonin reuptake and M channel inhibitor,is highly effective in the treatment-resistant depression and cognitive deficits,thus holding potential for development as therapy of depression with cognitive deficits.

关键词： SERT 5-HT Kv7/KCNQ/M current D01 Depression Cognition

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Catechins promoted Enterococcus faecalis to alleviate related indices of nonalcoholic steatohepatitis mice induced by high-fat diet

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Food Science and Human Wellness 2024年

作者： Ying Zhang yaqin Zhou Ming Zhou Xiao Guan School of Health Science and Engineering， University of Shanghai for Science and Technology National Grain Industry (Urban Grain and Oil Security) Technology Innovation Center MDO Smarter Grain Technology Co.， Ltd.

This study provides different opinion for exploring the mechanism of catechin (CAT) relieving nonalcoholic steatohepatitis (NASH)， it is more innovative to explore from the perspective of intestinal microorganism. Through in vitro fermentation experiments， CAT could improve the abundance of Enterococcus， and Enterococcus faecalis (EF) accounts for the vast majority of Enterococcus in human gut. The experimental results in vivo showed that EF group and CAT+EF group could reduce the body weight， liver weight and epididymal fat weight of NASH mice， and improve the changes of serum and liver indexes. HE staining observation showed that these two groups have greatly improved the fatty degeneration， balloon degeneration and necrotic focus caused by NASH. The alleviation of CAT+EF group was more obvious. Results of targeted metabonomics showed that CAT could promote EF to produce more methyl palmitate (MP， C16:0)， which plays a great role in relieving NASH. Our results indicated that EF could alleviate NASH and CAT+EF group had better alleviation may due to more production of MP by EF. This study provides a new idea for CAT to alleviate NASH.

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Oat arabinoxylan promoted Lactobacillus gasseri to alleviate metabolic disorders in high-fat diet-induced obese mice

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Food Science and Human Wellness 2024年

作者： Ying Zhang Ming Zhou yaqin Zhou Xiao Guan School of Health Science and Engineering， University of Shanghai for Science and Technology National Grain Industry (Urban Grain and Oil Security) Technology Innovation Center MDO Smarter Grain Technology Co.， Ltd.

Arabinoxylan (AX) has been found to improve an imbalanced gut microbiota. Lactobacillus gasseri is a beneficial endogenous bacterium that has been shown to have several health benefits in the human gut， particularly its lipid-lowering activity. However， it is not known whether AX can promote the action of L. gasseri. The results of in vitro experiments showed that AX promoted biofilm formation in L. gasseri， its acid and bile salt resistance could be enhanced， and enabled better colonization of L. gasseri in the intestinal tract of mice. In vivo experiments showed that the AX+ L. gasseri group could effectively ameliorate weight gain and fat accumulation in high-fat diet-induced obese mice， and the L. gasseri group or AX+L. gasseri alleviated liver injury in mice. 16S rRNA sequencing showed that L. gasseri can colonize the mice intestine and AX+L. gasseri can ameliorate gut microbiota dysbiosis in obese mice by increasing Lactobacillus spp. and Coriobacteriaceae＿UCG-002 and decreasing Peptococcaceae. In addition， metabolomics results indicated that the L. gasseri group and the AX+L. gasseri group could alleviate metabolic disorders by decreasing the levels of L-phenylalanine， L-tyrosine， kynurenine acid， and arachidonic acid in obese mice. The effect of AX+L. gasseri group was better than that of the L. gasseri group， suggesting that AX promotes the lipid-lowering activity of L. gasseri， and the mechanism may be due to the activation of retrograde endocannabinoid signaling. AX can be used as a functional food ingredient to potentially alleviate obesity and metabolic syndrome.

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Subsoil tillage enhances wheat productivity,soil organic carbon and available nutrient status in dryland fields

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Journal of Integrative Agriculture 2024年第1期23卷 251-266页

作者： Qiuyan Yan Linjia Wu Fei Dong Shuangdui Yan Feng Li yaqin Jia Jiancheng Zhang Ruifu Zhang Xiao Huang Institute of Wheat Research Shanxi Agricultural UniversityLinfen 041000China State Key Laboratory of Sustainable Dryland Agriculture(in preparation) Shanxi Agricultural UniversityTaiyuan 030031China College of Resources and Environment Shanxi Agricultural UniversityTaigu 030801China Jiangsu Key Lab and Engineering Center for Solid Organic Waste Utilization National Engineering Research Center for Organicbased FertilizersNanjing Agricultural UniversityNanjing 210095China

Tillage practices during the fallow period benefit water storage and yield in dryland wheat ***,there is currently no clarity on the responses of soil organic carbon(SOC),total nitrogen(TN),and available nutrients to tillage practices within the growing *** study evaluated the effects of three tillage practices(NT,no tillage;SS,subsoil tillage;DT,deep tillage)over five years on soil physicochemical *** samples at harvest stage from the fifth year were analyzed to determine the soil aggregate and aggregate-associated C and N *** results indicated that SS and DT improved grain yield,straw biomass and straw carbon return of wheat compared with *** contrast to DT and NT,SS favored SOC and TN concentrations and stocks by increasing the soil organic carbon sequestration rate(SOCSR)and soil nitrogen sequestration rate(TNSR)in the 0-40 cm *** SOC levels under SS and NT were associated with greater aggregate-associated C fractions,while TN was positively associated with soluble organic nitrogen(SON).Compared with DT,the NT and SS treatments improved soil available nutrients in the 0-20 cm *** findings suggest that SS is an excellent practice for increasing soil carbon,nitrogen and nutrient availability in dryland wheat fields in North China.

关键词： tillage dryland wheat fields soil aggregate size soil nutrients soil carbon and nitrogen fractions

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Exploration of the Integration of Ethnic Music Elements into Modern Piano Art Creation

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Journal of Contemporary Educational Research 2024年第7期8卷 216-220页

作者： yaqin Liu St Paul University of Manila College of Music and the Performing Arts Manila 0900Philippines

Piano originated in Western countries,so a large number of Western cultural elements are used in piano art creation,mainly to present Western humanistic thoughts and spiritual cultural cores to the *** recent years,with the modernization of piano art and culture in China,many Chinese listeners have begun to demand more ethnic and folk piano pieces with Chinese *** order to meet the audience’s pursuit of modern Chinese piano art,more and more creators are integrating ethnic music elements into modern piano art *** article explores the integration significance of ethnic music elements in modern piano art creation and the current situation of Chinese modern piano art creation,and finds that ethnic music elements have positive help in enhancing the novelty,ethnic characteristics,and timeliness of piano art *** on this,this article proposes several strategies for integrating traditional ethnic music elements into modern piano art creation,including adapting traditional ethnic music elements,creating pentatonic tunes,and modifying work *** aim is to provide references and inspiration for the development of Chinese piano art creation and culture.

关键词： Piano Modern art creation Ethnic music elements

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Coexisting fast–slow dendritic traveling waves in a 3D-array electric field coupled neuronal network

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Chinese Physics B 2024年第6期33卷 614-626页

作者：魏熙乐任泽宇卢梅丽樊亚琴常思远 The Tianjin Key Laboratory of Process Measurement and Control School of Electrical and Information EngineeringTianjin UniversityTianjin 300072China School of Information Technology Engineering Tianjin University of Technology and EducationTianjin 300074China

Coexistence of fast and slow traveling waves without synaptic transmission has been found in hhhippocampal tissues,which is closely related to both normal brain activity and abnormal neural activity such as epileptic discharge. However, the propagation mechanism behind this coexistence phenomenon remains unclear. In this paper, a three-dimensional electric field coupled hippocampal neural network is established to investigate generation of coexisting spontaneous fast and slow traveling waves. This model captures two types of dendritic traveling waves propagating in both transverse and longitude directions: the N-methyl-D-aspartate(NMDA)-dependent wave with a speed of about 0.1 m/s and the Ca-dependent wave with a speed of about 0.009 m/s. These traveling waves are synaptic-independent and could be conducted only by the electric fields generated by neighboring neurons, which are basically consistent with the in vitro data measured experiments. It is also found that the slow Ca wave could trigger generation of fast NMDA waves in the propagation path of slow waves whereas fast NMDA waves cannot affect the propagation of slow Ca waves. These results suggest that dendritic Ca waves could acted as the source of the coexistence fast and slow waves. Furthermore, we also confirm the impact of cellular spacing heterogeneity on the onset of coexisting fast and slow waves. The local region with decreasing distances among neighbor neurons is more liable to promote the onset of spontaneous slow waves which, as sources, excite propagation of fast waves. These modeling studies provide possible biophysical mechanisms underlying the neural dynamics of spontaneous traveling waves in brain tissues.

关键词： hippocampal network epileptiform dendritic oscillation traveling wave electric field coupling

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Relationship between Seed Priming Mediated Seedling Vigor and Yield Performance of Spring Wheat

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Phyton-International Journal of Experimental Botany 2024年第6期93卷 1159-1177页

作者： Md.Parvez Anwar Masuma Akhter sharmin Aktar Sinthia Afsana Kheya A.K.M.Mominul Islam Sabina Yeasmin Ahmed Khairul Hasan Md.Harun Or Rashid Department of Agronomy Bangladesh Agricultural UniversityMymensingh2202Bangladesh

Seed priming is a pre-germinated technique that can enhance seed germination percentage,faster and synchro-nized germination,better seedling growth,and yield under stress *** ascertain the most effective seed priming method that would ensure the potential yield of wheat in Bangladesh,two experiments were carried out from December 2021 to March 2022 at the Department of Agronomy,Bangladesh Agricultural *** wheat varieties namely BARI Gom-28 and BWMRI Gom-1 were subjected to a range of priming chemicals in both lab and pot *** compounds included the following:control(no priming),hydropriming(distilled water),10000 ppm KNO_(3),15000 ppm KNO_(3),40000 ppm Mannitol,60000 ppm Mannitol,10000 ppm NaCl,20000 ppm NaCl,100 ppm PEG,150 ppm PEG,500 ppm NaOCl,1000 ppm NaOCl,10000 ppm CaCl_(2),20000 ppm CaCl_(2),10000 ppm KCl and 20000 ppm KCl.A complete randomized design(CRD)with three repli-cations was used to set up the *** results showed that BARI Gom-28 and BWMRI Gom-1 responded best to KCl priming in terms of rapid seed germination and strong seedling *** the other hand,the best priming agents for plant growth and productivity turned out to be CaCl_(2) and *** results of this study support the possibility of using seed priming as a technique to improve wheat plant development and output by raising seed emergence and survival rates.

关键词： Priming seedling percentage germination growth yield wheat

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