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Advances in environmental DNA monitoring:standardization,automation,and emerging technologies in aquatic ecosystems

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science china(Life sciences) 2024年第7期67卷 1368-1384页

作者： Suxiang Lu Honghui Zeng fan Xiong Meng yao Shunping He State Key Laboratory of Freshwater Ecology and Biotechnology Institute of HydrobiologyChinese Academy of SciencesWuhan 430072China Institute of Ecology College of Urban and Environmental SciencesPeking UniversityBeijing 100871China School of Life sciences Peking UniversityBeijing 100871China Institute of Deep Sea science and Engineering Chinese Academy of SciencesSanyaChina Center for Excellence in Animal Evolution and Genetics Chinese Academy of SciencesKunmingChina

Environmental DNA(eDNA)monitoring,a rapidly advancing technique for assessing biodiversity and ecosystem health,offers a noninvasive approach for detecting and quantifying species from various environmental *** this review,a comprehensive overview of current eDNA collection and detection technologies is provided,emphasizing the necessity for standardization and automation in aquatic ecological ***,the intricacies of water bodies,from streams to the deep sea,and the associated challenges they pose for eDNA capture and analysis are *** paper delineates three primary eDNA survey methods,namely,bringing back water,bringing back filters,and bringing back data,each with specific advantages and constraints in terms of labor,transport,and data ***,innovations in eDNA sampling equipment,including autonomous drones,subsurface samplers,and in-situ filtration devices,and their applications in monitoring diverse taxa are ***,recent advancements in species-specific detection and eDNA metabarcoding are addressed,highlighting the integration of novel techniques such as CRISPR-Cas and nanopore sequencing that enable precise and rapid detection of *** implications of environmental RNA and epigenetic modifications are considered for future applications in providing nuanced ecological ***,the review stresses the critical role of standardization and automation in enhancing data consistency and comparability for robust long-term *** propose that the amalgamation of these technologies represents a paradigm shift in ecological monitoring,aligning with the urgent call for biodiversity conservation and sustainable management of aquatic ecosystems.

关键词： eDNA methodology sampler environment biomonitoring ecogenomic sensors ocean observation instrument

（＊）-Serial coalgebras

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Frontiers of Mathematics in china 2012年第5期7卷 955-970页

作者： hailou yao {2. fan Yanru PING college of applied {2.s Beijing University of TechnologyBeijing 100124China

In this paper, we introduce the notion of （＊）-serial coalgebras which is a generalization of serial coalgebras. We investigate the properties of （＊）-serial coalgebras and their comodules, and obtain sufficient a... 详细信息

关键词： Coalgebra biserial comodule (,)-serial coalgebra quiver

The Earth Summit Mission-2.2.:Successful ozone soundings contribute to source identification in the north *** region

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Journal of Environmental sciences 2024年第2期136卷 412-421页

作者： Jinqiang Zhang Chunxiang Ye Yuejian Xuan Zhixuan Bai weili Lin Dan Li Lingkun Ran Baofeng Jiao yaomingMa Weiqiang Ma Nan yao Yunshu Zeng Daren Lv Tong Zhu Key Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China college of Environmental sciences and Engineering Center for Environment and HealthPeking UniversityBeijing 100871China Key Laboratory of Ecology and Environment in Minority Areas(Minzu University of china) National Ethnic Affairs CommissionBeijing 100081China Key Laboratory of Cloud-Precipitation Physics and Severe Storms Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Land-Atmosphere Interaction and Its Climatic Effects Group State Key Laboratory of Tibetan Plateau Earth SystemResources and Environment(TPESRE)Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China college of Earth and Planetary sciences University of Chinese Academy of SciencesBeijing 100049China college of Atmospheric science Lanzhou UniversityLanzhou 730000China National Observation and Research Station for Qomolongma Special Atmospheric Processes and Environmental Changes Dingri 858200China Kathmandu Center of Research and Education Chinese Academy of SciencesBeijing 100101China china-Pakistan Joint Research Center on Earth sciences Chinese Academy of SciencesIslamabad 45320Pakistan Electronic Engineering college Chengdu University of Information TechnologyChengdu 610225China

As part of“The Earth Summit Mission-2.2.”during the second Tibetan Plateau Scientific Expedition and Research(STEP)in April and May 2.2.,we conducted the ozone sounding experiment(an ozonesonde mated to a radiosonde)at *** Base Camp(MQBC;86.85°E,2..14°N;52.0 m),a location at an extremely high altitude.A total of ten sounding profiles were obtained between April 30 and May 06,2.2.,of which seven profiles were above35 km in altitude,with a maximum detection altitude up to 39.0 *** study presents the temporal variation and vertical distributions of atmospheric temperature,humidity,and ozone during the MQBC *** averaged ozone concentration was high(68.3 ppbv)at the surface and then increased smoothly until peaking(~110 ppbv)in the middle troposphere(approximately 10 km),and afterward,the ozone concentration increased rapidly from the upper troposphere to a maximum of~10 ppmv at~30 *** enhanced ozone concentration in the middle troposphere was associated with the blocking high pressure,and transport from the southern flank of the Himalayas occurred during the campaign *** average total ozone column was 2.1.9±2..4 DU for the seven profiles exceeding 35km in *** ozonesonde measurements were also compared with the vertical ozone profiles retrieved from the space-borne ozone products from the Microwave Limb Sounder(MLS)onboard the Aura satellite and the Atmospheric Infrared Sounder(AIRS)onboard the Aqua satellite.

关键词： Ozone soundings Mt.Qomolangma Vertical ozone structure Ozone source Satellite data

A review of solid-state lithium metal batteries through in-situ solidification

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science china Chemistry 2024年第1期67卷 67-86页

作者： Pan Xu Zong-yao Shuang Chen-Zi Zhao Xue Li Li-Zhen fan Aibing Chen Haoting Chen Elena Kuzmina Elena Karaseva Vladimir Kolosnitsyn Xiaoyuan Zeng Peng Dong Yingjie Zhang Mingpei Wang Qiang Zhang beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China National and Local Joint Engineering Laboratory for Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093China Institute of Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China college of Chemical and Pharmaceutical Engineering Hebei University of Science and TechnologyShijiazhuang 050018China Ordos Carbon Neutral Research and Application Co. Ltd.Ordos City 017010China Ufa Institute of Chemistry UFRC RAS Ufa 450054Russia Institute for Carbon Neutrality Tsinghua UniversityBeijing 100084China Shanxi Research Institute for Clean Energy Tsinghua UniversityTaiyuan 030032China

High-energy-density lithium metal batteries are the next-generation battery systems of choice,and replacing the flammable liquid electrolyte with a polymer solid-state electrolyte is a prominent conduct towards realizing the goal of high-safety and high-specific-energy ***,the inherent intractable problems of poor solid-solid contacts between the electrode/electrolyte and the growth of Li dendrites hinder their practical *** in-situ solidification has demonstrated a variety of advantages in the application of polymer electrolytes and artificial interphase,including the design of integrated polymer electrolytes and asymmetric polymer electrolytes to enhance the compatibility of solid–solid contact and compatibility between various electrolytes,and the construction of artificial interphase between the Li anode and cathode to suppress the formation of Li dendrites and to enhance the high-voltage stability of polymer *** review firstly elaborates the history of in-situ solidification for solid-state batteries,and then focuses on the synthetic methods of solidified ***,the recent progress of in-situ solidification technology from both the design of polymer electrolytes and the construction of artificial interphase is summarized,and the importance of in-situ solidification technology in enhancing safety is ***,prospects,emerging challenges,and practical applications of in-situ solidification are envisioned.

关键词： in-situ solidification polymer electrolyte artificial solid electrolyte interphase rechargeable lithium metal batteries dendrite-free lithium metal anode

On adjacent-vertex-distinguishing total coloring of graphs

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science china Mathematics 2005年第3期48卷 289-299页

作者： ZHANG Zhongfu, CHEN Xiang’en, LI Jingwen, yao Bing, LU Xinzhong & WANG Jianfang {2. of Mathematics and Information science, Northwest Normal University, Lanzhou 730070,{2. Department of Computer, Lanzhou Normal {2., Lanzhou 730070,{2. Institute of applied Mathematics, Lanzhou Jiaotong University, Lanzhou 730070,{2. {2. of Information and Electrical Engineering, Lanzhou Jiaotong University, Lanzhou 730070,{2. Institute of applied Mathematics, Chinese Academy of sciences, beijing 100080,{2. 1. college of Mathematics and Information science Northwest Normal University 730070 Lanzhou China 2. Department of Computer Lanzhou Normal College 730070 Lanzhou China 3. Institute of applied Mathematics Lanzhou Jiaotong University 730070 Lanzhou China 4. college of Information and Electrical Engineering Lanzhou Jiaotong University 730070 Lanzhou China 5. Institute of applied Mathematics Chinese Academy of Sciences 100080 Beijing China

In this paper, we present a new concept of the adjacent-vertex-distinguishing total coloring of graphs (briefly, AVDTC of graphs) and, meanwhile, have obtained the adjacent-vertex-distinguishing total chromatic number... 详细信息

关键词： graph, proper total coloring, adjacent-vertex-distinguishing total coloring, adjacent-vertex-distinguishing total chromatic number.

A three-way electrolyte with ternary solvents for high-energy-density and long-cycling lithium-sulfur pouch cells

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SusMat 2024年第2期4卷 1-12页

作者： Zheng Li Legeng Yu Chen-Xi Bi Xi-yao Li JinMa Xiang Chen Xue-Qiang Zhang Aibing Chen Haoting Chen Zuoru Zhang Li-Zhen fan Bo-Quan Li Cheng Tang Qiang Zhang Tsinghua Center for Green Chemical Engineering Electrification Beijing Key Laboratory of Green Chemical Reaction Engineering and TechnologyDepartment of Chemical EngineeringTsinghua UniversityBeijingChina School of Materials science and Engineering Beijing Institute of TechnologyBeijingChina Institute of Advanced Materials and Technology University of Science and TechnologyBeijingChina Shanxi Research Institute for Clean Energy Tsinghua UniversityTaiyuanChina Center for Next-Generation Energy Materials and School of Chemical Engineering Sungkyunkwan UniversityJangan-GuSuwon-SiGyeonggi-DoRepublic of Korea college of Chemical and Pharmaceutical Engineering Hebei University of Science and TechnologyShijiazhuangChina Ordos Carbon Neutral Research and Application Co. Ltd.Kangbashi DistrictOrdos CityInner MongoliaChina Institute for Carbon Neutrality Tsinghua UniversityBeijingChina

Lithium–sulfur(Li–S)batteries promise high-energy-density potential to exceed the commercialized lithiumion batteries but suffer from limited cycling lifespan due to the side reactions between lithium polysulfides(LiPSs)and Li metal ***,a three-way electrolyte with ternary solvents is proposed to enable high-energy-density and long-cycling Li–S pouch ***,ternary solvents composed of 1,2.dimethoxyethane,di-isopropyl sulfide,and 1,3,5-trioxane are employed to guarantee smooth cathode kinetics,inhibit the parasitic reactions,and construct a robust solid electrolyte interphase,*** cycling lifespan of Li–S coin cells with 50μm Li anodes and 4.0 mg cm^(−2. sulfur cathodes is prolonged from88 to 2.2.cycles using the three-way ***-heterogeneous solvation structure of LiPSs and organic-rich solid electrolyte interphase are identified to improve the cycling stability of Li metal ***,a 3.0 Ah-level Li–S pouch cell with the three-way electrolyte realizes a high energy density of 405 Wh kg^(−1) and undergoes 2. *** affords a three-way electrolyte recipe for suppressing the side reactions of LiPSs and inspires rational electrolyte design for practical high-energy-density and long-cycling Li–S batteries.

关键词： lithium metal anodes lithium-sulfur batteries pouch cells solid electrolyte interphase three-way electrolyte

SYNTHESIS OF PERFLUORO-1-OCTANESULFONATED FULLERENE AND THE FRICTION PROPERTIES OF ITS THIN FILM

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Chinese Journal of Polymer science 2002年第5期20卷 397-400页

作者： Lan Huang Shuang fan fang Wei Xin-sheng Zhao Jin-xin Xiao Bu-{2. Zhu college of Chemistry and Molecular Engineering Peking University beijing 100871,{2. Peking Univ Coll Chem & Mol Engn Beijing 100871 Peoples R China

A star-shaped compound of perfluoro-1-octanesulfonated fullerene was synthesized. The measurement of the friction for its spin-coating film by friction force microscopy (FFM) reveals that the films possess lower frict... 详细信息

关键词： perfluoro-1-octanesulfonated fullerene thin film friction force microscopy (FFM)

In situ forming injectable MSC-loaded GelMA hydrogels combined with PD for vascularized sweat gland regeneration

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Military Medical Research 2024年第1期11卷 152-155页

作者： Enhe Jirigala Bin yao Zhao Li Yi-Jie Zhang Chao Zhang Li-Ting Liang fan-Liang Zhang Xing-Yu Yuan Xian-Lan Duan Wei Song Meng-De Zhang Yi Kong Xiao-Bing Fu Sha Huang Research Center for Tissue Repair and Regeneration Medical Innovation Research DepartmentChinese PLA General Hospital and PLA Medical CollegeBeijing 100048China Institute of Basic Medical Research Inner Mongolia Medical UniversityHohhot 010110China Academy of Medical Engineering and Translational Medicine Tianjin UniversityTianjin 300072China School of Medicine Nankai UniversityTianjin 300071China

Dear Editor,Three dimensional(3D)bioprinted extracellular matrix(ECM)can be used to provide both biochemical and biophysical cues to direct mesenchymal stem cells(MSCs)differentiation,and then differentiated cells were isolated for implantation in vivo using surgical ***,the reduced cell activity after cell isolation from 3D constructs and low cell retention in injured sites limit its application[1].Methacrylated gelatin(GelMA)hydrogel has the advantage of fast crosslinking,which could resemble complex architectures of tissue construct in vivo[2..Here,we adopted a noninvasive bioprinting procedure to imitate the regenerative microenvironment that could simultaneously direct the sweat gland(SG)and vascular differentiation from MSCs and ultimately promote the replacement of glandular tissue in situ(Fig.1a).

关键词： Sweat gland GelMA In situ niche Cell differentiation Tissue incorporation Vascularization

Trialkylsilyl-thiophene-conjugated acceptor for efficient organic solar cells compatible with spin-coating and blade-coating technologies

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science china Chemistry 2024年

作者： Tengfei Li Qiang Wu Zefan yao Hairui Bai Wenyan Su Rui Sun Lingxiao Tang Zhaozhao Bi Xiaojun Li Weiguo Zhu Jie Min Qunping fan Wei Ma State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong University college of Chemistry and Molecular Engineering Peking University School of Materials science and Engineering Xi'an University of Science and Technology Jiangsu Engineering Research Center of Light-Electricity-Heat Energy-Converting Materials and Applications School of Materials Science and Engineering and Changzhou University The Institute for Advanced Studies Wuhan University beijing National Laboratory for Molecular sciences CAS Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of Sciences

Sidechain engineering as an efficient and convenient strategy has been widely used to optimize molecular structure of photovoltaic materials for boosting power conversion efficiency(PCE) of organic solar cells(OSCs). Herein, a new Y-series acceptor named Y-ThSi with trialkylsilyl-substituted thiophene as conjugated sidechain is developed. Compared with its parental Y6 with multiple intermolecular interactions, Y-ThSi has a unitary molecular packing due to the additional steric hindrance from twodimensional(2.)-conjugated trialkylsilyl-thiophene. Therefore, Y-ThSi shows an obviously blue-shifted absorption with an onset of ～850 nm but significantly up-shifted lowest unoccupied molecular orbital energy level. For the PM6:Y-ThSi pair, the spin-coating OSCs achieve a decent PCE of 14.56% with an impressively high photovoltage(VOC) of 0.936 V. Inspired by its high VOCand narrow absorption, Y-ThSi is introduced into near-infrared absorbing binary PM6:BTP-eC9 host to construct ternary OSCs. Thanks to the complementary absorption, optimized morphology, and minimized energy loss properties, the PM6:BTP-eC9:Y-ThSi-based OSCs offer a higher PCE of 18.34%. Moreover, our developed strategy can overcome the commonly existed PCE drop when the blade-coating towards large-scale printing is used instead. Therefore, a comparable PCE of 18.34% is achieved, which is one of the best values for the blade-coating OSCs so far.

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