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Reasonable Designing of Free-standing MnO_(2)/Graphene Composite Membrane for Lithium-ion Storage

Chemical Research in chinese Universities 2024年第3期40卷 508-512页

作者： SHI Junye YU Chenxi ZOU Zewei ZheNG Shumin zhang {3. WANG Bao institute of Refrigeration and Cryogenics Shanghai Jiao Tong University Shanghai 200433P.R.China state key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190P.R.China key Laboratory of Biopharmaceutical Preparation and Delivery Institute of Process EngineeringChinese Academy of SciencesBeijing 100190P.R.China CAS key Laboratory of Molecular Nanostucture and Nanotechnology Institute of ChemistryChinese Academy of SciencesBeijing 100190P.R.China

Free-standing membranes show extraordinary promise in energy storage applications,however are usually limited by low capacity and poor rate ***,we assembled a series of free-standing MnO_(2)/GO composite membranes with ZIF67 particles embedded between two-dimensional(2D)*** particle size of ZIF67 can be adjusted to achieve tunable interlayer *** lithium storage performance of the as-obtained membranes with different interlayer spaces was systematically *** MnO_(2)/GO composite membrane embedded with ZIF67 particles with an average diameter of 3. nm(denoted as MnO_(2)/nZIF67/GO)delivers a good long cycling performance,and it retains a capacity of 3.0.7 mA·h·g^(−1) after 400 cycles at 0.05 A/*** MnO_(2)/GO composite membrane embedded with ZIF67 particles with an average diameter of 500 nm(denoted as MnO_(2)/mZIF67/GO)exhibits good rate *** of the size of the ZIF67 particles,the performance of the membrane containing ZIF67 is significantly better than that of the membrane without ZIF67,indicating that the ZIF67 particles can enhance the lithium storage performance of the assembled *** work provides a method to fabricate a free-standing membrane for lithium storage with tunable electrochemical performance.

关键词： Lithium-ion battery Membrane Free-standing ZIF67

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Underestimated benefits of NO_(x) control in reducing SNA and O_(3. based on missing heterogeneous HONO sources

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Frontiers of Environmental Science & Engineering 2024年第3期18卷 57-67页

作者： Shuping zhang Haotian Zheng Jun Liu Yao Shi Tianzeng Chen Chao{3. Xue Fenfen zhang Yueqi Jiang Xiangping zhang Shovan Kumar Sahu Biwu Chu Jia xing state key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China china academy of Civil Aviation Science and Technology Beijing 100028China state key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Yellow River institute of Hydraulic Research Zhengzhou 450003China Centre for Climate Research Singapore Meteorological Service SingaporeSingapore 537054Singapore

Substantial NO_(x) emission mitigation is crucial for the synergistic reduction of particulate matter and ozone(O_(3.)pollution in *** traditional air quality model does not consider heterogeneous HONO chemistry,leading to uncertainties in estimating the benefits of NO_(x) *** studies have shown that the parameterization of heterogeneous HONO formation increases both the simulated value of sulfate–nitrate–ammonium(SNA)and that of O_(3.,thus adding the heterogeneous reactions of HONO into air quality models inevitably leads to changes in the estimated benefits of NO_(x) *** we investigated the changes in SNA and O_(3.concentrations from NO_(x) emission reduction before and after adding heterogeneous HONO reactions in the Community Multi-Scale Air Quality(CMAQ)*** heterogeneous HONO reactions in the simulation improved the benefits of NO_(x) reduction in terms of SNA control in *** 80%NO_(x) reduction,the reduction in SNA increased from 3..9%without considering heterogeneous HONO reactions to 42.8%with heterogeneous HONO *** reduction in the maximum daily 8h average(MDA8)O_(3.in summer caused by NO_(x) reduction increased slightly from 4.7%to 5.2%after adding heterogeneous HONO *** results in this study highlight the enhanced effectiveness of NO_(x) controls for the reduction of SNA and O_(3.after considering heterogeneous HONO formation in a complex chemical ambient,demonstrating the importance of NO_(x) controls in reducing PM2.5 and O_(3.pollution in china.

关键词： heterogeneous HONO NO_(x) reduction PM_(2.5) O_(3.

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Cut marks and terminal Pleistocene hominids in the Ma'anshan site:Evidence for meat-eating

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chinese Science Bulletin 2009年第19期54卷 3872-3879页

作者： zhang Yue1,2,3. WANG ChunXue1,2, zhang ShuangQuan1,2 & GAO xing1,2? 1 {3. of Vertebrate Paleontology and Paleoanthropology, chinese academy of sciences, beijing 100044, china 2 Joint Laboratory of Human Evolution and Archaeometry, chinese academy of sciences, beijing 100044, china 3.state key Laboratory of Palaeobiology and Stratigraphy, Nanjing 210008, china institute of Vertebrate Paleontology and Paleoanthropology Chinese Academy of Sciences Beijing 100044 China Joint Laboratory of Human Evolution and Archaeometry Chinese Academy of Sciences Beijing 100044 China state key Laboratory of Palaeobiology and Stratigraphy Nanjing 210008 China

In this paper, cut marks on the long bones of class Ⅱ sized animals in the Ma'anshann site are studied. Based on the location and frequencies of the long bone cut marks, the distribution characteristics are analyzed as follows: (1) cut mark frequencies in the lower layer (LL) are much higher than those of the upper; (2) in the LL cut mark frequency of the upper limbs is the highest, and that of the middle and lower limbs is lower and the lowest; (3. In the upper layer (UL) the cut mark frequency, does not spread as orderly as in the LL. The data are compared to those of the experiment and it is demonstrated that values of the LL all fall into the experimental 95% confidence intervals, and the cut mark frequencies of the upper, middle and lower limbs coincide with those of the experiment; while the values of the UL are much lower, of which, those of the humerus, femur and radius are out of the intervals, and the frequencies of the upper, middle and lower limbs are far more different from those of the experiment. It implies that the earlier hominids (of the LL) defleshed the limbs of the class Ⅱ sized animals with stone tools more completely than the later hominids. With the evidence of burning marks, it is suggested that the difference on the roasting behaviors derived the cut mark difference of the Ma'anshan UL and LL.

关键词：原始人类马鞍山证据网站痕迹切口更新世肉类

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Computing Power Network:A Survey

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china Communications 2024年第9期21卷 109-145页

作者： Sun Yukun Lei Bo Liu Junlin Huang Haonan zhang xing Peng Jing Wang Wenbo School of Information and Communications Engineering Beijing University of Posts and TelecommunicationsBeijing 100876China Research institute of china Telecom Co. Ltd.Beijing 102209China beijing Branch of china Telecom Co. Ltd.Beijing 100032China

With the rapid development of cloud computing,edge computing,and smart devices,computing power resources indicate a trend of ubiquitous *** traditional network architecture cannot efficiently leverage these distributed computing power resources due to computing power island *** overcome these problems and improve network efficiency,a new network computing paradigm is proposed,i.e.,Computing Power Network(CPN).Computing power network can connect ubiquitous and heterogenous computing power resources through networking to realize computing power scheduling *** this survey,we make an exhaustive review on the state-of-the-art research efforts on computing power *** first give an overview of computing power network,including definition,architecture,and ***,a comprehensive elaboration of issues on computing power modeling,information awareness and announcement,resource allocation,network forwarding,computing power transaction platform and resource orchestration platform is *** computing power network testbed is built and *** applications and use cases in computing power network are ***,the key enabling technologies for computing power network are ***,open challenges and future research directions are presented as well.

关键词： computing power modeling computing power network computing power scheduling information awareness network forwarding

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Portable fluorogenic probe for monitoring of volatile amine vapour and food spoilage

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chinese Chemical Letters 2024年第3期35卷 257-261页

作者： Jian-Hao Zhao Wen-xing Xu Bin Li Wei Xu Wu-Kun zhang Ming-Shuai Yuan Hui-Zi Li Qing-Guo he Xiang Ma Jian-Gong Cheng Yan-Yan Fu state key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of the Chinese Academy of SciencesBeijing 100039China School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center Frontiers Science Center for Materiobiology and Dynamic Chemistry School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China

There are urgent needs of volatile amine gas sensors with high-performance in food quality control,disease monitoring and environmental ***-film fluorescent probe is suitable for amine vapour sensing due to its high sensitivity,high selectivity,and no polluting ***,a novel fluorescent probe based on indacenodithiophene structure withπconjugated system was designed and *** experimental results show that the films prepared by this material exhibit rapid and distinct fluorescence quenching after being exposed to saturated vapours of primary amine,secondary amine and tertiary amine represented by n-propylamine,diethylamine and trimethylamine,*** quenching of fluorescence is 84%,87%and 96%,respectively,within 10 *** detection mechanism of probe for primary amine is based on specific chemical reaction,while the detection mechanism for secondary amine and tertiary amine is intramolecular charge *** experiments show that the detection limit of the fluorescent probe for trimethylamine,an important marker of food spoilage,could reach 4.610 ***-site detection based on spoilage of small yellow croaker suggests the material possesses the potential for food freshness *** simple fluorogenic probe is an original approach to simplify real-time visual monitoring of volatile amine vapour.

关键词： Fluorescent probe Volatile amine Gas sensing Trimethylamine Food spoilage

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Tuning the Surface Field by Embedding Cations into Metals to Direct the Reaction Pathway of CO_(2) Electroreduction

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CCS Chemistry 2024年第3期6卷 631-640页

作者： Pei zhang Meng Zhou Shiqiang Liu Xueqing xing Jiahao yang Peng C{3.n Yaoyu Yin Yingying C{3.ng xing Tong Jun Ma Qinggong Zhu Xiaofu Sun ZhongJun C{3.n Xinc{3.n Kang Buxing Han beijing National Laboratory for Molecular sciences CAS Laboratory of Colloid and Interface and ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesCenter for Carbon Neutral ChemistryInstitute of ChemistryChinese Academy of SciencesBeijing 100190 beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049 Shanghai key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062 School of Chemistry University of Chinese Academy of SciencesBeijing 100049

The creation of universal strategies to affect the reaction route of the electroreduction of CO_(2) is ***,we report the first work to introduce cations into diverse metals such as Cu,Bi,In,and Sn via the electroreduction of related metallic oxides in quaternary ammonium surfactant *** to their physical adsorption,cations embedded into the electrodes have a more pronounced impact on the electrical field,which effectively influences the adsorption state of *** the increase of surface field,the hydrogen evolution reaction and*COOH route are significantly reduced,favouring the*OCHO pathway *** a result,hydrogen,CO,and C_(2+)products almost completely vanish at−0.5 V versus Rhe in 0.1 M Na_(2)SO_(4)in an H-type cell after enough cations are embedded into the Cu electrode,and the faradaic efficiency of formate rises from 18.0%to 99.5%simultaneously.

关键词： CO_(2)electroreduction tuneable products electrical field reaction pathway cations embedding

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PRaG 3.0 therapy for human epidermal growth factor receptor 2-positive metastatic pancreatic ductal adenocarcinoma:A case report

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World Journal of Gastroenterology 2024年第9期30卷 1237-1249页

作者： Yue-Hong Kong Mei-Ling Xu Jun-Jun zhang Guang-Qiang Chen Zhi-Hui Hong Hong zhang Xiao-Xiao Dai Yi-Fu Ma Xiang-Rong Zhao Chen-yang zhang Rong-Zheng Chen Peng-Fei xing Li-Yuan zhang Center for Cancer Diagnosis and Treatment The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Department of Radiotherapy&Oncology The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Institution of Radiotherapy&Oncology Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Department of Radiology The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Department of Nuclear Medicine The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Department of Clinical Laboratory The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina Department of Pathology The Second Affiliated Hospital of Soochow UniversitySuzhou 215000Jiangsu ProvinceChina

BACKGROUND Pancreatic ductal adenocarcinoma(PDAC)is a highly fatal disease with limited effective treatment especially after first-line *** human epidermal growth factor receptor 2(heR-2)immunohistochemistry(IHC)positive is associated with more aggressive clinical behavior and shorter overall survival in *** SUMMARY We present a case of multiple metastatic PDAC with IHC mismatch repair proficient but heR-2 IHC weakly positive at diagnosis that didn’t have tumor regression after first-line nab-paclitaxel plus gemcitabine and PD-1 inhibitor treatment.A novel combination therapy PRaG 3.0 of RC48(heR2-antibody-drug conjugate),radio-therapy,PD-1 inhibitor,granulocyte-macrophage colony-stimulating factor and interleukin-2 was then applied as second-line therapy and the patient had confirmed good partial response with progress-free-survival of 6.5 months and overall survival of 14.2 *** had not developed any grade 2 or above treatment-related adverse events at any *** of peripheral CD8^(+) Temra and CD4^(+) Temra were increased during first two activation cycles of PRaG 3.0 treatment containing radiotherapy but deceased to the baseline during the maintenance cycles containing no *** PRaG 3.0 might be a novel strategy for heR2-positive metastatic PDAC patients who failed from previous first-line approach and even PD-1 immunotherapy but needs more data in prospective trials.

关键词： Pancreatic ductal adenocarcinoma PRaG 3.0 therapy Human epidermal growth factor receptor 2 Novel combination therapy Case report

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Ultrasonic focusing and scanning with multiple waves

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chinese Physics B 2013年第1期22卷 312-317页

作者：张碧星刘冬冬师芳芳 hefeng Dong state key Laboratory of Acoustics Institute of Acoustics Chinese Academy of Sciences Department of Electronics and Telecommunications Norwegian University of Science and Technology

This paper presents a new focusing and scanning method which focuses multiple waves on a target. The key of the method is to control excitation pulses for each element of the transducer array. The excitation pulse on each array element is obtained by time reversing the signal received by the same element, which is generated by an imaginary source at the target. The excitation pulses from all array elements are transmitted and arrive at the target simultaneously, and focusing is achieved. The performance of the two methods is compared in numerical examples, and it is demonstrated that the proposed method achieves a satisfactory focusing and a good signal-to-noise ratio no matter where the target location is.

关键词： ultrasonic focusing and scanning multiple waves transducer array

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Corrosion and electrochemical behavior of as-cast Mg-5Y-7Gd-1Nd-0.5Zr magnesium alloys in 5%NaCl aqueous solution

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Progress in Natural Science:Materials International 2011年第4期21卷 314-321页

作者： Xin zhang~(1,2,3.,Kui zhang~1,xing-gang LI~1,Cong WANG~4,Hong-wei LI~(2,3.,Chang-shun WANG~(2,3.,Xia DENG~1 1.{3. key Laboratory for Fabrication and Processing of Nonferrous Metals, beijing General Research institute for Nonferrous Metals,beijing 100088,china 2.beijing Engineering Research Center for Advanced Manufacturing and Evaluation of Special Vehicle Parts,beijing 100072,china 3.institute of Technology,beijing North Vehicle Group Corporation,beijing 100072,china 4.Fengtai Military Representative Office,beijing Military Representative Office,PLA,beijing 100072,china [a] state key Laboratory for Fabrication and Processing of Nonferrous Metals Beijing General Research Institute for Nonferrous Metals Beijing 100088 China [b] beijing Engineering Research Center for Advanced Manufacturing and Evaluation of Special Vehicle Parts Beijing 100072 China [c] institute of Technology Beijing North Vehicle Group Corporation Beijing 100072 China [d] Fengtai Military Representative Office Beijing Military Representative Office PLA Beijing 100072 China

The corrosion mechanism of the as-cast Mg-5Y-7Gd-1Nd-0.5Zr magnesium alloy immersed in 5%NaCl aqueous solution was investigated by electrochemical test and *** electrochemical results indicate that the corrosion resistance of Mg-5Y-7Gd-1Nd-0.5Zr alloy in 5%NaCl aqueous solution gradually deteriorates with immersion time increasing from 2 h,24 h,60 h,to 108 h,which is consistent with the SEM observation of corrosion *** Cl-anion leads to the initiation and development of the corrosion pits,and Mg-5Y-7Gd-1Nd-0.5Zr alloy exhibits filiform type of attack under significant anodic control of magnesium solution *** corrosion potential becomes noble with increasing immersion time.

关键词： magnesium alloys Mg-5Y-7Gd-1Nd-0.5Zr corrosion electrochemical behavior

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Spatial-Temporal Changes of Soil Organic Carbon During Vegetation Recovery at Ziwuling, china

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Pedosphere 2005年第5期15卷 601-610页

作者： LI Yu-Yuan SHAO Ming-An ZheNG Ji-Yong zhang xing-Chang key Laboratory of Water Cycle and Related Land Surface Processes Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences Beijing 100101 （China） state key Laboratory of Soil Erosion and Dryland Farming on the Loess Plateau Institute of Soil and Water Conservation Chinese Academy of Sciences and Ministry of Water Resources Yangling 712100 （China）

To probe the processes and mechanisms of soil organic carbon (SOC) changes during forest recovery, a 150-yearchronosequence study on SOC was conducted for various vegetation succession stages at the Ziwuling area, in the centralpart of the Loess Plateau, china. Results showed that during the 150 years of local vegetation rehabilitation SOC increasedsignificantly (P he initial period of 55-59 years, but slightly decreased afterwards. Average SOCdensities for the 0-100 cm layer of farmland, grassland, shrubland and forest were 4.46, 5.05, 9.95, and 7.49 kg C m-3.respectively. The decrease in SOC from 60 to 150 years of abandonment implied that the soil carbon pool was a sink forCO2 before the shrubland stage and became a source in the later period. This change resulted from the spatially variedcomposition and structure of the vegetation. Vegetation recovery had a maximum effect on the surface (0-20 cm) SOCpool. It. was concluded that vegetation recovery on the Loess Plateau could result in significantly increased sequestrationof atmospheric CO2 in soil and vegetation, which was ecologically important for mitigating the increase of atmosphericconcentration of CO2 and for ameliorating the local eco-environment.

关键词： soil organic carbon density spatial-temporal change vegetation recovery vegetation succession

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