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Facile Surface engineering of NiCo_(2.O_(4) to Boost Propane Oxidation Activity

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china Petroleum Processing & Petrochemical Technology 2024年第1期26卷 19-26页

作者： yang Jialei Wang Fengyi lei yang zhang Mingchao Sun Shiqiang xu Wenfan ke Jiaxiang Wu Haojie Li Xingyun Qi Jian institute of Materials for Energy and Environment College of Materials Science and EngineeringQingdao UniversityQingdao 266071China School of Chemistry and Chemical engineering Hubei Key Laboratory of Coal Conversion and New Carbon MaterialsWuhan University of Science and TechnologyWuhan 430081China Department of Burn and Plastic Surgery Qingdao Municipal Hospital Affiliated to Rehabilitation UniversityQingdao 266000China State key Laboratory of Biochemical engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Spinel oxide(NiCo_(2.O_(4))has demonstrated great potential to replace noble metal catalysts for the oxidation reaction of air *** further boost the oxidation ability of such catalysts,in this study,a facile surface-engineering strategy wherein NiCo_(2.O_(4) was treated with different alkali solvents was *** obtained catalyst(NiCo_(2.O_(4)-OH)showed a higher surface alkalinity and more surface defects compared to the pristine spinel oxide,including enhanced structural distortion as well as promoted oxygen *** propane oxidation ability of NiCo_(2.O_(4)-OH was greatly enhanced,with a propane conversion rate that was approximately 6.4 times higher than that of pristine NiCo_(2.O_(4) at a reaction temperature 193℃.This work sets a valuable paradigm for the surface modulation of spinel oxide via alkali treatment to ensure a high-performance oxidation catalyst.

关键词： NiCo_(2.O_(4) surface defects alkali treatment propane oxidation

Bionic lightweight design of limb leg units for hydraulic quadruped robots by additive manufacturing and topology optimization

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Bio-Design and Manufacturing 2024年第1期7卷 1-13页

作者： Huaizhi Zong Junhui zhang lei Jiang Kun zhang Jun Shen Zhenyu Lu ke Wang Yanli Wang Bing xu The State key Laboratory of Fluid Power and Mechatronic Systems Zhejiang UniversityHangzhou 310058China Unmanned Vehicle Research and Development Center China North Vehicle Research InstituteBeijing 100072China School of Mechatronic engineering Nanchang UniversityNanchang 330031China Auclean High-Tech Ltd. Wuxi 214108China

Galloping cheetahs,climbing mountain goats,and load hauling horses all show desirable locomotion capability,which motivates the development of quadruped *** various quadruped robots,hydraulically driven quadruped robots show great potential in unstructured environments due to their discrete landing positions and large *** the most critical movement unit of a quadruped robot,the limb leg unit(LLU)directly affects movement speed and reliability,and requires a compact and lightweight *** by the dexterous skeleton–muscle systems of cheetahs and humans,this paper proposes a highly integrated bionic actuator system for a better dynamic performance of an *** propose that a cylinder barrel with multiple element interfaces and internal smooth channels is realized using metal additive manufacturing,and hybrid lattice structures are introduced into the lightweight design of the piston *** addition,additive manufacturing and topology optimization are incorporated to reduce the redundant material of the structural parts of the *** mechanical properties of the actuator system are verified by numerical simulation and experiments,and the power density of the actuators is far greater than that of cheetah *** mass of the optimized LLU is reduced by 2..5%,and the optimized LLU shows better response time performance when given a step signal,and presents a good trajectory tracking ability with the increase in motion frequency.

关键词： Additive manufacturing Bionic lightweight design Limb leg unit Quadruped robot Trajectory tracking

Latest Scientific Results of china's Lunar and Deep Space Exploration(2.2.–2.2.)

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空间科学学报 2024年第4期44卷 622-632页

作者： xu Lin LI lei LIU {2. LIN Honglei LI yang LIU yang XIE Lianghai zhang Jinhai QIAO Fuhao HAN Juanjuan ZOU Yongliao General Office of the Lunar and Deep Space Exploration Chinese Academy of SciencesBeijng 100190 State key Laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190 institute of Geochemistry Chinese Academy of SciencesGuiyang 550081 institute of Geology and Geophysics Chinese Academy of SciencesBeijing 100029

china has successfully launched six lunar probes so *** Chang'E-1 to Chang'E-4,they completed the circling,landing and roving exploration,of which Chang'E-4 was the first landing on the far side of the Moon in human ***'E-5 was launched in December 2.2.,bringing back 1731 g of lunar soil *** the detailed analysis of the samples,the scientists understand the history of late lunar volcanism,specifically extending lunar volcanism by about 800 million to 1 billion years,and proposed possible *** addition,there are many new understandings of space weathering such as meteorite impacts and solar wind radiation on the ***'s first Mars exploration mission Tianwen-1 was successfully launched in July *** the study of scientific data,a number of important scientific achievements have been made in the topography,water environment and shallow surface structure of *** paper introduces the main scientific achievements of Chang'E-4,Chang'E-5 and Tianwen-1 in the past two years,excluding technical and engineering *** to the large number of articles involved,this paper only introduces part of the results.

关键词： Lunar and deep space exploration of china Chang’E-4 mission Chang’E-5 mission Tianwen-1 mission

Exploring formation mechanism and source attribution of ozone during the 2.19 Wuhan Military World Games:Implications for ozone control strategies

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Journal of Environmental Sciences 2024年第2期136卷 400-411页

作者： lei zhang Lili Wang Runyu Wang Nan Chen Yuan {2. ke Li Jie Sun Dan Yao Yuesi Wang Minghui Tao {2. Sun institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China University of the chinese academy of Sciences Beijing 100049China Hubei Ecological Environment Monitoring Center Station Wuhan 430072China Guizhou Research and Designing institute of Environmental Sciences Guizhou Academy of Environmental Science and DesignGuiyang 550081China Jiangsu key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China School of Environment Key Laboratory for Yellow River and Huai River Water Environment and Pollution ControlMinistry of EducationHenan Normal UniversityXinxiang 453007China key Laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China

A series of emission reduction measures were conducted in Wuhan,Central china,to ensure good air quality during the 7th Military World Games(MWG)in October *** better understand the implications for ozone(O_(3))pollution control strategies,we applied integrated analysis approaches based on the de-weathered statistical model,parameterization methods,chemical box model,and positive matrix factorization *** the MWG,concentrations of O_(3),NO_x,and volatile organic compound(VOCs),OFP(O_(3)formation potential),L_(OH)(OH radical loss rate)were 83μg/m^(3),43μg/m^(3),2. ppbv,188μg/m^(3),and 3.9 s^(-1),respectively,which were 2.%,18%,3%,15%,and 13%lower than pre-MWG values and 6%,39%,30%,33%,and 50%lower than post-MWG values,*** removing meteorological influence,O_(3)and its precursors during the MWG decreased largely compared with post-MWG values,and only O_(3),NO_(2.,and oxygenated VOCs(OVOCs)declined compared with pre-MWG values,which revealed the emission reduction measures during the MWG played an important role for O_(3)*** six VOCs sources,the mass contributions of biomass burning and solvents usage during the MWG decreased largely compared with pre-MWG values.O_(3)production was sensitive to VOCs and the key species were aromatics,OVOCs,and alkenes,which originated mainly from solvents usage,biomass burning,industrial-related combustion,and vehicle *** O_(3)concentration during the strict control was mainly caused by OVOCs reduction due to biomass burning ***,the O_(3)abatement strategies of Wuhan should be focused on the mitigation of high-reactivity VOCs.

关键词： VOCs Ozone Wuhan Military World Games Source apportionment Relative incremental reactivity Random forest

Highly Strong,Tough,and Cryogenically Adaptive Hydrogel Ionic Conductors via Coordination Interactions

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Research 2024年第3期2024卷 703-713页

作者： Zhuomin Wang Siheng Wang lei zhang He Liu {2. {2. institute of Chemical Industry of Forestry Products Key Laboratory of Biomass Energy and MaterialJiangsu ProvinceKey Laboratory of Chemical Engineering of Forest ProductsNational Forestry and Grassland AdministrationNational Engineering Research Center of Low-Carbon Processing and Utilization of Forest BiomassJiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesChinese Academy of ForestryNanjing 210042China College of Chemical engineering Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesNanjing Forestry UniversityNanjing 210037China.

Despite the promise of high flexibility and conformability of hydrogel ionic conductors,existing polymeric conductive hydrogels have long suffered from compromises in mechanical,electrical,and cryoadaptive properties due to monotonous functional improvement strategies,leading to lingering ***,we propose an all-in-one strategy for the preparation of poly(acrylic acid)/cellulose(PAA/Cel)hydrogel ionic conductors in a facile yet effective manner combining acrylic acid and salt-dissolved cellulose,in which abundant zinc ions simultaneously form strong coordination interactions with the two polymers,while free solute salts contribute to ionic conductivity and bind water molecules to prevent ***,the developed PAA/Cel hydrogel simultaneously achieved excellent mechanical,conductive,and cryogenically adaptive properties,with performances of 42.5 MPa for compressive strength,1.6 MPa for tensile strength,896.9%for stretchability,9.2.MJ m^(−3)for toughness,59.5 kJ m^(−2.for fracture energy,and 13.9 and 6.2.mS cm^(−1)for ionic conductivity at 2. and−70°C,*** by these features,the resultant hydrogel ionic conductor is further demonstrated to be assembled as a self-powered electronic skin(e-skin)with high signal-to-noise ratio for use in monitoring movement and physiological signals regardless of cold temperatures,with hinting that could go beyond high-performance hydrogel ionic conductors.

关键词： Highly freezing salts

Machine Learning for Signal Demodulation in Underwater Wireless Optical Communications

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china Communications 2024年第5期21卷 297-313页

作者： Ma Shuai yang lei Ding Wanying Li Hang {2. Zhongdan xu Jing Li Zongyan xu Gang Li Shiyin Department of Strategic and Advanced Interdisciplinary Research Peng Cheng LaboratoryShenzhen 518055China School of Information and Control engineering China University of Mining and TechnologyXuzhou 221116China Data-driven Intelligent Information System Laboratory Shenzhen Research Institute of Big DataShenzhen 518172China Ocean College Zhejiang UniversityZhoushan 316021China State key Laboratory of Millimeter Waves Southeast UniversityNanjing 210096China

The underwater wireless optical communication(UWOC)system has gradually become essential to underwater wireless communication *** other existing works on UWOC systems,this paper evaluates the proposed machine learningbased signal demodulation methods through the selfbuilt experimental *** on such a platform,we first construct a real signal dataset with ten modulation ***,we propose a deep belief network(DBN)-based demodulator for feature extraction and multi-class feature *** also design an adaptive boosting(Ada Boost)demodulator as an alternative scheme without feature filtering for multiple modulated ***,it is demonstrated by extensive experimental results that the Ada Boost demodulator significantly outperforms the other *** also reveals that the demodulator accuracy decreases as the modulation order increases for a fixed received optical power.A higher-order modulation may achieve a higher effective transmission rate when the signal-to-noise ratio(SNR)is higher.

关键词： AdaBoost DBN machine learning signal demodulation

Chronic administration of triclosan leads to liver fibrosis through hepcidin-ferroportin axis-mediated iron overload

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Journal of Environmental Sciences 2024年第3期137卷 144-154页

作者： Jing Liu Lecong zhang Fang xu Ping zhang yang Song College of Eco-Environmental engineering Guizhou Minzu UniversityGuiyang 550025China The institute of Karst Wetland Ecology Guizhou Minzu UniversityGuiyang 550025China State key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Triclosan(TCS)has been manufactured as an antibacterial compound for half a ***,it is widely used in various personal care products;however,its potential adverse effects raise a lot of ***,we create a long-term oral administration mouse model and identify the corresponding hepatotoxicity of *** discover that daily intragastric administration of 10 mg/kg TCS to mice for 12.weeks results in severe hepatic *** study displays that hepatic iron increased 18%,2.%and 2.%upon oral TCS treatment for4,8 and 12.weeks,*** by hepatic iron variation,splenic and duodenal iron are increased,which indicates systemic iron *** only excessive iron accumulated in the liver,abnormal hepatic malondialdehyde,prostaglandin synthase 2.and glutathione peroxidase 4 are pointed to *** study uncovers that hepcidin expression increases 7%,10%,4%in serum and 2.4-,4.8-,and 2.3-fold on transcriptional levels upon TCS exposure for 4,8 and 12.weeks,*** together,the mice in the TCS-treated group show disordered systemic iron homeostasis via the upregulated hepatic hepcidin-ferroportin ***,both hepatic iron overload(systemic level)and hepatocyte ferroptosis(cellular level)are accused of TCS-induced liver ***■,an iron scavenger,significantly ameliorates TCS-induced liver *** summary,this study confirms the impact of TCS on liver fibrosis;a critical signal pathway is also *** significance of the current study is to prompt us to reevaluate the“pros and cons”of TCS applications.

关键词： Triclosan Iron metabolism Hepcidin Hepatotoxicity Liver fibrosis

Ionic Liquid-Enhanced Assembly of Nanomaterials for Highly Stable Flexible Transparent Electrodes

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Nano-Micro Letters 2024年第7期16卷 441-455页

作者： Jianmin yang Li Chang Xiqi zhang Ziquan Cao {2. Jiang key Laboratory of Bio-Inspired Materials and Interfacial Science Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China University of chinese academy of Sciences Beijing 100049People’s Republic of China College of Chemistry and Chemical engineering Chongqing University of TechnologyChongqing 400054People’s Republic of China Binzhou institute of Technology Binzhou 256600People’s Republic of China Nanomics Biotechnology Co. Ltd.HangzhouPeople’s Republic of China

The controlled assembly of nanomaterials has demon-strated significant potential in advancing technological ***,achieving highly efficient and low-loss assembly technique for nanomate-rials,enabling the creation of hierarchical structures with distinctive func-tionalities,remains a formidable ***,we present a method for nanomaterial assembly enhanced by ionic liquids,which enables the fabrication of highly stable,flexible,and transparent electrodes featuring an organized layered *** utilization of hydrophobic and non-volatile ionic liquids facilitates the production of stable interfaces with water,effectively preventing the sedimentation of 1D/2. nanomaterials assembled at the ***,the interfacially assembled nanomaterial monolayer exhibits an alternate self-climbing behavior,enabling layer-by-layer transfer and the formation of a well-ordered MXene-wrapped silver nanowire network *** resulting composite film not only demonstrates exceptional photoelectric performance with a sheet resistance of 9.4Ωsq^(-1) and 93%transmittance,but also showcases remarkable environmental stability and mechanical *** noteworthy is its application in transparent electromagnetic interference shielding materials and triboelectric nanogenerator *** research introduces an innovative approach to manufacture and tailor functional devices based on ordered nanomaterials.

关键词： Ionic liquids Assembly Silver nanowires MXene nanosheets Flexible transparent electrodes

In-situ coupling construction of interface bridge to enhance electrochemical stability of all solid-state lithium metal batteries

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Journal of Energy Chemistry 2024年第2期89卷 18-26,I0003页

作者： Qianwei zhang Rong yang Chao Li {2. Mao Bohai Wang Meng Luo Yinglin Yan Yiming Zou Lisheng Zhong Yunhua xu International Research Center for Composite and Intelligent Manufacturing Technology Institute of Chemical Power SourcesXi’an University of TechnologyXi’an 710048ShaanxiChina School of Materials Science and engineering Xi’an University of TechnologyXi’an 710048ShaanxiChina School of Electrical engineering Xi’an University of TechnologyXi’an 710048ShaanxiChina Yulin University Yulin 719000ShaanxiChina

Polymer-based composite electrolytes composed of three-dimensional Li_(6.4)La_(3)Zr_(2.Al_(0.2.O_(12.(3D-LLZAO)have attracted increasing attention due to their continuous ion conduction and satisfactory mechanical ***,the organic/inorganic interface is incompatible,resulting in slow lithium-ion transport at the ***,the compatibility of organic/inorganic interface is an urgent problem to be *** by the concept of“gecko eaves”,polymer-based composite solid electrolytes with dense interface structures were *** bridging of organic/inorganic interfaces was established by introducing silane coupling agent(3-chloropropyl)trimethoxysilane(CTMS)into the PEO-3D-LLZAO(PL)*** in-situ coupling reaction improves the interface affinity,strengthens the organic/inorganic interaction,reduces the interface resistance,and thus achieves an efficient interface ion transport *** prepared PEO-3D-LLZAO-CTMS(PLC)electrolyte exhibits enhanced ionic conductivity of 6.04×10^(-4)S cm^(-1)and high ion migration number(0.61)at 60℃and broadens the electrochemical window(5.1 V).At the same time,the PLC electrolyte has good thermal stability and high mechanical ***,the Li Fe PO_(4)|PLC|Li battery has excellent rate performance and cycling stability with a capacity decay rate of 2.2.after 100 cycles at 60℃and 0.1 *** advantages of PLC membranes indicate that this design approach is indeed practical,and the in-situ coupling method provides a new approach to address interface compatibility issues.

关键词： Organic/inorganic interphase Coupling effect Composite electrolyte Interface compatibility