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Facile Surface engineering of NiCo_(2)O_(4) to Boost Propane Oxidation Activity

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china Petroleum Processing & Petrochemical Technology 2024年第1期26卷 19-26页

作者： yang Jialei Wang Fengyi lei yang zhang Mingchao Sun Shiqiang xu Wenfan ke Jiaxiang Wu Haojie Li Xingyun Qi Jian institute of Materials for Energy and Environment College of Materials Science and EngineeringQingdao UniversityQingdao 266071China School of Chemistry and Chemical engineering Hubei Key Laboratory of Coal Conversion and New Carbon MaterialsWuhan University of Science and TechnologyWuhan 430081China Department of Burn and Plastic Surgery Qingdao Municipal Hospital Affiliated to Rehabilitation UniversityQingdao 266000China State key Laboratory of Biochemical engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Spinel oxide(NiCo_(2)O_(4))has demonstrated great potential to replace noble metal catalysts for the oxidation reaction of air *** further boost the oxidation ability of such catalysts,in this study,a facile surface-engineering strategy wherein NiCo_(2)O_(4) was treated with different alkali solvents was *** obtained catalyst(NiCo_(2)O_(4)-OH)showed a higher surface alkalinity and more surface defects compared to the pristine spinel oxide,including enhanced structural distortion as well as promoted oxygen *** propane oxidation ability of NiCo_(2)O_(4)-OH was greatly enhanced,with a propane conversion rate that was approximately 6.4 times higher than that of pristine NiCo_(2)O_(4) at a reaction temperature 193℃.This work sets a valuable paradigm for the surface modulation of spinel oxide via alkali treatment to ensure a high-performance oxidation catalyst.

关键词： NiCo_(2)O_(4) surface defects alkali treatment propane oxidation

Bionic lightweight design of limb leg units for hydraulic quadruped robots by additive manufacturing and topology optimization

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Bio-Design and Manufacturing 2024年第1期7卷 1-13页

作者： Huaizhi Zong Junhui zhang lei Jiang Kun zhang Jun Shen Zhenyu Lu ke Wang Yanli Wang Bing xu The State key Laboratory of Fluid Power and Mechatronic Systems Zhejiang UniversityHangzhou 310058China Unmanned Vehicle Research and Development Center China North Vehicle Research InstituteBeijing 100072China School of Mechatronic engineering Nanchang UniversityNanchang 330031China Auclean High-Tech Ltd. Wuxi 214108China

Galloping cheetahs,climbing mountain goats,and load hauling horses all show desirable locomotion capability,which motivates the development of quadruped *** various quadruped robots,hydraulically driven quadruped robots show great potential in unstructured environments due to their discrete landing positions and large *** the most critical movement unit of a quadruped robot,the limb leg unit(LLU)directly affects movement speed and reliability,and requires a compact and lightweight *** by the dexterous skeleton–muscle systems of cheetahs and humans,this paper proposes a highly integrated bionic actuator system for a better dynamic performance of an *** propose that a cylinder barrel with multiple element interfaces and internal smooth channels is realized using metal additive manufacturing,and hybrid lattice structures are introduced into the lightweight design of the piston *** addition,additive manufacturing and topology optimization are incorporated to reduce the redundant material of the structural parts of the *** mechanical properties of the actuator system are verified by numerical simulation and experiments,and the power density of the actuators is far greater than that of cheetah *** mass of the optimized LLU is reduced by 24.5%,and the optimized LLU shows better response time performance when given a step signal,and presents a good trajectory tracking ability with the increase in motion frequency.

关键词： Additive manufacturing Bionic lightweight design Limb leg unit Quadruped robot Trajectory tracking

Latest Scientific Results of china's Lunar and Deep Space Exploration(2022–2024)

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空间科学学报 2024年第4期44卷 622-632页

作者： xu Lin LI lei LIU jianzhong LIN Honglei LI yang LIU yang XIE Lianghai zhang Jinhai QIAO Fuhao HAN Juanjuan ZOU Yongliao General Office of the Lunar and Deep Space Exploration Chinese Academy of SciencesBeijng 100190 State key Laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190 institute of Geochemistry Chinese Academy of SciencesGuiyang 550081 institute of Geology and Geophysics Chinese Academy of SciencesBeijing 100029

china has successfully launched six lunar probes so *** Chang'E-1 to Chang'E-4,they completed the circling,landing and roving exploration,of which Chang'E-4 was the first landing on the far side of the Moon in human ***'E-5 was launched in December 2020,bringing back 1731 g of lunar soil *** the detailed analysis of the samples,the scientists understand the history of late lunar volcanism,specifically extending lunar volcanism by about 800 million to 1 billion years,and proposed possible *** addition,there are many new understandings of space weathering such as meteorite impacts and solar wind radiation on the ***'s first Mars exploration mission Tianwen-1 was successfully launched in July *** the study of scientific data,a number of important scientific achievements have been made in the topography,water environment and shallow surface structure of *** paper introduces the main scientific achievements of Chang'E-4,Chang'E-5 and Tianwen-1 in the past two years,excluding technical and engineering *** to the large number of articles involved,this paper only introduces part of the results.

关键词： Lunar and deep space exploration of china Chang’E-4 mission Chang’E-5 mission Tianwen-1 mission

Biodegradable amphiphilic block copolymers containing functionalized PEO blocks:Controlled synthesis and biomedical potentials

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Science china Chemistry 2010年第3期53卷 519-527页

作者： zhang Yu1,2,SUN PeiJian1,2 & GAN ZhiHua1 1CAS key Laboratory of engineering Plastics,institute of Chemistry,chinese academy of sciences,beijing 100190,china 2Graduate University of chinese academy of sciences,beijing 100039,china CAS key Laboratory of engineering Plastics Institute of Chemistry Chinese Academy of Sciences Beijing China Graduate University of chinese academy of sciences Beijing China

A series of controllable amphiphilic block copolymers composed of poly(ethylene oxide)(PEO) as the hydrophilic block and poly(ε-caprolactone)(PCL) as the hydrophobic block with the amino terminal group at the end of the PEO chain(PCL-b-PEO-NH2) were *** on the further reaction of reactive amino groups,diblock copolymers with functional carboxyl groups(PCL-b-PEO-COOH) and functional compounds RGD(PCL-b-PEO-RGD) as well as the triblock copolymers with thermosensitive PNIPAAm blocks(PCL-b-PEO-b-PNIPAAM) were *** well-controlled structures of these copolymers with functional groups and blocks were characterized by gel permeation chromatography(GPC) and 1H NMR *** copolymers with functionalized hydrophilic blocks were fabricated into microspheres for the examination of biofunctions via cell culture experiments and in vitro drug *** results indicated the significance of introducing functional groups(e.g.,NH2,COOH and RGD) into the end of the hydrophilic block of amphiphilic block copolymers for biomedical potentials in tissue engineering and controlled drug release.

关键词： amphiphilic block copolymers biodegradable polymers functional terminal group cell growth drug release

Exploring formation mechanism and source attribution of ozone during the 2019 Wuhan Military World Games:Implications for ozone control strategies

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Journal of Environmental sciences 2024年第2期136卷 400-411页

作者： lei zhang Lili Wang Runyu Wang Nan Chen Yuan yang ke Li Jie Sun Dan Yao Yuesi Wang Minghui Tao yang Sun institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China University of the chinese academy of sciences Beijing 100049China Hubei Ecological Environment Monitoring Center Station Wuhan 430072China Guizhou Research and Designing institute of Environmental sciences Guizhou Academy of Environmental Science and DesignGuiyang 550081China Jiangsu key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China School of Environment Key Laboratory for Yellow River and Huai River Water Environment and Pollution ControlMinistry of EducationHenan Normal UniversityXinxiang 453007China key Laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China

A series of emission reduction measures were conducted in Wuhan,Central china,to ensure good air quality during the 7th Military World Games(MWG)in October *** better understand the implications for ozone(O_(3))pollution control strategies,we applied integrated analysis approaches based on the de-weathered statistical model,parameterization methods,chemical box model,and positive matrix factorization *** the MWG,concentrations of O_(3),NO_x,and volatile organic compound(VOCs),OFP(O_(3)formation potential),L_(OH)(OH radical loss rate)were 83μg/m^(3),43μg/m^(3),26 ppbv,188μg/m^(3),and 3.9 s^(-1),respectively,which were 26%,18%,3%,15%,and 13%lower than pre-MWG values and 6%,39%,30%,33%,and 50%lower than post-MWG values,*** removing meteorological influence,O_(3)and its precursors during the MWG decreased largely compared with post-MWG values,and only O_(3),NO_(2),and oxygenated VOCs(OVOCs)declined compared with pre-MWG values,which revealed the emission reduction measures during the MWG played an important role for O_(3)*** six VOCs sources,the mass contributions of biomass burning and solvents usage during the MWG decreased largely compared with pre-MWG values.O_(3)production was sensitive to VOCs and the key species were aromatics,OVOCs,and alkenes,which originated mainly from solvents usage,biomass burning,industrial-related combustion,and vehicle *** O_(3)concentration during the strict control was mainly caused by OVOCs reduction due to biomass burning ***,the O_(3)abatement strategies of Wuhan should be focused on the mitigation of high-reactivity VOCs.

关键词： VOCs Ozone Wuhan Military World Games Source apportionment Relative incremental reactivity Random forest

Application of three-dimensional discrete element face-to-face contact model with fissure water pressure to stability analysis of landslide in Panluo iron mine

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Science china(Technological sciences) 2005年第z1期48卷 146-156页

作者： zhang lei1,2, WEI Zuoan1, LIU Xiaoyu1 & LI Shihai1 1.institute of Mechanics, chinese academy of sciences, beijing 100080, china 2.Graduate School, chinese academy of sciences, beijing 100060, china institute of Mechanics Chinese Academy of Sciences Beijing 100080 China

Three-dimensional discrete element face-to-face contact model with fissure water pressure is established in this paper and the model is used to simulate three-stage process of landslide under fissure water pressure in the opencast mine, according to the actual state of landslide in Panluo iron mine where landslide happened in 1990 and was fathered in 1999. The calculation results show that fissure water pressure on the sliding surface is the main reason causing landslide and the local soft interlayer weakens the stability of slope. If the discrete element method adopts the same assumption as the limit equilibrium method, the results of two methods are in good agreement; while if the assumption is not adopted in the discrete element method, the critical φ numerically calculated is less than the one calculated by use of the limit equilibrium method for the sameC. Thus, from an engineering point of view, the result from the discrete element model simulation is safer and has more widely application since the discrete element model takes into account the effect of rock mass structures.

关键词： face-to-facecontactmodel, fissure water pressure, three-dimensional discrete element method,landslide.

Highly Strong,Tough,and Cryogenically Adaptive Hydrogel Ionic Conductors via Coordination Interactions

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Research 2024年第3期2024卷 703-713页

作者： Zhuomin Wang Siheng Wang lei zhang He Liu xu xu institute of Chemical Industry of Forestry Products Key Laboratory of Biomass Energy and MaterialJiangsu ProvinceKey Laboratory of Chemical Engineering of Forest ProductsNational Forestry and Grassland AdministrationNational Engineering Research Center of Low-Carbon Processing and Utilization of Forest BiomassJiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesChinese Academy of ForestryNanjing 210042China College of Chemical engineering Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesNanjing Forestry UniversityNanjing 210037China.

Despite the promise of high flexibility and conformability of hydrogel ionic conductors,existing polymeric conductive hydrogels have long suffered from compromises in mechanical,electrical,and cryoadaptive properties due to monotonous functional improvement strategies,leading to lingering ***,we propose an all-in-one strategy for the preparation of poly(acrylic acid)/cellulose(PAA/Cel)hydrogel ionic conductors in a facile yet effective manner combining acrylic acid and salt-dissolved cellulose,in which abundant zinc ions simultaneously form strong coordination interactions with the two polymers,while free solute salts contribute to ionic conductivity and bind water molecules to prevent ***,the developed PAA/Cel hydrogel simultaneously achieved excellent mechanical,conductive,and cryogenically adaptive properties,with performances of 42.5 MPa for compressive strength,1.6 MPa for tensile strength,896.9%for stretchability,9.2 MJ m^(−3)for toughness,59.5 kJ m^(−2)for fracture energy,and 13.9 and 6.2 mS cm^(−1)for ionic conductivity at 25 and−70°C,*** by these features,the resultant hydrogel ionic conductor is further demonstrated to be assembled as a self-powered electronic skin(e-skin)with high signal-to-noise ratio for use in monitoring movement and physiological signals regardless of cold temperatures,with hinting that could go beyond high-performance hydrogel ionic conductors.

关键词： Highly freezing salts

Conceptual design and simulation analysis of thermal behaviors of TGR blast furnace and oxygen blast furnace

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Science china(Technological sciences) 2010年第1期53卷 85-92页

作者： zhang Hui1,2,LI HuiQuan1,TANG Qing1 & BAO WeiJun1 1 National engineering Laboratory for Hydrometallurgical Cleaner Production Technology,institute of Process engineering,chinese academy of sciences,beijing 100190,china 2 Graduate University of chinese academy of sciences,beijing 100049,china National engineering Laboratory for Hydrometallurgical Cleaner Production Technology Institute of Process Engineering Chinese Academy of Sciences Graduate University of chinese academy of sciences

Extensive use of carbon based fuel is the main inducement for global warming and more extreme *** carbon dioxide emission and enhancing energy use is a common subject in steel *** the integrated steel plant,decreasing carbon dioxide emission must consider energy balance in the whole iron and steel works,and secondary energy must be actively *** promising blast-furnaces,top gas recovery blast furnace(TGR-BF) and oxygen blast furnace have been *** this paper,conceptual TGR blast furnace and oxygen blast furnace are *** on the idea of blast furnace gas de-CO2 circulating as reducing agent and the idea of pure oxygen blast decreasing the thermal reserve zone temperature,process modeling is conducted with ASPEN *** is shown that the developed model reasonably describes the energy balance and mass balance feature of the furnace,and provides basic thermodynamic condition for *** effects of changes in different operation conditions are studied by sensitivity analysis and reference data from simulation.

关键词： TGR blast-furnace thermal behavior simulation analysis CO2 emission decreasing

Remote sensing based shrub above-ground biomass and carbon storage mapping in Mu Us desert,china

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Science china(Technological sciences) 2010年第S1期53卷 176-183页

作者： xu Min 1,2,CAO ChunXiang 1,TONG QingXi 1,LI ZengYuan 3,zhang Hao 1,HE QiSheng 1,2,GAO Mengxu 1,2,ZHAO Jian 1,2,ZHENG Sheng 1,2,CHEN Wei 1,2 & ZHENG LanFen 1 1State key Laboratory of Remote Sensing Science,Jointly Sponsored by the institute of Remote Sensing Applications of chinese academy of sciences and beijing Normal University,beijing 100101,china 2 Graduate School of the chinese academy of sciences,beijing 100049,china 3 Research institute of Forest Resources and Information Techniques,chinese academy of Forestry,beijing 10009,china State key Laboratory of Remote Sensing Science Jointly Sponsored by the Institute of Remote Sensing Applications of Chinese Academy of Sciences and Beijing Normal University Beijing China Graduate School of the chinese academy of sciences Beijing China Research institute of Forest Resources and Information Techniques Chinese Academy of Forestry Beijing China

The estimation of above-ground biomass(AGB) and carbon storage is very important for arid and semi-arid ***-1A/B satellite data combined with field measurement data was used for the estimation of shrub AGB and carbon storage in the Mu Us desert,*** correlations of shrub AGB and spectral reflectance of four bands as well as their combined vegetation indexes were respectively analyzed and stepwise regression analysis was employed to establish AGB prediction *** prediction equation based on ratio vegetation index(RVI)was proved to be more suitable for shrub AGB estimation in the Mu Us desert than *** AGB and carbon storage were mapped using the RVI based prediction model in *** statistics showed the western Mu Us desert has relatively high AGB and carbon storage,and that the gross shrub carton storage in Mu Us desert reaches 16 799 200 t,which has greatly contributed to the carbon fixation in northern china.

关键词： above-ground biomass carbon storage Mu Us desert HJ-1A/B remote sensing