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Electronic structure regulation and built-in electric field synergistically strengthen photocatalytic nitrogen fixation performance on Ti-BiOBr/TiO_(2)heterostructure

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Rare Metals 2024年第3期43卷 1125-1138页

作者： Ru-Qi Li Yu-Jie Bian Chun-ming yang Li Guo Tao-Xia Ma Chuan-Tao Wang Feng fu Dan-Jun Wang College of Chemistry and Chemical Engineering Yan’an UniversityYan’an Key Laboratory of Green Catalysis and Quality Improvement and Utilization of Low Rank CoalYan’an716000China

At present,industrial synthetic ammonia was still obtained through the Hubble-Bosch process,with large energy *** is a research hotspot to realize green synthetic ammonia by using solar *** difficulty of photocatalytic ammonia synthesis was that the photo-excited electrons have not enough energy to active N≡*** this study,Ti was doped into BiOBr by one-step hydrothermal method,which was oxidized into TiO_(2)when the doping amount reaches the maximum,in situ forming Ti_(0.31)B_(0.69)OB/TiO_(2)*** from the synergistic effect of Ti doping and S-scheme heterojunction,the synthetic ammonia efficiency of Ti_(0.31)B_(0.69)OB/TiO_(2)-11.96 reached 1.643 mmol·g_(cat)^(-1)at mild conditions and without hole scavenger for up to 7 h,the efficiency of synthetic ammonia is 115 times,10.5 times and 3.3 times of that of BiOBr,Ti_(0.31)B_(0.69)OB and TiO_(2),***,DFT calculation confirms that Ti doping accurately refine the electronic structure of BiOBr,facilitate nitrogen adsorption activation and reduce hydrogenation reaction energy barrier,thus accelerating the reaction kinetics of photocatalytic nitrogen reduction(NRR),Meanwhile,constructing S-scheme heterojunction boosts the separation and transfer of photogenerated electron-hole pairs,improving the reduction ability of electrons in the conduction band of TiO_(2)and the oxidation ability of holes in the valence band of Ti_(0.31)B_(0.69)OB.

关键词： S-scheme heterostructure Electronic structure regulation Built-in electric field Synergistical stren4gthening Photocatalytic nitrogen fixation

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Changes of coastline and tidal flat and its implication for ecological protection under human activities: Take China’s Bohai Bay as an example

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China Geology 2024年第1期7卷 26-35页

作者： Yong Li ming-zheng Wen Heng Yu Peng yang Fei-cui Wang fu Wang Tianjin Center China Geological SurveyMinistry of Natural ResourcesTianjin 300170China Key Laboratory of Coast Geo-environment China Geological SurveyMinistry of Natural ResourcesTianjin 300170China Tianjin Key Laboratory of Coast Geological Processes and Environmental Safety Tianjin 300170China Hebei University of Environmental Engineering Qinhuangdao 066102China Hebei Engineering Research Center for Ecological Restoration of seaward Rivers and Coastal Waters Qinhuangdao 066102China Department of Earth and Environment Boston UniversityBoston 02215USA

The change processes and trends of shoreline and tidal flat forced by human activities are essential issues for the sustainability of coastal area,which is also of great significance for understanding coastal ecological environment changes and even global *** on field measurements,combined with Linear Regression(LR)model and Inverse Distance Weighing(IDW)method,this paper presents detailed analysis on the change history and trend of the shoreline and tidal flat in Bohai *** shoreline faces a high erosion chance under the action of natural factors,while the tidal flat faces a different erosion and deposition patterns in Bohai Bay due to the impact of human *** implication of change rule for ecological protection and recovery is also *** should be taken to protect the coastal ecological *** models used in this paper show a high correlation coefficient between observed and modeling data,which means that this method can be used to predict the changing trend of shoreline and tidal *** research results of present study can provide scientific supports for future coastal protection and management.

关键词： Shoreline Tidal flat Erosion deposition patterns Changing trend Ecological protection Human activity Linear regression model Inverse distance weighing method Prediction Bohai Bay

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Inactivation of TGF-βsignaling in CAR-T cells

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Cellular & Molecular Immunology 2024年第3期21卷 309-310页

作者： Zaopeng yang yang-Xin fu Changping Laboratory Beijing102206China Department of Basic Medical Sciences School of MedicineTsinghua UniversityBeijing100084China

Accumulating evidence suggests that the transforming growth factor(TGF)-βpathway might be an ideal target for optimizing chimeric antigen receptor(CAR)-T-cell therapy for solid *** Cellular&Molecular Immunology,Liang et al.(2024)reported that CAR-T cells expressing SMAD7 displayed favorable antitumor efficacy and a reduced risk of systemic toxicity.

关键词： CAR Immunology

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A Case of Energy and Ecology System Development and a New Approach to System Dynamics Modeling

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Systems Science and Systems Engineering 2002年第4期11卷 462-470页

作者： JIA Ren-an, yang Bo, WU fu-ming, HU Ling Institute of Systems Engineering, Nanchang University, Nanchang 330047, China Institute of Systems Engineering Nanchang University Nanchang 330047 China

This paper uses SD rate variable fundamental in-tree modeling, SD branch-vector determinant method and systems archetype as tools to understand the structure and functions of energy and ecology system in Wangheqiu.

关键词： energy and ecology system feedback loop systems archetype

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SYNTHESIS,PHOTOCHROMIC PROPERTIES OF PYRRYL SUBSTITUTED HETEROCYCLIC fuLGIDES

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Chinese Chemical Letters 1993年第3期4卷 199-202页

作者： Lian He YU yang fu ming Mei Gong FAN Intitute of photographic chemistry,Academia Sinica Beijing 100101

Nine new 3-acetyl pyrrole derivatives and corresponding 3-pyrryl substituted heterocyclic fulgides:3-pyrryl-ethylidene(isopropylidene)succinic anhydrides have been synthesized and *** photochromic behavour in several organic solvents were *** coloured form of fulgide Ⅱc,(E)-α-(1,2,4-trimethyl- 3-pyrryl)-ethylidene(isopropylidene)succinic anhydride,shows absorption maxmium at 715nm in *** is the longest absorption among the known photochromic fulgides

关键词：加加加比 SYNTHESIS,PHOTOCHROMIC PROPERTIES OF PYRRYL SUBSTITUTED HETEROCYCLIC fuLGIDES 创口

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Low-temperature NH_(3) abatement via selective oxidation over a supported copper catalyst with high Cu^(+) abundance

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Journal of Environmental Sciences 2024年第9期143卷 12-22页

作者： Zhiming yang Lin Peng Leneng yang mingli fu Daiqi Ye Peirong Chen Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control National Engineering Laboratory for VOCs Pollution Control Technology and EquipmentSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Guangdong Chengyi Environmental Technology Corp. Shaoguan 512158China

Selective catalytic NH_(3)-to-N_(2) oxidation(NH_(3)-SCO)is highly promising for abating NH_(3) emissions slipped from stationary flue gas after-treatment *** practical application,however,is limited by the non-availability of low-cost catalysts with high activity and N_(2) ***,using defect-rich nitrogen-doped carbon nanotubes(NCNT-AW)as the support,we developed a highly active and durable copper-based NH_(3)-SCO catalyst with a high abundance of cuprous(Cu^(+))*** obtained Cu/NCNT-AW catalyst demonstrated outstanding activity with a T_(50)(*** temperature to reach 50% NH_(3) conversion)of 174℃ in the NH_(3)-SCO reaction,which outperformed not only the Cu catalyst supported on N-free O-functionalized CNTs(OCNTs)or NCNT with less surface defects,but also those most active Cu catalysts in open *** kinetics measurements and temperature-programmed surface reactions using NH_(3)as a probe molecule revealed that the NH_(3)-SCO reaction on Cu/NCNT-AW follows an internal selective catalytic reaction(i-SCR)route involving nitric oxide(NO)as a key *** to mechanistic investigations by X-ray photoelectron spectroscopy,Raman spectroscopy,and X-ray absorption spectroscopy,the superior NH_(3)-SCO performance of Cu/NCNT-AW originated from a synergy of surface defects and ***,surface defects promoted the anchoring of Cu O nanoparticles on N-containing sites and,thereby,enabled efficient electron transfer from N to Cu O,increasing significantly the fraction of SCR-active Cu^(+)sites in the *** study puts forward a new idea for manipulating and utilizing the interplay of defects and N-dopants on carbon surfaces to fabricate Cu^(+)-rich Cu catalysts for efficient abatement of slip NH_(3)emissions via selective oxidation.

关键词： NH_(3)-SCO XANES Localized etching N-doping N_(2) selectivity i-SCR

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Composite Converter Combined APFC with Switched-capacitor Converter

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 281-291页

作者： Qing fu Yishan Chen Yixing Su yang Hang School of Physics Sun Yat-Sen UniversityGuangzhou 510275China

To reduce switch numbers and voltage stress in semiconductor devices,this paper proposes a novel single-phase converter combined Active Power Factor Correction(APFC)with switched-capacitor *** addition,dynamic voltage regulation and voltage gain are improved by integrating the boost converter and switching capacitor *** interstage bulk capacitor is no longer *** average current control with redistribution of voltage in cells is proposed to obtain voltage lift ability of the switching capacitor cells and maintain a high-power *** study and verify the proposed converter preliminarily,theoretical analysis and simulation are presented in the ***,a 50o W prototype with two different configurations is built for experimental *** proposed converter can reach 95.62%of maximum efficiency,0.99 of power factor,and 3.55%of THD with 600 V output voltage,simultaneously.

关键词： AC-DC converter composite conveter power factor correction switched capacitor

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Irreducible anteromedial radial head dislocation without fracture caused by transposed biceps tendon in an adult:A case report and literature review

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Chinese Journal of Traumatology 2024年第3期27卷 180-186页

作者： ming-fu fu Hai-Ning Zuo Tao Sun ming-Zhang Mu Zhi-Yong Zhou Department of Orthopedic Surgery Yantaishan HospitalYantaiShandong Province264003China

Irreducible anteromedial radial head dislocation(IARHD)caused by transposed biceps tendon is *** diagnosis and surgical failure often occur.A 46-year-old fisherman presented with 10 days history of painful swelling and restricted movement of his right elbow due to strangulation injury by a fishing boat *** examination,the images of the right elbow reveals in a"semi-extended and pronated"elastic fixation *** and 3-dimensional reconstruction CT reveals an isolated anteromedial radial head dislocation with extreme protonation of the radius and the bicipital tuberosity towards the posterior aspect of the elbow joint,and MRI shows biceps tendon wrapping around the radial neck,similar to umbilical cord wrapping seen in *** Henry approach was applied for the first time to reduce the biceps *** patient achieved a good functional recovery at 26 months,which represents the first reported case of IARHD without fracture caused by biceps tendon in an *** treatment of IARHD,attention should be paid to the phenomenon of biceps tendon *** clinical examination,comprehensive imaging modalities,and appropriate surgical approach are the keys to successful management.

关键词： Biceps tendon Henry approach Irreducible Anteromedial dislocation Radial head Elbow Adult

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Effects of cement-enhanced soil on the ultimate lateral resistance of composite pile in clayey soil

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第1期16卷 183-191页

作者： Zhijun yang Kexin Chen Xudong fu Zhiyan Zou School of Civil Engineering Wuhan UniversityWuhan430000China Changjiang Design Group Co. Ltd.Wuhan430000China Institute of Geotechnical Engineering College of Civil Engineering and ArchitectureMOE Key Laboratory of Soft Soils and Geoenvironmental EngineeringZhejiang UniversityHangzhou310000China

The composite pile consisting of core-pile and surrounding cement-enhanced soil is a promising pile foundation in recent ***,how and to what extent the cement-enhanced soil influences the ultimate lateral resistance has not been fully *** this paper,the ultimate lateral resistance of the composite pile was studied by finite element limit analysis(FELA)and theoretical upper-bound *** results of FELA and theoretical analysis revealed three failure modes of laterally loaded composite *** effects of the enhanced soil thickness,strength,and pile-enhanced soil interface characteristics on the ultimate lateral resistance were *** results show that increasing the enhanced soil thickness leads to a significant improvement on ultimate lateral resistance factor(N P),and there is a critical thickness beyond which the thickness no longer affects the N *** the enhanced soil strength induced 6.2%-232.6%increase of N ***,no noticeable impact was detected when the enhanced soil strength was eight times higher than that of the natural *** maximum increment of N P is only 30.5%caused by the increase of interface adhesion factor(a).An empirical model was developed to calculate the N P of the composite pile,and the results show excellent agreement with the analytical results.

关键词： Composite pile Ultimate soil resistance Finite element limit analysis(FELA) Plasticity theory Failure mode

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Improvement of Film Cooling Design for Turbine Vane Leading Edge Considering Combustor Outflow

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Journal of Thermal Science 2024年第1期33卷 311-327页

作者： WANG Xinyu LIU Cunliang fu Zhongyi LI yang ZHU Huiren School of Power and Energy Northwestern Polytechnical UniversityXi'an 710072China AECC Hunan Aviation Powerplant Research Institute Zhuzhou 412002China

As the interaction between the combustor and the turbine in the aero-engine continues to increase,the film cooling design considering the combustor swirling outflow has become the research *** swirling inflow and high-temperature gas first affect the vane leading edge(LE).However,no practical improved solution for the LE cooling design has been proposed considering the combustor swirling *** this paper,the improved scheme of showerhead cooling is carried out around the two ways of adopting the laid-back-fan-shaped hole and reducing the coolant outflow *** film cooling effectiveness(η) and the coolant flow state are obtained by PSP(pressure-sensitive-paint) and numerical simulation methods,*** research results show that the swirling inflow increases the film distribution inhomogeneity by imposing the radial pressure gradient on the vane to make the film excessively gather in some *** showerhead film cooling adopts the laid-back-fan-shaped hole to reduce the momentum when the coolant flows *** this cooling scheme improves the film attachment and increases the surface-averaged film cooling effectiveness(η_(sur)) by as much as15.4%,the film distribution inhomogeneity *** reducing the coolant outlet angle,the wall-tangential velocity of the coolant increases,and the wall-normal velocity *** the swirl intake condition,both ηand the film distribution uniformity are significantly increased,and the growth of η_(sur) is up to 16.5%.This paper investigates two improved schemes to improve the showerhead cooling under the swirl intake condition to provide a reference for the vane cooling design.

关键词： turbine vane showerhead cooling swirling inflow laid-back-fan-shaped hole film hole inclination

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