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基于原位交联增容策略的增强PLA/NR共混物界面相容性和发泡性能研究

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陕西科技大学学报 2025年第1期43卷 73-80,100页

作者：王广静邵亮苏晨阳马春燕姬占有陕西科技大学化学与化工学院中国轻工业轻化工助剂重点实验室陕西西安710021

聚乳酸(PLA)是目前最具发展潜力的生物材料之一,但其韧性差,极大的限制了在塑料领域的发展与应用.已有研究发现天然橡胶(NR)的引入可以改善其韧性差的缺陷,但二者为不相容体系,发泡性能差.因此,本文基于原位交联增容原理,采用1,4-双(叔... 详细信息

聚乳酸(PLA)是目前最具发展潜力的生物材料之一,但其韧性差,极大的限制了在塑料领域的发展与应用.已有研究发现天然橡胶(NR)的引入可以改善其韧性差的缺陷,但二者为不相容体系,发泡性能差.因此,本文基于原位交联增容原理,采用1,4-双(叔丁基过氧异丙基)苯(BIPB)增强PLA和NR的界面相容性,并以超临界二氧化碳(scCO_(2))发泡技术制备了PLA/NR复合发泡材料.探究了不同BIPB含量对复合材料界面相容性、韧性及复合材料发泡行为的影响.结果表明,BIPB的引入显著增强了PLA/NR复合材料的相容性、韧性及发泡性能.当BIPB含量为0.25 phr时,PLA/NR复合材料的断裂伸长率从原来的25.75%增加到35.24%,提升了1.37倍;表观密度从初始的0.565 g·cm^(-3)下降至0.373 g·cm^(-3);平均泡孔尺寸从7.5μm下降至5.0μm.

关键词：聚乳酸天然橡胶 1,4-双(叔丁基过氧异丙基)苯超临界发泡相容性

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Using kin discrimination to construct synthetic microbial communities of Bacillus subtilis strains impacts the growth of black soldier fly larvae

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Insect Science 2024年第6期31卷 1943-1959页

作者： Jun-Hui Zhao Ping Cheng Yi Wang Xun yan Zhi-min Xu Dong-Hai Peng Guo-Hui Yu ming-Wei shao Key Laboratory of Green Prevention and Control on Fruits and Vegetables in South China Ministry of Agriculture and Rural AffairsGuangdong University Key Laboratory for Sustainable Control of Fruit and Vegetable Diseases and PestsInnovative Institute for Plant HealthCollege of Agriculture and BiologyZhongkai University of Agriculture and EngineeringGuangzhouChina State Key Laboratory of Agricultural Microbiology National Engineering Research Center of Microbial PesticidesCollege of Life Science and TechnologyHuazhong Agricultural UniversityWuhanChina Hubei Hongshan Laboratory WuhanChina College of Resources and Environment Zhongkai University of Agriculture and EngineeringGuangzhouChina

Using synthetic microbial communities to promote host growth is an effective ***,the construction of such communities lacks theoretical *** discrimination is an effective means by which strains can recognize themselves from non-self,and construct competitive microbial communities to produce more secondary ***,the construction of cooperative communities benefits from the widespread use of beneficial *** used kin discrimination to construct synthetic communities(SCs)comprising 13 Bacillus subtilis strains from the surface and gut of black soldier fly(BSF)*** assessed larval growth promotion in a pigeon manure system and found that the synthetic community comprising 4 strains(SC 4)had the most profound *** analyses of these 4 strains revealed that their complementary functional genes underpinned the robust functionality of the cooperative synthetic community,highlighting the importance of strain *** analyzing the bacterial composition of BSF larvae and the pigeon manure substrate,we observed that SC 4 altered the bacterial abundance in both the larval gut and pigeon *** also influenced microbial metabolic functions and co-occurrence network *** discrimination facilitates the rapid construction of synthetic *** positive effects of SC 4 on larval weight gain resulted from the functional redundancy and complementarity among the ***,SC 4 may enhance larval growth by inducing shifts in the bacterial composition of the larval gut and pigeon *** elucidated how the SC promoted larval growth by regulating bacterial composition and provided theoretical guidance for the construction of SCs.

关键词： community construction genomic analysis gut bacteria pigeon manure

Amplitude Oscillations of the Resonant Phenomena in a Frenkel-Kontorova Model with an Incommensurate Structure

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Chinese Physics Letters 2012年第6期29卷 68-71页

作者： yan yan-Zong WANG Cang-Long shao Zhi-Gang yanG Lei College of Mathematics and Statistics Longdong UniversityQingyang 745000 Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000 College of Physics and Electronic Engineering and Joint Laboratory of Atomic and Molecular Physics of NWNU&IMP CAS Northwest Normal UniversityLanzhou 730070 Laboratary of Quantum Information Technology Institute of Condensed Matter PhysicsSchool of Physics and Telecommunication EngineeringSouth China Normal UniversityGuangzhou 510006 Department of Physics Lanzhou UniversityLanzhou 730000

Dynamical mode locking phenomena in incommensurate structures of the dc- and ac-driven overdamped FrenkelKontorova model are studied by molecular-dynamics *** is found that the Shapiro steps exhibit significantly different amplitude and frequency dependences from the ones observed in the commensurate *** step widths still oscillate with the amplitude,but the form is no longer Bessel-like,i.e.,the anomaly appears in our *** same type of anomalies is also exhibited by the critical depinning *** oscillatory behavior and the anomalies are also revealed in the ((F),Fac) phase diagram where three phases are *** oscillations are directly correlated with the existence and the stability of interference phenomena in real systems.

关键词： force steps commensurate

Purification and studies on characteristics of cholinesterases from Daphnia magna

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2013年第4期14卷 325-335页

作者： yan-xia yanG Li-zhi NIU shao-nan LI Institute of Pesticide and Environmental Toxicology College of Agriculture and BiotechnologyZhejiang University

Due to their significant value in both economy and ecology,Daphnia had long been employed to investigate in vivo response of cholinesterase(ChE) in anticholinesterase exposures,whereas the type constitution and property of the enzyme remained unclear.A type of ChE was purified from Daphnia magna using a three-step procedure,i.e.,Triton X-100 extraction,ammonium sulfate precipitation,and diethylaminoethyl(DEAE)-Sepharose Fast-Flow *** to sodium dodecyl sulfate polyacrylamide gel electrophoresis(SDS-PAGE),molecular mass of the purified ChE was estimated to be 84 *** on substrate studies,the purified enzyme preferred butyrylthiocholine iodide(BTCh) [with maximum velocity(Vmax)/Michaelis constant(Km)=8.428 L/(min·mg protein)] to acetylthiocholine iodide(ATCh) [with V max /Km =5.346 L/(min·mg protein)] as its *** of the purified enzyme was suppressed by high concentrations of either ATCh or *** studies showed that the purified enzyme was more sensitive towards inhibition by tetraisopropylpyrophosphoramide(iso-OMPA) than by 1,5-bis(4-allyldimethylammoniumphenyl) pentan-3-one dibromide(BW284C51).Result of the study suggested that the purified ChE was more like a type of pseudocholinesterase,and it also suggested that Daphnia magna contained multiple types of ChE in their bodies.

关键词： Crustacea Pseudocholinesterase Cholinesterase Substrate preference Selective inhibitors

Controllable synthesis and photocatalytic activities of rod-shaped mesoporous titanosilicate composites with varied aspect ratios

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Chinese Chemical Letters 2014年第6期25卷 962-966页

作者： Feng-Jiao Chen Chang-Wang shao min-Nan Zhao Zhao-Sheng Bu yan Zhang Xiao-Nan Dai Guo-Wei Zhou Key Laboratory of Fine Chemicals in Universities of Shandong School of Chemistry and Pharmaceutical EngineeringQilu University of Technology School of Chemical Engineering and Environment Weifang University of Science and Technology

Rod-shaped mesoporous titanosilicate composites （RMTSs） with controllable aspect ratios （ARs） were fabricated using cetyltrimethylammonium bromide （CTAB） and ammonium hydroxide （NH4OH） at a continuous stirring rate, resulting in ARs ranging from 1 to 5. Slowing the stirring rate or increasing the concentration of CTAB mainly impacted the length growth, whereas NH4OH affected the width growth. Photocatalytic activity studies revealed that the length of RMTSs played a more significant role than the width at lower ARs in their photocatalytic activity.

关键词： Titanosilicate Aspect ratio Growth direction Photocatalytic activity

Modified k-ω model using kinematic vorticity for corner separation in compressor cascades

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Science China(Technological Sciences) 2016年第5期59卷 795-806页

作者： LIU yangWei yan Hao FANG Le LULiPeng LI QiuShi shao Liang National Key Laboratory of Science and Technology on Aero-Engine Aero-thermodynamics School of Energy and Power Engineering Beihang University Beijing 100191 China Collaborative Innovation Center of Advanced Aero-Engine Beihang University Beijing 100191 China Laboratory of Mathematics and Physics Ecole Centrale de Pekin Beihang University Beijing 100191 China Laboratoire de Mecanique ties Fluides et d'Acoustique Ecole Centrale de Lyon Ecullv 69134 France

A new method of modifying the conventional k-w turbulence model for comer separation is proposed in this paper. The production term in the w equation is modified using kinematic vorticity considering fluid rotation and deformation in complex geometric boundary conditions. The corner separation flow in linear compressor cascades is calculated using the original k-w model, the modified k-w model and the Reynolds stress model （RSM）. The numerical results of the modified model are compared with the available experimental data, as well as the corresponding results of the original k-w model and RSM. In terms of accuracy, the modified model, which significantly improves the performance of the original k-w model for predicting comer separation, is quite competitive with the RSM. However, the modified model, which has considerably lower computational cost is more robust than the RSM.

关键词： k-w comodel kinematic vorticity corner separation compressor cascades

A continuous-discontinuous cellular automaton method for cracks growth and coalescence in brittle material

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Acta Mechanica Sinica 2014年第1期30卷 73-83页

作者： Fei yan Xia-Ting Feng Peng-Zhi Pan shao-Jun Li State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChinese Academy of Science

A method of continuous-discontinuous cellular automaton for modeling the growth and coalescence of multiple cracks in brittle material is presented. The method uses the level set to track arbitrary discontinuities, and calculation grids are independent of the discontinuities and no remeshing are required with the crack growing. Based on Grif- fith fracture theory and Mohr-Coulumb criterion, a mixed fracture criterion for multiple cracks growth in brittle mate- rial is proposed. The method treats the junction and coales- cence of multiple cracks, and junction criterion and coales- cence criterion for brittle material are given, too. Besides, in order to overcome the tracking error in the level set ap- proximation for crack junction and coalescence, a dichotomy searching algorithm is proposed. Introduced the above the- ories into continuous-discontinuous cellular automaton, the present method can be applied to solving multiple crack growth in brittle material, and only cell stiffness is needed and no assembled global stiffness is needed. Some numerical examples are given to shown that the present method is efficient and accurate for crack junction, coalescence and percolation problems.

关键词： Continuous-discontinuous cellular automatonmethod Multiple crack growth Discontinuous cellular au-tomaton Junction criterion - Coalescence criterion

Analysis of Penetration Depth of Pipeline on Cohesive Soil Seabed

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China Ocean Engineering 2019年第6期33卷 739-745页

作者： ZHANG Qi-yi ZHANG Yuan yan Yun-qiang WU shao-xuan College of Engineering Ocean University of ChinaQingdao 266100China Key Laboratory of Marine Engineering in Shandong Province Qingdao 266100China

This paper conducts laboratory tests to investigate detailedly the soil deformation law around the pipeline and its penetration depth under self-gravity. The seabed model is prepared by consolidating saturated soil using vacuum pressure technology, and the pipeline models are specifically designed to possess different radii. Based on the experimental results and digital images, the soil deformation process is analyzed and summarized, a kinematic admissible velocity field is given and an upper bound solution of pipeline penetration depth and soil reaction force is derived and proposed in this paper. In order to verify the accuracy of the upper bound solution deduced in this paper,a comparison is made among some published results and the solution suggested in this paper, the comparison results confirm that the upper bound solution and the soil failure mode are reasonable. Finally two empirical formulas are given in this paper to estimate the soil reaction force of seabed and the penetration depth of pipeline. The empirical formulas are in agreement with the upper bound solution derived in this paper, and the conclusion of this paper could provide some theoretical reference for the further study of the interaction between the pipeline and the soil.

关键词： upper bound solution kinematic admissible velocity field soil reaction force penetration depth

Ru Nanoparticles Supported on Co-Embedded N-Doped Carbon Nanotubes as Efficient Electrocatalysts for Hydrogen Evolution in Basic Media

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Chemical Research in Chinese Universities 2020年第3期36卷 425-430页

作者： yan Baolin LIU Dapeng FENG Xilan shao mingzhe ZHANG Yu Key Laboratory of Bio-inspired SniaH Interfacial Science and Techiology of Ministry of EducationSchool of ChemistryBeihang UniversityBeijing 100191P.R.China Inteniational Research Institute for Multidisciplinary Science Beihang UniversityBeijing 100191P.R.China Beijing Advanced Innovation Center for Biomedical Engineering Beihang UniversityBeijing 100191P.R.China

A challenging but urgent task is to construct efficient and robust hydrogen evolution reaction(HER)electrocatalysts for practically feasible and sustainable hydrogen production through alkaline water *** we report a simple and mild pyrolysis method to synthesize the efficient Ru nanoparticles(NPs) supported on Co-embedded N-doped carbon nanotubes(Ru/Co-NCNTs)catalyst for HER in basic *** Ru/Co-NCNTs display remarkable performance with a low overpotential of only 35mV at 10mA/cm^2,a small Tafel slope(36mV/dec),and a high mass activity in 1mol/L KOH,which is superior to commercial 20% Pt/C *** excellent performance is benefited from the enhanced conductivity of N-doped carbon nanotubes(NCNTs)and high intrinsic activity triggered by synergistic coupling between Ru NPs and Co-embedded N-doped carbon nanotubes(Co-NCNTs).

关键词： Carbon nanotube Ru nanoparticle Hydrogen evolution reaction(HER) Electrocatalyst