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Innovative Solutions for High-Performance Silicon Anodes in Lithium-Ion Batteries:Overcoming Challenges and Real-World Applications

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Nano-Micro Letters 2024年第9期16卷 341-384页

作者： Mustafa Khan Suxia Yan Mujahid Ali Faisal Mahmood Yang zheng Guochun Li Junfeng Liu Xiaohui Song yong Wang Institute for Energy Research Jiangsu UniversityZhenjiang 212013JiangsuPeople’s Republic of China School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013JiangsuPeople’s Republic of China School of Materials Science and Engineering Hefei University of TechnologyHefei 230009AnhuiPeople’s Republic of China

Silicon(Si)has emerged as a potent anode material for lithium-ion batteries(LIBs),but faces challenges like low electrical conductivity and significant volume changes during lithiation/delithiation,leading to material pulverization and capacity *** research on nanostructured Si aims to mitigate volume expansion and enhance electrochemical performance,yet still grapples with issues like pulverization,unstable solid electrolyte interface(SEI)growth,and interparticle *** review delves into innovative strategies for optimizing Si anodes’electrochemical performance via structural engineering,focusing on the synthesis of Si/C composites,engineering multidimensional nanostructures,and applying non-carbonaceous *** a stable SEI is vital to prevent electrolyte decomposition and enhance Li^(+)transport,thereby stabilizing the Si anode interface and boosting cycling Coulombic *** also examine groundbreaking advancements such as self-healing polymers and advanced prelithiation methods to improve initial Coulombic efficiency and combat capacity *** review uniquely provides a detailed examination of these strategies in real-world applications,moving beyond theoretical *** offers a critical analysis of these approaches in terms of performance enhancement,scalability,and commercial *** conclusion,this review presents a comprehensive view and a forward-looking perspective on designing robust,high-performance Si-based anodes the next generation of LIBs.

关键词： Silicon anode Energy storage Nanostructure Prelithiation Binder

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Multi-scale persistent spatiotemporal transformer for long-term urban traffic flow prediction

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Journal of Electronic Science and Technology 2024年第1期22卷 53-69页

作者： Jia-Jun Zhong yong Ma Xin-zheng Niu Philippe Fournier-Viger Bing Wang Zu-kuan Wei School of Computer Science and Engineering University of Electronic Science and Technology of ChinaChengdu611731China College of Computer Science&Software Engineering Shenzhen UniversityShenzhen518060China School of Computer Science Southwest Petroleum UniversityChengdu610500China

Long-term urban traffic flow prediction is an important task in the field of intelligent transportation,as it can help optimize traffic management and improve travel *** improve prediction accuracy,a crucial issue is how to model spatiotemporal dependency in urban traffic *** recent years,many studies have adopted spatiotemporal neural networks to extract key information from traffic ***,most models ignore the semantic spatial similarity between long-distance areas when mining spatial *** also ignore the impact of predicted time steps on the next unpredicted time step for making long-term ***,these models lack a comprehensive data embedding process to represent complex spatiotemporal *** paper proposes a multi-scale persistent spatiotemporal transformer(MSPSTT)model to perform accurate long-term traffic flow prediction in *** adopts an encoder-decoder structure and incorporates temporal,periodic,and spatial features to fully embed urban traffic data to address these *** model consists of a spatiotemporal encoder and a spatiotemporal decoder,which rely on temporal,geospatial,and semantic space multi-head attention modules to dynamically extract temporal,geospatial,and semantic *** spatiotemporal decoder combines the context information provided by the encoder,integrates the predicted time step information,and is iteratively updated to learn the correlation between different time steps in the broader time range to improve the model’s accuracy for long-term *** on four public transportation datasets demonstrate that MSPSTT outperforms the existing models by up to 9.5%on three common metrics.

关键词： Graph neural network Multi-head attention mechanism Spatio-temporal dependency Traffic flow prediction

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Refining the Factors Affecting N_(2)O Emissions from Upland Soils with and without Nitrogen Fertilizer Application at a Global Scale

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Advances in Atmospheric Sciences 2024年第9期41卷 1804-1820页

作者： Wenqian JIANG Siqi LI yong LI Meihui WANG Bo WANG Ji LIU Jianlin SHEN Xunhua zheng State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Key Laboratory for Agro-ecological Processes in Subtropical Regions Institute of Subtropical AgricultureChinese Academy of SciencesChangsha 410125China Changsha Research Station for Agricultural&Environmental Monitoring Chinese Academy of SciencesChangsha 410125China University of Chinese Academy of Sciences Beijing 100049China State Environmental Protection Key Laboratory of Formation and Prevention of the Urban Air Pollution Complex Shanghai Academy of Environment SciencesShanghai 200233China Institute of Carbon Neutrality Qilu ZhongkeJinan 251699China Hubei Province Key Laboratory for Geographical Process Analysis and Simulation Central China Normal UniversityWuhan 430079China Department of Ecohydrology Leibniz Institute of Freshwater Ecology and Inland FisheriesBerlin 12587Germany Key laboratory of Environment Change and Resources Use in Beibu Gulf Ministry of EducationNanning Normal UniversityNanning 530001China Golden Mantis school of Architecture Soochow UniversitySuzhou 215123China

Nitrous oxide(N_(2)O)is a long-lived greenhouse gas that mainly originates from agricultural *** and more studies have explored the sources,influencing factors and effective mitigation measures of N_(2)O in recent ***,the hierarchy of factors influencing N_(2)O emissions from agricultural soils at the global scale remains *** this study,we carry out correlation and structural equation modeling analysis on a global N_(2)O emission dataset to explore the hierarchy of influencing factors affecting N_(2)O emissions from the nitrogen(N)and non-N fertilized upland farming systems,in terms of climatic factors,soil properties,and agricultural *** results show that the average N_(2)O emission intensity in the N fertilized soils(17.83 g N ha^(-1)d^(-1))was significantly greater than that in the non-N fertilized soils(5.34 g N ha^(−1) d^(−1))(p<0.001).Climate factors and agricultural practices are the most important influencing factors on N_(2)O emission in non-N and N fertilized upland soils,*** different climatic zones,without fertilizer,the primary influence factors on soil N_(2)O emissions are soil physical properties in subtropical monsoon zone,whereas climatic factors are key in the temperate *** fertilizer,the primary influence factors for subtropical monsoon and temperate continental zones are soil physical properties,while agricultural measures are the main factors in the temperate monsoon *** enhanced agricultural practices,such as reduced N fertilizer rate combined with the addition of nitrification and urease inhibitors can potentially mitigate N_(2)O emissions by more than 60%in upland farming systems.

关键词： N_(2)O emissions influencing factors nitrogen cycling upland farming systems

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CAOSA-extracted lignin improves enzymatic hydrolysis of cellulose

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Green Energy & Environment 2024年第7期9卷 1101-1111页

作者： Sen Ma zheng Li Jonathan Sperry Xing Tang yong Sun Lu Lin Jian Liu Xianhai Zeng College of Energy State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University Fujian Engineering and Research Centre of Clean and High-valued Technologies for Biomass Xiamen Key Laboratory of Clean and High-valued Utilization of Biomass Centre for Green Chemical Science University of Auckland

The conversion of biomass into sugar platform compounds is very important for the biorefinery industry. Pretreatment is essential to the biomass of the sugar platform, however, the lignin obtained by pretreatment, as a key part of lignocellulose, generally has a passive effect on the enzymatic hydrolysis of cellulose into sugars. In this study, p-TsOH(p-toluenesulfonic acid), DES(Deep eutectic solvent) and CAOSA(cooking with active oxygen and solid alkali) pretreatment ways were used to fraction lignin from bamboo biomass. After CAOSA treatment, the hydrolysis efficiency of the pulp was 95.57%. Moreover, the effect of different treatment methods on lignin properties was studied and the promotion effect of lignin was investigated by adding it to the cellulose enzymatic hydrolysis system. In this work, the results showed that CAOSA-extracted lignin with lower ?(1.31–1.25) had a better adsorption effect on the enzyme protein. p-TsOH-extracted lignin with a larger S/G ratio enhanced the inhibition of enzymatic hydrolysis. In addition, the presence of-COOHs in lignin could reduce its inhibitory effect on cellulose saccharification.

关键词： Biomass pretreatment CAOSA Cellulose hydrolysis Lignin Enzyme

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A Confined Two-peaked Solar Flare Observed by EAST and SDO

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Research in Astronomy and Astrophysics 2024年第4期24卷 71-83页

作者： Liang Zhang Ruisheng zheng Zhike xue Changhui Rao Qing Lin Zhimao Du Jiawen Yao Libo Zhong Yao Chen Institute of Space Sciences Shandong UniversityWeihai 264209China Yunnan Key Laboratory of the Solar physics and Space Science Kunming 650011China Institute of Frontier and Interdisciplinary Science.Shandong University Qingdao266237China Institute of Optics and Electronics Chinese Academy of SciencesChengdu 610209China National Laboratory on Adaptive Optics Chengdu610209China University of Chinese Academy of Sciences Beijing 100049China Shanghai Astronomy Museum Shanghai201306China

The solar flare is one of the most violent explosions,and can disturb the near-Earth space *** for commonly single-peaked solar flares in soft X-ray,some special flares show intriguing a two-peak feature that is deserved much more ***,we reported a confined two-peaked solar flare and analyzed the associated eruptions using high-quality observations from Educational Adaptive-optics Solar Telescope and Solar Dynamics *** the flare,a magnetic flux rope(MFR)formed through partially tether-cutting reconnection between two sheared *** flare occurred after the MFR eruption that was confined by the overlying strong ***,a small underlying filament immediately erupted,which was possibly destabilized by the flare *** successive eruptions were confirmed by the analysis of the emission measure and the reconnection ***,we suggest that the two peaks of the confined solar flare are corresponding to two episodes of magnetic reconnection during the successive eruptions of the MFR and the underlying filament.

关键词： Sun:activity Sun:corona Sun:flares Sun:magnetic fields Sun:filaments prominences Online material:animations

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Modification, application and expansion of electrode materials based on cobalt telluride

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Journal of Energy Chemistry 2024年第10期97卷 710-737页

作者： Huilin Fan Yao Dai Xiaoyun xue Runguo zheng Yuan Wang Hamidreza Arandiyan Zhiyuan Wang Zongping Shao Hongyu Sun Yanguo Liu School of Materials Science and Engineering Northeastern University School of Resources and Materials Northeastern University at Qinhuangdao Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Northeastern University at Qinhuangdao Department of Chemical Engineering The University of Melbourne Centre for Advanced Materials and Industrial Chemistry (CAMIC) School of Science RMIT University Laboratory of Advanced Catalysis for Sustainability School of Chemistry University of Sydney WA School of Mines: Minerals Energy and Chemical Engineering Curtin University

Metal(Li,Na,K,Al)-ion batteries and lithium-sulfur and lithium-tellurium batteries are gaining recognition for their eco-friendly characteristics,substantial energy density,and sustainable ***,the overall performance of rechargeable batteries heavily depends on their electrode *** metal tellurides have recently gained significant attention due to their high electrical conductivity and *** telluride has received the most extensive research due to its catalytic activity,unique magnetic properties,and diverse composition and crystal ***,its limited conductivity and significant volume variation contribute to electrode structural deterioration and rapid capacity *** review comprehensively summarizes recent advances in rational design and synthesis of modified cobalt telluride-based electrodes,encompassing defect engineering(Te vacancies,cation vacancies,heterointerfaces,and homogeneous interfaces) and composite engineering(derived carbon from precursors,carbon fibers,Mxene,graphene nanosheets,etc.).Particularly,the intricate evolution mechanisms of the conversion reaction process during cycling are ***,these modified strategies applied to other transitional metal tellurides,such as iron telluride,nickel telluride,zinc telluride,copper telluride,molybdenum telluride,etc.,are also thoroughly ***,their application extends to emerging aqueous zinc-ion ***,potential challenges and prospects are discussed to further propel the development of transition metal tellurides electrode materials for next-generation rechargeable batteries.

关键词： Rechargeable batteries Transition metal tellurides Cobalt telluride Defect engineering Composite engineering

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Machine learning prediction model for gray-level co-occurrence matrix features of synchronous liver metastasis in colorectal cancer

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World Journal of Gastrointestinal Surgery 2024年第6期16卷 1571-1581页

作者： Kai-Feng Yang Sheng-Jie Li Jun Xu yong-Bin zheng Department of Gastrointestinal Surgery Renmin Hospital of Wuhan UniversityWuhan 430030Hubei ProvinceChina Department of Gastrointestinal Surgery The First College of Clinical Medical ScienceChina Three Gorges UniversityYichang Central People’s HospitalYichang 443008Hubei ProvinceChina

BACKGROUND Synchronous liver metastasis(SLM)is a significant contributor to morbidity in colorectal cancer(CRC).There are no effective predictive device integration algorithms to predict adverse SLM events during the diagnosis of *** To explore the risk factors for SLM in CRC and construct a visual prediction model based on gray-level co-occurrence matrix(GLCM)features collected from magnetic resonance imaging(MRI).METHODS Our study retrospectively enrolled 392 patients with CRC from Yichang Central People’s Hospital from January 2015 to May *** were randomly divided into a training and validation group(3:7).The clinical parameters and GLCM features extracted from MRI were included as candidate *** prediction model was constructed using a generalized linear regression model,random forest model(RFM),and artificial neural network *** operating characteristic curves and decision curves were used to evaluate the prediction *** Among the 392 patients,48 had SLM(12.24%).We obtained fourteen GLCM imaging data for variable screening of SLM prediction *** difference,mean sum,sum entropy,sum variance,sum of squares,energy,and difference variance were listed as candidate variables,and the prediction efficiency(area under the curve)of the subsequent RFM in the training set and internal validation set was 0.917[95%confidence interval(95%CI):0.866-0.968]and 0.09(95%CI:0.858-0.960),*** A predictive model combining GLCM image features with machine learning can predict SLM in *** model can assist clinicians in making timely and personalized clinical decisions.

关键词： Colorectal cancer Synchronous liver metastasis Gray-level co-occurrence matrix Machine learning algorithm Prediction model

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Quaternary integrative stratigraphy, biotas, and paleogeographical evolution of the Qinghai-Tibet Plateau and its surrounding areas

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Science China Earth Sciences 2024年

作者： yong WANG Mianping zheng Yuan LING Shuyuan XIANG Zhaogang SHAO Kexin ZHANG xue KE Xiao LIN Fang HAN Jian'en HAN Institute of Geology Chinese Academy of Geological Sciences School of Earth Sciences East China University of Technology Chinese Academy of Geological Sciences Institute of Geological Survey China University of GeosciencesWuhan Institute of Geomechanics Chinese Academy of Geological Sciences Institute of Mineral Resources Chinese Academy of Geological Sciences Faculty of Earth Sciences China University of Geosciences

The Quaternary strata on the Qinghai-Tibet Plateau contain rich information about the paleoclimate and environmental evolution, record the evolution process of the Quaternary regional tectonics, paleogeography, and geomorphology of the plateau, and are extremely important areas for studying the Quaternary geological events and regional environmental *** to a comprehensive analysis of the regional stratigraphic data and the development and evolution characteristics of the biota, based on the differences in the lithostratigraphic units, sedimentary characteristics, landforms, and drainage systems, the Quaternary strata on the Qinghai-Tibet Plateau and its surrounding areas are divided into five stratigraphic regions: the Tarim region, Loess Plateau region, Qinghai-Tibet Plateau region, Yunnan-Guizhou Plateau region, and India-Ganges region. The Qinghai-Tibet Plateau stratigraphic region is divided into seven stratigraphic sub-regions: the West Kunlun-Karakorum, AltunQilian Mountains, Qaidam-Hehuang, East Kunlun-Bayan Har, Qiangtang, East Xizang-West Yunnan-West Sichuan, and Gangdise-Himalayan sub-regions. This paper briefly describes the lithostratigraphic units of the seven stratigraphic sub-regions of the Qinghai-Tibet Plateau. According to the lithostratigraphic sequence and its sedimentary characteristics, stratigraphic contact relationship, formation age, and evolution of the biota in each stratigraphic sub-region, the Quaternary tectonic paleogeographic evolution of the Qinghai-Tibet Plateau is divided into four stages.(1) The inherited differential uplift stage since the Pliocene(2.6–1.8/1.5 Ma): the regional sedimentary differences were significant, and the stratigraphic distribution was limited,the alluvial-proluvial sandy conglomerate was widely developed along the piedmont, and fluvial and lacustrine deposits were developed in the low-lying areas between the mountains.(2) The mountain range flattening stage(1.8/1.5–1.2/0.8 Ma): the erosion u

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Strengthening and control of second-phase particle precipitation in ferritic/austenitic/martensitic heat-resistant alloys:a review

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Journal of Iron and Steel Research International 2024年第1期31卷 3-23页

作者： xue-cheng Peng Han-jie Guo Xin-fang Zhang Yi-wa Luo Ye Sun Jing Guo Rong-guang Yang Xiao-dan zheng School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China Beijing Key Laboratory of Special Melting and Preparation of High-End Metal Materials University of Science and Technology Beijing(USTB)Beijing100083China Beijing Shougang Gitane New MATERIALS Co. Ltd.Beijing102206China

Heat-resistant alloys with excellent mechanical properties are widely used in various fields,and further improvement in their properties is essential to meet the requirements in new-generation advanced supercritical boilers,nuclear reactors,superheaters,and other new materials *** effectively enhance the comprehensive performance of heat-resistant alloys,second-phase particle strengthening has been widely studied,and in the face of different service envi-ronments of advanced heat-resistant steels,the selection of suitable second-phase particles is essential to maximize the performance of these *** this end,three major types of reinforcing phases in heat-resistant alloys such as carbides,rare earth oxides,and intermetallic compounds are summarized.A comparative analysis of the precipitation behavior of the reinforcing phases with different types as well as the risks and means of controlling their use in service,is *** parameters for the application of various types of second-phase particles in heat-resistant alloys are provided to support the design and preparation of new ultrahigh-performance heat-resistant alloys.

关键词： Heat-resistant alloy Second-phase particle Carbide Rare earth oxide Intermetallic compound Strengthening

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Different mechanisms underlie similar species-area relationships in two tropical archipelagoes

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Plant Diversity 2024年第2期46卷 238-246页

作者： Shengchun Li Tieyao Tu Shaopeng Li Xian Yang yong zheng Liang-Dong Guo Dianxiang Zhang Lin Jiang Key Laboratory of Plant Resources Conservation and Sustainable Utilization South China Botanical GardenChinese Academy of SciencesGuangzhou 510650China ECNU-Alberta Joint Lab for Biodiversity Study Tiantong Forest Ecosystem National Observation and Research StationSchool of Ecological and Environmental SciencesEast China Normal UniversityShanghai 200241China School of Biological Sciences Georgia Institute of TechnologyAtlantaGA 30332USA Jiangxi Academy of Forestry Nanchang 330032China Institute of Eco-Chongming(IEC) Shanghai 202162China State Key Laboratory of Biocontrol School of EcologySun Yat-sen UniversityGuangzhou 510275China School of Geographical Sciences Fujian Normal UniversityFuzhou 350007China State Key Laboratory of Mycology Institute of MicrobiologyChinese Academy of SciencesBeijing 100101China

Despite much research in the field of island biogeography,mechanisms regulating insular diversity remain ***,we aim to explore mechanisms underlying plant species-area relationships in two tropical archipelagoes in the South China *** found positive plant species-area relationships for both coral and continental ***,our results showed that different mechanisms contributed to similar plant species-area relationships between the two *** coral islands,soil nutrients and spatial distance among communities played major roles in shaping plant community structure and species *** contrast,the direct effect of island area,and to a lesser extent,soil nutrients determined plant species richness on continental ***,increasing soil nutrients availability(N,P,K)had opposite effects on plant diversity between the two *** summary,the habitat quality effect and dispersal limitation are important for regulating plant diversity on coral islands,whereas the passive sampling effect,and to a lesser extent,the habitat quality effect are important for regulating plant diversity on continental *** generally,our findings indicate that island plant species-area relationships are outcomes of the interplay of both niche and neutral processes,but the driving mechanisms behind these relationships depends on the type of islands.

关键词： Coral and continental islands Plant diversity Soil nutrients Species-area relationships The sampling effect

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