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Remote,selective,and in situ manipulation of liquid droplets on a femtosecond laser-structured superhydrophobic shape-memory polymer by near-infrared light

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Science China Chemistry 2021年第5期64卷 861-872页

作者： xue Bai Jiale Yong Chao Shan yao Fang Xun Hou feng Chen State Key Laboratory for Manufacturing System Engineering and Shaanxi Key Laboratory of Photonics Technology for Information School of Electronic Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China

Droplet manipulation plays a significant role in the fields of biomedical detection,microfluidics,and chemical ***,it still remains a great challenge to simultaneously achieve remote,selective,and in situ droplet manipulation on the same ***,Fe_(3)O_(4)nanoparticles were doped in a shape-memory polymer(SMP)to prepare a photothermal-responsive Fe_(3)O_(4)-SMP composite which showed remarkable near-infrared(NIR)light-triggered shape-memory *** micropillar array was constructed on such Fe_(3)O_(4)-SMP composite through femtosecond laser microfabrication and fluoroalkylsilane *** surface wettability of the as-prepared surface can transform from a low-adhesive sliding state to a high-adhesive pinning state as the micropillars are deformed by ***,the deformed micropillars can stand up and restore to their original morphology under remote NIR light irradiation,resulting in the reversible and repeatable recovery of the ultralow-adhesive *** such light-triggered wettability switching,the droplets pinning on the sample surface can be remotely,selectively,and in situ ***,the superhydrophobic Fe_(3)O_(4)-SMP surface is successfully applied in lossless liquid transfer,selective droplet release,and droplet-based *** as-fabricated superhydrophobic surfaces with NIR light-controlled reversible wettability will hold great promise in the fields of liquid manipulation,lab-on-a-chip,and microfluidics.

关键词： droplet manipulation superhydrophobicity shape-memory polymer femtosecond laser light responsive

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Self-Powered Flexible Multicolor Electrochromic Devices for Information Displays

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Research 2024年第2期2023卷 529-540页

作者： Wenzhao xue Yun Zhang feng Liu yao Dou Mei Yan Wenshou Wang School of Chemistry and Chemical Engineering University of JinanJinan 250022P.R.China

The development of self-powered flexible multicolor electrochromic(EC)systems that could switch different color without an external power supply has remained extremely ***,a new trilayer film structure for achieving self-powered flexible multicolor EC displays based on self-charging/discharging mechanism is proposed,which is simply assembled by sandwiching an ionic gel film between 2 cathodic nickel hexacyanoferrate(NiHCF)and Prussian blue(PB)nanoparticle films on indium tin oxide *** display exhibits independent self-powered color switching of NiHCF and PB films with fast responsive time and high reversibility by selectively connecting the Al wire as anodes with the 2 EC *** switching is thus achieved through a color overlay effect by superimposing the 2 EC films,including green,blue,yellow,and *** bleaching/coloration process of the displays is driven by the discharging/self-charging mechanism for NiHCF and PB films,respectively,ensuring the self-powered color switching of the displays reversibly without an external power *** is further demonstrated that patterns can be easily created in the self-powered EC displays by the spray-coating method,allowing multicolor changing to convey specific ***,a self-powered ionic writing board is demonstrated based on the self-powered EC displays that can be repeatedly written freehand without the need of an external power *** believe that the design concept may provide new insights into the development of self-powered flexible multicolor EC displays with self-recovered energy for widespread applications.

关键词： connecting repeatedly powered

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UNIX平台基于Motif环境的图形用户界面开发技术

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江南大学学报（自然科学版） 2002年第1期1卷 38-41页

作者：朱雪峰顾耀林曹莹江南大学信息工程学院江苏无锡214036

通过对UNIX系统图形用户界面开发技术的研究 ,提出了GUI的体系结构 ,并在此基础上进行了开发层次和面向对象技术的分析。

关键词： UNIX平台 Motif环境图形演示图形上下文图形用户界面

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Effects of straw size in buried straw layers on water movement in adjacent soil layers

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International Journal of Agricultural and Biological Engineering 2016年第2期9卷 74-84页

作者： yao Mingze Li Bo Wang Tieliang feng xue College of Water Conservation Shenyang Agricultural UniversityShenyang 110866China

Deeply buried straw retention can improve the soil content of organic matter,its capacity for moisture preservation,the agroecological environment utilization efficiency of water resources,ensuring a stable crop yield;at the same time,the quantitative effects of deeply buried straw retention on soil moisture have a direct influence on the promotion and application of the *** an infiltration and evaporation experiment of a one-dimensional soil column,the effects of straw size on the water content of the straw and the adjacent soil were evaluated when the straw was deeply buried in soil;the infiltration and evaporation features of different sized straw and its adjacent soil were analyzed;the hydraulic conductivity,sorptivity and saturated water content of the straw were obtained;in the end,the water distribution laws of straw and adjacent soil under the same conditions were *** experiment was comprised of rod-shaped straw(RS),segment-shaped straw(SS)and filament-shaped straw(FS)to control treatment(CK).The results indicated that from the perspective of infiltration,the infiltration rate of filament-shape straw was the lowest at the stage of straw *** hydraulic conductivities of rod-shaped,filament-shaped and segment-shaped straws are 4.01 mm/min,1.33 mm/min and 0.03 mm/min at the stage of straw and adjacent soil saturation,*** is a strong effect on preventing infiltration from segment-shaped straw;with the help of the Philip model of long duration,the sorptivity of the soil with rod-shaped,filament-shaped and segment-shaped straws was 12.31 mm/min0.5,11.02 mm/min0.5 and 24.26 mm/min0.5 at the unsaturation stage,*** segment-shape straw improved the water absorption capacity of the soil and straw *** water retention capacities indicated that the saturated water contents of sandy loam,filament-shaped straw,segment-shaped straw and rod-shaped straw were 0.38 cm^(3)/cm^(3),0.29 cm^(3)/cm^(3),0.26 cm^(3)

关键词： deeply buried straw straw size soil moisture infiltration evaporation water retention

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Identifying the dynamic behaviors in complete reconstruction of Co-based complex precatalysts during electrocatalytic oxygen evolution

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Journal of Energy Chemistry 2025年第1期100卷 226-233页

作者： Jingfang Zhang Danyang Wu Linke Cai Youluan Lu Fanpeng Cheng Lijuan Shi Qun Yi yao Liu Yi Huang Key Laboratory of Green Chemical Engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Hubei Key Laboratory of Novel Reactor and Green Chemical Technology School of Chemical Engineering & Pharmacy Wuhan Institute of Technology Key Laboratory of Pesticide & Chemical Biology of Ministry of Education Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction of Ministry of Education College of Chemistry Central China Normal University College of Materials Science and Engineering Fuzhou University

Transition metal-based nanomaterials have emerged as promising electrocatalysts for oxygen evolution reaction（OER）. Considerable research efforts have shown that self-reconstruction occurs on these nanomaterials under operating conditions of OER process. However, most of them undergo incomplete reconstruction with limited thickness of reconstruction layer, leading to low component utilization and arduous exploration of real catalytic mechanism. Herein, we identify the dynamic behaviors in complete reconstruction of Co-based complexes during OER. The hollow phytic acid（PA） cross-linked CoFe-based complex nanoboxes with porous nanowalls are designed because of their good electrolyte penetration and mass transport ability, in favor of the fast and complete reconstruction. A series of experiment characterizations demonstrate that the reconstruction process includes the fast substitution of PA by OH-to form Co（Fe）(OH)xand subsequent potential-driven oxidation to Co（Fe）OOH. The obtained CoFeOOH delivers a low overpotential of 290 mV at a current density of 10 mA cm-2and a long-term *** experiment results together with theory calculations reveal that the Fe incorporation can result in the electron rearrangement of reconstructed CoFeOOH and optimization of their electronic structure,accounting for the enhanced OER activity. The work provides new insights into complete reconstruction of metal-based complexes during OER and offers guidelines for rational design of high-performance electrocatalysts.

关键词： Complete reconstruction Co-based complex Precatalysts Oxygen evolution reaction

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植物源外泌体样纳米囊泡刺激成骨细胞、抑制破骨细胞并促进成骨

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中国组织工程研究 2025年第31期29卷 6765-6771页

作者：药文鑫王毅蔡林冯晓波武汉大学中南医院疼痛科湖北省武汉市430071 武汉大学中南医院脊柱与骨肿瘤科湖北省武汉市430071

背景:骨质疏松症易引发病理性骨折且严重影响患者的生活质量,植物源外泌体样纳米囊泡在调节骨质疏松症骨平衡方面发挥着重要作用。目的:综述不同植物源外泌体样纳米囊泡在骨质疏松症治疗中的研究现状与展望。方法:通过计算机在PubMed、W... 详细信息

背景:骨质疏松症易引发病理性骨折且严重影响患者的生活质量,植物源外泌体样纳米囊泡在调节骨质疏松症骨平衡方面发挥着重要作用。目的:综述不同植物源外泌体样纳米囊泡在骨质疏松症治疗中的研究现状与展望。方法:通过计算机在PubMed、Web of Science、中国知网中检索1995年1月至2024年3月发表的相关文献,以“osteoporosis,plant-derived exosome-like nanovesicles,exosomes,osteoblasts,osteoclasts”为英文检索词,以“骨质疏松症,植物源外泌体样纳米囊泡,外泌体,成骨细胞,破骨细胞”为中文检索词,最终纳入53篇文献进行分析。结果与结论:植物源外泌体样纳米囊泡具有生物相容性、低毒性和天然靶向性等优点,这些特性不仅确保了其在体内的稳定存在与有效作用,还避免了不必要的免疫反应,为长期治疗策略的设计奠定了基础。植物源外泌体样纳米囊泡可以通过刺激成骨细胞增殖、抑制破骨细胞分化以及促进成骨-抑制破骨双重作用抗骨质疏松症;此外,部分植物源外泌体样纳米囊泡因具有骨靶向性,未来或将成为新型示踪靶标和治疗方案广泛应用于骨质疏松症治疗过程中。

关键词：骨质疏松症植物源性外泌体样纳米囊泡外泌体成骨细胞破骨细胞工程化外泌体

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Boosting Oxygen Evolution Reaction Performance on NiFe‑Based Catalysts Through d‑Orbital Hybridization

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Nano-Micro Letters 2025年第1期17卷 281-292页

作者： Xing Wang Wei Pi Sheng Hu Haifeng Bao Na yao Wei Luo State Key Laboratory of New Textile Materials and Advanced Processing Technology Key Laboratory of New Textile Materials and Applications of Hubei ProvinceSchool of Materials Science and EngineeringWuhan Textile UniversityWuhan 430200People’s Republic of China College of Chemistry and Molecular Sciences Wuhan UniversityWuhan 430072People’s Republic of China

Anion-exchange membrane water electrolyzers(AEMWEs)for green hydrogen production have received intensive attention due to their feasibility of using earth-abundant NiFe-based *** introducing a third metal into NiFe-based catalysts to construct asymmetrical M-NiFe units,the d-orbital and electronic structures can be adjusted,which is an important strategy to achieve sufficient oxygen evolution reaction(OER)performance in ***,the ternary NiFeM(M:La,Mo)catalysts featured with distinct M-NiFe units and varying d-orbitals are reported in this *** and theoretical calculation results reveal that the doping of La leads to optimized hybridization between d orbital in NiFeM and 2p in oxygen,resulting in enhanced adsorption strength of oxygen intermediates,and reduced rate-determining step energy barrier,which is responsible for the enhanced OER *** critically,the obtained NiFeLa catalyst only requires 1.58 V to reach 1 A cm^(−2) in an anion exchange membrane electrolyzer and demonstrates excellent long-term stability of up to 600 h.

关键词： NiFe-based catalysts d-orbital coupling Oxygen evolution reaction Anion exchange membrane electrolyzer

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BAK1-mediated phosphorylation of canonical G protein alpha during flagellin signaling in Arabidopsis

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Journal of Integrative Plant Biology 2020年第5期62卷 690-701页

作者： Jiao xue Ben-Qiang Gong Xinran yao Xiangjuan Huang Jian-feng Li Guangdong Provincial Key Laboratory of Plant Resources State Key Laboratory of BiocontrolMOE Key Laboratory of Gene Function and RegulationSchool of Life SciencesSun Yat-sen UniversityGuangzhou 510275China

Heterotrimeric G proteins consisting of Gα,Gβand Gγare conserved signaling hubs in *** analogs to canonical animal G protein-coupled receptors,plant cells are thought to use RGS1 and a yet unknown mechanism to regulate the activity of Gα.Meanwhile,the exact role of canonical Gαin plant innate immunity remains ***,we report multiple immune deficiencies in the null allele of Arabidopsis Gα(GPA1)in response to bacterial flg22 elicitor,clarifying a positive regulatory role of GPA1 in flg22 *** also detect overall increased phosphorylation of GPA1 but reduced phosphorylation at Thr^19 upon flg22 ***,flg22 could not induce phosphorylation of GPA1 T19 Aand GPA1 T19D,suggesting that the dynamic Thr^19 phosphorylation is required for GPA1 to respond to ***,flg22-induced GPA1 phosphorylation is largely abolished in the absence of BAK1 in vivo,and BAK1 could phosphorylate GPA1 but not GPA1^T19A in vitro at the phosphorylation sites identified in vivo,suggesting BAK1 is likely the kinase for GPA1 phosphorylation in response to ***,the T19A mutation could promote flg22-induced association,rather than dissociation,between GPA1 and *** together,our findings shed new insights into the function and regulation of GPA1 in Arabidopsis defense signaling.

关键词： phosphorylation Arabidopsis immunity

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Burden of mental disorders and risk factors in the Western Pacific region from 1990 to 2021

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World Journal of Psychiatry 2025年第1期15卷 93-105页

作者： Ya-Xin Xu Xiao-Xuan Niu Wen-Chang Jia Jing Wen xue-Lin Cheng Yan Han Ming-Hui Peng Jing Zhou yao Liu Sun-Fang Jiang Xiao-Pan Li Department of Health Management Centre Zhongshan HospitalFudan UniversityShanghai 200030China Department of General Practice Zhongshan HospitalFudan UniversityShanghai 200030China Department of Nutrition Zhongshan HospitalFudan UniversityShanghai 200032China School of Public Health Fudan UniversityShanghai 200032China

BACKGROUND The burden of mental disorders(MD)in the Western Pacific Region(WPR)re-mains a critical public health concern,with substantial variations across demogra-phics and *** To analyze the burden of MD in the WPR from 1990 to 2021,along with associated risk factors,to reveal changing trends and emerging *** We used data from the Global Burden of Disease 2021,analyzing prevalence,incidence,and disability-adjusted life years(DALYs)of MD from 1990 to *** methods included age-standardisation and uncertainty analysis to address variations in population structure and data *** Between 1990 and 2021,the prevalence of MD rose from 174.40 million cases[95%uncertainty interval(UI):160.17-189.84]to 234.90 million cases(95%UI:219.04-252.50),with corresponding DALYs increasing from 22.8 million(95%UI:17.22-28.79)to 32.07 million(95%UI:24.50-40.68).During this period,the burden of MD shifted towards older age *** and anxiety disorders were predominant,with females showing higher DALYs for depressive and anxiety disorders,and males more affected by conduct disorders,attention-deficit hyperactivity disorder,and autism spectrum ***,New Zealand,and Malaysia reported the highest burdens,whereas Vietnam,China,and Brunei Darussalam reported the ***,childhood sexual abuse and bullying,and intimate partner violence emerged as significant risk *** This study highlights the significant burden of MD in the WPR,with variations by age,gender,and *** coronavirus disease 2019 pandemic has exacerbated the situation,emphasizing the need for a coordinated response.

关键词： Mental disorders Western pacific region Global Burden of Disease Risk factors Disability-adjusted life years

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Fiber Nonlinearity Post-Compensation by Optical Phase Conjugation for 40Gb/s CO-OFDM Systems

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Chinese Physics Letters 2011年第6期28卷 164-167页

作者： QIAO yao-Jun LIU xue-Jun JI Yue-feng Key Laboratory of Information Photonics and Optical Communications(Ministry of Education) Beijing University of Posts and TelecommunicationsBeijing 100876

Fiber nonlinearity impairments in a 40-Gb/s coherent optical orthogonal frequency division multiplexing(CO-OFDM)system are post-compensated for by a new method of fiber nonlinearity post-compensation(FNPC).The FNPC located before the CO-OFDM receiver includes an optical phase conjugation(OPC)unit and a subsequent 80-km-high nonlinear fiber(HNLF)as a fiber nonlinearity *** OPC unit is based on a four wave mixing effect in a semiconductor optical *** fiber nonlinearity impairments in the transmission link are post-compensated for after OPC by transmission through the HNLF with a large nonlinearity *** results show that the nonlinear threshold(NLT)(for Q>10 dB)can be increased by about 2.5 dB and the maximum Q factor is increased by about 1.2 dB for the single−channel 40-Gb/s CO-OFDM system with periodic dispersion *** the 50-GHz channel spacing wavelength-division-multiplexing system,the NLT increases by 1.1 dB,equating to a 0.7 dB improvement for the maximum Q factor.

关键词： fiber amplifier nonlinearity

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