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Defect Engineering and Carbon Supporting to Achieve Ni‑Doped CoP_(3) with High Catalytic Activities for Overall Water Splitting

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Nano-Micro Letters 2024年第11期16卷 569-584页

作者： Daowei Zha Ruoxing Wang Shijun Tian Zhong‑Jie Jiang Zejun xu Chu qin Xiaoning Tian Zhongqing Jiang Department of Physics Zhejiang Sci-Tech UniversityHangzhou 310018People’s Republic of China Department of Materials and Chemical Engineering Ningbo University of TechnologyNingbo 315211People’s Republic of China Guangzhou Key Laboratory for Surface Chemistry of Energy Materials Guangdong Engineering and Technology Research Center for Surface Chemistry of Energy MaterialsCollege of Environment and EnergySouth China University of TechnologyGuangzhou 510006People’s Republic of China

This work reports the use of defect engineering and carbon supporting to achieve metal-doped phosphides with high activities and stabilities for the hydrogen evolution reaction(HER)and the oxygen evolution reaction(OER)in alkaline ***,the nitrogen-doped carbon nanofiber-supported Ni-doped CoP_(3) with rich P defects(Pv·)on the carbon cloth(p-NiCoP/NCFs@CC)is synthesized through a plasma-assisted phosphorization *** p-NiCoP/NCFs@CC is an efficient and stable catalyst for the HER and the *** only needs overpotentials of 107 and 306 mV to drive 100 mA cm^(-2) for the HER and the OER,*** catalytic activities are higher than those of other catalysts reported *** high activities of the p-NiCoP/NCFs@CC mainly arise from its peculiar structural *** density functional theory calculation indicates that the Pv·richness,the Ni doping,and the carbon supporting can optimize the adsorption of the H atoms at the catalyst surface and promote the strong electronic couplings between the carbon nanofiber-supported p-NiCoP with the surface oxide layer formed during the OER *** gives the p-NiCoP/NCFs@CC with the high activities for the HER and the *** used in alkaline water electrolyzers,the p-NiCoP/NCFs@CC shows the superior activity and excellent stability for overall water splitting.

关键词： Plasma Electrocatalysis Hydrogen evolution reaction Oxygen evolution reaction Water splitting

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Effects of Co and Nb on the Crack of Additive Manufacturing Nickel-Based Superalloys

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Acta Metallurgica Sinica(English Letters) 2024年第9期37卷 1601-1610页

作者： Kejie Tan Jinli Xie Hailong qin Bin xu Guichen Hou Jinguo Li Zhongnan Bi Ji Zhang Beijing Key Laboratory of Advanced High Temperature Materials Central Iron&Steel Research InstituteBeijing100081China Beijing GAONA Materials&Technology Co. LTDBeijing100081China Superalloys Division Institute of Metal ResearchChinese Academy of SciencesShenyang110016China

Increasing the print quality is the critical requirement for the additive manufactured complex part of aero-engines of nickel-based superalloys.A study of the effects of Co and Nb on the crack is performed focusing on the selective laser melting(SLM)nickel-based *** this paper,the solvus temperature of γ',crack characteristics,microstructure,thermal expansion,and mechanical properties of SLM nickel-based superalloy are investigated by varying the content of Co and *** alloy with 15Co/0Nb shows the highest comprehensive *** increases the crack risk and thermal deformation,and then Co accelerates the stress ***,Co is an extremely important alloying element for improving the quality of SLM nickel-based ***,the crack growth kinetics and the strain difference are discussed to reveal the SLM crack regular that is affected by time or *** analysis work on the effect of alloying elements can obtain an effective foundational theory to guide the composition optimization of SLM nickel-based superalloys.

关键词： Nickel-based superalloys Selective laser melting Element effect Crack

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Automatically identifying imperfections and attacks in practical quantum key distribution systems via machine learning

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Science China(Information Sciences) 2024年第10期67卷 359-372页

作者： Jiaxin xu Xiao MA Jingyang LIU Chunhui ZHANG Hongwei LI Xingyu ZHOU qin WANG Institute of Quantum Information and Technology Nanjing University of Posts and Telecommunications Telecommunication and Networks National Engineering Research CenterNanjing University of Posts and Telecommunications Henan Key Laboratory of Quantum Information and Cryptography Strategic Support Force Information Engineering University

The realistic security of quantum key distribution(QKD) systems is currently a hot research topic in the field of quantum communications. There are always defects in practical devices, and eavesdroppers can make use of the security risk points of various devices to obtain key information. To date, current types of security analysis tend to analyze each security risk point individually, thereby posing great challenges for the overall security evaluation of QKD systems. In this paper, for the first time, we employ machine learning algorithms to identify the defects of different devices and certain attacks in real time, with an accuracy of 98%. It provides a novel solution for the practical security evaluation of QKD systems, thereby addressing the bottleneck problem of multiple risk points being difficult to address simultaneously in QKD systems,thus paving the way for the future large-scale application of quantum communication networks.

关键词： quantum key distribution device imperfections eavasdropping attacks real-time detection machine learning algorithms

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Transepithelial transport of nanoparticles in oral drug delivery:From the perspective of surface and holistic property modulation

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Acta Pharmaceutica Sinica B 2024年第9期14卷 3876-3900页

作者： Yaxian Zheng Shiqin Luo Min xu qin He Jiang Xie Jiawei Wu Yuan Huang Department of Pharmacy the Third People’s Hospital of Chengduthe Affiliated Hospital of Southwest Jiaotong UniversityCollege of MedicineSouthwest Jiaotong UniversityChengdu 610031China Department of Pharmacy Personalized Drug Therapy Key Laboratory of Sichuan ProvinceSichuan Academy of Medical Sciences&Sichuan Provincial People’s HospitalSchool of MedicineUniversity of Electronic Science and Technology of ChinaChengdu 610072China Key Laboratory of Drug-Targeting and Drug Delivery System of the Education Ministry and Sichuan Province Sichuan Engineering Laboratory for Plant-Sourced Drug and Sichuan Research Center for Drug Precision Industrial TechnologyWest China School of PharmacySichuan UniversityChengdu 610041China

Despite the promising prospects of nanoparticles in oral drug delivery,the process of oral administration involves a complex transportation pathway that includes cellular uptake,intracellular trafficking,and exocytosis by intestinal epithelial cells,which are necessary steps for nanoparticles to enter the bloodstream and exert therapeutic *** researchers have identified several crucial factors that regulate the interaction between nanoparticles and intestinal epithelial cells,including surface properties such as ligand modification,surface charge,hydrophilicity/hydrophobicity,intestinal protein corona formation,as well as holistic properties like particle size,shape,and *** these properties is essential for enhancing transepithelial transport efficiency and designing effective oral drug delivery ***,this review provides a comprehensive overview of the surface and holistic properties that influence the transepithelial transport of nanoparticles,elucidating the underlying principles governing their impact on transepithelial *** review also outlines the chosen of parameters to be considered for the subsequent design of oral drug delivery systems.

关键词： Oral delivery Nanoparticles Intestinal epithelial cells Surface property Holistic property Transepithelial transport

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β-Carboline alkaloids from the roots of Peganum harmala L.

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Chinese Journal of Natural Medicines 2024年第2期22卷 171-177页

作者： LI Shengge ZHANG qin WANG Yuetong LIN Bin LI Dahong HUA Huiming HU xu Henan Key Laboratory of Zhang Zhongjing Formulate and Herbs for Immunoregulation Zhang Zhongjing Traditional School of Chinese MedicineNanyang Institute of TechnologyNanyang 473004China Key Laboratory of Structure-Based Drug Design&Discovery Ministry of EducationShenyang Pharmaceutical UniversityShenyang 110016China Wuya College of Innovation Shenyang Pharmaceutical UniversityShenyang 110016China School of Pharmaceutical Engineering Shenyang Pharmaceutical UniversityShenyang 110016China

This study reports the isolation of four newβ-carboline alkaloids(1−4)and six previously identified alkaloids(5−10)from the roots of Peganum harmala *** these compounds,1 and 2 were characterized as rareβ-carboline-quinazoline dimers exhibiting axial *** 3 possessed a unique 6/5/6/7 tetracyclic ring system with an azepine ring,and compound 4 was a novel annomontineβ-*** structures of these compounds were elucidated by spectroscopic data and quantum mechanical *** biosynthetic pathways of 1−3 were ***,the cytotoxicity of some isolates against four cancer cell lines(HL-60,A549,MDA-MB-231,and DU145)was ***,compound 4 exhibited significant cytotoxicity against HL-60,A549,and DU145 cells with IC_(50) values of 12.39,12.80,and 30.65μmol·L^(−1),***,compound 2 demonstrated selective cytotoxicity against HL-60 cells with an IC_(50) value of 17.32μmol·L^(−1).

关键词： β-Carboline alkaloids Peganum harmala Structure elucidation Cytotoxic activity

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Systematic review and network meta-analysis of different nonsteroidal anti-inflammatory drugs for juvenile idiopathic arthritis

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World Journal of Clinical Cases 2024年第12期12卷 2056-2064页

作者： Tao Zeng Jian-Zhong Ye Hui qin Qian-Qian xu College of Medicine Jingchu University of Technology JingmenJingmen 448000Hubei ProvinceChina

BACKGROUND Various non-steroidal anti-inflammatory drugs(NSAIDs)have been used for juvenile idiopathic arthritis(JIA).However,the optimal method for JIA has not yet been *** To perform a systematic review and network meta-analysis to determine the optimal *** We searched for randomized controlled trials(RCTs)from PubMed,EMBASE,Google Scholar,CNKI,and Wanfang without restriction for publication date or language at August,*** RCTs that comparing the effectiveness of NSAIDs with each other or placebo for JIA were included in this network *** surface under the cumulative ranking curve(SUCRA)analysis was used to rank the treatments.P value less than 0.05 was identified as statistically *** We included 8 RCTs(1127 patients)comparing 8 different instructions including meloxicam(0.125 qd and 0.250 qd),Celecoxib(3 mg/kg bid and 6 mg/kg bid),piroxicam,Naproxen(5.0 mg/kg/d,7.5 mg/kg/d and 12.5 mg/kg/d),inuprofen(30-40 mg/kg/d),Aspirin(60-80 mg/kg/d,75 mg/kg/d,and 55 mg/kg/d),Tolmetin(15 mg/kg/d),Rofecoxib,and *** were no significant differences between any two NSAIDs regarding ACR Pedi 30 *** SUCRA shows that celecoxib(6 mg/kg bid)ranked first(SUCRA,88.9%),rofecoxib ranked second(SUCRA,68.1%),Celecoxib(3 mg/kg bid)ranked third(SUCRA,51.0%).There were no significant differences between any two NSAIDs regarding adverse *** SUCRA shows that placebo ranked first(SUCRA,88.2%),piroxicam ranked second(SUCRA,60.5%),rofecoxib(0.6 mg/kg qd)ranked third(SUCRA,56.1%),meloxicam(0.125 mg/kg qd)ranked fourth(SUCRA,56.1%),and rofecoxib(0.3 mg/kg qd)ranked fifth(SUCRA,56.1%).CONCLUSION In summary,celecoxib(6 mg/kg bid)was found to be the most effective NSAID for treating ***,piroxicam,and meloxicam may be safer options,but further research is needed to confirm these findings in larger trials with higher quality studies.

关键词： Non-steroidal anti-inflammatory drugs Juvenile idiopathic arthritis Network meta-analysis Systematic review

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Regulating zinc ion transport behavior and solvated structure towards stable aqueous Zn metal batteries

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Journal of Energy Chemistry 2024年第6期93卷 609-626,I0015页

作者： Qiang Ma Aoen Ma Shanguang Lv Bowen qin Yali xu Xianxiang Zeng Wei Ling Yuan Liu Xiongwei Wu College of Materials Engineering Henan International Joint Laboratory of Rare Earth Composite MaterialsHenan University of EngineeringZhengzhou 451191HenanChina Nanozyme Medical Center School of Basic Medical SciencesZhengzhou UniversityZhengzhou 450001HenanChina School of Chemistry and Materials Science Hunan Agricultural UniversityChangsha 410125HunanChina College of Electrical and Information Engineering Hunan UniversityChangsha 410082HunanChina Hunan Province Yin Feng New Energy Co.Ltd. Changsha 410019HunanChina

Aqueous Zn metal batteries(AZMBs)with intrinsic safety,high energy density and low cost have been regarded as promising electrochemical energy storage ***,the parasitic reaction on metallic Zn anode and the incompatibility between electrode and electrolytes lead to the deterioration of electrochemical performance of AZMBs during the *** critical point to achieve the stable cycling of AZMBs is to properly regulate the zinc ion solvated structure and transfer behavior between metallic Zn anode and *** recent years,numerous achievements have been made to resolve the formation of Zn dendrite and interface incompatible issues faced by AZMBs via optimizing the sheath structure and transport capability of zinc ions at electrode-electrolyte *** this review,the challenges for metallic Zn anode and electrode-electrolyte interface in AZMBs including dendrite formation and interface characteristics are *** the influences of different strategies involving designing advanced electrode structu re,artificial solid electrolyte interphase(SEI)on Zn anode and electrolyte engineering to regulate zinc ion solvated sheath structure and transport behavior are summarized and ***,the perspectives for the future development of design strategies for dendrite-free Zn metal anode and long lifespan AZMBs are also given.

关键词： aqueous Zn metal batteries Zn metal anode Transport behavior Solvated structure Dendrite-free

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Reversibly Tuning Electrochemiluminescence with Stimulated Emission Route for Single-Cell Imaging

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Research 2024年第3期2023卷 205-215页

作者： Cheng Ma Xiaodan Gou Zejing Xing Min-xuan Wang Wenlei Zhu qin xu Dechen Jiang Jun-Jie Zhu School of Chemistry and Chemical Engineering Yangzhou University.Yangzhou 225002P.R.China State Key Laboratory of Analytical Chemistry for Life Science State Key Laboratory of Pollution Control and Resource ReuseSchool of Chemistry and Chemical EngineeringSchool of the EnvironmentNanjing UniversityNanjing 210023P.R.China.

Electrochemiluminescence (ECL) has established itself as an excellent transduction technique in biosensing and light-emitting device, while conventional ECL mechanism depending on spontaneous emission of luminophores lacks reversibility and tunable emission characters, limiting the universality of ECL technique in the fields of fundamental research and clinical applications. Here, we report the first observation of stimulated emission route in ECL and thus establish a reversible tuning ECL microscopy for single-cell imaging. This microscopy uses a focused red-shifted beam to transfer spontaneous ECL into stimulated ECL, which enables selective and reversible tuning of ECL emission from homogeneous solution, single particles, and single cells. After excluding other possible competitive routes, the stimulated ECL emission route is confirmed by a dual-objective system in which the suppressed spontaneous ECL is accompanied by the enhanced stimulated ECL. By incorporating a commercial donut-shaped beam, the sharpness of single-cell matrix adhesion is improved 2 to 3 times compared with the counterpart in confocal ECL mode. The successful establishment of this stimulated emission ECL will greatly advance the development of light-emitting device and super-resolution ECL microscopy.

关键词： tuning beam limiting

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MicroR-9c-5p and novel-mir50 co-target Akt to regulate Lasioderma serricorne reproduction

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Insect Science 2024年第1期31卷 106-118页

作者： Yi Yan Dong-Dong qin Hong Yang Kang-Kang xu Can Li Wen-Jia Yang Provincial Key Laboratory for Agricultural Pest Management of Mountainous Region Institute of EntomologyGuizhou UniversityGuiyangChina Guizhou Provincial Key Laboratory for Rare Animal and Economic Insect of the Mountainous Region College of Biology and Environmental EngineeringGuiyang UniversityGuiyangChina

High fecundity is a common characteristic of insect pests which increases the difficulty of population ***/threonine kinase Akt is an indispensable component of the insulin signaling *** of LsAkt severely hinders reproduction in Lasioderma serricorne,a stored product insect ***,the post-transcriptional pathway of LsAkt in *** remains *** study identified 2 binding sites of miR-9c-5p and novel-mir50 in the coding sequences of *** expression profiles of 2 microRNAs(miRNAs)and LsAkt displayed an opposite pattern during the adult *** reporter assay showed that novel-mir50 and miR-9c-5p could downregulate the expression of *** of miR-9c-5p and novel-mir50 by injection of mimics inhibited the expression of LsAkt and reduced oviposition,decreased egg hatchability,and blocked ovarian *** also decreased the expression of genes involved in ovarian development(LsVg and LsVgR)and the nutritional signaling pathway(LsTOR,LsS6K,and Ls4EBP),and reduced the phosphorylation of ***,injection of miR-9c-5p and novel-mir50 inhibitors induced the expressions of LsAkt,LsVg,LsVgR,LsTOR,LsS6K,and Ls4EBP,enhanced Akt phosphorylation level,and accelerated ovarian *** of bovine insulin downregulated the expression of miR-9c-5p and novel-mir50 and upregulated the LsAkt *** also rescued the reproductive development defects associated with miR-9c-5p/novel-mir50 overexpression,forming a positive regulatory loop of insulin *** results indicate that miR-9c-5p/novel-mir50 regulates the female reproduction of *** by targeting Akt in response to insulin *** data also demonstrate the effects of the insulin/miRNA/Akt regulatory axis in insect reproduction.

关键词： Akt insulin Lasioderma serricorne microRNA reproduction

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Photometric Analysis for Asteroid(81)Terpsichore using Convex Inversion and Phase Function Fitting Methods

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Research in Astronomy and Astrophysics 2024年第6期24卷 201-208页

作者： Ao Wang Xiaobin Wang Xiaoyun xu Longhua qin Quangui Gao Huaizhen Li Yong Xiao Hairu Zhao Department of Physics Yuxi Normal UniversityYuxi 653100China Yunnan Observatories Chinese Academy of SciencesKunming 650216China Key Laboratory for the Structure and Evolution of Celestial Objects Chinese Academy of SciencesKunming 650216China University of Chinese Academy of Sciences Beijing 100049China

The shapes and rotation states(periods and pole orientations)of main-belt asteroids are important for understanding their formation and *** order to obtain sufficient photometric data covering different apparitions for asteroid(81)Terpsichore,ground-based photometric observations in 2020 and 2021 were carried *** combining published and newly obtained photometric data,we calculated the shape and spin parameters for(81)Terpsichore using the convex inversion *** this method,we have derived a best fitted pole orientation—(22.2±_(3.1)^(3.3°),17.5±_(5.5)^(10.8°))with a spin period of 10.94±_(0.01)^(0.01)*** on the derived convex shape of(81)Terpsichore,we have fitted the H,G+1,G_(2)phase function using the calibrated TESS data and Gaia data after accounting for the lightcurve amplitude *** a result,we have derived its absolute magnitude H=8.68±_(0.19)^(0.22)mag with corresponding phase function parameters G_(1)=0.82±_(0.10)^(0.09)and G_(2)=0.02±_(0.02)^(0.03).

关键词： asteroids:general minor planets asteroids:individual(Terpsichore) techniques:photometric

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