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Journal of Environmental Sciences 2024年第1期135卷 433-448页

作者： Xiang Meng Pierre désesquelles Lejin xu department of Nuclear Engineering and Technology School of Energy and Power EngineeringHuazhong University of Science&TechnologyWuhan 430074China CNRS Laboratoire de Physique des Gaz et des PlasmasUniversitéParis-SaclayOrsay 91405France State Key Laboratory of Coal Combustion School of Energy and Power EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The treatment and disposal of radioactive waste are presently facing great *** ion exchange resins have become a focus of attention due to their high production and serious environmental *** this paper,a simplified model of cationic exchange resin is proposed,and the degradation processes of cationic resin monomer initiated by hydroxyl radicals(·OH)are clarified by combining statistical molecular fragmentation(SMF)model and density functional theory(dFT)*** prediction of active sites indicates that the S-O bonds and the C-S bond of the sulfonic group are more likely to react during the *** meta-position of the sulfonic group on the benzene ring is the most active site,and the benzene ring without the sulfonic group has a certain *** C11-C14 and C17-C20 bonds,on the carbon skeleton,are the most easily *** is also found that dihydroxy ad.ition and elimination reactions play a major role in the process of desulfonation,carbon skeleton cleavage and benzene ring *** decomposition mechanisms found through the combination of physical models and chemical calculations,provide theoretical guidance for the treatment of complex polycyclic aromatic hydrocarbons.

关键词： Cationic exchange resin Statistical molecular fragmentation model density functional theory Hydroxyl radical decomposition mechanism

From 0d to 3d:Hierarchical structured high-performance free-standing silicon anodes based on binder-induced topological network architecture

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Journal of Energy Chemistry 2024年第6期93卷 16-23,I0002页

作者： Yihong Tong Ruicheng Cao Guanghui xu Yifeng Xia Hongyuan xu Hong Jin Hui xu Xi’an Jiaotong University Suzhou Academy Suzhou 215123JiangsuChina Nano Science and Technology institute University of Science and Technology of ChinaSuzhou 215123JiangsuChina

Free-standing silicon anodes with high proportion of active materials have aroused great attention;however,the mechanical stability and electrochemical performance are severely ***,to resolve the appeal issues,a free-standing anode with a"corrugated paper"shape on micro-scale and a topological crosslinking network on the submicron and nano-scale is ***,an integrated three-dimensional electrode structure is constructed based on robust carbon nanotubes network with firmly anchored SiNPs via forming interlocking *** which,the hierarchical interlocking structure is achieved by directional induction of the binder,which ensures well integration during cycling so that significantly enhances mechanical stability as well as electronic and.ionic conductivity of *** from it,this anode exhibits outsta nding performance under harsh service conditions including high Si loading,ultrahigh areal capacity(33.2 mA h cm^(-2)),and high/low temperatures(-15-60℃),which significantly extends its practical ***,the optimization mechanism of this electrode is explored to verify the crack-healing and structure-integration maintaining along cycling via a unique self-stabilization ***,from both the fundamental and engineering views,this strategy offers a promising path to produce high-performance free-standing electrodes for flexible device applications especially facing volume effect challenges.

关键词： Topological network Self-stabilization Flexibility Free-standing Silicon anode

ARPES investigation of the electronic structure and.its evolution in magnetic topological insulator MnBi2+2nTe4+3n family

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National Science Review 2024年第2期11卷 81-93页

作者： Runzhe xu Lixuan xu Zhongkai Liu Lexian Yang Yulin Chen State Key Laboratory of Low dimensional Quantum Physics Department of PhysicsTsinghua University School of Physical Science and Technology Shanghai Tech University and CAS-Shanghai Science Research Center Shanghai Tech Laboratory for Topological Physics Frontier Science Center for Quantum information Collaborative innovation Center of Quantum Matter department of Physics Clarendon LaboratoryUniversity of Oxford

in the past 5 years,there has been significant research interest in the intrinsic magnetic topological insulator family compounds MnBi2+2nTe4+3n（where n=0,1,2…）.in particular,exfoliated thin films of MnBi2Te4have led to numerous experimental breakthroughs,such as the quantum anomalous Hall effect,axion insulator phase and high-Chern number quantum Hall effect without Landau ***,despite extensive efforts,the energy gap of the topological surface states due to exchange magnetic coupling,which is a key feature of the characteristic band structure of the system,remains experimentally *** electronic structure measured by using angle-resolved photoemission （ARPES） shows significant deviation from ab initio prediction and scanning tunneling spectroscopy measurements,making it challenging to understand the transport results based on the electronic *** paper reviews the measurements of the band structure of MnBi2+2nTe4+3nmagnetic topological insulators using ARPES,focusing on the evolution of their electronic structures with temperature,surface and bulk doping and film *** aim of the review is to construct a unified picture of the electronic structure of MnBi2+2nTe4+3ncompounds and explore possible control of their topological properties.

关键词： magnetic topological insulator MnBi2Te4 electronic structure angle-resolved photoemission spectroscopy

deep learning based water leakage detection for shield tunnel lining

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Frontiers of Structural and Civil Engineering 2024年第6期18卷 887-898页

作者： Shichang LiU xu xu Gwanggil JEON Junxin CHEN Ben-Guo HE College of Computer Science Sichuan UniversityChengdu 610065China School of Computer Science and Engineering Northeastern UniversityShenyang 110004China department of Embedded Systems Engineering Incheon National UniversityIncheon 22012Korea School of Software Dalian University of TechnologyDalian 116621China Key Laboratory of Ministry of Education on Safe Mining of deep Metal Mines Northeastern UniversityShenyang 110819China

Shield tunnel lining is prone to water leakage,which may further bring about corrosion and structural damage to the walls,potentially leading to dangerous *** avoid tedious and.inefficient manual inspection,many projects use artificial intelligence(Al)to detect cracks and water leakage.A novel method for water leakage inspection in shield tunnel lining that utilizes deep learning is introduced.in this *** proposal includes a ConvNeXt-S backbone,deconvolutional-feature pyramid network(d-FPN),spatial attention module(SPAM).and a detection *** can extract representative features of leaking areas to aid.inspection *** further improve the model's robustness,we innovatively use an inversed low-light enhancement method to convert normally illuminated.images to low light ones and.introduce them into the training *** experiments are performed,achieving the average precision(AP)score of 56.8%,which outperforms previous work by a margin of 5.7%.Visualization illustrations also support our method's practical effectiveness.

关键词： water leakage detection deep learning deconvolutional-feature pyramid spatial attention

dCVAE-adv:A Universal Adversarial Example Generation Method for White and Black Box Attacks

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Tsinghua Science and Technology 2024年第2期29卷 430-446页

作者： Lei xu Junhai Zhai College of Mathematics and.information Science Hebei UniversityBaoding 071002China

deep neural network(dNN)has strong representation learning ability,but it is vulnerable and easy to be fooled by adversarial *** order to handle the vulnerability of dNN,many methods have been *** general idea of existing methods is to reduce the chance of dNN models being fooled by observing some designed adversarial examples,which are generated by ad.ing perturbations to the original *** this paper,we propose a novel adversarial example generation method,called *** from the existing methods,dCVAE-adv constructs adversarial examples by mixing both explicit and.implicit perturbations without using original ***,the proposed method can be applied to both white box and black box *** ad.ition,in the inference stage,the adversarial examples can be generated without loading the original images into memory,which greatly reduces the memory *** compared dCVAE-adv with three most advanced adversarial attack algorithms:FGSM,AdvGAN,and AdvGAN++.The experimental results demonstrate that dCVAE-adv is superior to these state-of-the-art methods in terms of attack success rate and transfer ability for targeted *** code is available at https://***/xzforeverlove/dCVAE-adv.

关键词： deep neural network adversarial examples white box attack black box attack robustness

Highly elastic 2d covalent organic framework films of interwoven single crystals

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National Science Review 2024年第7期11卷 71-72页

作者： Tongwen xu Key Laboratory of Precision and.intelligent Chemistry Department of Applied ChemistrySchool of Chemistry and Materials ScienceUniversity of Science and Technology of China

Two-dimensional(2d) materials feature angstrom-scale pores and tunable pore chemistry, demonstrating great potential for applications including flexible electronics and *** ion/molecule transport in the sub-nanometer-sized pore confinement often reveals phenomena not seen in bulk materials [1]. Yet, the practical application of 2d materials is hindered by their poor mechanical properties.

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Biohythane production from two-stage anaerobic digestion of food waste:A review

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Journal of Environmental Sciences 2024年第5期139卷 334-349页

作者： Xiaona An Ying xu Xiaohu d.i State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai institute of Pollution Control and Ecological Security Shanghai 200092China

The biotransformation of food waste(FW)to bioenergy has attracted considerable research attention as a means to address the energy crisis and waste disposal *** this end,a promising technique is two-stage anaerobic digestion(TSAd),in which the FW is transformed to biohythane,a gaseous mixture of biomethane and *** review summarises the main characteristics of FW and describes the basic principle of ***,the factors influencing the TSAd performance are identified,and an overview of the research status;economic aspects;and strategies such as pre-treatment,co-digestion,and regulation of microbial consortia to increase the biohythane yield from TSAd.is ***,the challenges and future considerations associated with the treatment of FW by TSAd are *** paper can provide valuable reference for the improvement and widespread.implementation of TSAd-based FW treatment.

关键词： Two-stage anaerobic digestion(TSAd) Food waste(FW) Methane production Hydrogen production

Comparison of Microwave imaging Algorithms for Short-Range Scenarios

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Journal of Beijing institute of Technology 2024年第3期33卷 227-236页

作者： Zhengyue dong Ning xu Kuiwen xu Engineering Research Center of Smart Microsensors and Microsystems Ministry of EducationHangzhou Dianzi UniversityHangzhou 310018China

Three dimensional(3-d.imaging algorithms with irregular planar multiple-input-multiple-output(MiMO)arrays are discussed and compared with each *** on the same MiMO array,a modified back projection algorithm(MBPA)is accordingly proposed and four imaging algorithms are used for comparison,back-projection method(BP),back-projection one in time domain(BP-Td),modified back-projection one and fast Fourier transform(FFT)-based MiMO range migration algorithm(FFT-based MiMO RMA).All of the algorithms have been implemented.in practical application scenarios by use of the proposed.imaging *** to the practical applications,MiMO array-based.imaging system with wide-band.idth properties provides an efficient tool to detect objects hidden behind a *** MiMO imaging radar system,composed of a vector network analyzer(VNA),a set of switches,and an array of Vivaldi antennas,have been designed,fabricated,and ***,these algorithms have been applied to measured data collected.in different scenarios constituted by five metallic spheres in the absence and.in the presence of a wall between the antennas and the targets in simulation and pliers in free space for experimental ***,the focusing properties and time consumption of the above algorithms are compared.

关键词： multiple-input-multiple-output(MiMO) short-range imaging back projection modi-fied back propagation range migration algorithm(RMA) through-wall imaging

Enhanced photocatalytic hydrogen production from Co-MOF/CN by nitrogen and sulfur co-doped coal-based carbon quantum dots

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Journal of Rare Earths 2024年第5期42卷 838-850,I0002页

作者： Shiyong xu Mei Li Yijun Wang Caiyun Gao Rongsheng xu Zhiliang jin School of Chemistry and Chemical Engineering North Minzu UniversityYinchuan750021China Ningxia Key Laboratory of Solar Chemical Conversion Technology.North Minzu University.Yinchuan 750021China State Key Laboratory of National Ethnic Affairs Commission Chemical Technology.North Minzu University Yinchuan750021China

A novel composite photocatalyst for photocatalytic decomposition of water for hydrogen evolution was successfully synthesized by in-situ growth of nitrogen and sulfur co-doped coal-based carbon quantum dots(NSCQds)nanoparticles on the surface of sheet cobalt-based metal-organic framework(Co-MOF)and graphitic carbon nitride(g-C_(3)N_(4),CN).The structure and properties of the obtained catalysts were systematically *** effectively broaden the absorption of Co-MOF and CN in the visible *** new composite photocatalyst has high hydrogen production activity and the hydrogen production rate reaches 6254μmol/(g·h)at pH=*** the same time,NSCQds synergy Co-MOF/CN composites have good *** four cycles of hydrogen production,the performance remains relatively *** tran sient photocurrent response and Nyquist plot experimental results further demonstrate the improvement of carrier separation efficiency in composite *** semiconductor type(n-type semico nductor)of the single-phase catalyst was determined by the Mott-Schottky test,and the band structure was *** conductive and valence bands of CN are-0.99 and 1.72 eV,respectively,and the conduction and valence bands of Co-MOF are-1.85 and 1.33 eV,*** e mechanism of the photocatalytic reaction can be inferred,that is,Z-type heterojunction is formed between CN an d Co-MOF,and NSCQds was used as cocatalyst.

关键词： Nitrogen and sulfur co-doped Coal-based carbon quantum dots Co-MOF CN Photocatalytic hydrogen evolution Rare earths

Periodic Variation Studies of the Two Short Period W UMa-type Eclipsing Binaries: LX Lyn and V0853 Aur

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Research in Astronomy and Astrophysics 2024年第1期24卷 273-284页

作者： xu Zhang Bin Zhang School of Physics and Electronic Science Guizhou Normal UniversityGuiyang 550001China Guizhou Provincial Key Laboratory of Radio Astronomy and data Processing Guizhou Normal UniversityGuiyang 550025China

in this paper,new light curves(LCs) of contact eclipsing binary(CEB) systems LX Lyn and V0853 Aur are presented and analyzed by using the 2015 version of the Wilson-devinney(W-d) *** order to explain their asymmetric LCs,cool starspots on the components were *** is suggested that their fill-out degrees are f=12.0%(LX Lyn) and f=26.3%(V0853 Aur).At the same time,we found that LX Lyn is a W-type eclipsing binary(EB) with an orbital inclination of i=84°.88 and a mass ratio of q=2.31.V0853 Aur is also a W-type CEB with a mass ratio of q=2.77 and an orbital inclination of i= 79°.*** on all available times of light minimum,their orbital period changes are studied by using the O-C *** O-C diagram of LX Lyn reveals a cyclic oscillation with a period of about 14.84 yr and an amplitude of 0.0019 days,which can be explained by the light-travel time effect(LTTE) due to the presence of a third body with a minimum mass of0.06M_⊙.For V0853 Aur,it is discovered that the O-C diagram of the system also shows a cyclic oscillation with a period of 9.64 yr and an amplitude of 0.03365 *** cyclic oscillation of V0853 Aur can be attributed to the LTTE by means of a third body with a mass no less than 3.77M_⊙.The third body may play an important role in the formation and evolution of these systems.

关键词： stars:activity (stars:)binaries(including multiple):close (stars:)binaries:eclipsing (stars:)brown dwarfs stars:evolution stars:formation