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Greenhouse gas emissions from Daihai Lake,China:Should eutrophication and salinity promote carbon emission dynamics?

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Journal of Environmental Sciences 2024年第1期135卷 407-423页

作者： Xiangwei li Ruihong Yu Jun Wang Heyang Sun Xinyu liu Xiaohui Ren Shuai Zhuang Zhiwei Guo xixi Lu Inner Mongolia Key Laboratory of River and Lake Ecology School of Ecology and EnvironmentInner Mongolia UniversityHohhot 010070China Key Laboratory of Mongolian Plateau Ecology and Resource Utilization Ministry of EducationHohhot 010070China Autonomous Region Collaborative Innovation Center for Integrated Management of Water Resources and Water Environment in the Inner Mongolia Reaches of the Yellow River Hohhot 010018China Department of Geography National University of Singapore117570Singapore

Greenhouse gases(GHGs)emitted or absorbed by lakes are an important component of the global carbon cycle.However,few studies have focused on the GHG dynamics of eutrophic saline lakes,thus preventing a comprehensive understanding of the carbon cycle.Here,we conducted four sampling analyses using a floating chamber in Daihai Lake,a eutrophication saline lake in Inner Mongolia Autonomous Region,China,to explore its carbon dioxide(CO_(2))and methane(CH_(4))emissions.The mean CO_(2)emission flux(FCO_(2))and CH_(4)emission flux(FCH_(4))were 17.54±14.54 mmol/m^(2)/day and 0.50±0.50 mmol/m^(2)/day,respectively.The results indicated that Daihai Lake was a source of CO_(2)and CH_(4),and GHG emissions exhibited temporal variability.The mean CO_(2)partial pressure(p CO_(2))and CH_(4)partial pressure(p CH_(4))were 561.35±109.59μatm and 17.02±13.45μatm,which were supersaturated relative to the atmosphere.The regression and correlation analysis showed that the main influencing factors of p CO_(2)were wind speed,dissolved oxygen(DO),total nitrogen(TN)and Chlorophyll a(Chl.a),whereas the main influencing factors of p CH_(4)were water temperature(WT),Chl.a,nitrate nitrogen(NO_(3)^(-)-N),TN,dissolved organic carbon(DOC)and water depth.Salinity regulated carbon mineralization and organic matter decomposition,and it was an important influencing factor of p CO_(2)and p CH_(4).Additionally,the trophic level index(Tli)significantly increased p CH_(4).Our study elucidated that salinity and eutrophication play an important role in the dynamic changes of GHG emissions.However,research on eutrophic saline lakes needs to be strengthened.

关键词： Eutrophication Salinity Greenhouse gas emissions Inland lake Inner Mongolia Autonomous Region

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Preparation and Swelling Kinetic Analysis of Poly (HPMC-co-AA-co-AM) Super Absorbent Resin

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Journal of Wuhan University of Technology(Materials Science) 2024年第3期39卷 790-799页

作者：马砺 WANG Xin liU xixi WEI Gaoming GUO Ying School of Safety Science and Engineering Xi’an University of Science and TechnologyXi'an 710054China Key Laboratory of Coal Fire Disaster Prevention Xi’an University of Science and TechnologyXi'an 710054China School of Energy Engineering Xi’an Uni-versity of Science and TechnologyXi'an 710054China Yanzhou Coal Mining Co. Ltd.Zoucheng 237500China

Super absorbent resin(SAR)is prepared by aqueous high temperature polymerization using hydroxypropyl methylcellulose(HPMC)as monomer backbone material,acrylic acid(AA)and acrylamide(AM)as the graft copolymer monomer,potassium persulfate(KPS)as the initiator to generate free radicals,and N,N`-methylenebisacrylamide(MBA)as cross-linking agent for cross-linking reaction.Simutaneously,the influence of individual factors on the water absorption is investigated,and these factors are mainly AA,AM,KPS,MBA,HPMC,and reaction temperature.The optimized conditions are obtained by the experiment repeating for several times.The water absorption multiplicity and salt absorption multiplicity under the conditions are 782.4 and 132.5 g/g,respectivity.Furthermore,the effects of different temperatures and salt concentrations on its water absorption,as well as the swelling kinetics of SAR are studied.It is indicated the water-absorbing swelling process is mainly caused by the difference in water osmotic pressure and Na+concentration inside and outside the cross-linked molecular structure of the resin,which is not only consistent with the quasi-secondary kinetic model,but also with the Fick diffusion model.

关键词： super absorbent resin swelling kinetics water absorption graft copolymerization hydroxypropyl methyl cellulose

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Perspective on novel proteins encoded by circular RNAs in glioblastoma

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Cancer Biology & Medicine 2022年第3期19卷 278-283页

作者： xixi li Xinya Gao Nu Zhang Department of Neurosurgery Sun Yat-sen UniversityThe First Affiliated Hospital of Sun Yat-sen UniversityGuangzhou 510080China

Circular RNAs(circRNAs)are generated by the non-canonical back-splicing of pre-mRNA and have been shown to be present in a wide variety of tissues at lower expression levels than their associated linear RNAs1.The advent of high-throughput sequencing technologies has enabled the identification of circRNAs with biological functions in diseases,particularly cancers.Because their stable circular structures resist digestion by RNase R,circRNAs accumulate in the brain with aging in a conservative form wherein neurons seldom undergo mitosis;some of these RNAs have been reported to serve as prognostic biomarkers for central nervous system(CNS)disease2.

关键词： circular diseases conservative

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Spatiotemporal characteristics and driving mechanisms of land use/land cover(LULC)changes in the Jinghe River Basin,China

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Journal of Arid Land 2024年第1期16卷 91-109页

作者： WANG Yinping JIANG Rengui YANG Mingxiang XIE Jiancang ZHAO Yong li Fawen LU xixi State Key Laboratory of Eco-hydraulics in Northwest Arid Region of China Xi'an University of TechnologyXi'an 710048China State Key Laboratory of Simulation and Regulation of Water Cycle in River Basin China Institute of Water Resources and Hydropower ResearchBeijing 100038China State Key Laboratory of Hydraulic Engineering Simulation and Safety Tianjin UniversityTianjin 300072China Department of Geography National University of SingaporeSingapore 117570Singapore

Understanding the trajectories and driving mechanisms behind land use/land cover(LULC)changes is essential for effective watershed planning and management.This study quantified the net change,exchange,total change,and transfer rate of LULC in the Jinghe River Basin(JRB),China using LULC data from 2000 to 2020.Through trajectory analysis,knowledge maps,chord diagrams,and standard deviation ellipse method,we examined the spatiotemporal characteristics of LULC changes.We further established an index system encompassing natural factors(digital elevation model(DEM),slope,aspect,and curvature),socio-economic factors(gross domestic product(GDP)and population),and accessibility factors(distance from railways,distance from highways,distance from water,and distance from residents)to investigate the driving mechanisms of LULC changes using factor detector and interaction detector in the geographical detector(Geodetector).The key findings indicate that from 2000 to 2020,the JRB experienced significant LULC changes,particularly for farmland,forest,and grassland.During the study period,LULC change trajectories were categorized into stable,early-stage,late-stage,repeated,and continuous change types.Besides the stable change type,the late-stage change type predominated the LULC change trajectories,comprising 83.31% of the total change area.The period 2010-2020 witnessed more active LULC changes compared to the period 2000-2010.The LULC changes exhibited a discrete spatial expansion trend during 2000-2020,predominantly extending from southeast to northwest of the JRB.Influential driving factors on LULC changes included slope,GDP,and distance from highways.The interaction detection results imply either bilinear or nonlinear enhancement for any two driving factors impacting the LULC changes from 2000 to 2020.This comprehensive understanding of the spatiotemporal characteristics and driving mechanisms of LULC changes offers valuable insights for the planning and sustainable management of LULC in the JRB.

关键词： land use/land cover(LULC)changes driving mechanisms trajectory analysis geographical detector(Geodetector) Grain for Green Project Jinghe River Basin

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Enhanced activation of peroxymonosulfate by Fe/N co-doped ordered mesoporous carbon with dual active sites for efficient removal of m-cresol

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Chinese Journal of Chemical Engineering 2024年第1期65卷 130-144页

作者： Donghui li Wenzhe Wu Xue Ren xixi Zhao Hongbing Song Meng Xiao Quanhong Zhu Hengjun Gai Tingting Huang College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042China School of Chemical&Environmental Engineering China University of Mining&Technology-BeijingBeijing 100083China

The novel Fe-N co-doped ordered mesoporous carbon with high catalytic activity in m-cresol removal was prepared by urea-assisted impregnation and simple pyrolysis method.During the preparation of the Fe-NC catalyst,the complexation of N elements in urea could anchor Fe,and the formation of C3N4during urea pyrolysis could also prevent migration and aggregation of Fe species,which jointly improve the dispersion and stability of Fe.The FeN4sites and highly dispersed Fe nanoparticles synergistically trigger the dual-site peroxymonosulfate (PMS) activation for highly efficient m-cresol degradation,while the ordered mesoporous structure of the catalyst could improve the mass transfer rate of the catalytic process,which together promote catalytic degradation of m-cresol by PMS activation.Reactive oxygen species (ROS) analytic experiments demonstrate that the system degrades m-cresol by free radical pathway mainly based on SO_(4)^(-)·and·OH,and partially based on·OH as the active components,and a possible PMS activation mechanism by 5Fe-50 for m-cresol degradation was proposed.This study can provide theoretical guidance for the preparation of efficient and stable catalysts for the degradation of organic pollutants by activated PMS.

关键词： Degradation Peroxymonosulfate Fe(II)/Fe(III)/FeN4 Ordered mesopores carbon Catalyst Radical

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Highly robust zinc metal anode directed by organic–inorganic synergistic interfaces for wearable aqueous zinc battery

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SmartMat 2024年第1期5卷 135-146页

作者： xixi Zhang Chuanlin li Guangmeng Qu Chenggang Wang Shunshun Zhao Tongkai Wang Na li Xiaojuan li Xijin Xu School of Physics and Technology University of JinanJinanChina School of Chemistry and Chemical Engineering Shandong UniversityJinanChina State Key Laboratory of Chemical Resource Engineering Beijing Key Laboratory of Electrochemical Process and Technology of MaterialsBeijing University of Chemical TechnologyBeijingChina

Flexible aqueous zinc batteries(FAZBs)with high safety and environmental friendliness are promising smart power sources for smart wearable electronics.However,the bare zinc anode usually suffers from damnable dendrite growth and rampant side reaction on the surface,greatly impeding practical applications in FAZBs.Herein,a composite polymer interface layer is artificially self‐assembled on the surface of the zinc anode by graft‐modified fluorinated monomer(polyacrylic acid‐2‐(Trifluoromethyl)propenoic acid,PAA‐TFPA),on which an organic–inorganic hybrid(PAA‐Zn/ZnF2)solid electrolyte interface(SEI)with excellent ionic conductivity is formed by interacting with Zn2+.Both the pouch cell and fiber zinc anode exhibit excellent plating/stripping reversibility after protecting by this organic–inorganic SEI,which can be stably cycled more than 3000 h in symmetric Zn||Zn cells or 550 h in fiber Zn||Zn cells.Additionally,this interface layer preserves zinc anode with excellent mechanical durability under various mechanical deformation(stably working for another 1200 h after bending 100 h).The corresponding PAA‐Zn/ZnF2@Zn||MnO2 full cell displays an ultra‐long life span(79%capacity retention after 3000 cycles)and mechanical robustness(85%of the initial capacity for another 3000 cycles after bending 100 times).More importantly,the as‐assembled cells can easily power smart wearable devices to monitor the user's health condition.

关键词： hybrid SEI mechanical durability wearable zinc battery zinc anode

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Reversible solid-liquid conversion enabled by self-capture effect for stable non-flow zinc-bromine batteries

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Green Energy & Environment 2024年第6期9卷 1035-1044页

作者： xixi Zhang Xiaoke Wang Guangmeng Qu Tairan Wang Xiliang Zhao Jun Fan Cuiping Han Xijin Xu Chunyi Zhi Hongfei li School of Physics and Technology University of JinanShandong250022China Songshan Lake Materials Laboratory DongguanGuangdong523808China Department of Materials Science and Engineering City University of Hong Kong83 Tat Chee AvenueHong KongChina Faculty of Materials Science and Engineering and Low Dimensional Energy Materials Research Center Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenGuangdong518055China School of System Design and Intelligent Manufacturing Southern University of Science and TechnologyShenzhenGuangdong518055China

Non-flow aqueous zinc-bromine batteries without auxiliary components(e.g.,pumps,pipes,storage tanks)and ion-selective membranes represent a cost-effective and promising technology for large-scale energy storage.Unfortunately,they generally suffer from serious diffusion and shuttle of polybromide(Br^(-),Br^(3-))due to the weak physical adsorption between soluble polybromide and host carbon materials,which results in low energy efficiency and poor cycling stability.Here,we develop a novel self-capture organic bromine material(1,10-bis[3-(trimethylammonio)propyl]-4,4'-bipyridinium bromine,NVBr4)to successfully realize reversible solid complexation of bromide components for stable non-flow zinc-bromine battery applications.The quaternary ammonium groups(NV^(4+)ions)can effectively capture the soluble polybromide species based on strong chemical interaction and realize reversible solid complexation confined within the porous electrodes,which transforms the conventional“liquid-liquid”conversion of soluble bromide components into“liquid-solid”model and effectively suppresses the shuttle effect.Thereby,the developed non-flow zinc-bromide battery provides an outstanding voltage platform at 1.7 V with a notable specific capacity of 325 mAh g^(-1)NVBr4(1 A g^(-1)),excellent rate capability(200 mAh g^(-1)NVBr4 at 20 A g^(-1)),outstanding energy density of 469.6 Wh kg^(-1)and super-stable cycle life(20,000 cycles with 100%Coulombic efficiency),which outperforms most of reported zinc-halogen batteries.Further mechanism analysis and DFT calculations demonstrate that the chemical interaction of quaternary ammonium groups and bromide species is the main reason for suppressing the shuttle effect.The developed strategy can be extended to other halogen batteries to obtain stable charge storage.

关键词： Solid-liquid conversion Self-capture Non-ﬂow zinc-bromine batteries Quaternary ammonium

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Antioxidant peptides from Lateolabrax japonicus to protect against oxidative stress injury in Drosophila melanogaster via biochemical and gut microbiota interaction assays

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Food Science and Human Wellness 2024年

作者： Chen li lichan li Jing Cheng Xu Chen Mohamed A.Farag xixi Cai Shaoyun Wang College of Chemical Engineering College of Biological Science and Engineering Fuzhou University Pharmacognosy Department Faculty of Pharmacy Cairo University

Identification of natural substances with antioxidant properties is ongoing research for addressing issues related to oxidative stress especially attributed to environmental effects. Our previous study demonstrated that Lateolabrax japonicus peptides （LPH）， rich in Glu， Gly， and hydrophobic amino acids， exhibited remarkable antioxidant activity in vitro， with though its action mechanism yet to be revealed. Therefore， to assess the in vivo antioxidative properties of LPH， we employed H2O2to generate oxidative stress in Drosophila melanogaster model. Results indicated that LPH significantly prolonged the lifespan of Drosophila subjected to oxidative stress mostly mediated via LPH's enhancement of the antioxidant defense system and intestinal functions. Antioxidant effects were manifested by a decrease in malondialdehyde （MDA） levels， elevated superoxide dismutase （SOD）， catalase （CAT）， and glutathione peroxidase （GSH-Px） activities， decreased levels of reactive oxygen species （ROS） in intestinal epithelial cells， and the preservation of intestinal length. LPH effectively controlled the excessive proliferation and differentiation of oxidative stress-induced Drosophila intestinal stem cells. At the gene level， LPH upregulated the expression of antioxidant-related Nrf2 genes while concurrently downregulated mTOR expression level. Furthermore， high-throughput 16S rDNA sequencing revealed that the addition of LPH significantly influenced the diversity and abundance of the intestinal microbiota in H2O2-induced Drosophila. These findings provide a deeper understanding of the antioxidative mechanism of LPH， suggesting its potential applications in food industry and to be assessed using other in vivo oxidative stress models.

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Rocking-chair ammonium ion battery with high rate and long-cycle life

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Chinese Chemical Letters 2024年第1期35卷 563-567页

作者： Tongkai Wang Xiaojuan li Shunshun Zhao Hongxia Bu Chuanlin li Na li xixi Zhang Xijin Xu School of Physics and Technology University of JinanJi'nan 250022China State Key Laboratory of Chemical Resource Engineering Beijing Key Laboratory of Electrochemical Process and Technology of MaterialsBeijing University of Chemical TechnologyBeijing 100029China College of Physics and Electronic Engineering Qilu Normal UniversityJi'nan 250200China

Aqueous rechargeable ammonium-ion batteries(AIBs)have drew considerable attention because of their capacity for high rates,low cost,and high safety.However,developing desired electrodes requiring stable structure in the aqueous fast ammoniation/de-ammoniation becomes urgent.Herein,an ammonium ion full battery using Cu_(3)[Fe(CN)_(6)]_(2)(CuHCF)acting to be a cathode and barium vanadate(BVO)acting to be an anode is described.Its excellent electrochemical behavior of Prussian blue analogs and the perfectly matched lattice structure of NH_(4)^(+)is expected.And the open structure of vanadium compounds satisfies the fast ammoniation/de-ammoniation of NH4+is also achieved.As a result of these synergistic effects,the BVO//CuHCF full cell retains 80.5 percent of its capacity following 1000 cycling.These achievements provide new ideas for developing low-cost and long-life AIBs.

关键词： Copper hexacyanoferrate Vanadium-based compounds Aqueous ammonium ion batteries Long-term cyclability Ammonium ion storage mechanism

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“城市更新+文旅”的城市孤岛空间多维拓扑结构与功能重塑研究——以广州市黄埔古村为例

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干旱区资源与环境 2024年第1期38卷 69-74页

作者：唐夕汐夏青田里广东第二师范学院管理学院广州510303 云南大学工商管理与旅游管理学院昆明650500

从列斐伏尔都市社会理论、德勒兹褶子说、阿特金Q分析等理论动力源出发来分析城市孤岛与周边现代化城市排斥与包容的辩证关系,并构建了城市孤岛“C-B”空间4维拓扑结构集合。采用观察法、半结构访谈法、文本分析法等数据获取方法,从历... 详细信息

从列斐伏尔都市社会理论、德勒兹褶子说、阿特金Q分析等理论动力源出发来分析城市孤岛与周边现代化城市排斥与包容的辩证关系,并构建了城市孤岛“C-B”空间4维拓扑结构集合。采用观察法、半结构访谈法、文本分析法等数据获取方法,从历时性拓扑演化的过程中,提炼出黄埔古村“村港一体”的拓扑不变量;从共时性的角度聚焦第四次拓扑结构,探索出“城市更新+文旅”的空间功能重塑模式是黄埔古村为代表的城市孤岛有效实施新时代空间转型发展的具体路径之一。

关键词：城市孤岛空间多维拓扑结构功能重塑城市更新文旅发展

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