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Journal of Energy Chemistry 2024年第9期96卷 79-88页

作者： Xiaoke wang Titi li Xixi Zhang Yaxin wang Hongfei li Hai-Feng li Gang Zhao Cuiping Han Institute of Applied Physics and Materials Engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078China School of Physics and Technology University of JinanJinan 250022ShandongChina Songshan Lake Materials Laboratory Dongguan 523808GuangdongChina Faculty of Materials Science and Energy Engineering Shenzhen University of Advanced TechnologyShenzhen 518055GuangdongChina Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina

Magnesium ion batteries(MIBs)are a potential field for the energy storage of the future but are restricted by insufficient rate capability and rapid capacity ***-sodium hybrid ion batteries(MSHBs)are an effective way to address these ***,we report a new type of MSHBs that use layered sodium vanadate((Na,Mn)V_(8)O_(20)·5H_(2)O,Mn-NVO)cathodes coupled with an organic 3,4,9,10-perylenetetracarboxylic diimide(PTCDI)anode in Mg^(2+)/Na^(+)hybrid *** electrochemical cycling,Mg^(2+)and Na^(+)co-participate in the cathode reactions,and the introduction of Na^(+)promotes the structural stability of the Mn-NVO cathode,as cleared by several ex-situ ***,the Mn-NVO cathode presents great specific capacity(249.9 mA h g^(−1)at 300 mA g^(−1))and cycling(1500 cycles at 1500 mA g^(−1))in the Mg^(2+)/Na^(+)hybrid ***,full battery displays long lifespan with 10,000 cycles at 1000 mA g^(−1).The rate performance and cycling stability of MSHBs have been improved by an economical and scalable method,and the mechanism for these improvements is discussed.

关键词： Aqueous battery Hybrid ion battery Mg^(2+)/Na^(+)co-intercalation High-rate performance Organic-water hybrid electrolyte

Highly adaptive triboelectric tactile sensor on the foot of autonomous wall-climbing robots for detecting the adhesion state and avoiding the hazard

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Nano Research 2024年第7期17卷 6518-6526页

作者： Zhaoyang wang Jianhua liu Ziyu wang Chang liu Qingyu Chen Chaofan Zhang Wenbo Zhang Jicang Si xiu Xiao Peng Xu Minyi Xu Dalian Key Lab of Marine Micro/Nano Energy and Self-powered System Marine Engineering CollegeDalian Maritime UniversityDalian 116026China Information Science and Technology College Dalian Maritime UniversityDalian 116026China Navigation College Dalian Maritime UniversityDalian 116026China Intelligent Biomimetic Design Lab College of EngineeringPeking UniversityBeijing 100871China

Due to the excellent maneuverability and obstacle crossing of legged robots,it is possible for an autonomous legged wallclimbing robots to replace manual inspection of ship exterior ***,when the magnetic adsorption legged wallclimbing robot steps on the convex point or convex line of the wall,or even when the robot missteps,the robot is likely to detach from the ferromagnetic ***,this paper proposes a tactile sensor for the legged magnetic adsorption wall-climbing robot to detect the magnetic adsorption state and improve the safety of the autonomous crawling of the *** tactile sensor mainly comprises a three-dimensional(3D)-printed shell,a tactile slider,and three isometric sensing units,with an optimized *** experiment shows that the triboelectric tactile sensor can monitor the sliding depth of the tactile slider and control the light-emitting device(LED)signal *** addition,in the demonstration experiment of detecting the adsorption state of the robot's foot,the triboelectric tactile sensor has strong adaptability to various ferromagnetic wall ***,this study establishes a robot gait control system to verify the feedback control ability of the triboelectric tactile *** results show that the robot equipped with the triboelectric tactile sensor can recognize the dangerous area on the crawling wall and autonomously avoid the ***,the proposed triboelectric tactile sensor has great potential in realizing the tactile sensing ability of robots and enhancing the safety and intelligent inspection of ultra-large vessels.

关键词： legged wall-climbing robot ship inspection tactile perception triboelectric sensor

Variable Selection for Generalized linear Model with Highly Correlated Covariates

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Acta Mathematica Sinica,English Series 2024年第6期40卷 1458-1480页

作者： li li YUE Wei Tao wang Gao Rong li School of Statistics and Data Science Nanjing Audit UniversityNanjing 211815P.R.China School of Mathematics Statistics and MechanicsBeijing University of TechnologyBeijing 100124P.R.China School of Statistics Beijing Normal UniversityBeijing 100875P.R.China

The penalized variable selection methods are often used to select the relevant covariates and estimate the unknown regression coefficients simultaneously,but these existing methods may fail to be consistent for the setting with highly correlated *** this paper,the semi-standard partial covariance(SPAC)method with Lasso penalty is proposed to study the generalized linear model with highly correlated covariates,and the consistencies of the estimation and variable selection are shown in high-dimensional settings under some regularity *** simulation studies and an analysis of colon tumor dataset are carried out to show that the proposed method performs better in addressing highly correlated problem than the traditional penalized variable selection methods.

关键词： Generalized linear model highly correlated covariates Lasso penalty semi-standard partial covariance variable selection

Effect of kerosene injection states on mixing and combustion characteristics in a cavity-based supersonic combustor

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Chinese Journal of Aeronautics 2024年第4期37卷 308-320页

作者： Xu liU Peibo li Fei li Hongbo wang Mingbo SUN Chao wang Yixin YANG Dapeng XIONG Yanan wang Science and Technology on Scramjet Laboratory College of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China

It has been found that the static pressure distribution along the axial direction of liquid kerosene is lower than that of the gaseous kerosene under the same flow condition and overall equivalent ratio from previous *** further investigate this phenomenon,a compressible two-phase parallel simulation method is utilized to analyze the mixing and combustion characteristics of gaseous and liquid kerosene jets in a cavity-based supersonic *** numerical results are consistent with the experiments and demonstrate that gaseous injection leads to a cavity shear layer that dives deeper into the cavity,forming two recirculation zones in the front and rear of the *** contrast,the cavity shear layer is closer to the mainstream during liquid injection,and only a large recirculation zone is formed in the rear of the *** a result of the cavity shear layer and the recirculating flow,the fuel vapor of gaseous injection accumulates in the front of the cavity,while for the liquid injection,the fuel vapor disperses in the cavity,cavity shear layer,and the region above,and the rear of the cavity has a higher fuel vapor concentration than the *** unique fuel distribution causes the combustion area to be concentrated in the cavity during the gaseous injection but dispersed inside and downstream of the cavity during the liquid *** a result,forming a thermal throat under the same conditions is more challenging during liquid injection,and the generated static pressure distribution is lower than that during the gaseous injection.

关键词： Gaseous injection liquid injection Mixing process Combustion Supersonic flow

Mathematical Analysis on a General Delayed HBV Model with Capsids and Two Infection Routes

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 508-525页

作者： li-li liU Hong-gang wang Ya-zhi li Shanxi Key Laboratory of Mathematical Techniques and Big Data Analysis on Disease Control and Prevention Complex Systems Research CenterShanxi UniversityTaiyuan 030006China School of Mathematics and Statistics Qiannan Normal University for NationalitiesDuyun 558000China

Considering that HBV belongs to the DNA virus family and is hepatotropic,we model the HBV DNA-containing capsids as a *** this paper,a delayed HBV infection model is established,where the general incidence function and two infection routes including cell-virus infection and cell-cell infection are *** to some preliminaries,including well-posedness,basic reproduction number and existence of two equilibria,we obtain the threshold dynamics for the *** illustrate numerical simulations to verify the above theoretical results,and furthermore explore the impacts of intracellular delay and cell-cell infection on the global dynamics of the model.

关键词： delayed HBV model capsids general incidence function two infection routes global stability

Mechanism research progress on transition metal compound electrode materials for supercapacitors

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Rare Metals 2024年第9期43卷 4076-4098页

作者： Zhi-Hui Xu Xue-Lei li Qing-Wen li Kai Lv Jing-Shun liu xiu-Kun Hang Aruuhan Bayaguud School of Materials Science and Engineering Inner Mongolia University of Technology School of Materials Science and Engineering Tianjin University of Technology College of Chemistry and Chemical Engineering Inner Mongolia University

Supercapacitors(SCs) have remarkable energy storage capabilities and have garnered considerable interest due to their superior power densities and ultra-long cycling characteristics. However, their comparatively low energy density limits their extensive application in large-scale commercial applications. Electrode materials directly affect the performance of SCs. Thus, the development of cutting-edge electrode materials and modification of their morphological and structural properties are vital for advancing the performance of SCs. Transition metal compounds have a high specific capacity and good cycling durability, making them the most promising electrode active materials for high-energy density SCs. Nevertheless,their inadequate conductivity, unfavorable ion diffusion rates, substantial volume expansion and phase transitions during charging and discharging are obstacles to their stable and efficient integration into SCs. To address these challenges, this study provides a comprehensive summary of the current advancements in transition metal nanomaterials as electrode materials for SCs, an overview of the current research status, and the prevailing ***, this study highlights synthetic techniques and management strategies for electrode materials derived from transition metal compounds, targeting the resolution of the aforementioned challenges. Finally, a concise discussion is provided on the future directions of SC development, with an emphasis on the utilization of transition metal compound electrode materials.

关键词： Electrodes

Thermofluidic investigations of oil natural transformer:Closed-loop modelling and experimental validation

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High Voltage 2024年第1期9卷 230-240页

作者： Yuan li Yiran Gao Chen wang Chao Zhu Ying li Yuankai wang Guanjun Zhang State Key Laboratory of Electrical Insulation and Power Equipment Xi'an Jiaotong UniversityXi'anChina Electric Power Research Institute of State Grid Shaanxi Electric Power Co. Ltd.Xi'anChina TBEA Hengyang Transformer Co. Ltd.HengyangChina

Excessively high temperatures inside a power transformer can accelerate the ageing rate and even cause unplanned *** estimating the hot-spot temperature(HST)of a power transformer is important for regulating the load and ensuring long-term *** this study,a closed-loop model of a 110-kV product transformer with an oil natural/air forced(ONAF)cooling mode is built to predict HST,in which the compression ratio of windings,equivalent heat source and radiator geometry are *** to the flow field of the winding,the‘dead oil zone’and reverse oil flow are observed in the horizontal oil *** accuracy of the proposed model is experimentally validated by temperature-rise *** results show that the absolute errors between the measured results and simulation are below 5°C,and the average error is~2°***,the arrangements of windings and radiators are studied to enhance the oil *** adding 5 washers to the high-voltage winding,the average temperature can be decreased by 6°C compared with the case without a *** the radiator can also mitigate the characteristic temperatures,and the optimal height difference between the radiator and winding centre is suggested to be 0.66 m.

关键词： winding arrangement adding

Molecular design of recyclable thermosetting polyimide and its composite with excellent mechanical and tribological properties

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Friction 2024年第3期12卷 452-461页

作者： Xiaoyue wang Zenghui YANG Tingmei wang Qihua wang Xinrui ZHANG Song li Key Laboratory of Science and Technology on Wear and Protection of Materials Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Recyclability of thermosetting polymers and their composites is a challenge for alleviating environmental pollution and resource *** this study,solvent-recyclable thermosetting polyimide(PI)and its composite were successfully *** tensile strength,elongation at break,and Young’s modulus of PI are 108.70±7.29 MPa,19.35%±3.89%,and 2336.42±128.00 MPa,*** addition of reduced graphene oxide(RGO)not only enhances the mechanical properties of PI but also endows it with excellent tribological *** PI illustrates a high recycling efficiency of 94.15%,but the recycled composite exhibits inferior mechanical *** recycling and utilization of PI and its composite are realized through imine bonds(-C=N),which provides new guidance for solving the problem of environmental pollution and resource waste and is potential application in the field of sustainable tribology.

关键词： thermosetting polyimide(PI) recyclability dynamic covalent bonds friction and wear polymer composites

Multidimensional regulation of Ti-Zr-Cr-Mn hydrogen storage alloys via Y partial substitution

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Nano Research 2024年第5期17卷 4211-4220页

作者： Haixiang xiu Wanqiang liu Dongming Yin Nan Ding Wenfeng Qiao Shaolei Zhao Long liang Cong liu Shaohua wang Qingshuang wang Bingbing Chen limin wang Yong Cheng School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resources Utilization Changchun Institute of Applied ChemistryChinese Academy of Sciences(CAS)Changchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China Department of Energy Science and Engineering Nanjing Tech UniversityNanjing 211816China National Engineering Research Center of Nonferrous Metals Materials and Products for New Energy GRINM Group Co.Ltd.Beijing 100088China GRIMAT Engineering Institute Co. Ltd.Beijing 101407China College of life Science and Technology Changchun University of Science and TechnologyChangchun 130022China

High density and safe storage of hydrogen are the preconditions for the large-scale application of hydrogen ***,the hydrogen storage properties of Ti_(0.6)Zr_(0.4)Cr_(0.6)Mn_(1.4) alloys are systematically studied by introducing Y element instead of Ti element through vacuum arc *** the partial substitution of Y,a second phase of rare earth oxide is added in addition to the main suction hydrogen phase,C14 Laves *** to the unique properties of rare earth elements,the partial substitution of Y can not only improve the activation properties and plateau pressure of the alloys,but also increase the effective hydrogen storage capacity of the *** comprehensive properties of hydrogen storage alloys are improved by multidimensional regulation of rare earth *** them,Ti_(0.552)Y_(0.048)Zr_(0.4)Cr_(0.6)Mn_(1.4) has the best comprehensive *** alloy can absorb hydrogen without activation at room temperature and 5 MPa,with a maximum hydrogen storage capacity of 1.98 wt.%.At the same time,it reduces the stability of the hydride and the enthalpy change value,making it easier to release *** theoretical analysis and first-principle simulation,the results show that the substitution of Y element reduces the migration energy barrier of hydrogen and the structural stability of the system,which is conducive to hydrogen *** alloy has superior durability compared to the original alloy,and the capacity retention rate was 96.79%after 100 hydrogen absorption/desorption cycles.

关键词： AB_(2)-type hydrogen storage alloy rare earth element first-principles simulation multidimensional regulation

Progress of gaseous arsenic removal from flue gas by adsorption:Experimental and theoretical calculations

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Journal of Environmental Sciences 2024年第2期136卷 470-485页

作者： Xuelei Yan Qingzhu li Xiaowei Huang Bensheng li Shengtu li Qingwei wang School of Metallurgy and Environment Central South UniversityChangsha 410083China National Engineering Research Centre for Control and Treatment of Heavy Metal Pollution Central South UniversityChangsha 410083China National Engineering Research Center for Rare Earth Materials General Research Institute for Non-Ferrous MetalsBeijing 100088China

Because of its high mobility and difficult capture,gaseous arsenic pollution control has become the focus of arsenic pollution *** mainly exists in the form of highly toxic As_(2)O_(3)in the flue ***,removing gaseous As_(2)O_(3)from flue gas is of great practical significance for arsenic pollution *** gaseous As_(2)O_(3)on the surface of adsorbents by physical or chemical adsorption is an effective way to reduce the content of arsenic in the flue gas and alleviate arsenic *** the past few decades,various adsorbents have been developed to capture gaseous As_(2)O_(3)in the flue gas,and their adsorption mechanisms have been studied in ***,it is necessary to review the strategies of arsenic removal from flue gas by adsorption,which can inspire further *** on summarizing the morphological distribution of gaseous As_(2)O_(3)in the flue gas,this review further summarizes the removal of gaseous As_(2)O_(3)by several adsorbents and the effect of temperature and the main components of the flue gas on arsenic *** addition,the mechanism of arsenic removal based on adsorption in the flue gas is discussed in depth through theoretical calculations,which is the particular focus of this ***,prospects based on the present research state of arsenic removal by adsorption are proposed to provide ideas for developing effective and stable adsorbents for arsenic removal from flue gas.

关键词： Gaseous arsenic Flue gas Adsorption Theoretical calculation Mechanism