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Asymmetric Electrolytes Design for Aqueous Multivalent Metal Ion Batteries

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Nano-Micro Letters 2024年第3期16卷 227-253页

作者： Xiaochen Yang xinyu Wang yue Xiang Longtao Ma Wei Huang Frontiers Science Center for Flexible Electronics Institute of Flexible ElectronicsNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China School of Materials Science and Engineering Guangdong Provincial Key Laboratory of Advanced Energy Storage MaterialsSouth China University of TechnologyGuangzhou 510641People’s Republic of China

With the rapid development of portable electronics and electric road vehicles,high-energy-density batteries have been becoming front-burner ***,homogeneous electrolyte cannot simultaneously meet diametrically opposed demands of high-potential cathode and low-potential anode,which are essential for high-voltage ***,homogeneous electrolyte is difficult to achieve bi-or multi-functions to meet different requirements of *** comparison,the asymmetric electrolyte with bi-or multi-layer disparate components can satisfy distinct requirements by playing different roles of each electrolyte layer and meanwhile compensates weakness of individual ***,the asymmetric electrolyte can not only suppress by-product sedimentation and continuous electrolyte decomposition at the anode while preserving active substances at the cathode for high-voltage batteries with long cyclic *** this review,we comprehensively divide asymmetric electrolytes into three categories:decoupled liquid-state electrolytes,bi-phase solid/liquid electrolytes and decoupled asymmetric solid-state *** design principles,reaction mechanism and mutual compatibility are also studied,***,we provide a comprehensive vision for the simplification of structure to reduce costs and increase device energy density,and the optimization of solvation structure at anolyte/catholyte interface to realize fast ion transport kinetics.

关键词： Asymmetric electrolyte Aqueous multivalent metal ion batteries Electrochemical stability windows Electrolyte interface

User Profiling for CSDN:Keyphrase Extraction,User Tagging and User Growth Value Prediction

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Data Intelligence 2019年第2期1卷 137-159页

作者： Guoliang Xing Hao Gao Qi Cao xinyu yue Bingbing Xu Keting Cen Huawei Shen Key Laboratory of Network Data Science and Technology Institute of Computing TechnologyChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The Chinese Software Developer Network(CSDN)is one of the largest information technology communities and service platforms in *** paper describes the user profiling for CSDN,an evaluation track of SMP Cup *** contains three tasks:(1)user document keyphrase extraction,(2)user tagging and(3)user growth value *** the first task,we treat keyphrase extraction as a classification problem and train a Gradient-Boosting-Decision-Tree model with comprehensive *** the second task,to deal with class imbalance and capture the interdependency between classes,we propose a two-stage framework:(1)for each class,we train a binary classifier to model each class against all of the other classes independently;(2)we feed the output of the trained classifiers into a softmax classifier,tagging each user with multiple *** the third task,we propose a comprehensive architecture to predict user growth *** contributions in this paper are summarized as follows:(1)we extract various types of features to identify the key factors in user value growth;(2)we use the semi-supervised method and the stacking technique to extend labeled data sets and increase the generality of the trained model,resulting in an impressive performance in our *** the competition,we achieved the first place out of 329 teams.

关键词： User profiling Keyphrase extraction User tagging Growth value prediction Word embedding

Regulating photothermal properties of near-infrared croconaine dyes by supramolecular assembly

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Nano Research 2024年第9期17卷 8560-8570页

作者： Yangge Ren yue Lu Juanjuan Gao Yi Ding Bo Zhu xinyu Hou Lin Jia Department of Polymer Materials School of Materials Science and EngineeringShanghai UniversityShanghai 200444China Department of Electronic Information Materials School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

The photochemical and photophysical properties of near-infrared(NIR)dyes are significantly influenced by their aggregation state and mesoscopic ***,beyond chemical synthesis,the regulation mechanisms for the properties of NIR dyes,particularly with respect to photothermal properties of the aggregates,are not yet fully ***,we investigate the photothermal behaviors of croconaine-based(CroA)NIR dyes containing dipeptide or amino acids *** introduction of hydrogen bonding promotesπ-πstacking of croconaine center,which can efficiently regulate aggregation states and assembly structures in *** laser irradiation,CroA aggregates undergo aggregation-dissociation transition,the in-situ monomer generation process regulates two parameters of photothermal performance:heating rates and plateau photothermal *** study reveals the regulation effect of non-covalent bonding interactions on CroA aggregates,highlighting supramolecular assembly strategy not only facilitates to construct of photothermal nanomaterials with well-defined structures,but also provides an alternative and effective method for regulating photothermal performance of NIR dyes.

关键词： croconaine dye hydrogen bonding photothermal performance supramolecular assembly chirality

Thienothiophene-centered ladder-type π-systems that feature distinct quinoidal π-extension

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Chinese Chemical Letters 2024年第5期35卷 249-253页

作者： Jiaxiang Guo Zeyi Li Tianyu Zhang xinyu Tian yue Wang Chuandong Dou State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun 130012China Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials Soochow UniversitySuzhou 215123China

Quinoidalπ-conjugated structures,a kind of fundamental subunits for organicπ-systems,may produce some intriguing optical,electronic and magnetic properties of polycyclic hydrocarbons(PHs).Herein,we report two thienothiophene-centered ladder-type polycyclic molecules(1 and 2),which possess one quinoidal thienothiophene moiety and two para-quinodimethane(p-QDM)subunits,*** theoretically and experimentally studied,while 1 is a fully closed-shell molecule,2 owns an open-shell structure along with partial contribution of tetraradical state that is induced by the resonance of ***,although 2 has a largerπ-conjugated skeleton and open-shell electronic state,it exhibits larger bandgap and blue-shifted *** the other hand,the reversible oxidation activity of 1 enables the preparation of its dication 1^(2+),and the studies on its single-crystal and aromatic structures demonstrate that its two positive charges are delocalized onto the oxygen atoms,thus achieving fullyπ-extended structure and near-infrared *** study not only gains insight into quinoidalπ-subunits,but also provides an important basis for the development of antiaromatic and open-shellπ-electron materials.

关键词： Thienothiophene Quinoidal conjugation Open-shell structure Aromaticity Photophysical properties

Enhancing stability of diradical polycyclic hydrocarbons via P=O-attaching

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Chinese Chemical Letters 2024年第8期35卷 309-313页

作者： Jingyuan Yang xinyu Tian Liuzhong Yuan Yu Liu yue Wang Chuandong Dou State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun 130012China Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials Soochow UniversitySuzhou 215123China

Diradical polycyclic hydrocarbons(PHs)have unique open-shell structures and interesting physical ***,owing to high reactivity of unpaired electrons,such open-shell organic diradicaloids are usually less stable than closed-shell systems,limiting their practical *** this study,we report P=O-attaching of diradical PHs as a new strategy to enhance their stability while maintaining diradi-cal *** P=O-attached PHs containing the indeno[1,2-b]fluorene,fluoreno[3,2-b]fluorene and indeno[2,1-b]fluoreneπ-skeletons,respectively,were designed and *** theoretically and ex-perimentally proved,two of them have the relatively large diradical characters and open-shell singlet diradical *** comparison to their all-carbon analogues,the attached electron-withdrawing P=O groups endow them with much lower LUMO/HOMO energy levels but preserved magnetic activities and physical properties,such as thermally accessible triplet species and multi-redox ***,the P=O groups effectively decrease their oxidation activities and thereby lead to their remarkably excellent ambient ***,this P=O-attaching strategy will be applicable to other diradical PH systems and may promote the generation of stable organic diradicaloids for radical chemistry and materials.

关键词： Polycyclic hydrocarbons Open-shell structure Diradical character Stability Oxidation activity

Tumor biomarkers for diagnosis,prognosis and targeted therapy

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Signal Transduction and Targeted Therapy 2024年第6期9卷 2391-2476页

作者： yue Zhou Lei Tao Jiahao Qiu Jing Xu xinyu Yang Yu Zhang xinyu Tian Xinqi Guan Xiaobo Cen Yinglan Zhao Department of Biotherapy Cancer Center and State Key Laboratory of BiotherapyWest China HospitalSichuan UniversityChengdu 610041China West China School of Pharmacy Sichuan UniversityChengdu 610041China School of Medicine Tibet UniversityLhasa 850000China National Chengdu Center for Safety Evaluation of Drugs State Key Laboratory of BiotherapyWest China HospitalSichuan UniversityChengdu 610041China

Tumor biomarkers,the substances which are produced by tumors or the body’s responses to tumors during tumorigenesis and progression,have been demonstrated to possess critical and encouraging value in screening and early diagnosis,prognosis prediction,recurrence detection,and therapeutic efficacy monitoring of *** the past decades,continuous progress has been made in exploring and discovering novel,sensitive,specific,and accurate tumor biomarkers,which has significantly promoted personalized medicine and improved the outcomes of cancer patients,especially advances in molecular biology technologies developed for the detection of tumor ***,we summarize the discovery and development of tumor biomarkers,including the history of tumor biomarkers,the conventional and innovative technologies used for biomarker discovery and detection,the classification of tumor biomarkers based on tissue origins,and the application of tumor biomarkers in clinical cancer *** particular,we highlight the recent advancements in biomarker-based anticancer-targeted therapies which are emerging as breakthroughs and promising cancer therapeutic *** also discuss limitations and challenges that need to be addressed and provide insights and perspectives to turn challenges into opportunities in this ***,the discovery and application of multiple tumor biomarkers emphasized in this review may provide guidance on improved precision medicine,broaden horizons in future research directions,and expedite the clinical classification of cancer patients according to their molecular biomarkers rather than organs of origin.

关键词： diagnosis breakthrough biomarkers

Effects of axylitol-casein complex on insulin resistance and gut microbiota composition in high-fat-diet+streptozotocin-induced type 2 diabetes mellitus mice

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Food Science and Human Wellness 2024年第5期13卷 2741-2753页

作者： Fanhua Kong Juan Zhang Shimo Kang xinyu Shen Aicheng Liu Yan Zheng Junhua Shao Xiqing yue College of Food Science Shenyang Agriculture UniversityShenyang 110866China

This study investigated the effects of a xylitol-casein non-covalent complex(XC)on parameters related to type 2 diabetes mellitus(T2DM),in addition to related changes in gut microbiome composition and ***-fat-diet(HFD)+streptozotocin(STZ)-induced T2DM mice were treated with xylitol(XY),casein(CN),and XC,after which fecal samples were collected for gut microbiota composition and diversity analyses based on 16S rRNA high-throughput sequencing and multivariate *** decreased body weight and improved glucose tolerance,insulin sensitivity,pancreas impairment,blood lipid levels,and liver function in T2DM mice compared to XY-and CN-treated ***,XC modulated theα-diversity,β-diversity and gut microbiota *** on Spearman’s correlation analysis,the relative abundances of Alistipes,Bacteroides,and Faecalibaculum were positively correlated and those of Akkermansia,Lactobacillus,Bifidobacterium,and Turicibacter were negatively correlated with the phenotypes related to the improvement of *** conclusion,we found that XC alleviated insulin resistance by restoring the gut microbiota of T2DM *** results provide strong evidence for the beneficial effects of XC on T2DM and motivation for further investigation in animal models and,eventually,human trials.

关键词： Xylitol-casein complex Type 2 diabetes mellitus Insulin resistance Gut microbiota

Disparity map optimization based on edge detection

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Disparity map optimization based on edge detection

DNA methylation of SMPD3-based diagnostic biomarkers of NASH and mild fibrosis

第30届中国控制与决策会议

作者： xinyu yue Fangrong Wang Baicang Guo Pengzhi Xu Jian Shi College of Communication Engineering Jilin University College of Transportation Jilin University

In stereo vision, disparity map after stereo matching using projection model can get the depth information and 3D information of the original image. In order to improve the accuracy and speed of stereo matching, improving the quality of disparity map becomes the core problem of stereo matching. Firstly, the paper extracted edge information of binocular images using Canny, Scharr and Sobel edge detection algorithm. On this basis, the paper use SGBM algorithm（Semi-global block Matching） and DP algorithm（Dynamic Programming）and CSCA algorithm（Cross-scale Cost Aggregation） respectively calculated the disparity map and its error rate. After analysis, the combination of Canny detection algorithm and CSCA algorithm can eliminate a large number of number of irrelevant information and reduce the amount of data processing. The real scene image is selected to validate the *** on the above research results, the method improved the quality of disparity map.

关键词： Computer application Stereo vision Edge detection stereo matching Disparity map

来源： cnki会议评论

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Genes & Diseases 2024年第1期11卷 99-102页

作者： Na Wu Mofan Feng Siran yue xinyu Shi Nan Tang Yalan Xiong Jianying Wang Lei Zhang Hualing Song Yi Shi Guang He Guang Ji Baocheng Liu Shanghai Innovation Center of Traditional Chinese Medicine Health Service School of Public HealthShanghai University of Traditional Chinese MedicineShanghai 201203China Institute of Digestive Diseases Longhua HospitalShanghai University of Traditional Chinese MedicineShanghai 200032China Bio-X Institutes Key Laboratory for the Genetics of Developmental and Neuropsychiatric DisordersShanghai Jiao Tong UniversityShanghai 200030China Institute for Advancing Translational Medicine in Bone and Joint Diseases School of Chinese MedicineHong Kong Baptist UniversityHong Kong SAR 999077China

Non-alcoholic fatty liver disease(NAFLD)is a liver condition that is widely prevalent across the world.A considerable number of people with NAFLD have the potential to progress to a more severe form of the condition known as nonalcoholic steatohepatitis(NASH),accompanied by bridging *** advancement is more likely if the patient has metabolic risk factors such as obesity or type 2 diabetes that deteriorate over ***,even slight inflammation or fibrosis in NAFLD can significantly increase the likelihood of progression compared to steatosis *** underscores the importance of revising the present methods of monitoring NAFLD patients to ensure early detection and effective management of the disease.

关键词： NAFLD inflammation NASH