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Printing perovskite and graphene parallel structure-based optical-mechanical sensors for human-machine interaction

Science China Technological Sciences 2025年

作者： Sisi CHEN Jiemin ZHANG Nan CHENG Wenbo LI Jing LIU Hongfei XIE Jie ZHANG Yueying CHENG Xiaotong ZHAO meng SU Yanlin SONG Key Laboratory of Green Printing CAS Research/Education Center for Excellence in Molecular Sciences Institute of ChemistryChinese Academy of Sciences (ICCAS) University of Chinese Academy of Sciences Weiyang College Tsinghua University Department of Cardiovascular Surgery First Medical Center PLA General Hospital AECC Beijing Institute of Aeronautical Materials Beijing Institute of Graphene Technology Beijing Engineering Research Centre of Graphene Application School of Integrated Circuit & Beijing National Research Center for Information Science and Technology (BNRist) Tsinghua University

Surgical robots are designed to provide enhanced precision and dexterity compared to manual surgical procedures,which mainly rely on multimodal sensing technologies for the surgeon to seamlessly operate the robotic arms and *** with single-mode sensors, optical and mechanical bi-modal sensors provide improved precision, enhanced safety,and robustness of human-machine interaction systems. Here, the template-guided and pneumatic printing technologies are combined to construct perovskite and graphene parallel structures with both optical and mechanical sensing capabilities. The printed uniformly crystallized perovskite microstructure exhibits fast and sensitive photoelectric response characteristics,enabling shadow recognition functionality. The combination of graphene and elastic rubber endows the great printability to prepare parallel structures near the perovskite arrays for force sensing capabilities. Thus, the printed perovskite and graphene structures possess non-contact optical sensing capabilities to detect hand position by recognizing shadows between the hand and the sensor, as well as contact mechanical sensing capabilities to detect touch force applied by the hand. It provides a synergistic platform for real-time and multidimensional feedback to improve human-machine interaction.

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Alleviating the anisotropic microstructural change and boosting the lithium ions diffusion by grain orientation regulation for Ni-rich cathode materials

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Journal of Energy Chemistry 2024年第1期88卷 213-222,I0005页

作者： xinyou He Shilin Su Bao Zhang Zhiming Xiao Zibo Zhang Xing Ou Engineering Research Center of the Ministry of Education for Advanced Battery Materials School of Metallurgy and EnvironmentCentral South UniversityChangsha 410083HunanChina Zhejiang Power New Energy Co.Ltd Zhuji 311899ZhejiangChina

Generally,layered Ni-rich cathode materials exhibit the morphology of polycrystalline secondary sphere composed of numerous primary *** the arrangement of primary particles plays a very important role in the properties of Ni-rich *** disordered particle arrangement is harmful to the cyclic performance and structural stability,yet the fundamental understanding of disordered structure on the structural degradation behavior is ***,we have designed three kinds of LiNi_(0.83)Co_(0.06)Mn_(0.11)O_(2) cathode materials with different primary particle orientations by regulating the precursor coprecipitation *** finite element simulation and in-situ characterization,the Li^(+)transport and structure evolution behaviors of different materials are ***,the smooth Li^(+)diffusion minimizes the reaction heterogeneity,homogenizes the phase transition within grains,and mitigates the anisotropic microstructural change,thereby modulating the crack evolution ***,the optimized structure evolution ensures radial tight junctions of the primary particles,enabling enhanced Li^(+)diffusion during dynamic ***-loop bidirectional enhancement mechanism becomes critical for grain orientation regulation to stabilize the cyclic *** precursor engineering with particle orientation regulation provides the useful guidance for the structural design and feature enhancement of Ni-rich layered cathodes.

关键词： Ni-rich cathode Grain orientation regulation Anisotropic microstructural change Precursor engineering Li~+-ions diffusion

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Defect-mode and Fabry-Perot resonance induced multi-band nonreciprocal thermal radiation

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Science China(Technological Sciences) 2024年第8期67卷 2405-2412页

作者： CHEN ZiHe YU ShiLv YUAN Cheng CUI xinyou HU Run School of Energy and Power Engineering Huazhong University of Science and TechnologyWuhan 430074China Wuhan Fiberhome Fuhua Electric Co. Ltd.Wuhan 430074China

According to Kirchhoff's radiation law,the spectral-directional absorptivity(α)and spectral-directional emissivity(e)of an object are widely believed to be identical,which places a fundamental limit on photonic energy conversion and *** introduction of Weyl semimetals and magneto-optical(MO)materials into photonic crystals makes it possible to violate Kirchhoff's law,but most existing work only report the unequal absorptivity and emissivity spectra in a single band,which cannot meet the requirements of most practical ***,we introduce a defect layer into the structure composed of one-dimensional(1D)magnetophotonic crystal and a metal layer,which realizes dual-band nonreciprocal thermal radiation under a 3-T magnetic field with an incident angle of 60°.The realization of dual-band nonreciprocal radiation is mainly due to the Fabry-Perot(FP)resonance occurring in the defect layer and the excitation of Tamm plasmon,which is proved by calculating the magnetic field *** addition,the effects of incident angle and structural parameters on nonreciprocity are also *** is more,the number of nonreciprocal bands could be further increased by tuning the defect layer *** the defect layer thickness increases to 18.2μm,tri-band nonreciprocal thermal radiation is realized due to the enhanced number of defect modes in the photonic band gap and the FP resonance occurring in the defect ***,the effect of defect location on nonreciprocity is also *** present work provides a new way for the design of multi-band or even broad-band nonreciprocal thermal emitters.

关键词： Kirchhoff's law multi-band nonreciprocal thermal radiation magnetophotonic crystal Tamm plasmon defect layer Fabry-Perot resonance

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A New Type of Li Deposit:Hydrothermal Crypto-Explosive Breccia Pipe Type

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Journal of Earth Science 2022年第5期33卷 1095-1113页

作者： Shao-Yong Jiang Huimin Su xinyou Zhu Kangyu Zhu Zhenpeng Duan State Key Laboratory of Geological Processes and Mineral Resources School of Earth Resources and Collaborative Innovation Center for Exploration of Strategic Mineral ResourcesChina University of GeosciencesWuhan 430074China Beijing Institute of Geology and Mineral Resource Co. LtdBeijing 100012China

Lithium is one of the important strategic energy metals,which is in short supply in *** are three major types of lithium deposits:brine and salt lake type,highly differentiated granite or pegmatite type,and carbonate-clay *** recent years,some new types of lithium deposits have also begun to receive great attention and subject recent *** are many crypto-explosive breccia pipe type deposits in the world,including copper,gold,lead,zinc,tungsten and tin deposits,but little is known about this type of lithium *** paper introduces the latest research results of the Weilasituo Sn-Li-Rb polymetallic deposit in Inner Mongolia(NE China),which occurs in the middlesouthern section of the Great Xing’an Range metallogenic belt.A remarkable feature of this deposit is the coexistence of various mineralization types,including granite type Rb and Sn-Zn,hydrothermal crypto-explosive breccia pipe type Li-Rb,quartz vein type Sn-Zn and sulfide vein type Pb-Zn-Ag *** them,hydrothermal crypto-explosive breccia pipe type Li-Rb deposit is currently very rare at home and abroad,which is likely a new type of rare metal deposit that worthy of our *** paper systematically summarizes the geology,alteration and mineralization,geochemistry,isotopes and geochronology of the Weilasituo deposit,and establishes a new petrogenic and metallogenic model.

关键词： lithium deposit hydrothermal crypto-explosive breccia pipe type petrogenic and metallogenic model Weilasituo deposit Inner Mongolia mineral deposits

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Responses of Lowland, Upland and Aerobic Rice Genotypes to Water Limitation During Different Phases

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Rice science 2020年第4期27卷 345-354页

作者： Preethi VIJAYARAGHAVAREDDY YIN xinyou Paul CSTRUIK Udayakumar MAKARLA Sheshshayee SREEMAN Department of Crop Physiology University of Agricultural SciencesBengaluru 560065India Centre for Crop Systems Analysis Wageningen University&ResearchPO Box 4306700AK Wageningenthe Netherlands

Rice yield reduction due to water limitation depends on its severity and duration and on the phenological stage of its *** exposed three contrasting rice genotypes,IR64,UPLRi7 and Apo(adapted to lowland,upland and aerobic conditions,respectively),to three water regimes(puddle,100%and 60%field capacity)in pots during the vegetative(GSI),flowering(GSII)and grain filling(GSIII)*** at all the three stages significantly reduced yield especially in lowland genotype *** of water limitation was more severe at GSII than at the other two *** at GSI stage reduced both source activity(leaf area and photosynthetic rate)and sink capacity(tiller number or panicle number per pot).When stress was imposed at GSII,spikelet fertility was most affected in all the three *** both GSII and GSIII,although leaf area was constant in all the three water regimes,estimated relative whole-plant photosynthesis was strongly associated with yield *** photosynthesis due to stress at any given stage was found to have direct impact on *** to the other genotypes,Apo had deeper roots and maintained a better water relation,thus,higher carbon gain and spikelet viability,and ultimately,higher biomass and productivity under water-limited ***,screening for these stage-dependent adaptive mechanisms is crucial in breeding for sustained rice production under water limitation.

关键词： water limitation phenology upland aerobic Oryza sativa yield

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Facile synthesis of the dodecahydridododecaborate (B12H122-) from borane Lewis base adducts

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Science China Chemistry 2025年

作者： Yi Jing Xin-Ran Liu Xing-Hua Wang Hui Han Sha-Sha Liang Xi-meng Chen Dong-Hui Wei Lai-Sheng Wang Xue-Nian Chen College of Chemistry Zhengzhou University School of Chemistry and Chemical Engineering Henan Key Laboratory of Boron Chemistry and Advanced MaterialsHenan Normal University Department of Chemistry Brown University

Polyhedral boranes are a class of well-known boron molecular clusters widely used in energy,chemistry,medicine,and materials science because of their unique physical and chemical *** efforts have been made in the past decades to find more effective synthetic methods for this important class of boron ***,existing synthetic methods suffer from low efficiency and low ***,we report a facile one-pot synthesis of[（CH3）3S]2B12H12with moderate yields at mild *** mechanisms for the multi-step chemoselective synthesis of B12H122-without other by-products are elucidated based on theoretical results and our previous *** Lewis base used in B–H bond condensation reaction,which acts as a hydrogen or to balance the newly generated polyhedral borane charges,is proposed and studied in *** current study has led to a more effective and selective synthetic method for B12H122-and has also implicated the syntheses of other new polyhedral boranes.

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Understanding the failure mechanism towards developing high-voltage single-crystal Ni-rich Co-free cathodes

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Green Energy & Environment 2024年第6期9卷 1045-1057页

作者： Jixue Shen Bao Zhang Changwang Hao Xiao Li Zhiming Xiao xinyou He Xing Ou Engineering Research Center of the Ministry of Education for Advanced Battery Materials School of Metallurgy and EnvironmentCentral South UniversityChangsha410083China Zhejiang Power New Energy Co. Ltd.Zhuji311899China Material Science and Chemistry Engineering College China University of GeosciencesWuhan430074China

Benefited from its high process feasibility and controllable costs,binary-metal layered structured LiNi_(0.8)Mn_(0.2)O_(2)(NM)can effectively alleviate the cobalt supply crisis under the surge of global electric vehicles(EVs)sales,which is considered as the most promising nextgeneration cathode material for lithium-ion batteries(LIBs).However,the lack of deep understanding on the failure mechanism of NM has seriously hindered its application,especially under the harsh condition of high-voltage without sacrifices of reversible ***,singlecrystal LiNi_(0.8)Mn_(0.2)O_(2) is selected and compared with traditional LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM),mainly focusing on the failure mechanism of Cofree cathode and illuminating the significant effect of Co element on the Li/Ni antisite defect and dynamic ***,the presence of high Li/Ni antisite defect in NM cathode easily results in the extremely dramatic H2/H3 phase transition,which exacerbates the distortion of the lattice,mechanical strain changes and exhibits poor electrochemical performance,especially under the high cutoff ***,the reaction kinetic of NM is impaired due to the absence of Co element,especially at the single-crystal ***,the negative influence of Li/Ni antisite defect is controllable at low current densities,owing to the attenuated ***,Co-free NM can exhibit better safety performance than that of NCM *** findings are beneficial for understanding the fundamental reaction mechanism of single-crystal Ni-rich Co-free cathode materials,providing new insights and great encouragements to design and develop the next generation of LIBs with low-cost and high-safety performances.

关键词： Li/Ni antisite defect Dynamic characteristic High-voltage Single-crystal Ni-rich Co-free cathodes Lithium-ion batteries

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Influence of Sb_2O_3 doping on the properties of KBT-NBT-BT lead-free piezoelectric ceramics

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Rare Metals 2011年第1期30卷 72-75页

作者： HUANG xinyou GAO Chunhua WEI Minxian CHEN Zhigang CUI Yongzhen School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China

0.144（K0.5Bi0.5）TiO3-0.85（Na0.5Bi0.5）TiO3-0.006BaTiO3（KBT-NBT-BT） lead-free piezoelectric ceramics were prepared using a conventional solid state *** influence of Sb2O3 doping on the crystal phase,surface microstructure and properties of the KBT-NBT-BT lead-free piezoelectric ceramics were investigated using X-ray diffraction（XRD）,scanning electron microscope（SEM） and other analytical *** results show that all compositions are of pure perovskite structure solid ***2O3 doping does not influence the microstructure of KBT-NBT-BT lead-free piezoelectric ceramics obviously in the Sb2O3 doping range of 0.1-0.5 wt.%.Sb2O3 functions as a donor when doped small amount,while functions as a acceptor when doped large *** piezoelectric strain constant（d33） increases first and then decreases;the dielectric constant（ε33^T/ε0） and the dielectric loss（tanδ） decrease continuously when the amount of Sb2O3 dopant *** the doping amount of Sb2O3 is 0.1 wt.%,the KBT-NBT-BT piezoelectric ceramics with good comprehensive properties are obtained,whose d33,ε33^T/ε0 and tanδ are 147 pC/N,1510 and 4.2%,respectively.

关键词： nonmetallic materials piezoelectric ceramics doping piezoelectricity dielectric properties

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Pulp health and calcific healing of a complicated crown–root fracture with additional root fracture in a maxillary incisor: A case report

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World Journal of Clinical Cases 2025年第3期13卷 42-49页

作者： Na Li Yue-Yue Ren Ying Tang Qi Yang Tian-Tian meng Song Li Jing Zhang Stomatological Hospital and College Anhui Medical UniversityHefei 230032Anhui ProvinceChina Department of Endodontics The Affiliated Stomatological Hospital of Xuzhou Medical UniversityXuzhou 221000Jiangsu ProvinceChina

BACKGROUND Complicated crown–root fracture (CRF) involves severe injury to the crown, root,and pulp, and may be accompanied by multiple root fractures. The loss of a toothhas lifelong consequences for children and teenagers, but the maintenance of pulphealth and the calcific healing of multiple root fractures are rarely reported in *** SUMMARY This case reports healing of a permanent tooth with complicated crown–root andadditional root fractures, in which pulp health was maintained. A 10-year-old girlfell and fractured the root of her maxillary left central incisor at the cervical *** the coronal fragment was repositioned, the tooth was splinted until thetooth was no longer mobile, 2 years later. Eight years after treatment, the toothhas remained asymptomatic with vital pulp and localized gingival ***-beam computed tomography revealed not only calcified healing of the CRFbut also spontaneous healing in an additional undiagnosed root fracture. Thefracture line on the enamel could not be healed by hard tissue and formed agroove in the cervical crown. It was speculated that the groove was related to thelocalized gingival *** This case provides a clinical perspective of the treatment of a tooth with acomplicated CRF and an additional root fracture.

关键词： Complicated crown-root fracture Multiple root fracture Spontaneous healing Cone-beam computed tomography Long-term follow-up Case report

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内卷感知对大学生积极心理健康的影响:一项短期追踪研究

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黑龙江高教研究 2025年第2期43卷 115-123页

作者：周昱昊张萌中国人民公安大学北京100038

采用问卷调查法,通过5个月两阶段的纵向追踪探讨了627名中国大学生内卷感知对其积极心理健康的影响以及内在机制和边界条件。研究结果表明,内卷感知负向预测大学生的积极心理健康,自我调节疲劳在内卷感知和积极心理健康之间起中介作用,... 详细信息

采用问卷调查法,通过5个月两阶段的纵向追踪探讨了627名中国大学生内卷感知对其积极心理健康的影响以及内在机制和边界条件。研究结果表明,内卷感知负向预测大学生的积极心理健康,自我调节疲劳在内卷感知和积极心理健康之间起中介作用,且自我调节疲劳和积极心理健康存在相互预测作用;自我概念清晰性调节了内卷感知对自我调节疲劳和积极心理健康的作用。为高等教育内卷现象中大学生心理健康的干预提供了理论依据,强调了大学生群体积极应对内卷压力、发展清晰的自我概念和保护自我调节资源的重要性。

关键词：大学生内卷感知自我调节疲劳积极心理健康自我概念清晰性

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