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Humic acid-mediated transport of a typical soil passivation remediation product(chloropyromorphite)in saturated porous media

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Journal of Environmental Sciences 2024年第7期141卷 51-62页

作者： xinying Li Mengjia Zhang Siyuan Li Wei Wei School of Environment Jiangsu Engineering Lab of Water and Soil Eco-remediationJiangsu Province Engineering Research Center of Environmental Risk Prevention and Emergency Response TechnologyNanjing Normal UniversityNanjing 210023China Jiangsu Center for Collaborative Innovation in Geographical Information Resource Development and Application Nanjing 210023China

Conversion of labile Pb species into chloropyromorphite(CPY)using phosphorus-bearing amendments was considered to be an ideal strategy in soil passivation ***,the fate and transport of CPY in the soil are poorly *** study aims to fill the knowledge gap by evaluating the fate and transport of CPY under environmentally relevant conditions of humic acid(HA),pH,electrolyte concentration,and species through the saturated sandy *** showed that bare CPY colloids are basically immobile in sandy porous media while the co-existence of HA made the transport of CPY improved by30%-93.5%.Facilitated transport of CPY was attributed to the increased stability of CPY and the repulsive interaction between CPY particles and sands due to HA *** mobility of CPY was also increased with increasing pH from 5.0 to *** the pH was 9 with a10 mmol/L NaCl background solution,the stronger energy barrier between CPY and sand led to enhanced transport *** divalent Ca^(2+)had a more dramatic effect than monovalent Na^(+)on the aggregation and sedimentation of CPY colloids due to its effectivescreening of the surface charge of CPY and bridging interaction with CPY ***-LandauVerwey-Overbeek theory and attachment efficiency calculation indicated that high energy barriers were responsible for the high mobility of CPY colloids,while the retention of CPY in sands was mainly caused by secondary energy minimum and physically *** findings of this work can help to evaluate the fate of soil passivation remediation products in natural water and soil.

关键词： Chloropyromorphite DLVO theory Stability Saturated porous medium Transport

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Cigarette Use and Secondhand Smoke Exposure Among Secondary School Students—China,2023

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China CDC weekly 2024年第22期6卷 509-515页

作者： xinying Zeng Shiwei Liu Lin Xiao Tobacco Control Office Chinese Center for Disease Control and PreventionBeijingChina

What is already known about this topic?In 2021,the prevalence of experimental and current cigarette use among secondary school students in China stood at 16.7%and 4.7%,***,39.9%of these students were exposed to secondhand smoke at *** is added by this report?In comparison to 2021,the prevalence of current cigarette use remained unchanged at 4.2%in 2023,whereas experimental use declined to 13.7%.Notably,rates were significantly higher among vocational senior high school(VSHS)students relative to their peers in senior high school(SHS)and junior high school(JHS).Furthermore,exposure to secondhand smoke in schools decreased to 35.4%in 2023 from previously recorded levels,with more pronounced reductions observed in JHS and SHS populations and no notable change among VSHS *** are the implications for public health practice?Targeted tobacco control policies are imperative for secondary school students,including the establishment of smoke-free school ***,it is crucial to pay close attention to the needs of VSHS students.

关键词： smoke unchanged senior

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Wood use and forest management by Neolithic millet farmers at the Xinglong site,northern China

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Science China Earth Sciences 2024年第6期67卷 1910-1921页

作者： Hui SHEN Zhenwei QIU Keliang ZHAO xinying ZHOU Xiaoqiang LI Key Laboratory of Vertebrate Evolution and Human Origins Institute of Vertebrate Paleontology and PaleoanthropologyChinese Academy of SciencesBeijing 100044China National Museum of China Beijing 100006China University of Chinese Academy of Sciences Beijing 100049China

The origin and development of agriculture and its relationship with climate change are hotly debated topics among environmental *** this study,we analyzed wood charcoal materials from the Neolithic Xinglong site in northern China in order to understand the woody vegetation around the site and how early millet farmers shaped local *** results suggest that the area around the Xinglong sites during 8700-7000 yr BP was primarily woodlands,including Prunus sibirica shrubs,Ulmus and Acer forests,and Populus stands near *** 8000 to 7000 yr BP,the warm and humid climate probably contributed to the expansion of Acer,Rhamnus,and Juniperus,and may have facilitated the development of early millet *** these ancient wood fragments that we studied,the high percent of Prunus charcoal appears to indicate an abundance of fruit trees,which might have constituted the main component of local ***,the wood taxa illustrate the existence of a variety of ecological habitats,and it is logical to assume that people made full use of the locally available wood ***,Populus and Ulmus were the dominant sources of *** results of tree-ring curvature analyses indicate that people mainly collected trunks or large branches of Ulmus,Populus,Acer,and Juniperus *** interpret the increasing use of Prunus twigs and the declining percentage of Prunus charcoal in the period between 8000-7000 yr BP as indicating that people started to protect and manage wild fruit *** may have started pruning to acquire more food resources as part of the cultural responses and adaptation strategies employed by these early millet cultivators.

关键词： Xinglong site Wood charcoal Wood use Woodland management

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The Trend of Smoking-Related Cognition and Its Association with Smoking Behaviors Among Junior High School Students—China,2013–2021

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China CDC weekly 2024年第22期6卷 503-508页

作者： Wenzhao Liu xinying Zeng Qi Su Lin Xiao Shiwei Liu Tobacco Control Office Chinese Center for Disease Control and PreventionBeijingChina

What is already known about this topic?In 2013,31.61%of students perceived quitting smoking as difficult,61.73%considered smoking less attractive,and 73.89%believed that secondhand smoke is definitely harmful to *** is added by this report?The percentage of students who perceived quitting smoking as difficult increased from 31.61%in 2013 to 38.83%in 2021,while the percentage of students who found smoking less attractive rose from 61.73%to 69.40%.Conversely,there was a decrease in the percentage of students who perceived secondhand smoke as harmful,from 73.89%to 68.46%.An increased awareness of the hazards of secondhand smoke was associated with a reduction in smoking *** are the implications for public health practice?It is imperative to enhance health education efforts that aim to raise awareness of the hazards of secondhand smoke.

关键词： smoke attractive Junior

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Cobalt-Catalyzed Switchable[4+1]and[4+1+1]Spirocyclization of Aromatic Amides with 2-Diazo-1H-indene-1,3(2H)-dione:Access to Spiro Indene-2,1'-isoindolinones and Spiro Isochroman-3,1'-isoindolinones

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Chinese Journal of Chemistry 2024年第4期42卷 363-369页

作者： Bin Li Mengmeng Xie Jingyu Li Nana Shen xinying Zhang Xuesen Fan State Key Laboratory of Antiviral Drugs Pingyuan LaboratoryKey Laboratory of Green Chemical Media and ReactionsKey Laboratory for Yellow River and Huai River Water Environmental Pollution ControlMinistry of EducationSchool of EnvironmentSchool of Chemistry and Chemical EngineeringHenan Normal UniversityXinxiangHenan453007 China

Herein,we report a condition-controlled divergent synthesis of spiro indene-2,1'-isoindolinones and spiro isochroman-3,1'-isoindolinones through cobalt-catalyzed formal[4+1]and[4+1+1]spirocyclization of aromatic amides with 2-diazo-1H-indene-1,3(2H)-*** the reaction is carried out under air in ethyl acetate,spiro indene-2,1'-isoindolinones are formed through Co(II)-catalyzed C—H/N—H[4+1]*** the reaction is run under O2 in CH3CN,on the other hand,spiro isochroman-3,1'-isoindolinones are generated through Baeyer-Villiger oxidation of the in situ formed spiro indene-2,1'-isoindolinones with O2 as a cheaper and environmental-friendly oxygen *** general,these protocols have advantages such as using non-precious and earth-abundant metal catalyst,no extra additive,high efficiency and regioselectivity.A gram-scale synthesis and the removal of the directing group further highlight its utility.

关键词： Spiro indene-2,1'-isoindolinones Spiro isochroman-3,1'-isoindolinones 3d Transition metals Cobalt-catalyzed C-H Activation Switchable[4+1]and[4+1+1]spirocyclization Aromatic amides 2-Diazo-1H-indene-1,3(2H)-dione

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Hierarchical Game Approach for Optimization of Regional Integrated Energy System Clusters Considering Bounded Rationality

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 302-313页

作者： Lei Dong Mengting Li Junjie Hu Sheng Chen Tao Zhang xinying Wang Tianjiao Pu school of Electrical and Electronic Engineering North China Electric Power UniversityBeijing 102206China Department of Artificial Intelligence Application Research China Electric Power Research InstituteBeijing 100192China Key Laboratory of Smart Grid of Ministry of Education Key Laboratory of Smart Energy&Information Technology of Tianjin MunicipalityTianjin UniversityTianjin 300072China

Regional integrated energy system(RIES)cluster,i.e.,multi-source integration and multi-region coordination,is an effective approach for increasing energy utilization *** hierarchical architecture and limited information sharing of RIES cluster make it difficult for traditional game theory to accurately describe their game ***,a hierarchical game approach considering bounded rationality is proposed in this paper to balance the interests of optimizing RIES cluster under privacy protection.A Stackelberg game with the cluster operator(CO)as the leader and multiple RIES as followers is developed to simultaneously optimize leader benefit and RIES utilization ***,a slight altruistic function is introduced to simulate the game behavior of each RIES agent on whether to cooperate or *** introducing an evolutionary game based on bounded rationality in the lower layer,the flaw of the assumption that participants are completely rational can be ***,for autonomous optimal dispatching,each RIES is treated as a prosumer,fexibly switching its market participation role to achieve cluster coordination *** studies on a RIES cluster verify effectiveness of the proposed approach.

关键词： Bounded rationality coordinated optimization evolutionary game regionaIilntegrated energysystem stackelberg game

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Synergistic effects of peroxydisulfate on UV/O_(3) process for tetracycline degradation:Mechanism and pathways

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Chinese Chemical Letters 2024年第10期35卷 408-413页

作者： Fengrui Yang Debing Wang xinying Zhang Jie Zhang Zhichao Wu Qiaoying Wang State Key Laboratory of Pollution Control and Resource Reuse Shanghai Institute of Pollution Control and Ecological SecuritySchool of Environmental Science and EngineeringTongji UniversityShanghai 200092China Fujian Provincial Engineering Research Center of Rural Waste Recycling Technology College of Environment&Safety EngineeringFuzhou University.Fuzhou 350108China

Tetracycline(TC)as a typical emerging pollutant is becoming a serious threat to the environment and human health.A combined advanced oxidation technology of UV/Ozone(O_(3))/peroxydisulfate(PDS)process was developed to explore an efficient and economic treatment process of TC in ***,the reactive sites and transformation pathways of TC were explored and the toxicity of the intermediates was quantified with a quantitative structure-activity relationship(QSAR)*** degradation performance of TC was substantially enhanced in UV/O_(3)/PDS process with a kobsof 0.0949 min-1,which was 2.3 times higher than UV/O_(3)and 3.2 times than sole *** results demonstrated that there was a superior synergistic effect of PDS on UV/O_(3)processes for the degradation of *** paramagnetic resonance(EPR)analysis and quenching experiments show that·OH,SO_(4)·-,O_(2)·-and1O_(2)all contributed to TC degradation in the UV/O_(3)/PDS process and exhibited a synergistic effect,which inhibited the generation of harmful *** addition,the UV/O_(3)/PDS system can effectively degrade TC in a wide range of substrate concentrations and pH,and also showed excellent adaptability to various concentrations of anions(Cl-and HCO_(3)-).This study proves the feasibility of UV/O_(3)/PDS process for treating TC contaminated wastewater with complicated water matrix.

关键词： UV/ozonation/peroxydisulfate Synergistic effect Tetracycline Degradation Wastewater

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Voltage-dependent P-Q Reserve Capacity Evaluation for TSO-DSO Interface Considering Uncertainties of DGs and FLs

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CSEE Journal of Power and Energy Systems 2024年第5期10卷 1935-1954页

作者： Yeyan Xu Liangzhong Yao Tianjiao Pu Siyang Liao Fan Cheng Ye Li xinying Wang School of Electrical Engineering and Automation Wuhan UniversityWuhan 430072China China Electric Power Research Institute Beijing 100085China. China Electric Power Research Institute Beijing 100192China.

Increasing distributed generators(DGs)and flexible loads(FLs)enable distribution systems to provide both active and reactive power reserves(P-Q reserves)in supporting the frequency and voltage regulations of transmission ***,such requirements at the interface between the transmission system operator(TSO)and distribution system operator(DSO)affect the distribution system operation security,considering the uncertainties of DGs and *** exploit the reserve potential of distribution systems,this paper investigates the voltagedependent P-Q reserve capacity(V-PQRC)of such types of distribution systems.V-PQRC reflects the feasible space of PQ reserves that the DSO can provide to the TSO taking the voltage deviation limit at TSO-DSO interface into consideration,while ensuring the distribution system operation security under uncertainties of DGs and *** evaluation method for VPQRC at the TSO-DSO interface is *** improve the robust performance of the evaluation method,the DG uncertainty is captured by a generalized ambiguity set and the FL uncertainty is addressed by designing a constrained sliding mode controller(CSMC).Three objectives are considered in the evaluation,i.e.,P reserve capacity,Q reserve capacity,and the voltage deviation limit at the TSO-DSO ***,a multiobjective optimization model integrating the generalized robust chance-constrained optimization and CSMC(GRCC-CSMC)is established for V-PQRC evaluation to obtain the Pareto optimal reserve ***,a non-approximated selecting(NAS)method is proposed to build up a simplified V-PQRC linear model,which can be convenient to apply in the transmissiondistribution system *** results reveal that the V-PQRC evaluation method can achieve a good performance of accuracy and robustness against uncertainties.

关键词： Generalized robust chance-constrained optimization reserve capacity evaluation sliding mode control transmission-distribution system coordination voltage-dependent P-Q reserve capacity

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Analyzing and engineering of the biosynthetic pathway of mollemycin A for enhancing its production

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Synthetic and Systems Biotechnology 2024年第3期9卷 445-452页

作者： Shixue Jin Huixue Chen Jun Zhang Zhi Lin Xudong Qu xinying Jia Chun Lei School of Pharmacy Fudan UniversityShanghai201203China State Key Laboratory of Microbial Metabolism and School of Life Sciences and Biotechnology Shanghai Jiao Tong UniversityShanghai200240China Australian Institute for Bioengineering and Nanotechnology The University of QueenslandSt LuciaQLD4072Australia Department of Biochemistry National University of Singapore14 Medical DrSingapore117599

Mollemycin A(MOMA)is a unique glyco-hexadepsipeptide-polyketide that was isolated from a Streptomyces *** from the Australian marine *** exhibits remarkable inhibitory activity against both drug-sensitive and multidrug-resistant malaria *** MOMA through structural modifications or product enhancements is necessary for the development of effective ***,modifying MOMA using chemical approaches is challenging,and the production titer of MOMA in the wild-type strain is *** study identified and characterized the biosynthetic gene cluster of MOMA for the first time,proposed its complex biosynthetic pathway,and achieved an effective two-pronged enhancement of MOMA *** fermentation medium was optimized to increase the yield of MOMA from 0.9 mg L^(-1)to 1.3 mg L^(-1),a 44%***,a synergistic mutant strain was developed by deleting the momB3 gene and overexpressing momB2,resulting in a 2.6-fold increase from 1.3 mg L^(-1)to 3.4 mg L^(-1).These findings pave the way for investigating the biosynthetic mechanism of MOMA,creating opportunities to produce a wide range of MOMA analogues,and developing an efficient strain for the sustainable and economical production of MOMA and its analogues.

关键词： Mollemycin A Gene cluster Biosynthetic pathway Biosynthetic engineering Production enhancement Azinothricin

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Composition optimization and performance prediction for ultra-stable water-based aerosol based on thermodynamic entropy theory

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Defence Technology（防务技术） 2024年第3期33卷 437-446页

作者： Tingting Kang Canjun Yan xinying Zhao Jingru Zhao Zixin Liu Chenggong Ju Xinyue Zhang Yun Zhang Yan Wu College of Chemical Engineering and Materials Science Tianjin University of Science and TechnologyNo.29 13th AvenueEconomic and Technologic Development ZoneTianjin 300457China Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization Tianjin University of Science and TechnologyTianjin 300457China College of Meteorology and Oceanography National University of Defense TechnologyChangsha 410073China

Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and ***,the stability of the water-based aerosol is always unsatisfactory due to the rapid evaporation and sedimentation of the aerosol *** efforts have been devoted to improve the stability of water-based aerosol by using additives with different composition and ***,the lack of the criterion and principle for screening the effective additives results in excessive experimental time consumption and *** the stabilization time of the aerosol is still only 30 min,which could not meet the requirements of the perdurable ***,to improve the stability of water-based aerosol and optimize the complex formulation efficiently,a theoretical calculation method based on thermodynamic entropy theory is *** the factors that influence the shielding effect,including polyol,stabilizer,propellant,water and cosolvent,are considered within *** ultra-stable water-based aerosol with long duration over 120 min is obtained with the optimal fogging agent composition,providing enough time for fighting the electro-optic *** design guideline for choosing the additives with high phase transition temperature and low phase transition enthalpy is also proposed,which greatly improves the total entropy change and reduce the absolute entropy change of the aerosol cooling process,and gives rise to an enhanced stability of the water-based *** theoretical calculation methodology contributes to an abstemious time and space for sieving the water-based aerosol with desirable performance and stability,and provides the powerful guarantee to the homeland security.

关键词： Ultra-stable Water-based aerosol Thermodynamic entropy Composition optimization Performance prediction

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