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Edge and lithium concentration effects on intercalation kinetics for graphite anodes

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Journal of Energy Chemistry 2024年第3期90卷 337-347,I0009页

作者： Keming zhu Denis Kramer Chao Peng School of Mechanical and Precision Instrument Engineering Xi'an University of TechnologyXi'an 710048ShanxiChina Faculty of Mechanical Engineering Helmut-Schmidt UniversityHamburg 22043Germany School of Engineering University of SouthamptonSouthampton SO171BJUK Multiscale Crystal Materials Research Center Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina

Graphite interfaces are an important part of the anode in lithium-ion batteries(LIBs),significantly influencing Li intercalation *** anodes adopt different stacking sequences depending on the concentration of the intercalated Li *** this work,we performed first-principles calculations to comprehensively address the energetics and dynamics of Li intercalation and Li vacancy diffusion near the no n-basal edges of graphite,namely the armchair and zigzag-edges,at high Li *** find that surface effects persist in stage-Ⅱ that bind Li strongly at the edge ***,the pronounced effect previously identified at the zigzag edge of pristine graphite is reduced in LiC_(12),penetrating only to the subsurface site,and eventually disappearing in LiC_(6).Consequently,the distinctive surface state at the zigzag edge significantly impacts and restrains the charging rate at the initial lithiation of graphite anodes,whilst diminishes with an increasing degree of *** diffusion time for Li hopping to the bulk site from either the zigzag edge or the armchair edge in LiC_(6) was observed during high state of charge due to charge *** controlling Li occupation and diffusion kinetics at this stage is also crucial for enhancing the charge rate.

关键词： Graphite anode Edge Interface Lithium-ion batteries Density functional theory

Morphology of impact fragmentation distribution of single spherical and ellipsoidal particles in drop weight experiments

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Particuology 2024年第3期86卷 137-148页

作者： Qiuhua Miao Peng Huang Wenchang zhu School of Mechanical Engineering Southeast UniversityNanjing211189China

Particle shape is an important factor affecting the fragmentation distribution of the ore *** investigate the influence of particle shape on the morphological fragmentation distribution characteristics,the crushable ore particles are defined as prolate,oblate ellipsoid and spherical particles,which have different aspect ratios(AR)and sphericity(S).Based on the drop weight experiment,the influence of the net drop height on the macroscopic mechanical behavior and crushing distribution characteristics of the single spherical and ellipsoidal particles is *** results show that different peak-shifting characteristics exist during particle *** fragmentation distribution peak shifts left when the increased impact energy is eventually only enough to break medium-sized ***,it shifts right when impact energy is increased enough to break largest-sized ***,regardless of whether the net drop height changes,the maximum continuous fragmentation degree presents"M"-shaped characteristic with the increased *** with the ellipsoid particles,the single spherical particle is more difficult to be broken by impact,with wider equivalent particle fragmentation *** the increase of particle sphericity,the maximum continuous fragmentation degree of a single ellipsoid particle has an overall trend of initial increase and subsequent *** when particle sphericity is 0.9

关键词： Ellipsoid particles Fragmentation distribution Drop weight experiment Numerical simulation

Distributed Least Squares Algorithm of Continuous-Time Stochastic Regression Model Based on Sampled Data

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Journal of Systems Science & Complexity 2024年第2期37卷 609-628页

作者： zhu Xinghua GAN Die LIU Zhixin The Key Laboratory of Systems and Control Academy of Mathematics and Systems ScienceChinese Academy of Sciencesand School of Mathematical SciencesUniversity of Chinese Academy of SciencesBeijing 100190China Zhongguancun Laboratory Beijing 100094China

In this paper,the authors consider the distributed adaptive identification problem over sensor networks using sampled data,where the dynamics of each sensor is described by a stochastic differential *** minimizing a local objective function at sampling time instants,the authors propose an online distributed least squares algorithm based on sampled data.A cooperative non-persistent excitation condition is introduced,under which the convergence results of the proposed algorithm are established by properly choosing the sampling time *** upper bound on the accumulative regret of the adaptive predictor can also be ***,the authors demonstrate the cooperative effect of multiple sensors in the estimation of unknown parameters by computer simulations.

关键词： Cooperative excitation condition distributed least squares regret sampled data stochastic differential equation

Compositional evolution for mixed aerosols containing gluconic acid and typical nitrate and the effect of multiply factors on hygroscopicity

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Journal of Environmental Sciences 2024年第5期139卷 206-216页

作者： Yue zhu Shufeng Pang Yunhong Zhang School of Chemistry and Chemical Engineering Beijing Institute of TechnologyBeijing 100081China

The aging process of atmospheric aerosols usually leads to a mixture of inorganic salts and organic compounds of anthropogenic *** organic compounds,polyhydroxy organic acids are important components,however,the study on composition and hygroscopic properties of the mixture containing inorganics and polyhydroxy organic acids is *** this study,gluconic acid,the proxy of polyhydroxy organic acids,is mixed with the representative nitrate(Mg(NO_(3))_(2),Ca(NO_(3))_(2))to form ***-FTIR and optical microscopy are employed to study the component changes and hygroscopicity as a function of relative *** relative humidity fluctuates,the FTIR-ATR spectra display that the internal mixed gluconic acid(CH_(2)(CH)_(4)(OH)_(5)COOH)and nitrate can react to release acidic gases,forming relevant gluconate and further affecting the *** specific presentation is particles cannot be recovered to their original size after the dehydration-hydration process and there will be some disparities in GF for mixed *** the gluconic acid-Ca(NO_(3))_(2)/Mg(NO_(3))_(2)mixtures with molar ratios of 1:1,higher degree of reaction resulting in the production of large amounts of gluconate should be responsible to the lower hygroscopicity compared to ZSR *** 1:2 gluconic acid-nitrate mixed systems(with higher nitrate content),the hygroscopicity of mixtures are higher than the ZSR prediction.A possible reason could be‘salt-promoting effect’on the organic fractions of the surplus inorganic salt in the *** data can improve the chemical composition list evaluation,in turn hygroscopic properties and phase state of atmospheric aerosol,and then the climate effect.

关键词： Hygroscopicity Gluconic acid Reaction ZSR simulation Size growth factors

Measuring Financial Systemic Risk:Net Liability Clearing Mechanism and Contagion Effect

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Journal of Systems Science & Complexity 2024年第3期37卷 1114-1146页

作者： MA Jiali zhu Shushang LI Duan College of Big Data Statistics Guizhou University of Finance and EconomicsGuiyang 550025China School of Business Sun Yat-Sen UniversityGuangzhou 510275China School of Data Science City University of Hong KongHong Kong 999077China

Following the framework of E-N model(Eisenberg and Noe,2001),the authors consider a new clearing mechanism based on net liabilities among financial institutions since the liabilities between the counterparties should be deducted accordingly when clearing in *** the basis for systemic risk measurement,similar to the original E-N model,the authors first establish some good properties for the clearing payment vector according to a more general ***,the authors investigate how risk spreads among institutions through the liability network forming the risk contagion ***,the authors illustrate with a specific example that the original E-N clearing mechanism may misidentify the systemic important institutions,and theoretically show that it may also overestimate the risk compared with the netting clearing mechanism.

关键词： Clearing mechanism contagion net liability network systemic risk

Analysis and Design of Time-Delay Impulsive Systems Subject to Actuator Saturation

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IEEE/CAA Journal of Automatica Sinica 2024年第1期11卷 196-204页

作者： Chenhong zhu Xiuping Han Xiaodi Li IEEE the School of Mathematics and Statistics Shandong Normal UniversityJi'nan 250014China the Center for Control and Engineering Computation Shandong Normal UniversityJi'nan 250014China

This paper investigates the exponential stability and performance analysis of nonlinear time-delay impulsive systems subject to actuator saturation. When continuous dynamics is unstable, under some conditions, it is shown that the system can be stabilized by a class of saturated delayed-impulses regardless of the length of input delays. Conversely, when the system is originally stable, it is shown that under some conditions, the system is robust with respect to sufficient small delayed-impulses. Moreover, the design problem of the controller with the goal of obtaining a maximized estimate of the domain of attraction is formulated via a convex optimization problem. Three examples are provided to demonstrate the validity of the main results.

关键词： Delayed impulses impulsive control impulsive disturbance nonlinear systems saturation

C@Ag core‒shell structure as lubricating additives towards high efficient lubrication

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Friction 2024年第9期12卷 1991-2003页

作者： Dong AO Xiaoqiang FAN Minhao zhu Key Laboratory of Advanced Technologies of Materials(Ministry of Education) School of Materials Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China Tribology Research Institute School of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China

Efficient cooperative lubrication can be achieved via the introduction of core‒shell structure lubricant additives with hard core and soft shell,for obtaining the expected anti-wear performance from the structural changes in the friction *** this study,C@Ag microspheres with a core‒shell structure were prepared by the redox method with carbon spheres as the core and Ag nanoparticles as the *** tribological behaviors as base oil(G1830)additive with different concentrations were investigated in *** with base oil,the addition of C@Ag particles at 0.5 wt%can reduce the coefficient of friction(COF)and wear volume(Wv)up to 15.5%and 88%,*** importantly,C@Ag particles provide superior lubrication performance to single additive(like carbon sphere(CS)and Ag nanoparticle).C@Ag core‒shell particles contribute to the formation of tribo-film by melt bonding of flexible Ag and carbon sphere(CS)toward excellent self-repair performance and high-efficiency ***,core‒shell structural nanoparticles with hard-core and soft-shell hold bright future for high-performance lubrication application.

关键词： C@Ag microspheres tribo-film self-repair performance high-efficiency lubrication

A physics-informed deep learning framework for spacecraft pursuit-evasion task assessment

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Chinese Journal of Aeronautics 2024年第5期37卷 363-376页

作者： Fuyunxiang YANG Leping YANG Yanwei zhu College of Aerospace Science and Engineering National University of Defense TechnologyChangsha 410073China

Qualitative spacecraft pursuit-evasion problem which focuses on feasibility is rarely studied because of high-dimensional dynamics,intractable terminal constraints and heavy computational *** this paper,A physics-informed framework is proposed for the problem,providing an intuitive method for spacecraft threat relationship determination,situation assessment,mission feasibility analysis and orbital game rules *** the first time,situation adjustment suggestions can be provided for the weak player in orbital ***,a dimension-reduction dynamics is derived in the line-of-sight rotation coordinate system and the qualitative model is determined,reducing complexity and avoiding the difficulty of target set presentation caused by individual ***,the Backwards Reachable Set(BRS)of the target set is used for state space partition and capture zone ***-time analysis can eliminate the influence of changeable initial state and enable the proposed framework to analyze plural situations ***,a time-dependent Hamilton-Jacobi-Isaacs(HJI)Partial Differential Equation(PDE)is established to describe BRS evolution driven by dimension-reduction dynamics,based on level set ***,Physics-Informed Neural Networks(PINNs)are extended to HJI PDE final value problem,supporting orbital game rules summarization through capture zone evolution ***,numerical results demonstrate the feasibility and efficiency of the proposed framework.

关键词： Spacecraft pursuit-evasion Qualitative differential game Physics-Informed Neural Networks(PINNs) Reachability analysis Hamilton-Jacobi-Isaacs(HJI) Partial Differential Equations(PDEs)

Optimal Operation Strategy Analysis with Scenario Generation Method Based on Principal Component Analysis,Density Canopy,and K-medoids for Integrated Energy Systems

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Journal of Modern Power Systems and Clean Energy 2024年第1期12卷 89-100页

作者： Bingtuan Gao Yunyu zhu Yuanmei Li School of Electrical Engineering Southeast UniversityNanjingChina

The operation of integrated energy systems(IESs)is confronted with great challenges for increasing penetration rate of renewable energy and growing complexity of energy *** generation is one of ordinary methods to alleviate the system uncertainties by extracting several typical scenarios to represent the original high-dimensional *** paper proposes a novel representative scenario generation method based on the feature extraction of panel *** original high-dimensional data are represented by an aggregated indicator matrix using principal component analysis to preserve temporal ***,the aggregated indicator matrix is clustered by an algorithm combining density canopy and *** with the proposed scenario generation method,an optimal operation model of IES is established,where the objective is to minimize the annual operation costs considering carbon trading ***,case studies based on the data of Aachen,Germany in 2019 are *** results indicate that the adjusted rand index(ARI)and silhouette coefficient(SC)of the proposed method are 0.6153 and 0.6770,respectively,both higher than the traditional methods,namely K-medoids,K-means++,and density-based spatial clustering of applications with noise(DBSCAN),which means the proposed method has better *** error between optimal operation results of the IES obtained by the proposed method and all-year time series benchmark value is 0.1%,while the calculation time is reduced from 11029 s to 188 s,which verifies that the proposed method can be used to optimize operation strategy of IES with high efficiency without loss of accuracy.

关键词： Scenario generation principal component analysis(PCA) density canopy K-medoids integrated energy system