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Chinese Chemical Letters 2024年第1期35卷 533-536页

作者： Mengjia Luo Xiaohui Li xingxing jiang Zheshuai Lin Zhengyang Zhou Nanchang Key Laboratory of Photoelectric Conversion and Energy Storage Materials Nanchang Institute of TechnologyNanchang 330099China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050China Functional Crystals Lab Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China Institute of Experimental Physics Free University BerlinBerlin D-14195Germany

It is challenging to cooperatively improve the nonlinear optical(NLO)efficiency and the laser-induced damage threshold(LIDT).This work reports a novel IR NLO materials CsInP_(2)S_(7)(CIPS)designed by combination the strategies of alkali metals substitution and microscopic NLO units PS4 introduction based on AgGaS_(2).CIPS was composed of strongly distorted[InS_(6)]^(9-)octahedra and[P_(2)S_(7)]4-dimers constructed by corner-sharing[PS_(4)]^(3-),which increase the NLO efficiency and decrease thermal expansion anisotropy simultaneously.Compared with AgGaS_(2),CIPS exhibited strong phase matchable NLO response ca.1.1×AGS@2.1μm,high LIDT ca.20.8×AgGaS_(2),and IR transparency up to 15.3μm.Structural analysis and theoretical investigation confirmed that large SHG effect and ultrahigh LIDT of CIPS originated from the synergistic contribution of[InS_(6)]^(9-)octahedra and[P_(2)S_(7)]4-dimers.These results indicate that CIPS is a promising NLO candidate in the mid-IR region,and this study provides a new approach for developing potential NLO-LIDT compatible materials.

关键词： Infrared nonlinear optics materials A novel thiophosphate Structure design Structure-activity relationship High laser-induced damage threshold

Improved Multi-Bandwidth Mode Manifold for Enhanced Bearing Fault Diagnosis

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Chinese Journal of Mechanical Engineering 2022年第1期35卷 179-191页

作者： Guifu Du Tao jiang Jun Wang xingxing jiang Zhongkui Zhu School of Rail Transportation Soochow UniversitySuzhou 215131China

Variational mode decomposition(VMD) has been proved to be useful for extraction of fault-induced transients of rolling bearings. Multi-bandwidth mode manifold(Triple M, TM) is one variation of the VMD, which units multiple fault-related modes with different bandwidths by a nonlinear manifold learning algorithm named local tangent space alignment(LTSA). The merit of the TM method is that the bearing fault-induced transients extracted contain low level of in-band noise without optimization of the VMD parameters. However, the determination of the neighborhood size of the LTSA is time-consuming, and the extracted fault-induced transients may have the problem of asymmetry in the up-and-down direction. This paper aims to improve the efficiency and waveform symmetry of the TM method.Specifically, the multi-bandwidth modes consisting of the fault-related modes with different bandwidths are first obtained by repeating the recycling VMD(RVMD) method with different bandwidth balance parameters. Then, the LTSA algorithm is performed on the multi-bandwidth modes to extract their inherent manifold structure, in which the natural nearest neighbor(Triple N, TN) algorithm is adopted to efficiently and reasonably select the neighbors of each data point in the multi-bandwidth modes. Finally, a weight-based feature compensation strategy is designed to synthesize the low-dimensional manifold features to alleviate the asymmetry problem, resulting in a symmetric TM feature that can represent the real fault transient components. The major contribution of the improved TM method for bearing fault diagnosis is that the pure fault-induced transients are extracted efficiently and are symmetrical as the real. One simulation analysis and two experimental applications in bearing fault diagnosis validate the enhanced performance of the improved TM method over the traditional methods. This research proposes a bearing fault diagnosis method which has the advantages of high efficiency, good waveform symmetry and enhanced in-band noise removal capab

关键词： Variational mode decomposition Manifold learning Natural nearest neighbor algorithm Rolling bearing Fault diagnosis Time-frequency signal decomposition

Unexpected giant negative area compressibility in palladium diselenide

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National Science Review 2023年第9期10卷 146-153页

作者： xingxing jiang Shengzi Zhang Dequan jiang Yonggang Wang Maxim S.Molokeev Naizheng Wang Youquan Liu Xingyu Zhang Zheshuai Lin New Functional Crystals Group Key Laboratory of Functional Crystals and Laser TechnologyTechnical Institute of Physics and ChemistryChinese Academy of Sciences 2. Center of Materials Science and Optoelectronics EngineeringUniversity of Chinese Academy of Sciences University of Chinese Academy of Sciences Center for High Pressure Science &Technology Advanced Research School of Materials Science and Engineering Peking University Laboratory of Crystal Physics Kirensky Institute of PhysicsSB RAS 7. Department of Physics Far Eastern State Transport University 8. International Research Center of Spectroscopy and Quantum ChemistrySiberian Federal University

Negative area compressibility(NAC) is a counterintuitive ’squeeze-expand’ behavior in solids that is very rare but attractive due to possible pressure-response applications and coupling with rich physicochemical properties.Herein,NAC behavior is reported in palladium diselenide with a large magnitude and wide pressure range.We discover that,apart from the rigid flattening of layers that has been generally recognized,the unexpected giant NAC effect in PdSe2largely comes from anomalous elongation of intralayer chemical bonds.Both structural variations are driven by intralayer-to-interlayer charge transfer with enhanced interlayer interactions under pressure.Our work updates the mechanical understanding of this anomaly and establishes a new guideline to explore novel compression-induced properties.

关键词： negative area compressibility Lifshitz mechanism charge transfer

Remediation of arsenic-contaminated paddy field by a new iron oxidizing strain(Ochrobactrum sp.)and iron-modified biochar

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Journal of Environmental Sciences 2022年第5期34卷 411-421页

作者： Kaikai Wu Chuan Wu xingxing jiang Rui Xue Weisong Pan Wai-Chin Li Xinghua Luo Shengguo Xue School of Metallurgy and Environment Central South UniversityChangsha 410083China Department of Science and Environmental Studies The Education University of Hong KongAdministrative RegionHong KongChina College of Environmental Sciences Sichuan Agricultural UniversityChengdu 611130China College of Bioscience and Biotechnology Hunan Agricultural UniversityChangsha 410125China

Iron-oxidizing strain(FeOB)and iron modified biochars have been shown arsenic(As)reme-diation ability in the environment.However,due to the complicated soil environment,few field experiment has been conducted.The study was conducted to investigate the potential of iron modified biochar(BC-FeOS)and biomineralization by a new found FeOB to remediate As-contaminated paddy field.Compared with the control,the As contents of G_(B)(BC-FeOS),G_(F)(FeOB),G_(FN)(FeOB and nitrogen fertilizer),G_(BF)(BC-FeOS and FeOB)and G_(BFN)(BC-FeOS,FeOB and nitrogen fertilizer)treatments in pore water decreased by 36.53%-80.03%and the microbial richness of iron-oxidizing bacteria in these treatments increased in soils at the rice maturation stage.The concentrations of available As of G_(B),G_(F),G_(FN),G_(BF) and G_(BFN) at the tillering stage were significantly decreased by 10.78%-55.48%.The concentrations of non-specifically absorbed and specifically absorbed As fractions of G_(B),G_(F),G_(FN),G_(BF) and G_(BFN) in soils were decreased and the amorphous and poorly crystalline hydrated Fe and Al oxidebound fraction was increased.Moreover,the As contents of G_(B),G_(F),G_(FN),G_(BF) and G_(BFN) in rice grains were significantly decreased(*P<0.05)and the total As contents of G_(FN),G_(BF) and G_(BFN) were lower than the standard limit of the National Standard for Food Safety(GB 2762-2017).Compared with the other treatments,G_(BFN) showed the greatest potential for the effective remediation of As-contaminated paddy fields.

关键词： Arsenic Iron-modified biochar Iron-oxidizing strain Field experiment

Retrieval and validation of long-term aerosol optical depth from AVHRR data over China

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International Journal of Digital Earth 2022年第1期15卷 1817-1832页

作者： Chunlin Jin Yong Xue xingxing jiang Shuhui Wu Yuxin Sun School of Environment and Spatial Informatics China University of Mining and TechnologyXuzhouPeople’s Republic of China School of Computing and Engineering College of Science and EngineeringUniversity of DerbyDerbyUK

Advanced Very High Resolution Radiometer(AVHRR)onboard National Oceanic and Atmospheric Administration(NOAA)satellites can provide over 40 years of global remote sensing observations,which can be used to retrieve long-term aerosol optical depth(AOD).This is of great significance to the study of global climate change.In this paper,we proposed an algorithm to jointly calculate AOD and land surface properties from AVHRR observations.With assumptions that AOD doesn’t vary in adjacent space and earth surface property doesn’t vary in two days,the algorithm considered non-Lambertian surface reflection based on the shape of bidirectional reflectance distribution function(BRDF shape)and obtained AOD and surface property by optimal estimation(OE)method.The algorithm has been applied to NOAA-7,9,11,14,16,18,and 19 satellites and AVHRR-retrieved AOD with 5×10 km over China(15°–60°N,70°–140°E)has been obtained from 1982 to 2016.Comparisons of AVHRR-retrieved AOD against AErosol RObotic NETwork(AERONET)(in and around China)and China Aerosol Remote Sensing Network(CARSNET)AOD show good consistency with 62.62%points within the uncertainty ofΔτ=±(0.05+0.25τ)and root-mean-square error(RMSE)of 0.26.Further comparison of the monthly mean AOD of multiple AOD datasets in the‘Beijing’,‘Dalanzadgad’,‘NCU_Taiwan’and‘Kanpur’stations shows that the results of the algorithm are stable.The yearly averaged AOD data also has similar agreements with MERRA-2(The Modern-Era Retrospective analysis for Research and Applications,Version 2)and AVHRRDB data(AVHRR‘Deep Blue’aerosol data set).The multi-year mean correlation coefficient is 0.70 and 0.61 and the percentages within the uncertainty are 80.01%and 67.29%compared with MERRA-2 AOD and AVHRRDB AOD respectively.

关键词： Long-term AOD AVHRR joint retrieval BRDF shape

Identification of a natural PLA2 inhibitor from the marine fungus Aspergillus sp.c1 for MAFLD treatment that suppressed lipotoxicity by inhibiting the IRE-1a/XBP-1s axis and JNK signaling

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Acta Pharmaceutica Sinica B 2024年第1期14卷 304-318页

作者： Yong Rao Rui Su Chenyan Wu xingxing Chai Jinjian Li Guanyu Yang Junjie Wu Tingting Fu Zhongping jiang Zhikai Guo Congjun Xu Ling Huang Key Laboratory of Tropical Biological Resources of Ministry of Education School of Pharmaceutical SciencesHainan UniversityHaikou 570200China Hainan Key Laboratory of Tropical Microbe Resources Institute of Tropical Bioscience and BiotechnologyChinese Academy of Tropical Agricultural Sciences&Key Laboratory for Biology and Genetic Resources of Tropical Crops of Hainan ProvinceHainan Institute for Tropical Agricultural ResourcesHaikou 571101China School of Pharmaceutical Sciences Guangdong Provincial Key Laboratory of New Drug Design and EvaluationSun Yat-sen UniversityGuangzhou 510275China Laboratory Animal Center of Guangdong Medical University Dongguan 523808China

Lipotoxicity is a pivotal factor that initiates and exacerbates liver injury and is involved in the development of metabolic-associated fatty liver disease(MAFLD).However,there are few reported lipotoxicity inhibitors.Here,we identified a natural anti-lipotoxicity candidate,HN-001,from the marine fungus Aspergillus sp.C1.HN-001 dose-and time-dependently reversed palmitic acid(PA)-induced hepatocyte death.This protection was associated with IRE-1a-mediated XBP-1 splicing inhibition,which resulted in suppression of XBP-1s nuclear translocation and transcriptional regulation.Knockdown of XBP-1s attenuated lipotoxicity,but no additional ameliorative effect of HN-001 on lipotoxicity was observed in XBP-1s knockdown hepatocytes.Notably,the ER stress and lipotoxicity amelioration was associated with PLA2.Both HN-001 and the PLA2 inhibitor MAFP inhibited PLA2 activity,reduced lysophosphatidylcholine(LPC)level,subsequently ameliorated lipotoxicity.In contrast,overexpression of PLA2 caused exacerbation of lipotoxicity and weakened the anti-lipotoxic effects of HN-001.Additionally,HN-001 treatment suppressed the downstream pro-apoptotic JNK pathway.In vivo,chronic administration of HN-001(i.p.)in mice alleviated all manifestations of MAFLD,including hepatic steatosis,liver injury,inflammation,and fibrogenesis.These effects were correlated with PLA2/IRE-1a/XBP-1s axis and JNK signaling suppression.These data indicate that HN-001 has therapeutic potential for MAFLD because it suppresses lipotoxicity,and provide a natural structural basis for developing anti-MAFLD candidates.

关键词： Lipotoxicity MAFLD ER stress IRE-1a XBP-1s JNK PLA2

Janus heterostructure of cobalt and iron oxide as dual-functional electrocatalysts for overall water splitting

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Nano Research 2023年第2期16卷 2245-2251页

作者： Xiaojie Li Huike Zhang Xuan Li Qi Hu Chen Deng xingxing jiang Hengpan Yang Chuanxin He College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China Institute of Microscale Optoelectronics Shenzhen UniversityShenzhen 518060China

In electrocatalytic water splitting,low-cost dual-functional catalysts can not only reduce costs but also avoid cross-contamination of cathode and anode.However,the orderly aggregation of active sites for hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)into a specific catalyst is very challenging.In this study,a Co/Fe_(3)O_(4)Janus heterojunction supported on carbon fiber paper(J-CoFe-CFP)is designed and successfully synthesized.Generally,Co-Fe oxides have preferable OER activity but weak HER activity.However,in J-CoFe-CFP,due to the intense and special electronic interaction of different substances(Co and Fe3O4)in the Janus heterogeneous interface,a huge number of tidy high-quality HER and OER active sites are uniformly distributed on the interface simultaneously,which endows the catalyst with both excellent HER and OER performance.In HER,the overpotential@10 mA·cm^(−2)(ηHER)is only 53.9 mV,and the Tafel slope is 43.7 mV·dec^(−1).In OER,theηis 272 mV,and the Tafel slope is 50.2 mV·dec^(−1),much lower than those of RuO_(2)/CFP.In the J-CoFe-CFP||J-CoFe-CFP two-electrode system,the required voltage is only 1.26 V at the beginning and 1.56 V@10 mA·cm^(−2),much lower than those of RuO_(2)/CFP||20%Pt/C/CFP.This work provides a Janus heterojunction pathway for bifunctional water electrolysis catalysts.

关键词： Janus bifunctional electrocatalytic water splitting CoFe

A hierarchically structured tin-cobalt composite with an enhanced electronic effect for high-performance CO_(2) electroreduction in a wide potential range

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Journal of Energy Chemistry 2023年第1期76卷 462-469,I0012页

作者： xingxing jiang Xuan Li Yan Kong Chen Deng Xiaojie Li Qi Hu Hengpan Yang Chuanxin He Institute of Microscale Optoelectronics College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060GuangdongChina

Earth-abundant and nontoxic Sn-based materials have been regarded as promising catalysts for the electrochemical conversion of CO_(2)to C1 products,e.g.,CO and formate.However,it is still difficult for Snbased materials to obtain satisfactory performance at low-to-moderate overpotentials.Herein,a simple and facile electrospinning technique is utilized to prepare a composite of a bimetallic Sn-Co oxide/carbon matrix with a hollow nanotube structure(Sn Co-HNT).Sn Co-HNT can maintain>90%faradaic efficiencies for C1 products within a wide potential range from-0.6 VRHE to-1.2 VRHE,and a highest 94.1%selectivity towards CO in an H-type cell.Moreover,a 91.2%faradaic efficiency with a 241.3 m A cm^(-2)partial current density for C1 products could be achieved using a flow cell.According to theoretical calculations,the fusing of Sn/Co oxides on the carbon matrix accelerates electron transfer at the atomic level,causing electron deficiency of Sn centers and reversible variation between Co^(2+)and Co^(3+)centers.The synergistic effect of the Sn/Co composition improves the electron affinity of the catalyst surface,which is conducive to the adsorption and stabilization of key intermediates and eventually increases the catalytic activity in CO_(2)electroreduction.This study could provide a new strategy for the construction of oxide-derived catalysts for CO_(2)electroreduction.

关键词： Hierarchic structure Tin-cobalt bimetallic oxide Electronic effect CO_(2)electroreduction Wide potential range

Synchronous chirp mode extraction: A promising tool for fault diagnosis of rolling element bearings under varying speed conditions

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Chinese Journal of Aeronautics 2022年第1期35卷 348-364页

作者： xingxing jiang Qiang HUANG Changqing SHEN Qian WANG Kun XU Jie LIU Juanjuan SHI Zhongkui ZHU School of Rail Transportation Soochow UniversitySuzhou 215131China Wenzheng College of Soochow University Suzhou 215104China College of Energy and Power Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China Sclool of Hydropower and Infonnation Engineering Huazhong University of Science and TechnologyWuhan 430074China

As critical components in modern aerospace productions,rolling element bearings(REBs)generally work under varying speed conditions,which brings great challenges to their operating health monitoring.Some novel time–frequency decomposition(TFD)algorithms are established recently to extract nonlinear features from the non-stationary signals effectively,which are promising for realizing fault diagnosis of REBs under varying speed conditions.However,numerous personal experiences must be incorporated and the anti-noise performance of these methods needs to be further enhanced.Given these issues,a synchronous chirp mode extraction(SCME)-based REB fault diagnosis method is proposed for the health monitoring of REBs under varying speed conditions in this study.It mainly consists of following two parts.(a)The shaft rotational frequency(SRF)is initially estimated from the low-frequency band of the vibration signal.Simultaneously,an adaptive refining strategy is incorporated to obtain a suitable bandwidth parameter.(b)A cycle-one-step estimation frame is constructed to extract synchronous modes from the envelope waveform of the vibration signal.Meanwhile,a synchronous mode spectrum(SMS)is generated using the information of the extracted synchronous modes,which is a novel REBs fault diagnosis technique with tacholess and resampling-free.In contrast to the current TFD algorithms,the proposed method needs fewer input parameters and owns a well anti-noise performance because there is no iterative optimization in the procedure of construction of SMS.As a result,the health conditions of REBs are evaluated by detecting the exhibited features in the SMS.Simulations and experiments are conducted to validate the effectiveness of the proposed method in terms of REB fault diagnosis.Analysis results demonstrate that the proposed method outperforms the current TFD algorithm and the conventional order tracking technique for fault diagnosis of REB under varying speed conditions.

关键词： Envelope analysis Fault diagnosis Order tracking Rolling element bearing Varying speed

Novel two-dimensional PdSe phase:A puckered material with excellent electronic and optical properties

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Frontiers of physics 2022年第5期17卷 65-73页

作者： Mingyun Huang xingxing jiang Yueshao Zheng Zhengwei Xu Xiong-Xiong Xue Keqiu Chen Yexin Feng Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics&Devices School of Physics and ElectronicsHunan UniversityChangsha 410082China School of Physics and Optoelectronics Xiangtan UniversityXiangtan 411105China

By combining structural search and first-principles calculations,we predict a new stable twodimensional PdSe monolayer,and systematically investigate its structural,electronic and optical properties.The calculated formation enthalpy,phonon spectra and molecular dynamic simulations confirm that PdSe monolayer possesses excellent thermodynamic and dynamic stability.PdSe monolayer is a semiconductor with an indirect band gap of∼1.10 eV.The carrier transport of PdSe monolayer is dominated by hole and exhibits remarkable anisotropy due to the intrinsic structure anisotropy.The optical properties also show obvious anisotropic characteristic with considerable absorption coefficient and broad absorption from the visible to ultraviolet regions.Benefiting from these excellent physical properties,PdSe monolayer is expected to be a promising candidate as electronic and optoelectronic devices.

关键词： first-principles calculation two-dimensional(2D) electronic structure structural search PdSe