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A flexible solid polymer electrolyte enabled with lithiated zeolite for high performance lithium battery

Nano Research 2023年第7期16卷 9443-9452页

作者： Zhiyu Ding Qiming Tang Qi Zhang Penghui Yao Xingjun Liu Junwei Wu Shenzhen Key Laboratory of Advanced Materials Department of Materials Science and EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China Maryland Energy Innovation Institute University of MarylandCollege ParkMD 20742USA Department of Chemical and Metallurgical Engineering Aalto UniversityKemistintie 1Aalto FI-00076Finland

Solid-state lithium batteries using composite polymer electrolytes(CPEs)have attracted much attention owing to their higher safety compared to liquid electrolytes and flexibility compared to ceramic electrolytes.However,their unsatisfactory lithium-ion conductivity still limits their development.Herein,a high ion conductive CPE with multiple continuous lithium pathways is designed.This new electrolyte consists of poly(vinylidene fluorideco-hexafluoropropylene)(PVDF-HFP)and lithiated X type zeolite(Li-X),which possesses a high ionic conductivity(1.98×10^(-4)S/cm),high lithium transference number(t_(Li^(+))=0.55),wide electrochemical window(4.7 V),and excellent stability against the lithium anode.Density functional theory(DFT)calculation confirms that the Lewis acid sites in zeolite can graft with N,N-dimethylformamide(DMF)and PVDF-HFP chains,resulting in decreased crystallinity of polymer and providing rapid Li+transmission channels.When used in a full cell,the solid Li|Li-X-3%|LiFePO_(4) cell displays excellent cycling stability and rate performance at room temperature and 60℃.Furthermore,pouch cells with the Li-X-3%electrolyte exhibit brilliant safety under extreme conditions,such as folding and cutting.Thus,this proposed zeolite-PVDF-HFP CPE represents a promising potential in the application of making a safer,higher performing,and flexible solid-state lithium battery.

关键词： solid-state lithium batteries composite polymer electrolytes zeolite poly(vinylidene fluorideco-hexafluoropropylene)(PVDF-HFP) flexible

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Phase-field simulation on microstructure evolution of D019 phase in γ/γ′structure of Co–Al–W superalloys

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Progress in Natural Science:Materials International 2020年第3期30卷 382-392页

作者： Xingjun Liu Hufan Kong Yong Lu Jianhong Huang Cuiping Wang College of Materials and Fujian Provincial Key Laboratory of Materials Genome Xiamen University Department of Materials Science and Engineering Harbin Institute of Technology Institute of Materials Genome and Big Data Harbin Institute of Technology

The morphological evolution and precipitation kinetics of γ′ and D0(CoW) phase in Co–Al–W alloys at 900 °C have been studied by applying Phase-field method and experiment in order to understand the transformation process of γ′ phase and D0phase. The growth processes of D0phase and precipitation of γ′ phase under elastic fields were simulated through coupling with thermodynamics and dynamics databases. The simulation results indicate that the misfit δ≥ 0.53% has a greater impact on γ′ particle morphology in γ/γ′ structure.Co–Al–W alloy with low Al and high W is one of the factors to promote the precipitation of D0phase. Three stages during aging, namely the γ′ phase incubation stage, the γ′ phase fast nucleation and growth stage, and the transformation from γ′ phase to D0phase stage can be observed with the non-constant coarsening rate that varying with the decrease of γ′ phase. The particle size distribution(PSD) during the precipitation of D0phase is more in line with MLSW theory than LSW theory. This simulation results are in good agreement with the experiment results to help analyze microstructure evolution of Co–Al–W alloy.

关键词： Phase-field Co–Al–W High-temperature alloys Coarsening kinetics

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SA-RSR:a read-optimal data recovery strategy for XOR-coded distributed storage systems

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Frontiers of Information Technology & Electronic Engineering 2022年第6期23卷 858-875页

作者： xingjun ZHANG Ningjing LIANG Yunfei liu Changjiang ZHANG Yang LI School of Computer Science and Technology Xi’an Jiaotong UniversityXi'an 710049China Beijing Electronic Engineering General Research Institute Beijing 100854China

To ensure the reliability and availability of data,redundancy strategies are always required for distributed storage systems.Erasure coding,one of the representative redundancy strategies,has the advantage of low storage overhead,which facilitates its employment in distributed storage systems.Among the various erasure coding schemes,XOR-based erasure codes are becoming popular due to their high computing speed.When a single-node failure occurs in such coding schemes,a process called data recovery takes place to retrieve the failed node’s lost data from surviving nodes.However,data transmission during the data recovery process usually requires a considerable amount of time.Current research has focused mainly on reducing the amount of data needed for data recovery to reduce the time required for data transmission,but it has encountered problems such as significant complexity and local optima.In this paper,we propose a random search recovery algorithm,named SA-RSR,to speed up single-node failure recovery of XOR-based erasure codes.SA-RSR uses a simulated annealing technique to search for an optimal recovery solution that reads and transmits a minimum amount of data.In addition,this search process can be done in polynomial time.We evaluate SA-RSR with a variety of XOR-based erasure codes in simulations and in a real storage system,Ceph.Experimental results in Ceph show that SA-RSR reduces the amount of data required for recovery by up to 30.0%and improves the performance of data recovery by up to 20.36%compared to the conventional recovery method.

关键词： Distributed storage system Data reliability and availability XOR-based erasure codes Single-node failure Data recovery

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Optimization of mechanical properties and corrosion resistance of Zn-0.4Mn-0.8Li alloy using the hot rolling process

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Journal of Materials Science & Technology 2023年第14期145卷 136-147页

作者： Xinxin Yang Peng Du Kun Li Weizong Bao Tao Xiang Jie Chen Xingjun Liu Guoqiang Xie School of Materials Science and Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

Zinc-based degradable metals are considered one of the most promising biodegradable materials due to their moderate corrosion rate,excellent mechanical properties,and good biocompatibility.In this work,biodegradable Zn-0.4Mn-0.8Li alloy was fabricated and rolled in multiple passes at different tem peratures.As the hot rolling temperature increases,the grain size of Zn-0.4Mn-0.8Li alloy was found to increase cor-respondingly.Further,a multi-scale structure with the coexistence of coarse grains and fine grains was obtained.The results demonstrated that the mechanical strength and corrosion resistance were improved by increasing the rolled temperature.It was observed that Zn-0.4Mn-0.8Li alloy with a total reduction of 90%after hot rolling at 325℃ exhibited excellent mechanical and corrosion properties.The cooperation of multi-scale microstructure and twinning was found to improve the strength and guarantee the duc-tility of Zn-0.4Mn-0.8Li alloy significantly so that the 325℃ hot-rolled Zn-0.4Mn-0.8Li alloy has optimal comprehensive properties.Further,yield strength,ultimate tensile strength,and elongation were found to be 449.7±5.3 MPa,505.1±6.5 MPa,and 40.5%±7.5%,respectively.Meanwhile,Zn-0.4Mn-0.8Li al-loy via 325℃ hot-rolled processes also exhibited excellent corrosion resistance.The corrosion current density and corrosion potential were found to be 8.8×10-5 mA cm^(-2)and−0.929 V,respectively.The preliminary study indicates that Zn-0.4Mn-0.8Li alloy is a promising candidate material for medical de-vice applications.

关键词： Zn-based degradable metal Hot rolling Mechanical property Corrosion behavior

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Characterization and modeling studies towards Al_(3)Ti/Mg interfaces in Ti reinforced AZ31 alloys

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Journal of Materials Science & Technology 2023年第16期147卷 197-206页

作者： Longke Bao Shengli Han Shengkun Xi Yuhui Zhang Cuiping Wang Kaihong Zheng Rongpei Shi Xingjun Liu Fusheng Pan State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyShenzhen 518055China College of Materials Science and Engineering and Institute of Materials Genome and Big DataHarbin Institute of TechnologyShenzhen 518055China Institute of New Materials Guangdong Academy of SciencesGuangzhou 510650China College of Materials Science and Engineering Xiamen UniversityXiamen 361005China College of Materials Science and Engineering Chongqing UniversityChongqing 400045China

The interfaces between in-situ Al3Ti particles and magnesium(Mg)matrix are crucial role in highperformance titanium(Ti)reinforced AZ31 alloy.Herein,the interfaces between Al3Ti particles and the Mg matrix are fabricated and investigated using advanced characterization tools and first-principles calculations.The orientation relationship(OR)and atomic interface structure between the Al_(3)Ti particles and matrix are characterized using a high-resolution transmission electron microscope.The OR is determined to be(1010)Mg//(001)Al3Ti;[1213]Mg//[100]Al3Ti.Based on the characterized OR,the interface properties(including atomic structure,work of adhesion,interface energy,and fracture mechanism)are investigated using first-principles calculations.The relaxed interface structure indicates that the TiAl-terminated bridge site configurations(MT1)and hollow site configurations(HCP1)are unstable and would convert into other bridge site configurations(MT).Furthermore,the work of adhesion and interface energy suggests that Al-terminated hollow site configurations(HCP)and bridge site configurations(MT)are more stable than other configurations.In addition,the calculations of work of fracture show that fracture of the interfaces with Al-MT1,Al-HCP,and TiAl-MT configurations may initiate from bulk Mg interior.The findings may help to understand and tailor the deformation mechanisms and mechanical properties of Ti-reinforced Mg alloys.

关键词： Ti/AZ31 alloy Mg/Al_(3)Ti interface HAADF-STEM First-principles computation

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Water-soluble brown carbon in atmospheric aerosols from the resource-dependent cities:Optical properties,chemical compositions and sources

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Journal of Environmental Sciences 2024年第4期138卷 74-87页

作者： Haoji Wang Yue Su Yangzheng liu Fei Xie xingjun Zhou Ruihong Yu Changwei Lü Jiang He School of Ecology and Environment Inner Mongolia UniversityHohhot 010021China Institute of Environmental Geology Inner Mongolia UniversityHohhot 010021China Environmental Monitoring Center of Inner Mongolia Hohhot 010011China

As a vital type of light-absorbing aerosol,brown carbon(BrC)presents inherent associations with atmospheric photochemistry and climate change.However,the understanding of the chemical and optical properties of BrC is limited,especially in some resource-dependent cities with long heating periods in northwest China.This study showed that the annual average abundances of Water-soluble BrC(WS-BrC)were 9.33±7.42 and 8.69±6.29μg/m^(3)in Baotou and Wuhai and the concentrations,absorption coefficient(Abs_(365)),and mass absorption efficiency(MAE365)of WS-BrC presented significant seasonal patterns,with high values in the heating season and low values in the non-heating season;while showing opposite seasonal trends for the Absorption Angstr?m exponent(AAE_(300-400)).Comparatively,the levels of WS-BrC in developing regions(such as cities in Asia)were higher than those in developed regions(such as cities in Europe and Australia),indicating the significant differences in energy consumption in these regions.By combining fluorescence excitation-emission matrix(EEM)spectra with the parallel factor(PARAFAC)model,humic-like(C1 and C2)and proteinlike(C3)substances were identified,and accounted for 61.40%±4.66%and 38.6%±3.78%at Baotou,and 60.33%±6.29%and 39.67%±4.17%at Wuhai,respectively.The results of source apportionment suggested that the potential source regions of WS-BrC varied in heating vs.non-heating seasons and that the properties of WS-BrC significantly depended on primary emissions(e.g.,combustion emissions)and secondary formation.

关键词： Water-soluble brown carbon Atmospheric aerosols Optical properties PARAFAC Source apportionment

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Production evolution patterns and development stage division of waterflooding oilfields

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Petroleum Exploration and Development 2023年第2期50卷 433-441页

作者： JI Bingyu XU Ting GAO xingjun YU Hongmin liu He Sinopec Petroleum Exploration and Production Research Institute Beijing 102206China Research Institute of Petroleum Exploration&Development PetroChinaBeijing 100083China

The continuous growth of recoverable reserves in a waterflooding oilfield has a significant impact on the patterns of production evolution. A new production evolution model is established by improving the Weng Cycle model. With the new model, the statistical correspondence between the production decline stage and the reserve-production imbalance is clarified,and the correlation of water cut with the recovery percent of recoverable reserves is discussed, providing quantitative basis of reservoir engineering for dividing development stages of oilfield and defining mature oilfields. According to the statistics of oilfields in eastern China, the time point corresponding to the reserve-production balance coefficient dropping to less than 1dramatically is well correlated the beginning point of production decline, thus the time when the reserve-production balance coefficient drops dramatically can be taken as the initiation point of production decline stage. The research results show that the water cut and the recovery percent of recoverable reserves have a good statistical match in the high water cut stage, and it is more rational to take both the start point of production decline stage and the water cut of 90%(or the recovery percent of recoverable reserves of 80%) as the critical criteria for defining a mature oilfield. Five production evolution patterns can be summarized as follows: growth–peak plateau–stepped decline, growth–stepped stabilizing–stepped decline, growth–stepped stabilizing–rapid decline, growth–peak plateau–rapid decline, and growth–continuous decline.

关键词： waterflooding oilfield production evolution development stage division recoverable reserves mature oilfield

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One-step synthesis of novel core-shell bimetallic hexacyanoferrate for high performance sodium-storage cathode

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Journal of Materials Science & Technology 2022年第19期114卷 180-190页

作者： Daxian Zuo Cuiping Wang Jiajia Han Qinghao Han Yanan Hu Junwei Wu Huajun Qiu Qian Zhang Xingjun Liu College of Materials and Fujian Key Laboratory of Materials Genome and Xiamen Key Laboratory of High Performance Metals and Materials Xiamen UniversityXiamen 361005China Institute of Materials Genome and Big Data Harbin Institute of TechnologyShenzhen 518055China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyShenzhen 518055China

Recently, the design of core-shell hierarchical architecture plays an important role in improving the electrochemical performance of Prussian blue analogue cathodes(PBAs). Unfortunately, the inconvenient stepwise preparation and the strict lattice-matching requirement have restricted the development of coreshell PBAs. Herein, we demonstrate a one-step synthesis strategy to synthesize core-shell manganese hexacyanoferrate(MnFeHCF@MnFeHCF) for the first time. And the formation mechanism of the core-shell hierarchical architecture is investigated by first-principles calculations. It is found that the as-obtained Mn FeHCF@MnFeHCF act out the superior intrinsic natures, which not only can obtain a larger specific surface area and lower Fe(CN)_(6) vacancies but also can activate more Na-storage sites. Compared with the manganese hexacyanoferrate(MnHCF), the iron hexacyanoferrate(FeHCF), and even the traditional coreshell nickel hexacyanoferrate(FeHCF@NiHCF) prepared by a stepwise method, the Mn Fe HCF@MnFeHCF demonstrates a superior rate performance, which achieves a high capacity of 131 mAh g^(−1) at 50 mA g^(−1) and delivers a considerable discharge capacity of about 100 mAh g^(−1) even at 1600 mA g^(−1). Meantime, the capacity retention can reach up to nearly 80% after 500 cycles. The improved performances could be mainly originated from two aspects: on the one hand, Mn substitution is helpful to enhance the material conductivity;on the other hand, the core-shell structure with matched lattice parameters is more favorable to enhance the diffusion coefficient of sodium ions. Beside, the structural transformation of MnFeHCF@MnFeHCF upon the extraction/insertion of sodium ions is instrumental in releasing the interior stress and effectively maintaining the integrity of the crystal structure.

关键词： Cathode Prussian blue analogue Core-shell structure First-principles calculations Electrochemical performance

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Enhanced spectral splitting in a novel solar spectrum optical splitter based on one dimensional photonic crystal heterostructure

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Journal of Materiomics 2021年第3期7卷 648-655页

作者： Dong Wei Feng Cao Zuoxu Wu Yijie liu Jian Wang Qingmei Wang Xingjun Liu Qian Zhang School of Science and Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information SystemHarbin Institute of TechnologyShenzhenGuangdong518055China Department of Materials Science and Engineering Harbin Institute of TechnologyShenzhenGuangdong518055China

Controlling the distribution of solar spectrum in different bands would boost the energy harvesting efficiency and optimize the energy dispatchability.1D photonic crystal with intrinsic optical band gap can be used to split the solar spectrum for hybrid photovoltaic/thermal solar applications.Here,we designed an efficient solar spectrum optical filter based on a cermet layer,Si/SiO_(2)1D photonic crystal,and top heterostructure layer.Compared with 1D photonic crystal structure,the 1D photonic crystal heterostructure with top YSZ layer can realize the reflectance of greater than 92%in PV band and the low average reflectance in two thermal bands by tuning the effective impedance of multilayer films.The enhanced reflectance in PV band results from the huge mismatching of impedance between free space and the heterostructure structure.The top dielectric layer can also be extended to other oxides.

关键词： Solar spectral splitting 1D photonic crystal heterostructure Solar absorptance Effective impedance

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Novel and durable composite phase change thermal energy storage materials with controllable melting temperature

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Journal of Materials Science & Technology 2021年第27期86卷 11-19页

作者： Haiting Wei Shuiyuan Yang Cuiping Wang Changrui Qiu Kairui Lin Jiajia Han Yong Lu Xingjun Liu College of Materials and Fujian Provincial Key Laboratory of Materials Genome Xiamen UniversityXiamen 361005China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyShenzhen 518055China Institute of Materials Genome and Big Data Harbin Institute of TechnologyShenzhen 518055China Shenzhen R&D Center for Al-based Hydrogen Hydrolysis Materials Shenzhen 518055China

The development of high temperature phase change materials(PCMs)with great comprehensive performance is significant in the future thermal energy storage system.In this study,novel and durable Al-Si/Al_(2)O_(3)-Al N composite PCMs with controllable melting temperature were successfully synthesized by using pristine Al powder as raw material and tetraethyl orthosilicate as SiO_(2)source.The Al_(2)O_(3)shell and Al-Si alloy were in-situ produced via the substitution reaction between molten Al and SiO_(2).Importantly,the crack caused by the incomplete encapsulation of the Al_(2)O_(3)shell could repair itself by the nitridation reaction of internal molten Al and thereby forming a highly dense Al_(2)O_(3)-Al N composite shell.The produced dense Al_(2)O_(3)-Al N composite shell could significantly improve the thermal cycling stability of composite PCMs,and thus,the thermal storage density decrease of the Al-Si/Al_(2)O_(3)-Al N(59.8 J/g to77.7 J/g)was far less than that of the Al-Si/Al_(2)O_(3)(118.5 J/g)after 3000 thermal cycles.Moreover,the synthesized Al-Si/Al_(2)O_(3)-Al N still exhibited a controllable melting temperature(571.5-637.9℃),relatively high thermal storage density(105.6-150.7 J/g),great dimensional stability and structural stability after3000 thermal cycles.Hence,the synthesized Al-Si/Al_(2)O_(3)-Al N composite PCMs,as promising preferential thermal energy storage materials,can be stably used in the energy utilization efficiency improvement of various systems for more than 6 years.

关键词： Al-Si Al_(2)O_(3)-AlN Durable Controllable melting temperature Phase change thermal storage material

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