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The δ^(15)n values of foxtail millet(Setaria italica)and common millet(Panicum miliaceum)are reliable indicators of manuring practices

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Science China Earth Sciences 2024年第9期67卷 2910-2923页

作者： Jishuai yang Xiaoyan yang Ting YOU Fahu CHEn Key Scientific Research Base of Bioarchaeology in Cold and Arid Regions(national Cultural Heritage Administration) Key Laboratory of Western China’s Environmental Systems(Ministry of Education)College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China Group of Alpine Paleoecology and Human Adaptation(ALPHA) State Key Laboratory of Tibetan Plateau Earth SystemResources and Environment(TPESRE)Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China State Key Laboratory of Herbage Improvement and Grassland Agro-ecosystems College of Pastoral Agriculture Science and TechnologyLanzhou UniversityLanzhou 730000China

Millet agriculture,which originated in northern China,alongside rice agriculture,have nurtured the Chinese *** manuring practices likely promoted and maintained sustainable millet agricultural production in the loess area of northern ***,ongoing controversy exists regarding the indicators of prehistoric manuring intensity of foxtail millet(Setaria italica)and common millet(Panicum miliaceum).Here,we present the results of pot and field fertilization experiments on two millet *** findings suggest that manuring can significantly increase the δ^(15)n values of foxtail millet,and its δ^(15)n values increase with increasing manuring *** δ^(15)n values of foxtail millet leaves are systematically greater than those of grains by approximately 1.6‰.Manuring could have a long-term residual impact on increasing the δ^(15)n values of soil and millet *** with previous crop fertilization experiment results,we propose that the impact of manuring on the δ^(15)n values of non-nitrogen-fixing crops is roughly *** δ^(15)n value and amount of manure are key factors determining the extent of change in plant δ^(15)n *** millet grain δ^(15)n values can serve as reliable indicators of manuring ***,we provide an interpretive framework for assessing the correlation between manuring levels and the δ^(15)n values of archaeological millet *** δ^(15)n values of ancient millet grains suggest widespread and intensive manuring practices in prehistoric millet agriculture in northern China,spanning from the early yangshao period to the Longshan period.

关键词： Millet farming Manuring experiment Farming system Archaeobotany north China

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Engineering Cu_(2)O/Cu/n-C interface to induce directional migration of charge for driving photocatalytic homo-coupling of terminal alkynes

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nano Research 2024年第8期17卷 6895-6902页

作者： Xiaoqin Yan Tianyi Xu Wenwen Zhan yang yang yang Yu Jianjian Yi Xiaoxiao He Lei yang Jianwei Zhao Liming Sun Xiguang Han Jiangsu Key Laboratory of Green Synthetic Chemistry for Functional Materials Department of ChemistrySchool of Chemistry&Materials ScienceJiangsu Normal UniversityXuzhou 221116China State Key Laboratory of Precision Spectroscopy East China Normal UniversityShanghai 200241China College of Environmental Science and Engineering Yangzhou UniversityYangzhou 225009China Shenzhen HUASUAn Technology Co. LtdShenzhen 518055China

The efficient utilization of visible light catalysts for organic reactions necessitates not only the effective separation of photogenerated electrons and holes to participate in the reaction,but also their ability to form key intermediates with reactant *** present study successfully synthesized a crusiform-like mesoporous structure of nitrogen-doped carbon-coated Cu_(2)O/Cu(Cu_(2)O/Cu/n-C)with a Cu_(2)O/dual electron acceptor interface using etched HKUST-1 as the precursor.A series of theoretical and experimental studies have demonstrated that the Cu_(2)O/Cu/n-C interface in the photocatalytic homo-coupling of terminal alkynes not only effectively enhances the separation of photogenerated electron−hole pairs,but also facilitates the formation of the key intermediate[Cu_(2)O/Cu/n-C]-phenylacetylide and promotes the rearrangement of its internal *** a result,the homo-coupling reaction can be effectively *** primary reason for the functional role of Cu_(2)O/Cu/n-C interface lies in the downward bending of energy band from Cu_(2)O to n-doped C layers,induced by the different work functions of Cu_(2)O,Cu and n-doped C ***,Cu_(2)O/Cu/n-C photocatalysts demonstrate exceptional photocatalytic activity in the homo-coupling reaction of terminal alkynes under blue-light irradiation and air *** present study presents a novel research methodology for the development of highly efficient visible light catalysts to facilitate organic reactions in future applications.

关键词： photocatalysis homo-coupling of terminal alkynes directional migration of charges heterojunction interface Cu_(2)O carbon coated

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Facile access to C-n bonds via unexpected side reactions of Knoevenagel condensation and their application in high-efficiency organic solar cells

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Science China Chemistry 2024年第1期67卷 323-329页

作者： Daobin yang Shuncheng yang Hongqian Wang Lin Xie Pengyu Yan Ziyi Ge Zhejiang Engineering Research Center for Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China School of Materials Science and Chemical Engineering Ningbo UniversityNingbo 315211China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

The construction of C-n bonds is of great importance in the fields of biology,medicine,chemistry and materials ***,the replacement of organic base from pyridine to piperidine in the Knoevenagel condensation process unexpectedly yields a series of novel organic molecules containing C-n ***,the synthesis method does not require any external transition-metals catalysis,and photo-/***,when the new compound 1b is added as a third component to a well-known binary system of PM6:Y6,the efficiency of the organic solar cell is significantly improved,resulting in an outstanding efficiency of 18.0%,which is one of the highest values reported to date for PM6:Y6-based ternary organic solar cells.

关键词： C-n bonds Knoevenagel condensation cross-coupling reaction third component organic solar cells

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Heterointerface engineering of assembled CoP_(2) on n-modified carbon as efficient trifunctional electrocatalysts for Zn-Air batteries and overall water splitting

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nano Research 2024年第5期17卷 3801-3809页

作者： Yan Chen Zhenrui yang Juan Wang Yun yang Xuedong He yang Wang Jiadong Chen Yaqing Guo Xin Wang Shun Wang Huile Jin Wenzhou Key Lab of Advanced Energy Storage and Conversion Zhejiang Province Key Lab of Leather EngineeringCollege of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China Zhejiang Engineering Research Center for Electrochemical Energy Materials and Devices Institute of New Materials and Industrial TechnologiesWenzhou UniversityWenzhou 325035China School of Chemical and Biomedical Engineering Nanyang Technological UniversitySingapore 637459Singapore

Enhancing catalytic activity through modulating the interaction between n-doped carbon and metal phosphides clusters is an effective ***,the electronic structure modulation of CoP_(2) supported n-modified carbon(CoP_(2)/nC)has been designed and prepared as efficient electrocatalysts for oxygen reduction reaction(ORR),oxygen evolution reaction(OER),and hydrogen evolution reaction(HER).notably,CoP_(2)/nC-1 catalyst exhibits impressive performance in alkaline media,with an ORR half-wave potential of 0.84 V,as well as OER and HER overpotentials of 290 and 129 mV(at 10 mA·cm^(−2)),*** addition,CoP_(2)/nC-1 produces a power density as high as 172.9 mW·cm^(−2),and excellent reversibility of 100 h at 20 mA·cm^(−2) in home-made Zn-air *** experimental results demonstrate that the synergistic interactions between n modified carbon substrate and CoP_(2) material significantly enhance the kinetics of ORR,OER,and *** functional theory(DFT)calculations reveal the strong electrons redistribution of CoP_(2) induced by high-density n atoms at the interface,thus optimizing the key intermediates and significantly lower the energy barrier of *** electronic adjustments of CoP_(2) greatly enhance its kinetics of ORR/OER/HER,leading to faster *** study provides profound insights into the specific modification of CoP_(2) by n-doped carbon,enabling the construction of efficient catalysts.

关键词： two-dimensional(2D)carbon metal-organic framework cobalt phosphide zinc air battery water splitting

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Color-kinematics duality and dual conformal symmetry for a four-loop form factor in n=4 SYM

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Science China(Physics,Mechanics & Astronomy) 2024年第4期67卷 64-71页

作者： Guanda Lin Gang yang Siyuan Zhang CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China School of Fundamental Physics and Mathematical Sciences Hangzhou Institute for Advanced StudyUCASHangzhou 310024China International Centre for Theoretical Physics Asia-Pacific Beijing/Hangzhou 310024China

We obtain the integrand of full-color four-loop three-point form factor of the stress-tensor supermultiplet in n=4 SYM,based on the color-kinematics(CK)duality and generalized unitarity *** result not only manifests all dual Jacobi relations via CK duality but also contains 133 free *** suggests the constructibility of the form factor at even higher loops via CK *** also find that the planar form factor has a hidden dual conformal symmetry in the lightlike limit of the operator momentum,which is checked up to four loops.

关键词： S-matrix supersymmetric model perturbative calculations

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Irreducible Representations of GL_(n)(C)of Minimal Gelfand-Kirillov Dimension

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Acta Mathematica Sinica,English Series 2024年第3期40卷 639-657页

作者： Zhan Qiang BAI yang yang CHEn Dong Wen LIU Bin Yong SUn School of Mathematical Sciences Soochow UniversitySuzhou 215006P.R.China School of Sciences JiangnanUniversityWui214122P.R.China School of Mathematical Sciences Zhejiang UniversityHangzhou 310058P.R.China Institute for Advanced Study in Mathematics Zhejiang UniversityHangzhou 310058P.R.China

In this article,by studying the Bernstein degrees and Goldie rank polynomials,we es-tablish a comparison between the irreducible representations of G=GL_(n)(C)possessing the minimal Gelfand-Kirillov dimension and those induced from finite-dimensional representations of the maximal parabolic subgroup of G of type(n-1,1).We give the transition matrix between the two bases for the corresponding coherent families.

关键词： Bernstein degree coherent continuation Gelfand-Kirillov dimension

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Asymmetric Zn-n4 atomic sites embedded hollow fibers as stable Zn anode for high-performance Zn-ion hybrid capacitor

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Journal of Energy Chemistry 2024年第10期97卷 460-469页

作者： Yukun Liu Bing Li Jin Wang Caiyun Li Hongrui yang yang Song Sen Zhang Chao Deng Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of Education College of Physics and Electronic Engineering Harbin Normal University College of Material Science and Chemical Engineering Harbin Engineering University

Zn based electrochemical energy storage systems（EES） have attracted tremendous interests owing to their low cost and high intrinsic ***,the uncontrolled growth of Zn dendrites and the side reactions of Zn metal anodes（ZMAs） severely restrict their *** address these issues,we design the asymmetric Zn-n4atomic sites embedded hollow fibers（AS-IHF） as the flexible host for stable *** introducing different nitrogen resources in the synthesis,two kinds of coordination,i,***-n（pyridinic） and Zn-n（pyrrolic）,are introduced in the Zn-n4atomic module *** asymmetric Zn-n4module with regulated micro-environment facilitates the superior zincophilic features and promotes the Zn ***,the highly porous structure of the hollow fiber effectively reduces local current density,homogenize Zn ion flux,and alleviate structure *** the advantages endow the high efficiency and good stability for Zn plating/*** theoretical and experimental results demonstrate the high reversibility,low nucleation overpotential,and dendritefree behavior of the AS-IHF@Zn anode,which afford the high stability in high-rate and long-term ***,the solid-state Zn-ion hybrid capacitor（ZIHC） based on AS-IHF@Zn anode shows the high flexibility,reliability,and superior long-term cycling capability in a wide-range of temperatures（-20-25℃）.Therefore,the present work not only gives a new strategy for modulating local environments of single atomic sites,but also propels the development of flexible power sources for diverse electronics.

关键词： Asymmetric coordination Dendrite free behavior Single atomic sites Zincophilic sites Zn-ion hybrid capacitor

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Inducible RnA targeting and n^(6)-methyladenosine editing by a split-Cas13 architecture

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Journal of Molecular Cell Biology 2024年第1期16卷 66-69页

作者： yang Li Qiang Sun Zhi yang Gang Yuan International Institutes of Medicine the Fourth Affiliated Hospital of Zhejiang University School of MedicineYiwu 322000China Department of Thoracic Surgery and Institute of Thoracic Oncology West China HospitalSichuan UniversityChengdu 610041China Future Health Laboratory Innovation Center of Yangtze River DeltaZhejiang UniversityJiaxing 314100China

Dear editor,Cas13,a class Ⅱ type Ⅵ CRISPR‒Cas endonuclease with two higher eukaryotes and prokaryotes nucleotide-binding(HEPn)domains,exclusively binds to and cleaves single-stranded RnA by a complementary guide RnA(gRnA)(Makarova et al.,2020).RfxCas13d(also known as CasRx)is an ortholog of CRISPR‒Cas13 with a relatively small size and robust RnA knockdown capability in mammalian cells(Konermann et al.,2018).Owing to its simplicity and high efficiency,CasRx has been applied for RnA targeting in various types of cells and ***,most of these studies failed to control the nuclease activity of CasRx *** re-engineered split-Cas9 system enables inducible genome editing and epigenetic modulation through chemical-induced reassembly of the Cas9 protein(Zetsche et al.,2015).However,tools that allow for efficient and controllable RnA knockdown by a split-Cas13 system remain to be established.

关键词： split system simplicity

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A Fractional-Order Ultra-Local Model-Based Adaptive neural network Sliding Mode Control of n-DOF Upper-Limb Exoskeleton With Input Deadzone

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 760-781页

作者： Dingxin He HaoPing Wang yang Tian Yida Guo the School of Automation Nanjing University of Science and TechnologyNanjing 210094China IEEE norinco Group Institute of navigation and Control Technology Beijing 100089China

This paper proposes an adaptive neural network sliding mode control based on fractional-order ultra-local model for n-DOF upper-limb exoskeleton in presence of uncertainties,external disturbances and input *** the model complexity and input deadzone,a fractional-order ultra-local model is proposed to formulate the original dynamic system for simple controller ***,the control gain of ultra-local model is considered as a *** fractional-order sliding mode technique is designed to stabilize the closed-loop system,while fractional-order time-delay estimation is combined with neural network to estimate the lumped ***,a fractional-order ultra-local model-based neural network sliding mode controller(FO-nnSMC) is ***,to avoid disadvantageous effect of improper gain selection on the control performance,the control gain of ultra-local model is considered as an unknown ***,the nussbaum technique is introduced into the FO-nnSMC to deal with the stability problem with unknown ***,a fractional-order ultra-local model-based adaptive neural network sliding mode controller(FO-AnnSMC) is ***,the stability analysis of the closed-loop system with the proposed method is presented by using the Lyapunov ***,with the co-simulations on virtual prototype of 7-DOF iReHave upper-limb exoskeleton and experiments on 2-DOF upper-limb exoskeleton,the obtained compared results illustrate the effectiveness and superiority of the proposed method.

关键词： Adaptive control input deadzone model-free control n-DOF upper-limb exoskeleton neural network

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Coupling n-doping and confined Co_(3)O_(4) on carbon nanotubes by polydopamine coating strategy for pleiotropic water purification

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Rare Metals 2024年第7期43卷 3146-3160页

作者： Wen-Long Tu Gang Wang Yue Zhang Hong-yang Zhu Rong-Rong Du Hong-Yao Zhao Sheng Tang Zeng-Jing Guo Jun yang Fu yang Cheng-Zhang Zhu School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China School of Chemistry and Chemical Engineering Liaocheng UniversityLiaocheng 252000China School of Material Science and Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China School of Environmental Science and Engineering Nanjing Tech UniversityNanjing 211816China

The development of effective and sustainable solutions for pleiotropic water purification becomes urgent and *** Fenton-like catalysts for activation of peroxymonosulfate(PMS)to purify organic wastewater show great *** this work,by tuning metal loading with an in-situ polydopamine coating strategy,oxygen vacancy-enriched Co_(3)O_(4) loading on n-doped carbon nanotubes(CnTs)were constructed to enhance PMS activation efficiency for pollutants ***,the obtained modified CnTs afford a well-developed n-containing network structure,which is further endowed with abundant Co(Ⅱ)/Co(Ⅲ)redox cycles and significant metal-carbon *** particular,the surface n doping in CnTs might induce the oriented enrichment of pollutants around the catalyst,which reduces the migration distance and correspondingly improves the utilization of reactive oxidative *** electron transfer efficiency of the catalyst can be further improved by incorporating oxygen vacancy-enriched Co_(3)O_(4).The performance results show that the optimal nC/Co-1 could mineralize 20×10^(-6)of bisphenol A(BPA)by almost 98%in 8 min.A low reaction activation energy(26.05 kJ·mol^(-1))in BPA degradation was demonstrated by the nC/*** importantly,nC/Co-1 can inherit excellent degradation performance towards oxytetracycline,2,4-dichlorophenol,and tetracycline,showing wide practical *** addition,by virtue of the photothermal conversion property,nC/Co-1 achieves an additive function for interfacial solar water evaporation(1.84 kg·m^(-2)·h^(-1),112.51%),showing impressive potential for clean water recovery under complicated environmental pollution conditions.

关键词： Carbon nanotube Advanced oxidation process Co_(3)O_(4) Photothermal conversion Solar water evaporation

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