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Science China Chemistry 2024年第10期67卷 3432-3437页

作者： Xianzhe Wei Jincheng Liu Yan Su Weitao wang Guixiang wang Gen Zhang Ping wang cheng Gu State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSouth China University of TechnologyGuangzhou 510640China College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065China Key Laboratory for Soft Chemistry and Functional Materials of Ministry of Education School of Chemistry and Chemical EngineeringNanjing University of Science and TechnologyNanjing 210094China

Designing efficient proton-conductive materials is crucial in fuel ***,it remains a substantial challenge because of the issues in proton mobility,proton-carrier amount,and orientation of proton host ***,we report an in-situ protonation strategy to produce a locally flexible porous coordination polymer(PCP)to enhance the proton-carrier loading and proton *** local dipole flipping of the ligand allows effective proton exchange with low activation energy,promoting interpore proton transport through the pore apertures and pore *** protonation induces substantial charges to the frameworks and enhances the interaction with proton carriers,thereby increasing the loading of the proton *** this design strategy,the resulting PCP exhibits enhanced phosphoric acid loading and extraordinary proton conductivities under both aqueous and anhydrous conditions compared to its isoreticular analog that features rigidity without proton-exchange *** work provides a new avenue for designing proton-conductive materials that combine structural dynamics with performance merits.

关键词： porous coordination polymers in-situ protonation local flexibility proton-exchange mechanism proton conduction

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Unlocking the potential of ultra-thin two-dimensional antimony materials:Selective growth and carbon coating for efficient potassium-ion storage

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Journal of Energy Chemistry 2024年第5期92卷 440-449页

作者： Dongyu Zhang Zhaomin wang Yabin Shen Yeguo Zou Chunli wang Limin wang Yong cheng State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of Sciences(CAS)Changchun 130022JilinChina School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026AnhuiChina

Antimony-based anodes have attracted wide attention in potassium-ion batteries due to their high theoretical specific capacities(∼660 mA h g^(-1))and suitable voltage ***,severe capacity fading caused by huge volume change and limited ion transportation hinders their practical ***,strategies for controlling the morphologies of Sb-based materials to improve the electrochemical performances have been *** these,the two-dimensional Sb(2D-Sb)materials present excellent properties due to shorted ion immigration paths and enhanced ion ***,the synthetic methods are usually tedious,and even the mechanism of these strategies remains elusive,especially how to obtain large-scale 2D-Sb ***,a novel strategy to synthesize 2D-Sb material using a straightforward solvothermal method without the requirement of a complex nanostructure design is *** method leverages the selective adsorption of aldehyde groups in furfural to induce crystal growth,while concurrently reducing and coating a nitrogen-doped carbon *** to the reported methods,it is simpler,more efficient,and conducive to the production of composite nanosheets with uniform thickness(3–4 nm).The 2D-Sb@NC nanosheet anode delivers an extremely high capacity of 504.5 mA h g^(-1) at current densities of 100 mA g^(-1) and remains stable for more than 200 *** characterizations and molecular dynamic simulations,how potassium storage kinetics between 2D Sb-based materials and bulk Sb-based materials are explored,and detailed explanations are *** findings offer novel insights into the development of durable 2D alloy-based anodes for next-generation potassium-ion batteries.

关键词： Antimony Two-dimensional materials Selective growth Nitrogen-doped carbon Potassium-ion batteries

A generalized nonlinear three-dimensional Hoek‒Brown failure criterion

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3149-3164页

作者： Jiaxin wang Shunchuan Wu Haiyong cheng Junlong Sun Xiaolong wang Yaxi Shen Faculty of Land Resource Engineering Kunming University of Science and TechnologyKunming650093China Key Laboratory of Geohazard Forecast and Geoecological Restoration in Plateau Mountainous Area Ministry of Natural ResourcesKunming650093China Yunnan Key Laboratory of Geohazard Forecast and Geoecological Restoration in Plateau Mountainous Area Kunming650093China

To understand the strengths of rocks under complex stress states,a generalized nonlinear threedimensional(3D)Hoek‒Brown failure(NGHB)criterion was proposed in this *** criterion shares the same parameters with the generalized HB(GHB)criterion and inherits the parameter advantages of *** new parameters,b,and n,were introduced into the NGHB criterion that primarily controls the deviatoric plane shape of the NGHB criterion under triaxial tension and compression,*** NGHB criterion can consider the influence of intermediate principal stress(IPS),where the deviatoric plane shape satisfies the smoothness requirements,while the HB criterion *** criterion can degenerate into the two modified 3D HB criteria,the Priest criterion under triaxial compression condition and the HB criterion under triaxial compression and tension *** criterion was verified using true triaxial test data for different parameters,six types of rocks,and two kinds of in situ rock *** comparison,three existing 3D HB criteria were selected for performance comparison *** result showed that the NGHB criterion gave better prediction performance than other *** prediction errors of the strength of six types of rocks and two kinds of in situ rock masses were in the range of 2.0724%-3.5091%and 1.0144%-3.2321%,*** proposed criterion lays a preliminary theoretical foundation for prediction of engineering rock mass strength under complex in situ stress conditions.

关键词： Rock mechanics HoekeBrown criterion Failure criterion Intermediate principal stress True triaxial test Smoothness and convexity

Silent information regulator sirtuin 1 ameliorates acute liver failure via the p53/glutathione peroxidase 4/gasdermin D axis

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World Journal of Gastroenterology 2024年第11期30卷 1588-1608页

作者： xing-Nian Zhou Quan Zhang Hong Peng Yu-Jie Qin Yu-Hong Liu Lu wang Ming-Liang cheng Xin-Hua Luo Hong Li Department of Infectious Diseases The Affiliated Hospital of Guizhou Medical UniversityGuizhou Medical UniversityGuiyang 550004Guizhou ProvinceChina Department of Infectious Diseases Guizhou Provincial People's HospitalGuiyang 550001Guizhou ProvinceChina

BACKGROUND Acute liver failure(ALF)has a high mortality with widespread hepatocyte death involving ferroptosis and *** silent information regulator sirtuin 1(SIRT1)-mediated deacetylation affects multiple biological processes,including cellular senescence,apoptosis,sugar and lipid metabolism,oxidative stress,and *** To investigate the association between ferroptosis and pyroptosis and the upstream regulatory *** This study included 30 patients with ALF and 30 healthy individuals who underwent serum alanine aminotransferase(ALT)and aspartate aminotransferase(AST)testing.C57BL/6 mice were also intraperitoneally pretreated with SIRT1,p53,or glutathione peroxidase 4(GPX4)inducers and inhibitors and injected with lipopolysaccharide(LPS)/D-galactosamine(D-GalN)to induce *** D(GSDMD)^(-/-)mice were used as an experimental *** changes in liver tissue were monitored by hematoxylin and eosin ***,AST,glutathione,reactive oxygen species,and iron levels were measured using commercial ***-and pyroptosis-related protein and mRNA expression was detected by western blot and quantitative real-time polymerase chain ***1,p53,and GSDMD were assessed by immunofluorescence *** Serum AST and ALT levels were elevated in patients with ***1,solute carrier family 7a member 11(SLC7A11),and GPX4 protein expression was decreased and acetylated p5,p53,GSDMD,and acyl-CoA synthetase long-chain family member 4(ACSL4)protein levels were elevated in human ALF liver *** the p53 and ferroptosis inhibitor-treated and GSDMD^(-/-)groups,serum interleukin(IL)-1β,tumour necrosis factor alpha,IL-6,IL-2 and C-C motif ligand 2 levels were decreased and hepatic impairment was *** mice with GSDMD knockout,p53 was reduced,GPX4 was increased,and ferroptotic events(depletion of SLC7A11,elevation of ACSL4,and iron accumulation)were *** vitro,knockdown of p53 and overexpression of GPX

关键词： Silent information regulator sirtuin 1 Ferroptosis Pyroptosis p53/glutathione peroxidase 4/gasdermin D Acute liver failure

Preventive effects of Bifidobacterium lactis Probio-M8 on ovalbumin-induced food allergy in mice

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Food Science and Human Wellness 2024年第4期13卷 2346-2352页

作者： Jialu Shi Yan Xu cheng Liu Shizhi wang Jin wang Vijaya Raghavan Key Laboratory of Environmental Medicine and Engineering Ministry of Educationand Department of Nutrition and Food HygieneSchool of Public HealthSoutheast UniversityNanjing 210009China Department of Bioresource Engineering Faculty of Agricultural and Environmental SciencesMcGill UniversitySainte-Anne-de-BellevueQC H9X3V9Canada

Food allergy is a significant public health concern *** probiotics have been found to enhance food allergy by regulating immune-microbe interactions in animal models and ***,the effects of Bifidobacterium lactis Probio-M8 on food allergy have not been thoroughly *** present study examined the anti-allergic properties of Probio-M8,particularly in relation to immune response and gut microbiota *** demonstrate that oral administration of Probio-M8 effectively mitigated the allergy symptoms triggered by ovalbumin(OVA)by ameliorating the morphological damage in the jejunum,reducing OVA-specific IgE and histamine levels in the serum,and suppressing Th2 cytokines(interleukin(IL)4 and IL-13)while increasing Th1 cytokines(interferon(IFN)γ)and regulatory T(Treg)cytokines(IL-10 and transforming growth factor(TGF)β1)in the culture supernatants of splenic ***,Probio-M8 effectively altered the diversity and composition of gut microbiota,particularly the relative abundances of Akkermansia_muciniphila in OVA-induced *** to the OVA group,the Probio-M8 group showed a decrease in the relative abundance of Akkermansia_*** conclusion,Probio-M8 demonstrates the potential to alleviate food allergy by regulating the Th1/Th2 response and modulating gut microbiota,thereby offering a novel therapeutic strategy for patients with food allergy.

关键词： Food allergy Bifidobacterium lactis Probio-M8 T cell immune response Gut microbiota

Convergence analysis for complementary-label learning with kernel ridge regression

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Applied Mathematics(A Journal of Chinese Universities) 2024年第3期39卷 533-544页

作者： NIE Wei-lin wang cheng XIE Zhong-hua School of Mathematics and Statistics Huizhou UniversityHuizhou 516007China School of Computer Science and Engineering Huizhou UniversityHuizhou 516007China

Complementary-label learning(CLL)aims at finding a classifier via samples with complementary *** data is considered to contain less information than ordinary-label *** transition matrix between the true label and the complementary label,and some loss functions have been developed to handle this *** this paper,we show that CLL can be transformed into ordinary classification under some mild conditions,which indicates that the complementary labels can supply enough information in most *** an example,an extensive misclassification error analysis was performed for the Kernel Ridge Regression(KRR)method applied to multiple complementary-label learning(MCLL),which demonstrates its superior performance compared to existing approaches.

关键词： multiple complementary-label learning partial label learning error analysis reproducing kernel Hilbert spaces

Time-dependent behavior and permeability evolution of limestone under hydro-mechanical coupling

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Journal of Mountain Science 2024年第5期21卷 1697-1714页

作者： wang Zhilong ZENG Zhengqiang LYU cheng wang Mingnian HU Xiongyu DONG Yucang School of Civil Engineering Southwest Jiaotong UniversityChengdu 61003China College of Civil Engineering Tongji UniversityShanghai 200092China College of Water Resource and Hydropower Sichuan UniversityChengdu 610065China Hebei GEO University Shijiazhuang 050031China

Excessively high pore water pressure presents unpredictable risks to the safety of rock tunnels in mountainous regions that are predominantly composed of limestone. Investigating the creep characteristics and permeability evolution of limestone under varying hydrated conditions is crucial for a better understanding of the delayed deformation mechanisms of limestone rock tunnels. To this end, this paper initially conducts a series of multi-stage triaxial creep tests on limestone samples under varying pore water pressures. The experiment examines how pore water pressure affects limestone’s creep strain, strain rate, long-term strength, lifespan, and permeability, all within the context of hydraulicmechanical(HM) coupling. To better describe the creep behavior associated with pore water pressure, this paper proposes a new nonlinear fractional creep constitutive model. This constitutive model depicts the initial, steady-state, and accelerated phases of limestone’s creep behavior. Finally, the proposed model is applied to the numerical realization of deformation in limestone tunnel, validating the effectiveness of the proposed constitutive model in predicting tunnel’s creep deformation. This research enhances our understanding of limestone’s creep characteristics and permeability evolution under HM coupling, laying a foundation for assessing the longterm stability of mountain tunnels.

关键词： Creep test Hydraulic-mechanical coupling Creep constitutive model Fractional derivatives Pore pressure

Monocular Distance Estimated Based on PTZ Camera

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Computers, Materials & Continua 2024年第5期79卷 3417-3433页

作者： Qirui Zhong Xiaogang cheng Yuxin Song Han wang Bell Honors School Nanjing University of Posts and Telecommunications Nanjing210003China College of Telecommunications and Information Engineering Nanjing University of Posts and TelecommunicationsNanjing210003China College of Automation and College of Artificial Intelligence Nanjing University of Posts and TelecommunicationsNanjing210003China

This paper introduces an intelligent computational approach for extracting salient objects fromimages and estimatingtheir distance information with PTZ (Pan-Tilt-Zoom) cameras. PTZ cameras have found wide applications innumerous public places, serving various purposes such as public securitymanagement, natural disastermonitoring,and crisis alarms, particularly with the rapid development of Artificial Intelligence and global infrastructuralprojects. In this paper, we combine Gauss optical principles with the PTZ camera’s capabilities of horizontal andpitch rotation, as well as optical zoom, to estimate the distance of the *** present a novel monocular objectdistance estimation model based on the Focal Length-Target Pixel Size (FLTPS) relationship, achieving an accuracyrate of over 95% for objects within a 5 km range. The salient object extraction is achieved through a simplifiedconvolution kernel and the utilization of the object’s RGB features, which offer significantly faster computingspeeds compared to Convolutional Neural Networks (CNNs). Additionally, we introduce the dark channel beforethe fog removal algorithm, resulting in a 20 dB increase in image definition, which significantly benefits distanceestimation. Our system offers the advantages of stability and low device load, making it an asset for public securityaffairs and providing a reference point for future developments in surveillance hardware.

关键词： Public security location information PTZ camera image processing

Statistical QoS Provisioning Architecture for 6G Satellite-Terrestrial Integrated Networks

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Journal of Communications and Information Networks 2024年第1期9卷 34-42页

作者： Jingqing wang Wenchi cheng Wei Zhang Hui Liang School of Telecommunications Engineering Xidian UniversityXi’an 710071China School of Electrical Engineering and Telecommunications the University of New South WalesSydneyAustralia School of Electrical Engineering and Intelligentization Dongguan University of TechnologyDongguan 523808China Peng cheng Laboratory Shenzhen 518055China.

The emergence of massive ultra-reliable and low latency communications (mURLLC) as a category of age/time/reliability-sensitive service over 6G wireless networks has received considerable research attention, which has presented unprecedented challenges. As one of the key enablers for 6G,satellite-terrestrial integrated networks (STIN) have been developed to offer more expansive connectivity and comprehensive 3D coverage in space-aerial-terrestrial domains for supporting 6G mission-critical mURLLC applications while fulfilling diverse and rigorous quality of service (QoS) requirements. In the context of these mURLLC-driven satellite services, data freshness assumes paramount importance, as outdated data may engender unpredictable or catastrophic *** effectively measure data freshness in satellite-terrestrial integrated communications,age of information(AoI)has recently surfaced as a new dimension of QoS metric to support time-sensitive applications. It is crucial to design new analytical models that ensure stringent and diverse QoS metrics bounded by different key parameters,including AoI,delay,and reliability,over 6G satellite-terrestrial integrated networks. However,due to the complicated and dynamic nature of satellite-terrestrial integrated network environments, the research on efficiently defining new statistical QoS provisioning schemes while taking into account varying degrees of freedom has still been in their infancy. To remedy these deficiencies, in this paper we develop statistical QoS provisioning schemes over 6G satellite-terrestrial integrated networks in the finite blocklength regime. Particularly, we firstly introduce and review key technologies for supporting ***,we formulate a number of novel fundamental statistical-QoS metrics in the finite blocklength ***,we conduct a set of simulations to validate and evaluate our developed statistical QoS provisioning schemes over satellite-terrestrial integrated networks.

关键词： statistical QoS provisioning mURLLC peak AoI satellite-terrestrial integrated networks QoS exponents hybrid automatic repeat request finite blocklength coding

Interfacial modification using the cross-linkable tannic acid for highly-efficient perovskite solar cells with excellent stability

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Journal of Energy Chemistry 2024年第4期91卷 236-244页

作者： xing Gao Lirong Rong Fei Wu Yen-Hung Lin Ye Zeng Junhong Tan Rongxing He cheng Zhong Linna Zhu Chongqing Key Laboratory for Advanced Materials and Technologies of Clean Energy School of Materials&EnergySouthwest UniversityChongqing 400715China Hubei Key Lab on Organic and Polymeric Optoelectronic Materials Department of ChemistryWuhan UniversityWuhan 430072HubeiChina Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationSchool of Chemistry and Chemical EngineeringSouthwest UniversityChongqing 400715China Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloon 999077Hong KongChina State Key Laboratory of Advanced Displays and Optoelectronics Technologies The Hong Kong University of Science and TechnologyClear Water BayKowloon 999077Hong KongChina

Although the performance of perovskite solar cells(PSCs)has been dramatically increased in recent years,stability is still the main obstacle preventing the PSCs from being *** device instability can be caused by a variety of reasons,including ions diffusion,surface and grain boundary defects,*** this work,the cross-linkable tannic acid(TA)is introduced to modify perovskite film through post-treatment *** numerous organic functional groups(–OH and C=O)in TA can interact with the uncoordinated Pb^(2+)and I^(-)ions in perovskite,thus passivating defects and inhibiting ions *** addition,the formed TA network can absorb a small amount of the residual moisture inside the device to protect the perovskite ***,TA modification regulates the energy level of perovskite,and reduces interfacial charge ***,following TA treatment,the device efficiency is increased significantly from 21.31%to 23.11%,with a decreased hysteresis ***,the treated device shows excellent air,thermal,and operational *** light of this,the readily available,inexpensive TA has the potential to operate as a multipurpose interfacial modifier to increase device efficiency while also enhancing device stability.

关键词： Tannic acid Defect passivation lons diffusion Hydrophilic Stability Perovskite solar cells