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A Strong,Tough,and Self-Healing Strengthening Thioctic Acid-based Elastomer for Highly Reliable Flexible Strain Sensor

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Chinese Journal of Polymer Science 2024年第10期42卷 1610-1618,I0016页

作者： xin-Yu Chen Yu-Bing fu Xue-Ling Yan Lan liu School of Materials Science and Engineering Key Lab of Guangdong Province for High Property and Functional Polymer MaterialsSouth China University of TechnologyGuangzhou510641China

Elastomers with high strength and toughness,excellent self-healing properties,and biocompatibility have broad application prospects in wearable electronics and other fields,but preparing it remains a *** this work,we propose a highly adaptable strategy by introducing the small molecule crosslinking agent of triethanolamine(TEA)to the poly(thioctic acid)(PTA)chains and preparing the PAx Ey elastomers using a simple synthesis *** strategy stabilizes the PTA chains by constructing multiple non-covalent cross-linked dynamic networks,endowing materials with excellent strength and toughness(tensile strength of 288 kPa,toughness of 278.2 kJ/m3),admirable self-healing properties(self-healing efficiency of 121.6%within 7 h at 70℃),and good *** PAx Ey elastomers can also be combined with MWNTs to become flexible strain sensors,which can be used to monitor human joint movements with high sensitivity,repeatable responses,and stability.

关键词： Thioctic acid Ion clusters Multiple dynamic networks Self-healing strengthening Flexible strain sensor

Coupling effect of micro-textured tools and cooling conditions on the turning performance of aluminum alloy 6061

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Advances in Manufacturing 2023年第4期11卷 663-681页

作者： Guo-Liang liu Jin-Tao Zheng Chuan-Zhen Huang Shu-Feng Sun xin-fu liu Long-Jie Dai De-Xiang Wang Xiang-Yu Wang Key Lab of Industrial Fluid Energy Conservation and Pollution Control Ministry of EducationKey Lab of Industrial Fluid Energy Conservation and Pollution ControlMinistry of EducationSchool of Mechanical and Automotive EngineeringQingdao University of TechnologyQingdao266520ShandongPeople’s Republic of China State Key Laboratory of High Performance Complex Manufacturing Central South UniversityChangsha410083People’s Republic of China Key Laboratory of High-Efficiency and Clean Mechanical Manufacture(Ministry of Education) School of Mechanical EngineeringShandong UniversityJinan250061People’s Republic of China School of Mechanical Engineering Yanshan UniversityQinhuangdao066004HebeiPeople’s Republic of China Qingdao Choho Ind Co Ltd Qingdao266705ShandongPeople’s Republic of China School of Mechanical Engineering University of JinanJinan250022People’s Republic of China

Micro-texturing has been widely proven to be an effective technology for achieving sustainable ***,the performance of micro-textured tools under different cooling conditions,especially their coupling effect on machined surface integrity,was scarcely *** this paper,the non-textured,linear micro-grooved,and curvilinear micro-grooved inserts were used to turn aluminum alloy 6061 under dry,emulsion,and liquid nitrogen cryogenic cooling *** coupling effects of different micro-textures and cooling conditions on cutting force,cutting temperature,and machined surface integrity,including the surface roughness,work hardening,and residual stress,were revealed and discussed in *** indicated that the micro-grooved tools,especially the curvilinear micro-grooved tools,not only reduced the cutting force and cutting temperature,but also improved the machined surface *** addition,the micro-grooved tools can cooperate with the emulsion or liquid nitrogen to reduce the cutting force,cutting temperature,and improve the machined surface integrity generally,although the combination of emulsion cooling condition and micro-grooved tools generated negative coupling effects on cutting forces and surface work ***,the combination of curvilinear micro-grooved cutting tools and cryogenic cooling condition resulted in the lowest cutting force and cutting temperature,which generated the surface with low roughness,weak work hardening,and compressive residual stress.

关键词： Micro-grooved cutting tool Cooling condition Cutting force Cutting temperature Surface integrity

Stable hydrogen-bonded organic frameworks and their photo-and electro-responses

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Nano Research 2024年第8期17卷 7675-7699页

作者： Ying Hou xin-Song Huang Sheng-Hao Gong Chen liu Yangyang liu Tian-fu liu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China University of Chinese Academy of Sciences Beijing 100049China Department of Chemistry and Biochemistry California State UniversityLos AngelesCalifornia 90032USA College of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350007China

Hydrogen-bonded organic frameworks(HOFs)are a recent class of porous materials that have garnered considerable research interest owing to their distinctive *** can be constructed through judicious selection of H-bonding motifs,which are further enforced by other weak intermolecular interactions such asπ–πstacking,van der Waals forces,and framework *** advantage of these interactions,we can expand the functional field of HOFs by introducing active ***,researchers have made substantial advancements in using HOFs for chemical sensing,catalysis,proton conduction,biological applications,and *** low bonding energy of H-bonds allows for precise control over the concentration of ligands in solvents,forming diverse HOF *** varied structures offer significant advantages for producing HOFs with photo-responsive and electro-responsive ***,the presence of H-bonds in HOFs results in their inherent lower stability compared to metal-organic frameworks(MOFs)and covalent-organic frameworks(COFs)formed via coordination and covalent bonds,*** a result,the pursuit of stable and innovative HOF materials with novel functional sites remains an ongoing *** review provides an overview of recent research progress in the development of new strategies for stable HOF synthesis and applications of HOFs with stimuli-responsive *** first classified all synthetic methods reported to date and discussed the stable HOFs synthesized,as well as their unique properties and *** addition,we summarized the applications of HOFs utilizing their synergistic responses to external stimuli,including photo,electrical,pressure,and chemical *** systematically reviewed stable HOF synthesis and applications,which may lead to a deeper understanding of the structure–activity relationship for these materials and guide future HOF design.

关键词： stable hydrogen-bonded organic frameworks(HOFs) photo-response electro-response photoelectric synergistic response

Non-symmetric distributions of solids deposition for solid-water stratified flow in deviated tubing strings

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Petroleum Science 2023年第5期20卷 3048-3061页

作者： xin-fu liu Chun-Hua liu Zhong-Xian Hao Ying Zheng Kai Zhang Jian-Feng Wang Song-Bo Wei Ai-Gang Hao Jun-Ling Tao Hui Cheng School of Mechanical and Automotive Engineering Qingdao University of TechnologyQingdaoShandong266520China College of Mechanical and Electronic Engineering China University of Petroleum(East China)QingdaoShandong266580China Research Institute of Exploration&Development PetroChinaBeijing100083China Department of Chemical and Biochemical Engineering Western UniversityOntarioN6A 3K7Canada Lusheng Petroleum Development Company Ltd. SINOPECDongyingShandong256657China

Dynamic performance on solids flow with water in deviated tubing is essential for the reliability of pump and normal operation of horizontal and directional *** with coal-water flow in vertical tubing and sand-oil flow with high production in deviated tubing,solids deposition with water shows obvious non-symmetric distributions in deviated tubing from simulations and *** mathematical model of two phase flow was developed under coupling conditions of deviated tubing,low flow rate and viscosity based on the kinetic theory of granular flow and first-order discrete *** results show that solid-water stratified flow in deviated tubing can be divided into two zones of suspension bed and the moving bed throughout the flow *** solid flowing velocity with water is negative and particles slide down at the bottom of moving bed *** process of solids flow with water in deviated tubing will produce pressure loss and consume the kinetic *** thickness of deposited layer and the flowing velocity of solids flow downward with water at the moving bed zone enhance with the decreased inlet flow rate and the increased particle size,tubing inside diameter(ID)and inclination *** are easier into suspension from the upper part of moving bed zone to suspension bed zone and more solid particles flow with water towards the tubing outlet with the increase of inlet flowing *** decision is made to reduce the screen width,tubing ID and inclination angle to maintain to be greater than critical deposition velocity in order to prevent solids *** it provides the theoretical basis and technical reserves for solid control and offers an effective approach to enhance tubing cleaning in deviated strings.

关键词： Deviated tubing Stratified flow Solid deposition Critical velocity Prevent solids settling

A novel multi-state bogie system reliability evaluation approach by extended d-MC model for high-speed trains

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Transportation Safety and Environment 2024年第3期6卷 35-46页

作者： Yong fu Ruoqu liu Jisheng Dai Wenlong Zhu xin liu Yong Qin Zhuzhou CRRC Times Electric Co. Ltd.Times RoadShifeng DistrictZhuzhouHunan 412001China Department of Statistics University of WarwickCoventry CV47ALUnited Kingdom State Key Lab of Rail Traffic Control&Safety Beijing Jiaotong UniversityHaidian DistrictBeijing 100044China

Bogie is a pivotal system and plays a critical part in the safety and reliability management of high-speed ***,the available bogie system reliability analysis methods lack the consideration of multi-state characteristics,and the common multi-state reliability analysis methods,being an NP-hard problem,lead to low *** order to overcome these drawbacks,this paper proposes a novel multi-state rail train bogie system reliability analysis approach based on the extended d-MC *** different function interactions within the bogie system are considered to build the multi-state bogie system flow network ***,an extended d-MC model is established to remove unnecessary d-MC candidates and duplicates,which greatly enhances the computing *** bogie system reliability is calculated,and examples are *** experiments are carried out for the different operational conditions of the bogie system and are used to test the practicability of the method proposed in this article;it is found that this method outperforms a newly developed method in solving multi-state reliability problems.

关键词： multi-state system reliability bogie flow network extended d-MC model

Development of MoS_(2)-stainless steel catalyst by 3D printing for efficient destruction of organics via peroxymonosulfate activation

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Journal of Environmental Sciences 2024年第1期135卷 108-117页

作者： Yufeng liu Jianhui Xu xin fu Pengxu Wang Dan Li Yunfei Zhang Shenggui Chen Chunhui Zhang Peng liu School of Environment and Civil Engineering Dongguan University of TechnologyDongguan 523808China School of Art and Design Guangzhou Panyu PolytechnicGuangzhou 511483China Dongguan Institute of Science and Technology Innovation Dongguan University of TechnologyDongguan 523808China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China

Herein,a novel MoS_(2)-stainless steel composite material was first synthetized via a 3D printing method(3DP MoS_(2)-SS)for peroxymonosulfate(PMS)activation and organics *** with MoS_(2)-SS powder/PMS system(0.37 g/(m^(2)/min)),4.3-fold higher k_(FLO)/S_(BET)value was obtained in 3DP MoS_(2)-SS/PMS system(1.60 g/(m^(2)/min),resulting from the superior utilization of active *** observed that 3DP MoS_(2)-SS significantly outperformed the 3DP SS due to the enhanced electron transfer rate and increased active ***,Mo^(4+)facilitated the Fe^(2+)/Fe^(3+)cycle,resulting in the rapid degradation of florfenicol(FLO).Quenching experiments and electron paramagnetic resonance spectra indicated that·OH,SO_(4)·^(-),O_(2)·^(-)and^(1)O_(2)were involved in the degradation of *** effect of influencing factors on the degradation of FLO were evaluated,and the optimized degradation efficiency of 98.69%was achieved at 1 mM PMS and pH of *** degradation products were detected by UPLC/MS analyses and several possible degradation pathways were proposed to be the cleavage of C-N bonds,dechlorination,hydrolysis,defluorination and *** addition,3DP MoS_(2)-SS/PMS system also demonstrated superior degradation performance for 2-chlorophenol,acetaminophen,ibuprofen and *** study provided deep insights into the MoS_(2)-SS catalyst prepared by 3DP technology for PMS activation and FLO-polluted water treatment.

关键词： 3D printing Stainless steel MoS_(2) Peroxymonosulfate activation Degradation mechanism

Calcium-chelating peptides from rabbit bone collagen:characterization,identification and mechanism elucidation

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Food Science and Human Wellness 2024年第3期13卷 1485-1493页

作者： fuhuan Yuan Yu fu Liang Ma Hankun Zhu Yong Yu xin Feng Yi Sun Hongjie Dai xin liu Zhengfang liu Yuhao Zhang College of Food Science Southwest UniversityChongqing 400715China Chongqing Key Laboratory of Speciality Food Co-Built by Sichuan and Chongqing Chongqing 400715China Key Laboratory of Luminescence Analysis and Molecular Sensing(Southwest University) Ministry of EducationChongqing 400715China Angel Yeast Co. Ltd.Yichang 443003China

This study aimed to characterize and identify calcium-chelating peptides from rabbit bone collagen and explore the underlying chelating *** peptides and calcium were extracted from rabbit bone by instant ejection steam explosion(ICSE)combined with enzymatic hydrolysis,followed by chelation reaction to prepare rabbit bone peptide-calcium chelate(RBCP-Ca).The chelating sites were further analyzed by liquid chromatography-tandem mass(LC-MS/MS)spectrometry while the chelating mechanism and binding modes were *** structural characterization revealed that RBCP successfully chelated with calcium ***,LC-MS/MS analysis indicated that the binding sites included both acidic amino acids(Asp and Glu)and basic amino acids(Lys and Arg),Interestingly,three binding modes,namely Inter-Linking,Loop-Linking and Mono-Linking were for the first time found,while Inter-Linking mode accounted for the highest proportion(75.1%),suggesting that chelation of calcium ions frequently occurred between two ***,this study provides a theoretical basis for the elucidation of chelation mechanism of calcium-chelating peptides.

关键词： Rabbit bone Collagen peptide Peptide-calcium chelate Chelation mechanism Liquid chromatography-tandem mass(LC-MS/MS)

Evaluation of 3D crustal seismic velocity models in southwest China:Model performance,limitation,and prospects

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Science China Earth Sciences 2024年第2期67卷 604-619页

作者： xin WANG Ling CHEN Qi-fu CHEN Key Laboratory of Earth and Planetary Physics Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing100049China State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China

Southwest China is a tectonically and seismically active region,witnessing strong deformation due to the collision between the Indian and Eurasian *** the subsurface velocity structure of this region is thus important in understanding the tectonics and geodynamic processes of continental collision and in mitigating seismic *** studies have provided various 3D seismic velocity models in southwest ***,discrepancies exist among these models,and less effort has been made to quantify the reliability and accuracy of these existing velocity *** this study,we use regional 3D waveform simulation to evaluate the performance of various regional crustal 3D velocity models in reproducing observed *** particularly focus on two recent earthquake sequence in the region,the 2021 Yunnan Yangbi MS_(6.4) earthquake sequence and the 2022 Sichuan Luding MS_(6.8) earthquake *** tested 3D velocity models include the Southwest China Community Velocity model V1.0,the Unified Seismic Tomography Models for Continental China Lithosphere V2.0,the adjoint full waveform tomography model of the crustal and upper mantle beneath Eastern Tibetan Plateau,and the shallow seismic structure model beneath continental *** results show that the tested 3D velocity models generally capture well long-period(full-waveform tomography model shows a slighter better performance than the other models,especially for the body-waves,highlighting the advantages

关键词： Southwest China Seismic tomography models Shallow Structures Waveform simulation Model evaluation

Metagenomic analysis revealing the metabolic role of microbial communities in the free amino acid biosynthesis of Monascus rice vinegar during fermentation

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Food Science and Human Wellness 2024年第4期13卷 2317-2326页

作者： Hang Gao Jian Zhang Li liu Lijun fu Yan Zhao Germán Mazza xin Zhang Beijing Academy of Food Sciences 100068 BeijingChina Institute for Research and Development in Process Engineering Biotechnology and Alternative Energies(PROBIENCONICET-UNCo)8300 NeuquénArgentina

Free amino acid(FAA)is the important component of vinegar that infl uences quality perception and consumer *** is one of the major metabolites produced by microorganisms;however,the microbial metabolic network on FAA biosynthesis remains *** metagenomic analysis,this work aimed to elucidate the roles of microbes in FAA biosynthesis during Monascus rice vinegar *** profiles from functional analyses showed 14 dominant genera with high contributions to the metabolism *** metabolic network for FAA biosynthesis was then constructed,and the microbial distribution in different metabolic pathways was *** results revealed that 5 functional genera were closely involved in FAA *** study illuminated the metabolic roles of microorganisms in FAA biosynthesis and provided crucial insights into the functional attributes of microbiota in vinegar fermentation.

关键词： Monascus rice vinegar Metagenomic analysis Free amino acid synthesis Metabolic pathway Microbial distribution