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Chemical Research in Chinese Universities 2024年第1期40卷 127-135页

作者： Yan Jiali Yang Kaiying Wang Xi Zhai Jinli Zhu Wenjie Yang Daoli Luo Yongming Gao xiaoya Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming650500P.R.China Innovation Team for Volatile Organic Compounds Pollutants Control and Resource Utilization of Yunnan Province Kunming650500P.R.China Higher Educational Key Laboratory for Odorous Volatile Organic Compounds Pollutants Control of Yunnan Province Kunming650500P.R.China

Maximizing the sustainable recycling of spent lithium-ion batteries(LIBs)shows economic and environmental *** study recovered lithium cobaltate(LiCoO_(2.,LCO)from spent LIBs cathode *** recovered LCO was then combined with NaHSO_(3)to remove refractory organic pollutants of carbamazepine(CBZ)in *** degradation of CBZ reached 80.0%within 60 min,by 1O_(2.,SO_(4),OH and O_(2.^(-)generated in the LCO/NaHSO_(3)*** electron transfer between Co(III)and Co(II)was beneficial to the generation of free *** LCO/NaHSO_(3)degraded CBZ effectively in both secondary outlet water and tap ***,high concentrations of inorganic ions(Cl^(−),HCO_(3)^(-),HPO_(4)^(2.),SO_(2.−4,NO_(3)^(-))and natural organic matter(humic acid,HA)could inhibit the degradation of *** three cycles,the stability of the LCO/NaHSO_(3)system was demonstrated by the maintained high efficiency in the degradation of *** obtained data indicate that the LCO/NaHSO_(3)system holds great application potential in the field of advanced oxidation degradation of pollutants.

关键词： Spent lithium-ion battery Lithium cobaltate Carbamazepine NaHSO_(3) Advanced oxidation

Measuring urban thermal environment from accessibility-based perspective:A case study in a populous city

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Geography and Sustainability 2024年第3期5卷 329-342页

作者： Xinyu Dong xiaoya Li Yanmei Ye Dan Su Runjia Yang Angela Lausch Department of Land Management Zhejiang UniversityHangzhou 310058China Department of Computational Landscape Ecology Helmholtz Centre for Environmental Research-UFZLeipzig 04318Germany Landscape Ecology Lab Geography DepartmentHumboldt-Universität zu BerlinBerlin 10099Germany Department of Physical Geography and Geoecology Martin Luther University Halle-WittenbergHalle 06120Germany Department of Architecture Facility Management and GeoinformationAnhalt University of Applied SciencesDessau 06846Germany

Understanding the spatial interaction among residents,cooling service,and heat risk area in complex urban areas is conducive to developing targeted ***,traditional urban thermal environment assessments typically relied on simple linear integration of associated indicators,often neglecting the spatial interaction *** explore the spatial interaction among the three elements,this study proposes an accessibility-based urban thermal environment assessment *** Zhengzhou,a rapidly urbanizing city,as an example,remotely sensed images from three periods(2.10,2.15 and 2.2.)were applied to extract urban green space(UGS)and hot island area(HIA).An improved two-step floating catchment area(2.FCA)method and bivariate local Moran’s I were employed to explore whether residents’clustering locations are more likely to access cooling service or to be exposed to heat *** results demonstrate that the UGS in the city has been expanding,whereas the HIA shrank within the inner city in 2.15 and then increased in *** though the urban thermal environment may have improved in the last decade,the spatial interaction among the residents,cooling service and heat risk area could be *** autocorrelation shows an increase in locations that are disadvantageous for resident *** when sufficient cooling services were provided,residents in these areas could still be exposed to high heat *** developed urban thermal environment framework provides a novel insight into the residents’heat risk exposure and cooling service accessibility,and the findings could assist urban planners in targeting the improvement of extra heat exposure risk locations.

关键词： Urban heat island Urban green space Accessibility Remote sensing Spatial autocorrelation analysis

High power tunable Raman fiber laser at 1.2.m waveband

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Frontiers of Optoelectronics 2024年第1期17卷 1-8页

作者： Yang Zhang Jiangming Xu Junrui Liang Jun Ye Sicheng Li xiaoya Ma Zhiyong Pan Jinyong Leng Pu Zhou College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China Hunan Provincial Key Laboratory of High Energy Laser Technology National University of Defense TechnologyChangsha 410073China

Development of a high power fiber laser at special waveband,which is difficult to achieve by conventional rare-earth-doped fibers,is a significant *** of the most common methods for achieving lasing at special wavelength is Raman ***-doped fiber(PDF),due to the phosphorus-related large frequency shift Raman peak at 40 THz,is a great choice for large frequency shift Raman ***,by adopting 150 m large mode area triple-clad PDF as Raman gain medium,and a novel wavelength-selective feedback mechanism to suppress the silica-related Raman emission,we build a high power cladding-pumped Raman fiber laser at 1.2.m waveband.A Raman signal with power up to 735.8 W at 12.2.7 nm is *** the best of our knowledge,this is the highest output power ever reported for fiber lasers at 1.2.m ***,by tuning the wavelength of the pump source,a tunable Raman output of more than 450 W over a wavelength range of 12.0.6–12.2.7 nm is *** work proves PDF’s advantage in high power large frequency shift Raman conversion with a cladding pump scheme,thus providing a good solution for a high power laser source at special waveband.

关键词： Phosphosilicate fiber Raman fiber laser 1.2.m waveband Wavelength tunable

Electronic structure engineering of single atomic sites by plasmoninduced hot electrons for highly efficient and selective photocatalysis

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Nano Research 2024年第8期17卷 6960-6967页

作者： xiaoya Huang Xinyuan Li Akang Chen Hongfei Gu Shouyuan Li Tailei Hou Shuwen Zhu Shuang Yu Yin Song Jiatao Zhang Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications MIIT Key Laboratory of Medical Molecule Science and Pharmaceutical EngineeringMOE Key Laboratory of Cluster ScienceSchool of Chemistry and Chemical EngineeringSchool of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China MIIT Key Laboratory of Complex-field Intelligent Exploration School of Optics and PhotonicsBeijing Institute of TechnologyBeijing 100081China

Single atom(SA)catalysts have achieved great success on highly selective heterogeneous catalysis due to their abundant and homogeneous active *** electronic structures of these active sites,restrained by their localized coordination environments,significantly determine their catalytic performances,which are difficult to ***,we investigated the effect of localized surface plasmon resonance(LSPR)on engineering the electronic structures of single atomic ***,core–shell structures consisted of Au core and transition metal SAs loaded N-doped carbon(CN)shell were constructed,namely Au@M-SA/CN(M=Ni,Fe,and Co).It was demonstrated that plasmon-induced hot electrons originated from Au were directionally injected to the M-SAs under visible light irradiation,which significantly changed their electronic structures and meanwhile facilitated improved overall charge separation *** as-prepared Au@Ni-SA/CN exhibited highly efficient and selective photocatalytic CO_(2. reduction to CO performance,which is 2..8,17.5,and 6.9 times those of Au nanoparticles,Au@CN,and Ni-SA/CN,*** spectroscopy analysis and theoretical calculations confirmed that the plasmon enhanced Ni-SA/CN sites featured increased charge density for efficient intermediate activation,contributing to the superb photocatalytic *** work provides a new insight on plasmon and atomic site engineering for efficient and selective catalysis.

关键词： single atom catalysts plasmon enhancement coupling effect photocatalysis CO_(2. reduction

Mode division multiplexing reconstructive spectrometer with an all-fiber photonics lantern

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Frontiers of Optoelectronics 2024年第3期17卷 29-38页

作者： Junrui Liang Jun Ye xiaoya Ma Yao Lu Jun Li Jiangming Xu Zilun Chen Jinyong Leng Zongfu Jiang Pu Zhou College of Advanced Disciplinary Studies National University of Defense TechnologyChangsha 410073China Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China Hunan Provincial Key Laboratory of High Energy Laser Technology National University of Defense TechnologyChangsha 410073China Space Engineering University Beijing 101416China

This study presents a high-accuracy,all-fber mode division multiplexing(MDM)reconstructive spectrometer(RS).The MDM was achieved by utilizing a custom-designed 3×1 mode-selective photonics lantern to launch distinct spatial modes into the multimode fber(MMF).This facilitated the information transmission by increasing light scattering processes,thereby encoding the optical spectra more comprehensively into speckle *** resolution of 2.pm and the recovery of 2.00 spectral channels were *** to methods employing single-mode excitation and two-mode excitation,the three-mode excitation method reduced the recovered error by 88%and 50%respectively.A resolution enhancement approach based on alternating mode modulation was proposed,reaching the MMF limit for the 3 dB bandwidth of the spectral correlation *** proof-of-concept study can be further extended to encompass diverse programmable mode *** is not only succinct and highly efcient but also well-suited for a variety of high-accuracy,high-resolution spectral measurement scenarios.

关键词： High-accuracy Resolution enhancement Reconstructive spectrometer Mode division multiplexing Photonics lantern

Melatonin improves synapse development by PI3K/Akt signaling in a mouse model of autism spectrum disorder

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Neural Regeneration Research 2024年第7期19卷 1618-1624页

作者： Luyi Wang Man Xu Yan Wang Feifei Wang Jing Deng xiaoya Wang Yu Zhao Ailing Liao Feng Yang Shali Wang Yingbo Li Institute of Neuroscience Department of PhysiologySchool of Basic Medical ScienceChongqing Medical UniversityChongqingChina Department of Pediatric Chongqing University Fuling HospitalChongqingChina Department of Neurosurgery Xinqiao HospitalArmy Medical UniversityChongqingChina Department of Pathology Affiliated Hospital of North Sichuan Medical CollegeNanchongSichuan ProvinceChina NHC Key Laboratory of Birth Defects and Reproductive Health Chongqing Population and Family Planning Science and Technology Research InstituteChongqingChina China National Clinical Research Center for Neurological Diseases Beijing Tiantan HospitalCapital Medical UniversityBeijingChina Advanced Innovation Center for Human Brain Protection Capital Medical UniversityBeijingChina

Autism spectrum disorders are a group of neurodevelopmental disorders involving more than 1100 genes,including Ctnnd2.as a candidate ***2.nockout mice,serving as an animal model of autis m,have been demonstrated to exhibit decreased density of dendritic *** role of melatonin,as a neuro hormone capable of effectively alleviating social interaction deficits and regulating the development of dendritic spines,in Ctnnd2.deletion-induced nerve injury remains unclea *** the present study,we discove red that the deletion of exon 2.of the Ctnnd2.gene was linked to social interaction deficits,spine loss,impaired inhibitory neurons,and suppressed phosphatidylinositol-3-kinase(PI3K)/protein kinase B(Akt) signal pathway in the prefrontal *** findings demonstrated that the long-term oral administration of melatonin for 2. days effectively alleviated the aforementioned abnormalities in Ctnnd2.gene-knockout ***,the administration of melatonin in the prefro ntal cortex was found to improve synaptic function and activate the PI3K/Akt signal pathway in this *** pharmacological blockade of the PI3K/Akt signal pathway with a PI3K/Akt inhibitor,wo rtmannin,and melatonin receptor antagonists,luzindole and 4-phenyl-2.propionamidotetralin,prevented the melatonin-induced enhancement of GABAergic synaptic *** findings suggest that melatonin treatment can ameliorate GABAe rgic synaptic function by activating the PI3K/Akt signal pathway,which may contribute to the improvement of dendritic spine abnormalities in autism spectrum disorders.

关键词： autism Ctnnd2.deletion GABAergic neurons melatonin PI3K/Akt signal pathway prefrontal cortex social behavior spine density synaptic-associated proteins

Twisted Phosphors that Violate Kasha's Exciton Model in Organic Systems

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Chinese Journal of Chemistry 2024年第11期42卷 1237-1246页

作者： Boyi Fu Guangming Wang Jiuyang Li Junbo Li Xun Li xiaoya Zhao Shuhui Ding Guoping Yan Qianqian Yan Kaka Zhang School of Materials Science and Engineering Wuhan Institute of TechnologyWuhanHubei430205 China Key Laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules Shanghai Institute of Organic ChemistryUniversity of Chinese Academy of SciencesChinese Academy of Sciences345 Lingling RoadShanghai200032 China

Kasha's exciton model proposes that T1 energy levels of organic compounds are insensitive to molecular aggregation and microenvironment change because of negligible small transition dipole moments of T1 *** model holds true in most organic systems till *** we report the fabrication of twisted organic phosphors with intramolecular charge transfer characters and flexible molecular *** doped into different organic matrices,the twisted phosphor adopts different conformation,exhibits distinct phosphorescence colors and T1 energy levels,which violates Kasha's exciton model in organic *** that the change of phosphorescence colors and maxima can be readily distinguished by human eyes and conventional instrument,the twisted phosphors would be exploited as a new type of molecular probe,which would exhibit potential application in optical sensing and stimuli-responsive systems.

关键词： Afterglow Twisted phosphor Triplet excited state Room-temperature phosphorescence Luminescence Spin-orbit coupling

Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou,China

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Journal of Environmental Sciences 2024年第4期138卷 62-73页

作者： Lijun Yun Chunlei Cheng Suxia Yang Zaihua Wang Mei Li Qi En Zhong LiyuanMao Sulin Liu xiaoya Cheng Duanying Chen Fan Yang Zhen Zhou Institute of Mass Spectrometry and Atmospheric Environment Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollutionJinan UniversityGuangzhou 510632China Guangdong-Hongkong-Macao Joint Laboratory of Collaborative Innovation for Environmental Quality Guangzhou 510632China State Key Laboratory of Loess and Quaternary Geology Institute of Earth EnvironmentChinese Academy ScienceXi’an 710061China Institute for Environment and Climate Research Jinan UniversityGuangzhou 510632China Guangdong Academy of Sciences Institute of Resources Utilization and Rare Earth DevelopmentGuangzhou 510650China Environmental Monitoring Station of Pudong New District Shanghai 201200China

Organic nitrogen(ON)compounds play a significant role in the light absorption of brown carbon and the formation of organic aerosols,however,the mixing state,secondary formation processes,and influencing factors of ON compounds are still *** paper reports on the mixing state of ON-containing particles based on measurements obtained using a highperformance single particle aerosol mass spectrometer in January 2.2. in *** ON-containing particles accounted for 2.% of the total detected single particles,and the particle count and number fraction of the ON-containing particles were two times higher at night than during the *** prominent increase in the content of ON-containing particles with the enhancement of NO_xmainly occurred at night,and accompanied by high relative humidity and nitrate,which were associated with heterogeneous reactions between organics and gaseous NO_(x)and/or NO_(3)*** synchronous decreases in ON-containing particles and the mass absorption coefficient of water-soluble extracts at 365 nm in the afternoon may be associated with photo-bleaching of the ON species in the *** addition,the positive matrix factorization analysis found five factors dominated the formation processes of ON particles,and the nitrate factor(33%)mainly contributed to the production of ON particles at *** results of this study provide unique insights into the mixing states and secondary formation processes of the ON-containing particles.

关键词： Organic nitrogen compounds Single particles Mixing state Secondary formation Nighttime chemistry

Spectral programmable mid-infrared optical parametric oscillator

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Photonics Research 2024年第8期12卷 1593-1603页

作者： JUNRUI LIANG JIANGMING XU YANZHAO KE SICHENG LI JUNHONG HE YIDONG GUO YANG ZHANG xiaoya MA JUN YE XIAO LI JINYONG LENG PU ZHOU College of Advanced Disciplinary Studies National University of Defense TechnologyChangsha 410073China Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China Hunan Provincial Key Laboratory of High Energy Laser Technology National University of Defense TechnologyChangsha 410073China

A spectral programmable,continuous-wave mid-infrared(MIR)optical parametric oscillator(OPO),enabled by a self-developed high-power spectral tailorable fiber laser,was proposed and *** operating at a singlewavelength,the maximum idler power reached 5.53 W at 302. nm,with a corresponding pump-to-idler conversion efficiency of 14.7%.The wavelength number switchable output was available from one to *** single idler was tunable in a range of 52. nm(2.52.3380 nm).In a dual-wavelength operation,the interval between two idlers could be flexibly tuned for 470 nm(53–52. nm),and the intensity of each channel was *** idler emission was realized,meanwhile exhibiting spectral custom-tailored ***,we balanced the parametric gain through the pre-modulating broadband multi-peak pump spectra,enabling a 10 d B bandwidth adjustment of the idler emission from 2. to 12. *** versatile mid-infrared laser,simultaneously featuring wide tuning,multi-wavelength operation,and broad bandwidth manipulation,has great application potential in composition detection,terahertz generation,and speckle-free imaging.

关键词： pump tuning parametric

Regulator of G protein signaling 2. contributes to radioresistance of non-small cell lung cancer cells by suppressing pyroptosis

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Radiation Medicine and Protection 2024年第3期5卷 178-184页

作者： Jialing Zhang Zhaoyan Jiang Xinglong Liu xiaoya Jin Yan Pan Yang Bai Jianghong Zhang Chunlin Shao Institute of Radiation Medicine Shanghai Medical CollegeFudan UniversityShanghai200032China

Objective:To investigate the potential role of the regulator of G protein signaling 2.(RGS2.)in radioresistance of non-small cell lung cancer(NSCLC).Methods:A total of 35 lung adenocarcinoma(LUAD)patients from The Cancer Genome Atlas(TCGA),who un-derwent radiotherapy,were enrolled and divided into radiosensitive(n=16)and radioresistant(n=19)groups based on clinical *** expression and prognosis of RGS2. were analyzed by Gene Expression Profiling Interactive Analysis(GEPIA)database.A radioresistant cell line(A549R)was constructed by irradiating A549 cells with 6 Gy X-rays for 10 *** survival was measured by colony formation *** regulatory effect of RGS2. on pyroptosis were verified by LDH release and Western blot assay,and the underlying mech-anism was investigated by transfecting RGS2. siRNA and applying a GSDMD ***:A total of 2.181 differentially expressed genes(DEGs)were identified by analyzing the data of radio-sensitive and radioresistant individuals from the TCGA-LUAD *** DEGs were enriched in G alpha(z)signalling events analyzed by Reactome ***2. exhibited significant upregulation among the DEGs,and its higher expression predicted poor prognosis in LUAD *** vitro,the expression of RGS2. protein was increased by irradiation in A549 cells,whereas it remained at much high levels in A549R cells regardless of *** irradiation,the expressions of pyroptosis-related proteins were significantly increased in A549 cells(P2. gene in A549R cells significantly increased LDH release(P2.(P<0.05).Meantime,the increased expression le

关键词： NSCLC Radioresistance RGS2. Pyroptosis