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Occurrence and vertical distribution of aluminum and rare earths in weathered crust elution-deposited rare earth ore:Effect of soil solution pH and clay minerals

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Journal of Rare Earths 2024年第7期42卷 1394-1402,I0007页

作者： Jiaxin Pan Longsheng Zhao Zheng Li xiaowei huang Zongyu Feng Jun Chen National Engineering Research Center for Rare Earth China GRINM Group Co.Ltd.Beijing100088China School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China GRIREM Hi–Tech Co. Ltd.Langfang065201China GRIREM Advanced Materials Co. Ltd.Beijing100088China GRIMAT Engineering Institute Co. Ltd.Beijing101407China

Weathered crust elution-deposited rare earth ore is crucial source of medium and heavy rare earths,with in-situ leaching being the most common mining *** high contents of impurity of aluminum in the leach solution are a significant challenge for the subsequent enrichment process of rare earths.A comprehensive understanding of the occurrences and vertical distribution of aluminum and rare earths within typical vertical profiles can provide valuable insights into entire design of the in-situ *** paper improves a five-step sequential extraction method to analyze the occurrence and vertical distribution of rare earths and aluminum in vertical profiles from Chongzuo and *** results demonstrate that soil solution pH is the main factor affecting the vertical distribution of ionexchangeable rare *** samples have distinct areas of enrichment for ion-exchangeable rare earths or ***-exchangeable rare earths are primary concentrated in the middle and lower parts of the ore layer(4-13 m in Chongzuo,14-22 m in Longyan),while the ion-exchangeable aluminum is mainly enriched in the upper part of the ore layer(1-5 m in Chongzuo,and 2-14 m in Longyan).The vertical distribution of inorganic hydroxy aluminum is likely influenced by the micromorphology and particle size of the clay *** inorganic hydroxy aluminum concentration in Chongzuo samples decreases continuously from 415.65 to 120.95 mg/kg with increasing sampling depth,whereas the concentration in Longyan samples(110.55-171.27 mg/kg)is almost independence with sampling *** results provide direct guidance for the entire design of the injection well depth and the leaching parameters,thereby inhibiting the leaching of impurity of aluminum and lower the consumption of leaching agent.

关键词： Weathered crust elution-deposited rare earth ore Sequential extraction Occurrence Aluminum Rare earth elements

Progress of gaseous arsenic removal from flue gas by adsorption:Experimental and theoretical calculations

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Journal of Environmental Sciences 2024年第2期136卷 470-485页

作者： Xuelei Yan Qingzhu Li xiaowei huang Bensheng Li Shengtu Li Qingwei Wang School of Metallurgy and Environment Central South UniversityChangsha 410083China National Engineering Research Centre for Control and Treatment of Heavy Metal Pollution Central South UniversityChangsha 410083China National Engineering Research Center for Rare Earth Materials General Research Institute for Non-Ferrous MetalsBeijing 100088China

Because of its high mobility and difficult capture,gaseous arsenic pollution control has become the focus of arsenic pollution *** mainly exists in the form of highly toxic As_(2)O_(3)in the flue ***,removing gaseous As_(2)O_(3)from flue gas is of great practical significance for arsenic pollution *** gaseous As_(2)O_(3)on the surface of adsorbents by physical or chemical adsorption is an effective way to reduce the content of arsenic in the flue gas and alleviate arsenic *** the past few decades,various adsorbents have been developed to capture gaseous As_(2)O_(3)in the flue gas,and their adsorption mechanisms have been studied in ***,it is necessary to review the strategies of arsenic removal from flue gas by adsorption,which can inspire further *** on summarizing the morphological distribution of gaseous As_(2)O_(3)in the flue gas,this review further summarizes the removal of gaseous As_(2)O_(3)by several adsorbents and the effect of temperature and the main components of the flue gas on arsenic *** addition,the mechanism of arsenic removal based on adsorption in the flue gas is discussed in depth through theoretical calculations,which is the particular focus of this ***,prospects based on the present research state of arsenic removal by adsorption are proposed to provide ideas for developing effective and stable adsorbents for arsenic removal from flue gas.

关键词： Gaseous arsenic Flue gas Adsorption Theoretical calculation Mechanism

Expanding the horizons of targeted protein degradation:A non-small molecule perspective

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Acta Pharmaceutica Sinica B 2024年第6期14卷 2402-2427页

作者： xiaowei huang Fengbo Wu Jing Ye Lian Wang Xiaoyun Wang Xiang Li Gu He Department of Pharmacy and Department of Dermatology&Venerology West China HospitalSichuan UniversityChengdu 610041China Department of Urology West China HospitalSichuan UniversityChengdu 610041China Laboratory of Dermatology Clinical Institute of Inflammation and ImmunologyFrontiers Science Center for Disease-Related Molecular Network and State Key Laboratory of BiotherapyWest China HospitalSichuan UniversityChengdu 610041China

Targeted protein degradation(TPD)represented by proteolysis targeting chimeras(PROTACs)marks a significant stride in drug discovery.A plethora of innovative technologies inspired by PROTAC have not only revolutionized the landscape of TPD but have the potential to unlock functionalities beyond ***-small-molecule-based approaches play an irreplaceable role in this field.A wide variety of agents spanning a broad chemical spectrum,including peptides,nucleic acids,antibodies,and even vaccines,which not only prove instrumental in overcoming the constraints of conventional small molecule entities but also provided rapidly renewing *** we summarize the burgeoning non-small molecule technological platforms inspired by PROTACs,including three major trajectories,to provide insights for the design strategies based on novel paradigms.

关键词： Targeted protein degradation Proteolysis targeting chimera Endocytosis Autophagy Proximity-inducing modality Post-translational modification

The structure–activity relationships of Rh/CeO_(2)-ZrO_(2) catalysts based on Rh metal size effect in the three-way catalytic reactions

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Nano Research 2024年第8期17卷 6870-6878页

作者： Dongming Chen Weixin Zhao Zihao Xu Zheng Zhao Juanyu Yang Yongke Hou Yongqi Zhang Zongyu Feng Meisheng Cui xiaowei huang National Engineering Research Center for Rare Earth Grirem Advanced Materials Co.Ltd.Beijing 100088China Grirem Hi-Tech Co. Ltd.Sanhe 065201China General Research Institute for Nonferrous Metals Beijing 100088China

With the continuous tightening of automotive emission regulations and the increasing promotion of energy-efficient hybrid vehicles,new challenges have arisen for the low-temperature performance of three-way catalysts(TWCs).To guide the design of next-generation TWCs,it is essential to further develop our understanding of the relationships between microstructure and catalytic ***,Rh/CeO_(2)–ZrO_(2) catalysts were synthesized with different Rh metal dispersion by using a combination of the wet impregnation method and reduction *** catalysts included Rh single-atom catalysts,cluster catalysts,and nanoparticle *** results showed that the Rh nanoparticle catalyst,with an average size of 1.9 nm,exhibited superior three-way catalytic performance compared to the other *** on the catalytic activity in a series of simple reaction atmospheres such as CO+O_(2),NO+CO,and hydrocarbons(HCs)+O_(2) and operando infrared spectroscopy,we found that metallic Rh sites on Rh nanoparticles are the key factor responsible for the low-temperature catalytic performance.

关键词： Rh/CeO_(2)-ZrO_(2) catalyst Rh metal size effect Rh nanoparticles three-way catalytic performance

Autophagy in hepatic progenitor cells modulates exosomal miRNAs to inhibit liver fibrosis in schistosomiasis

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Frontiers of Medicine 2024年第3期18卷 538-557页

作者： Yue Yuan Jiaxuan Li Xun Lu Min Chen Huifang Liang Xiao-ping Chen Xin Long Bixiang Zhang Song Gong xiaowei huang Jianping Zhao Qian Chen Division of Gastroenterology Department of Internal Medicine at Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan430030China Hepatic Surgery Center Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan430030China Hubei Key Laboratory of Hepato–Pancreato–Biliary Diseases Wuhan430030China Department of Trauma Surgery Tongji Trauma CenterTongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan430030China

Schistosoma infection is one of the major causes of liver *** roles of hepatic progenitor cells(HPCs)in the pathogenesis of liver fibrosis have been ***,the precise mechanism underlying the role of HPCs in liver fibrosis in schistosomiasis remains *** study examined how autophagy in HPCs affects schistosomiasis-induced liver fibrosis by modulating exosomal *** activation of HPCs was verified by immunohistochemistry(IHC)and immunofluorescence(IF)staining in fibrotic liver from patients and mice with Schistosoma japonicum *** coculturing HPCs with hepatic stellate cells(HSCs)and assessing the autophagy level in HPCs by proteomic analysis and in vitro phenotypic assays,we found that impaired autophagy degradation in these activated HPCs was mediated by lysosomal *** autophagy by the autophagy inhibitor chloroquine(CQ)significantly diminished liver fibrosis and granuloma formation in ***-infected ***-secreted extracellular vehicles(EVs)were further isolated and studied by miRNA ***-1306-3p,miR-493-3p,and miR-34a-5p were identified,and their distribution into EVs was inhibited due to impaired autophagy in HPCs,which contributed to suppressing HSC *** conclusion,we showed that the altered autophagy process upon HPC activation may prevent liver fibrosis by modulating exosomal miRNA release and inhibiting HSC activation in *** the autophagy degradation process may be a therapeutic strategy for liver fibrosis during Schistosoma infection.

关键词： schistosomiasis hepatic progenitor cell autophagy extracellular vesicle fibrosis miRNA

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2023年中国稀土研究综合评述

中国稀土学报 2024年第3期42卷 381-418页

作者：严纯华黄小卫兰州大学化学化工学院稀有同位素前沿科学中心甘肃省有色金属化学与资源利用重点实验室甘肃兰州730000 北京大学化学与分子工程学院北京分子科学国家研究中心北京大学稀土材料化学及应用国家重点实验室北京100871 中国有研科技集团有限公司稀土国家工程研究中心有研稀土新材料股份有限公司北京100088

稀土新材料作为现代工业和高新技术产业发展的关键基础材料,在未来的产业发展中将面临新的机遇和挑战。本文主要以中国2023年稀土领域研究发展状况为对象,总结归纳了近年来中国稀土光功能材料、催化材料、生物医用材料等10个稀土材料领... 详细信息

稀土新材料作为现代工业和高新技术产业发展的关键基础材料,在未来的产业发展中将面临新的机遇和挑战。本文主要以中国2023年稀土领域研究发展状况为对象,总结归纳了近年来中国稀土光功能材料、催化材料、生物医用材料等10个稀土材料领域以及中国在稀土提取和分离方面取得的研究成果及进展,并对未来发展趋势进行了研判和展望。

关键词：稀土新材料提取分离

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我国不同付费模式信用评级校验机制研究

北京工商大学学报（社会科学版） 2024年第1期39卷 90-103页

作者：黄晓薇安小雪对外经济贸易大学中国金融学院北京100105

我国债券市场刚性兑付被打破后,不断出现高评级债券违约事件。为此,监管部门积极发展多种评级,以期提高债券评级质量。通过理论建模与实证分析,研究了不同付费模式信用评级如何综合发挥校验作用。基于博弈模型的理论分析发现,不同付费... 详细信息

我国债券市场刚性兑付被打破后,不断出现高评级债券违约事件。为此,监管部门积极发展多种评级,以期提高债券评级质量。通过理论建模与实证分析,研究了不同付费模式信用评级如何综合发挥校验作用。基于博弈模型的理论分析发现,不同付费模式评级发挥校验作用的机制在于投资者的反应:当投资者付费和发行人付费两种模式评级差值增大,投资者不以单一评级结果进行债券定价,而是根据评级差值调整债券价格。基于2011—2020年企业债评级数据的经验证据显示,随着评级差值增大,发行人付费评级机构会降低后续评级,且评级差值对单一信用评级与债券信用利差之间的负向关系具有抑制作用。进一步检验发现,发行人付费评级机构提供的偏正面的私有信息会降低债券信用利差,而以中债资信为代表的投资者付费评级机构提供的私有信息则不会显著影响债券信用利差,均体现出单一评级模式在定价方面的弊端。因此,监管部门应继续鼓励发展投资者付费评级模式,并鼓励机构投资者发展内部评级,以充分发挥多种评级模式的交叉校验作用。

关键词：债券市场付费模式信用评级校验机制评级差值评级质量

“去美元化”背景下的人民币贸易计价研究——基于双边货币互换协议视角

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国际金融研究 2024年第1期 15-26页

作者：黄晓薇张卓识卞洋对外经济贸易大学中国金融学院

在美联储持续加息以及美欧对俄频繁金融制裁的背景下,各经济体加速“去美元化”,这为发展人民币贸易计价功能带来机遇。本文在允许第三方货币计价的条件下构建了基于厂商利润最大化的计价货币选择模型,分析表明:双边货币互换协议有助于... 详细信息

在美联储持续加息以及美欧对俄频繁金融制裁的背景下,各经济体加速“去美元化”,这为发展人民币贸易计价功能带来机遇。本文在允许第三方货币计价的条件下构建了基于厂商利润最大化的计价货币选择模型,分析表明:双边货币互换协议有助于增强人民币的贸易计价功能,其作用机制包括稳定人民币汇率和增强境外人民币信心两个方面。本文使用2005—2021年UNComtrade数据库构建了国家间贸易价格数据集,测算人民币的贸易计价功能。研究发现:双边货币互换协议对人民币的贸易计价功能有显著增强作用,剔除美元影响后该作用依然存在。机制检验结果表明,双边货币互换协议从稳定人民币对签署国货币汇率和增强境外人民币信心两个方面推进人民币的贸易计价功能。本文研究对“去美元化”背景下稳步发展人民币贸易计价功能具有重要的政策参考价值。

关键词：贸易计价功能双边货币互换协议 “去美元化” 人民币汇率

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熔喷机智能化控制系统的实践与应用

化工管理 2024年第5期 15-17页

作者：黄晓伟常州纺织服装职业技术学院江苏常州213164

文章针对熔喷机智能化控制系统控制流程长、工艺标准高、控制要求难等特点进行了详细的分析,并提出从物联网平台、PLC、变频器和伺服电机驱动自动化电气控制等系统进行优化设计,来满足生产过程实时和历史数据的采集与信息反馈,实现电气... 详细信息

文章针对熔喷机智能化控制系统控制流程长、工艺标准高、控制要求难等特点进行了详细的分析,并提出从物联网平台、PLC、变频器和伺服电机驱动自动化电气控制等系统进行优化设计,来满足生产过程实时和历史数据的采集与信息反馈,实现电气系统的高精度智能化控制应用措施。

关键词：熔喷机 PLC 物联网平台