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High‑Performance Silicon‑Rich Microparticle Anodes for Lithium‑Ion Batteries Enabled by Internal Stress Mitigation

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纳微快报:英文版 2023年第12期15卷 99-114页

作者： Yao Gao Lei Fan Rui Zhou xiaoqiong du Zengbao Jiao Biao Zhang Department of Applied Physics The Hong Kong Polytechnic UniversityKowloonHong KongPeople’s Republic of China Department of Mechanical Engineering The Hong Kong Polytechnic UniversityKowloonHong KongPeople’s Republic of China Department of Physics The Chinese University of Hong KongNew TerritoriesHong KongPeople’s Republic of China

Si is a promising anode material for Li ion batteries because of its high specific capacity,abundant reserve,and low cost.However,its rate performance and cycling stability are poor due to the severe particle pulverization during the lithiation/delithiation process.The high stress induced by the Li concentration gradient and anisotropic deformation is the main reason for the fracture of Si particles.Here we present a new stress mitigation strategy by uniformly distributing small amounts of Sn and Sb in Si micron-sized particles,which reduces the Li concentration gradient and realizes an isotropic lithiation/delithiation process.The Si8.5Sn0.5Sb microparticles(mean particle size:8.22μm)show over 6000-fold and tenfold improvements in electronic conductivity and Li diffusivity than Si particles,respectively.The discharge capacities of the Si_(8.5)Sn_(0.5)Sb microparticle anode after 100 cycles at 1.0 and 3.0 A g^(-1)are 1.62 and 1.19 Ah g^(-1),respectively,corresponding to a retention rate of 94.2%and 99.6%,respectively,relative to the capacity of the first cycle after activation.Multicomponent microparticle anodes containing Si,Sn,Sb,Ge and Ag prepared using the same method yields an ultra-low capacity decay rate of 0.02%per cycle for 1000 cycles at 1 A g^(-1),corroborating the proposed mechanism.The stress regulation mechanism enabled by the industry-compatible fabrication methods opens up enormous opportunities for low-cost and high-energy-density Li-ion batteries.

关键词： Silicon anodes Silicon microparticles Lithium-ion batteries Internal stress

Teaching Mode Reform of the Electrical Automation Control Course

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Journal of Electronic Research and Application 2024年第3期8卷 47-52页

作者： xiaoqiong Chen Wuhan Donghu University Wuhan 430212China

Under the background of the new era,higher requirements are put forward for colleges and universities to carry out teaching reform.Teachers of electrical automation control courses should update their teaching ideas regularly,innovate teaching methods,and take novel and effective measures to carry out related work.Because electrical automation control courses tend to be technology-oriented,teachers can help students consolidate basic knowledge.They should also focus on developing practical skills so students can easily adapt to future job positions.However,there are many problems in the actual teaching process,which hampers the improvement of the teaching quality to a certain extent.In view of this,this paper presents an in-depth exploration based on theories and practical experiences.It starts with an analysis of the current teaching status of electrical automation control courses in colleges and universities,followed by suggestions to improve them based on their characteristics and students’needs.

关键词： Universities Electrical automation technology Teaching status Optimization strategy

Accelerating the Digitalization Process in Rural China and Promoting Common Prosperity

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Asian Agricultural Research 2024年第3期16卷 8-13页

作者： Zhongxiong LAI xiaoqiong XU Institute of Horticultural Biotechnology Fujian Agriculture and Forestry UniversityFuzhou 350002China

Under the historical background of promoting agricultural and rural modernization in an all-round way,this paper deeply analyzes the practical significance of digital construction in rural China,and explores the problems in the digitalization level of rural infrastructure,farmers digitalization awareness and accomplishment,and agricultural digital system.Countermeasures and suggestions are put forward from four aspects:digital village construction policy system,rural digital infrastructure construction,rural digital talent cultivation system,and agricultural digital system,and the rural digital construction of Huzhou City is taken as an example,in order to further realize the goal of empowering rural farmers with digital technology for common prosperity.

关键词： Digital village Digital technology Rural farmer Common prosperity

Nitrogen-doped graphene hydrogel-supported NiPt-CeOx nanocomposites and their superior catalysis for hydrogen generation from hydrazine at room temperature

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Nano Research 2017年第8期10卷 2856-2865页

作者： xiaoqiong du Chao Liu Cheng du Ping Cai Gongzhen Cheng Wei Luo College of Chemistry and Molecular Sciences Wuhan University Wuhan 430072 China Key laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University Tianjin 300071 China

The safe and efficient storage and release of hydrogen is one of the key technological challenges for the fuel cell-based hydrogen economy. Hydrazine monohydrate has attracted considerable attention as a safe and convent chemical hydrogen-storage material. Herein, we report the facile synthesis of NiPt-CeOx nanocomposites supported by three-dimensional nitrogen-doped graphene hydrogels （NGHs） via a simple one-step co-reduction synthesis method. These catalysts were composition-dependent for hydrogen generation from an alkaline solution of hydrazine. （NisPt5）I-（CeOx）0.B/NGH exhibited the highest catalytic activity, with 100% hydrogen selectivity and turnover frequencies of 408 h^-1 at 298 K and 3,064 h^-1 at 323 K. These superior catalytic performances are attributed to the electronic structure of the NiPt centers, which was modified by the electron interaction between NiPt and CeOx and the strong metal-support interaction between NiPt-CeOx and the NGH.

关键词： nitrogen-doped graphene hydrogels NiPt-CeOx hydrogen storage hydrazine

Realizing high-performance Zn-ion batteries by a reduced graphene oxide block layer at room and low temperatures

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Journal of Energy Chemistry 2020年第4期29卷 1-7页

作者： Jian-Qiu Huang Xiuyi Lin Hong Tan xiaoqiong du Biao Zhang Department of Applied Physics The Hong Kong Polytechnic UniversityHong KongChina

Rechargeable aqueous Zn-ion batteries (ZIBs) have attracted great attention due to their costeffectiveness,high safety,and environmental friendliness.However,some issues associated with poor structural instability of cathode materials and fast self-discharge hinder the further development of ZIBs.Herein,a new configuration is introduced by placing a reduced graphene oxide film as a block layer between the separator and the V2O5·nH2O cathode.This layer prevents the free diffusion of dissolved active materials to the anode and facilitates the transport of Zn ion and electrons,largely improving the cyclic stability and alleviating the self-discharge.Accordingly,the optimized battery delivers a remarkable capacity of 191 mAh g^-1 after 500 cycles at 2 A g^-1.Moreover,a high capacity of 106 mAh g^-1 is achieved after 100 cycles at-20℃.The strategy proposed is expected to be applicable to other electrode systems,thus offering a new approach to circumvent the critical challenges facing aqueous batteries.

关键词： Block layer Dissolution Self-discharge Low temperatures Aqueous Zn-ion batteries

BioTreasury:a community-based repository enabling indexing and rating of bioinformatics tools

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Science China(Life Sciences) 2024年第2期67卷 221-229页

作者： Qi Zhao Xin Zhou Jingxing Wu Jieyi Cai xiaoqiong Bao Lin Tang Chaoye Wang Chunlei Liu Yukai Wang Yuyan Teng Mohan Zheng Weiping Mu Zhixiang Zuo Yubin Xie Xiaotong Luo Jian Ren School of Life Sciences State Key Laboratory of Oncology in South ChinaCancer CenterGuangdong Provincial Clinical Research Center for CancerSun Yat-sen UniversityGuangzhou 510060China Institute of Precision Medicine The First Affiliated HospitalSun Yat-sen UniversityGuangzhou 510080China Guangdong Institute of Gastroenterology Department of General SurgeryGuangdong Provincial Key Laboratory of Colorectal and Pelvic Floor DiseasesThe Sixth Affiliated HospitalSun Yat-sen UniversityGuangzhou 510275China

The exponential growth of bioinformatics tools in recent years has posed challenges for scientists in selecting the most suitable one for their data analysis assignments.Therefore,to aid scientists in making informed choices,a community-based platform that indexes and rates bioinformatics tools is urgently needed.In this study,we introduce Bio Treasury(http://***),an integrated communitybased repository that provides an interactive platform for users and developers to share their experiences in various bioinformatics tools.Bio Treasury offers a comprehensive collection of well-indexed bioinformatics software,tools,and databases,totaling over 10,000 entries.In the past two years,we have continuously improved and maintained Bio Treasury,adding several exciting features,including creating structured homepages for every tool and user,a hierarchical category of bioinformatics tools and classifying tools using large language model(LLM).Bio Treasury streamlines the tool submission process with intelligent auto-completion.Additionally,Bio Treasury provides a wide range of social features,for example,enabling users to participate in interactive discussions,rate tools,build and share tool collections for the public.We believe Bio Treasury can be a valuable resource and knowledge-sharing platform for the biomedical community.It empowers researchers to effectively discover and evaluate bioinformatics tools,fostering collaboration and advancing bioinformatics research.

关键词： bioinformatics tools index tool database rating system large language model tool collections shari

Newcastle disease virus suppresses antigen presentation via inhibiting IL-12 expression in dendritic cells

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2024年第3期25卷 254-270页

作者： Fulong NAN Wenlong NAN Xin YAN Hui WANG Shasha JIANG Shuyun ZHANG Zhongjie YU Xianjuan ZHANG Fengjun LIU Jun LI xiaoqiong ZHOU Delei NIU Yiquan LI Wei WANG Ning SHI Ningyi JIN Changzhan XIE Xiaoni CUI He ZHANG Bin WANG Huijun LU Department of Special Medicine Department of Pathogenic BiologySchool of Basic MedicineQingdao UniversityQingdao 266071China China Animal Health and Epidemiology Center Qingdao 266032China Academician Workstation of Jilin Province Changchun University of Chinese MedicineChangchun 130117China Institute of Virology Wenzhou UniversityWenzhou 325035China College of Veterinary Medicine Jilin UniversityChangchun 130012China Changchun Veterinary Research Institute Chinese Academy of Agricultural SciencesChangchun 130122China Sino-Cell Biomed Co. Ltd.Qingdao 266000China

As a potential vectored vaccine,Newcastle disease virus(NDV)has been subject to various studies for vaccine development,while relatively little research has outlined the immunomodulatory effect of the virus in antigen presentation.To elucidate the key inhibitory factor in regulating the interaction of infected dendritic cells(DCs)and T cells,DCs were pretreated with the NDV vaccine strain LaSota as an inhibitor and stimulated with lipopolysaccharide(LPS)for further detection by enzyme-linked immunosorbent assay(ELISA),flow cytometry,immunoblotting,and quantitative real-time polymerase chain reaction(qRT-PCR).The results revealed that NDV infection resulted in the inhibition of interleukin(IL)-12p40 in DCs through a p38 mitogen-activated protein kinase(MAPK)-dependent manner,thus inhibiting the synthesis of IL-12p70,leading to the reduction in T cell proliferation and the secretion of interferon-(IFN-),tumor necrosis factor-α(TNF-α),and IL-6 induced by DCs.Consequently,downregulated cytokines accelerated the infection and viral transmission from DCs to T cells.Furthermore,several other strains of NDV also exhibited inhibitory activity.The current study reveals that NDV can modulate the intensity of the innate-adaptive immune cell crosstalk critically toward viral invasion improvement,highlighting a novel mechanism of virus-induced immunosuppression and providing new perspectives on the improvement of NDV-vectored vaccine.

关键词： Newcastle disease virus Dendritic cells Interleukin-12(IL-12) T cells Immunosuppression

新时代区域协调发展的新态势、新问题与推进路径

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区域经济评论 2024年第3期 46-51页

作者：万晓琼中国人民大学书报资料中心北京100086

我国区域协调发展的演进历程可以分为四个阶段:改革开放前,公平导向的区域低水平均衡发展阶段(1949-1977年);改革开放后,增长极导向的区域非均衡发展阶段(1978-1999年);21世纪以来,全局统筹导向的区域协调发展阶段(2000-2011年);党的十... 详细信息

我国区域协调发展的演进历程可以分为四个阶段:改革开放前,公平导向的区域低水平均衡发展阶段(1949-1977年);改革开放后,增长极导向的区域非均衡发展阶段(1978-1999年);21世纪以来,全局统筹导向的区域协调发展阶段(2000-2011年);党的十八大以来,多元导向的区域高质量协调发展阶段(2012年至今)。进入新时代,区域协调发展呈现新的内涵、新的发展态势,也出现一些新的问题。宜从顶层设计层面,统筹协调推进区域发展总体战略;从政策实施层面,构建系统完备的区域政策体系;从制度保障层面,健全区域协调发展新机制;从驱动力层面,以全国统一大市场建设助力区域协调发展。

关键词：区域协调发展演进历程新态势新问题推进路径

碳纤维/不锈钢极薄带纤维金属层板制备工艺及其弯曲性能

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复合材料学报 2024年第2期41卷 1047-1057页

作者：马威管海陆张晓琼王涛太原理工大学机械与运载工程学院太原030024 太原理工大学先进成形与智能装备研究院太原030024

不锈钢极薄带这一新型精密带材具有质量轻(厚度仅为0.01~0.1 mm)、强度高、易成型、耐腐蚀等诸多优点,是一种极具应用前景的轻质高强材料。为了探讨不锈钢极薄带作为纤维金属层板组分材料的可行性及评估其力学性能优劣,通过对比6种不同... 详细信息

不锈钢极薄带这一新型精密带材具有质量轻(厚度仅为0.01~0.1 mm)、强度高、易成型、耐腐蚀等诸多优点,是一种极具应用前景的轻质高强材料。为了探讨不锈钢极薄带作为纤维金属层板组分材料的可行性及评估其力学性能优劣,通过对比6种不同的不锈钢极薄带表面处理工艺,探明了6种工艺中机械打磨+丙酮清洗+10wt%氢氧化钠溶液腐蚀+1wt%偶联剂是不锈钢极薄带与碳纤维预浸料复合的最优表面处理工艺,其单搭接拉伸剪切强度值为21.3 MPa。基于该工艺,采用T700碳纤维单向预浸料、T300编织布预浸料及0.1 mm厚软态、半硬态与硬态不锈钢极薄带分别制备出含不同层数与不同类型不锈钢极薄带的纤维金属层板。并通过三点弯曲实验对所制层板的弯曲性能与变形失效机制进行了系统研究。结果表明:碳纤维/不锈钢极薄带纤维金属层板弯曲失效模式主要受钢带强韧性变化影响,弯曲变形主要受钢带含量影响。

关键词：纤维金属层板不锈钢极薄带表面处理抗弯性能弯曲失效